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P. von Neumann-Cosel

Publications and source records attributed to P. von Neumann-Cosel.

At least 19 recordsLinked to original sources

Low-energy collective structure of $^{92,94}$Zr and $^{94}$Mo from ($e,e^{\prime}$) and ($p,p^{\prime}$) scattering I. Experimental results

This is the first of two papers discussing a new signature of quadrupole mixed-symmetry states in the vibrational nuclei $^{92,94}$Zr and $^{94}$Mo based on proton and neutron transition densities derived from the comparison of inelastic electron and proton scattering experiments. Results of the $(e,e^\prime)$ and $(p,p^\prime)$ experiments on these nuclei as well as $(p,p^\prime)$ data for other potential cases $^{96}$Mo and $^{70}$Zn are presented. Spin and parity quantum numbers of excited states are assigned based on angular distributions from the proton scattering data in comparison to calculations employing form factors from the collective model in distorted-wave Born approximation. Possible candidates of one-phonon fully symmetric and mixed-symmetry states as well as members of two-phonon multiplets are identified.

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Low-energy collective structure of $^{92,94}$Zr and $^{94}$Mo from ($e,e^{\prime}$) and ($p,p^{\prime}$) scattering II. Signatures of mixed-symmetry states and origin of collectivity

This is the second of two papers discussing a new experimental signature of mixed-symmetry states (MSS) in the vibrational nuclei $^{92,94}$Zr and $^{94}$Mo based on proton and neutron transition densities. Quasiparticle-phonon model calculations for these nuclei are extensively tested by comparison to ground-state properties, energies and moments of excited states, transition probabilities between them, and the momentum transfer dependence in $(e,e^\prime)$ and $(p,p^\prime)$ reactions. The overall very good agreement permits the extraction of information on the wave functions of the MSS and their fully symmetric (FSS) counterparts. MSS can be identified by a sign change between the leading proton and neutron two-quasiparticle configurations compared to the FSS. Possible candidates for $2^+$, $3^-$, and $4^+$ MSS are identified. The modification of proton and neutron transition densities, which can be derived from a combined analysis of inelastic electron and proton scattering, by the sign change provide a new experimental signature of MSS. The collectivity of ground-state excitations of predominantly one-phonon FSS and MSS is generated to a large extent by the coupling to high-lying states forming giant resonances with the same spin and parity.

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Exploring the statistical properties of the neutron-deficient $^{109}$In isotope with the Oslo method

The nuclear level density (NLD) and the $γ$-ray strength function (GSF) of the neutron-deficient $^{109}$In isotope were extracted for the first time with data from the $^{106}$Cd$(α,pγ)^{109}$In reaction using a combination of the Oslo and the shape methods. Both quantities are consistent with those of neighboring Cd and Sn nuclei, but show substantial discrepancies with currently available model predictions. In contrast to earlier observations in the neighboring isotopic chains, $^{109}$In does not exhibit any significant enhancement of the dipole strength near the neutron separation energy. To interpret this feature, random-phase time-blocking approximation calculations have been performed for $^{109}$In and the neighboring $^{110,112}$Sn nuclei. The experimental data were also employed to estimate cross sections and rates of the radiative neutron- and proton-capture reactions, $^{108}$In($n,γ)$$^{109}$In and $^{108}$Cd($p,γ)$$^{109}$In, respectively, with the reaction code TALYS. Our ($p,γ)$ cross section is in excellent agreement with direct measurements over a wide range of proton energies, while the ($n,γ)$ cross section demonstrates notable deviations from predictions in the JINA REACLIB library. The new results on the statistical properties of $^{109}$In provide valuable constraints that may help address the problem of large model uncertainties compromising the accuracy of astrophysical $p$-process simulations.

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Electric dipole strength in $sd$-shell nuclei from small-angle proton scattering

The present work reports new total photoabsorption cross sections for the $N=Z$ nuclei in the $sd$-shell $^{20}$Ne, $^{24}$Mg, $^{28}$Si, $^{32}$S, $^{36}$Ar, and for $^{26}$Mg. The results are compared to predictions of a data-driven artificial neural network application and to configuration-interaction shell-model calculations covering the excitation energy region of the isovector giant dipole resonance. Double-differential cross sections of the $(p,p^\prime)$ reaction at 295 MeV have been measured between $0^\circ$ and $14^\circ$. The angular distributions of the $E1$ parts due to Coulomb excitation have been extracted with a multipole decomposition analysis for excitation energies 12 to 24 MeV and converted to equivalent photoabsorption cross sections with the virtual photon method. Reasonable agreement of the photoabsorption cross sections with previous experiments is found for $^{24}$Mg and $^{28}$Si, while the present results diverge for $^{32}$S. For the first time, data are presented for $^{20}$Ne, $^{26}$Mg and $^{36}$Ar. Configuration-interaction shell-model calculations provide an overall satisfactory description of the fragmented $E1$ strength distributions. The same holds for absolute cross sections except for $^{26}$Mg and $^{36}$Ar, where the experimental results significantly exceed the expected exhaustion of the Thomas-Reiche-Kuhn energy-weighted sum rule. Fot light nuclei, there is a larger model dependence compared to previous analyses in heavy nuclei, in particular for excitation energies above 20 MeV, due to the need to constrain the continuum background with additional assumptions. The overall success of the shell-model approach to describe the features of the experimental photoabsorption cross sections motivates its application in large-scale reaction network calculations aiming at an understanding of the mass composition of ultrahigh-energy cosmic rays.

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Wavelet analysis of monopole strength in highly deformed $^{24}$Mg

Experimental data on $α$-particle inelastic scattering for monopole excitations in $^{24}$Mg in the excitation-energy region $E_{\rm x}$$=$$9$$-$$25$ MeV, obtained at the iThemba Laboratory for Accelerator Based Sciences (iThemba LABS), have been analyzed within a fully self-consistent quasiparticle random-phase approximation (QRPA) framework using two Skyrme parametrizations. A good overall agreement with the experimental data is achieved, particularly with the SkP$^δ$ force, which corresponds to a low nuclear incompressibility of $K_{\infty}$$=$$202$ MeV. Extraction of energy scales, by means of wavelet analysis, characterizing the observed fine structure of the isoscalar giant monopole resonance (ISGMR) as well as the low-energy region $10$$-$$18$ MeV of the deformation-induced monopole-quadrupole coupling (MQC) in order to investigate the damping mechanism contributing to their decay widths. Characteristic energy scales are extracted from the fine structure using continuous wavelet transforms. The experimental results are compared to QRPA calculations employing the Skyrme parameterizations SkP$^δ$ and SVbas. A significant, if not decisive, impact of the MQC strength on the wavelet power spectra is observed across the entire excitation-energy range of $10$$-$$24$ MeV. Wavelet features derived from the QRPA and from unperturbed two-quasiparticle (2qp) monopole strengths are compared. The results demonstrate that the residual interaction plays a key role in reproducing realistic wavelet powers and characteristic energy scales. Overall, a continuous range of scales $δE$$=$$200$$-$$1000$ keV is obtained rather than distinct isolated scales. The deformation softness of $^{24}$Mg is found to significantly influence both the monopole strength distribution and the wavelet characteristics.

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Electric dipole polarizability constraints on neutron skin and symmetry energy

We review the experimental knowledge on the dipole polarizability (DP) of nuclei and its relation to the neutron skin thickness and properties of the neutron-rich matter equation of state (EOS). The discussion focuses on recent experiments using relativistic Coulomb excitation in inelastic proton scattering at extreme forward angles covering a mass range from $^{40}$Ca to $^{208}$Pb. Constraints on the neutron skins and the density dependence of the symmetry energy are derived from systematic comparison to calculations based on density functional theory (DFT) and ab initio methods utilizing interactions derived from chiral effective field theory ($χ$EFT). The results consistently favor a soft EOS around or slightly below the saturation point. An outlook is given on possible improvements of the precision achievable in stable nuclei and studies of exotic neutron-rich unstable nuclei with upcoming experimental facilities.

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The Electron-Gamma Coincidence Setup DAGOBERT

The QCLAM electron spectrometer at the S-DALINAC electron accelerator at Technische Universität Darmstadt has been extended by the DAGOBERT $γ$-detector array consisting of fast timing and high efficiency LaBr$_3$:Ce detectors to perform electron-gamma coincidence measurements. The functionality of the setup and data acquisition system was demonstrated in a commissioning measurement on $^{12}\textrm{C}$ observing the $4.44\,$MeV and $15.11\,$MeV states. A medium-heavy nucleus, $^{96}\textrm{Ru}$, has been studied for the first time up to excitation energies of $15\,$MeV using the $(e,e'γ)$ reaction. In particular, the angular distribution of the $2_1^+$ state and the $γ$-decay branching ratios of the mixed-symmetric $2_3^+$ state were observed. DAGOBERT@QCLAM is a new and worldwide unique setup for nuclear structure studies of excitation and decay using purely electromagnetic probes, with a significantly improved sensitivity compared to previous experiments.

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Systematics of the low-energy electric dipole strength in the Sn isotopic chain

We present a systematic study of the mass dependence of the low-energy electric dipole strength (LEDS) in Sn isotopes in the range $ A = 111 - 124$ based on data obtained with the Oslo method and with relativistic Coulomb excitation in forward-angle ($p,p^\prime$) scattering. The combined data cover an energy range of $2 - 20$ MeV which permits, with minimal assumptions, a decomposition of the total strength into the contribution from the low-energy tail of the isovector giant dipole resonance (IVGDR) and possible resonance-like structures on top of it. In all cases, a resonance peaked at about 8.3 MeV is observed, exhausting an approximately constant fraction of the Thomas-Reiche-Kuhn (TRK) sum rule with a local maximum at $^{120}$Sn which might be related to shell structure effects. For heavier isotopes ($A \geq 118$) a consistent description of the data requires the inclusion of a second resonance centered at 6.5 MeV, representing the isovector response of the pygmy dipole resonance (PDR). Its strength corresponds to a small fraction of the total LEDS only and shows an approximately linear dependence on mass number. The experimental results are also compared to ab initio-based microscopic calculations to investigate the importance of an inclusion of quasiparticle vibration coupling (qPVC) for a realistic description of the LEDS. A possible interpretation of the experimentally observed two-bump structure is given.

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Candidate toroidal electric dipole mode in the spherical nucleus $^{58}$Ni

Dipole toroidal modes appear in many fields of physics. In nuclei, such a mode was predicted more than 50 years ago, but clear experimental evidence was lacking so far. Using a combination of high-resolution inelastic scattering experiments with photons, electrons and protons, we identify for the first time candidates for toroidal dipole excitations in the nucleus $^{58}$Ni and demonstrate that transverse electron scattering form factors represent a relevant experimental observable to prove their nature.

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Electric dipole polarizability of $^{58}$Ni

The electric dipole strength distribution in $^{58}$Ni between 6 and 20 MeV has been determined from proton inelastic scattering experiments at very forward angles at RCNP, Osaka. The experimental data are rather well reproduced by quasiparticle random-phase approximation calculations including vibration coupling, despite a mild dependence on the adopted Skyrme interaction. They allow an estimate of the experimentally inaccessible high-energy contribution above 20 MeV, leading to an electric dipole polarizability $α_\mathrm{D}(^{58}{\rm Ni}) = 3.48(31)$ fm$^3$. This serves as a test case for recent extensions of coupled-cluster calculations with chiral effective field theory interactions to nuclei with two nucleons on top of a closed-shell system.

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Electric and magnetic dipole strength in $^{58}$Ni from forward-angle inelastic proton scattering

The aim of the present work is a state-by-state analysis of possible E1 and M1 transitions in $^{58}$Ni with a high-resolution (p,p') experiment at 295 MeV and very forward angles including 0° and a comparison to results from studies of the dipole strength with the $(γ,γ')$ and (e,e') reactions. The E1 and M1 cross sections of individual peaks in the spectra are deduced with a multipole decomposition analysis and converted to reduced E1 and spin-M1 transition strengths using the virtual photon and the unit cross-section method, respectively. Despite the high level density good agreement is obtained for the deduced excitation energies of J = 1 states in the three types of experiments indicating that the same states are excited. The B(E1) and B(M1) strengths from the $(γ,γ^\prime)$ experiments are systematically smaller than in the present work because of the lack of information on branching ratios to lower-lying excited states and the competition of particle emission. Fair agreement with the B(M1) strengths extracted from the (e,e') data is obtained after removal of E1 transitions uniquely assigned in the present work, which belong to a low-energy toroidal mode with unusual properties mimicking M1 excitations in electron scattering. The experimental M1 strength distribution is compared to large-scale shell-model calculations with the effective GXPF1A and KB3G interactions. They provide a good description of the isospin splitting and the running sum of the M1 strength. A quenching factor 0.74 for the spin-isospin part of the M1 operator is needed to attain quantitative agreement with the data.

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Systematic study of the low-lying electric dipole strength in Sn isotopes and its astrophysical implications

The $γ$-ray strength functions (GSF) and nuclear level densities (NLD) below the neutron threshold have been extracted for $^{111-113,116-122,124}$Sn from particle-$γ$ coincidence data with the Oslo method. The evolution of bulk properties of the low-lying electric dipole response has been investigated on the basis of the Oslo GSF data and results of a recent systematic study of electric and magnetic dipole strengths in even-even Sn isotopes with relativistic Coulomb excitation. The obtained GSFs reveal a resonance-like peak on top of the tail of the isovector giant dipole resonance, centered at $\approx$8 MeV and exhausting $\approx$2\% of the classical Thomas-Reiche-Kuhn (TRK) sum. In contrast to predictions of the relativistic quasiparticle random-phase and time-blocking approximation calculations (RQRPA and RQTBA), no monotonous increase in the total low-lying $E1$ strength was observed in the experimental data from $^{111}$Sn to $^{124}$Sn, demonstrating rather similar strength distributions in these nuclei. The Oslo GSFs and NLDs were further used as inputs to constrain the cross sections and Maxwellian-averaged cross sections of $(n,γ)$ reactions in the Sn isotopic chain using TALYS. The obtained results agree well with other available experimental data and the recommended values from the JINA REACLIB, BRUSLIB, and KADoNiS libraries. Despite relatively small exhausted fractions of the TRK sum rule, the low-lying electric dipole strength makes a noticeable impact on the radiative neutron-capture cross sections in stable Sn isotopes. Moreover, the experimental Oslo inputs for the $^{121,123}$Sn$(n,γ)$$^{122,124}$Sn reactions were found to affect the production of Sb in the astrophysical $i$-process, providing new constraints on the uncertainties of the resulting chemical abundances from multi-zone low-metallicity Asymptotic Giant Branch stellar models.

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Nuclear level densities and $γ-$ray strength functions of $^{111,112,113}$Sn isotopes studied with the Oslo method

The $^{111,112,113}$Sn isotopes have been studied with ($p,d γ$), ($p,p^{\prime} γ$), and ($d,p γ$) reactions to extract the nuclear level densities (NLDs) and $γ$-ray strength functions (GSFs) of these nuclei below the neutron separation energy by means of the Oslo method. The experimental NLDs for all three nuclei demonstrate a trend compatible with the constant-temperature model below the neutron separation energy while also being in good agreement with the NLDs of neighboring Sn isotopes, obtained previously with the Oslo-type and neutron evaporation experiments. The extracted microcanonical entropies yield $\approx 1.5$ $k_B$ entropy of a valence neutron in both $^{111}$Sn and $^{113}$Sn. Moreover, the deduced microcanonical temperatures indeed suggest a clear constant-temperature behavior above $\approx$ 3 MeV in $^{111,113}$Sn and above $\approx$ 4.5 MeV in $^{112}$Sn. We observe signatures for the first broken neutron pairs between 2 and 4 MeV in all three nuclei. The GSFs obtained with the Oslo method are found to be in good agreement below the neutron threshold with the strengths of $^{112,114}$Sn extracted in the ($p,p^{\prime}$) Coulomb excitation experiments.

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Fine structure of the isoscalar giant monopole resonance in $^{58}$Ni, $^{90}$Zr, $^{120}$Sn and $^{208}$Pb

Over the past two decades high energy-resolution inelastic proton scattering studies were used to gain an understanding of the origin of fine structure observed in the isoscalar giant quadrupole resonance (ISGQR) and the isovector giant dipole resonance (IVGDR). Recently, the isoscalar giant monopole resonance (ISGMR) in $^{58}$Ni, $^{90}$Zr, $^{120}$Sn and $^{208}$Pb was studied at the iThemba Laboratory for Accelerator Based Sciences (iThemba LABS) by means of inelastic $α$-particle scattering at very forward scattering angles (including $0\circ$). The good energy resolution of the measurement revealed significant fine structure of the ISGMR.~To extract scales by means of wavelet analysis characterizing the observed fine structure of the ISGMR in order to investigate the role of different mechanisms contributing to its decay width. Characteristic energy scales are extracted from the fine structure using continuous wavelet transforms. The experimental energy scales are compared to different theoretical approaches performed in the framework of quasiparticle random phase approximation (QRPA) and beyond-QRPA including complex configurations using both non-relativistic and relativistic density functional theory. All models highlight the role of Landau fragmentation for the damping of the ISGMR especially in the medium-mass region. Models which include the coupling between one particle-one hole (1p-1h) and two particle-two hole (2p-2h) configurations modify the strength distributions and wavelet scales indicating the importance of the spreading width. The effect becomes more pronounced with increasing mass number. Wavelet scales remain a sensitive measure of the interplay between Landau fragmentation and the spreading width in the description of the fine structure of giant resonances.

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Electric dipole polarizability of $^{40}$Ca

The electric dipole strength distribution in $^{40}$Ca between 5 and 25 MeV has been determined at RCNP, Osaka, from proton inelastic scattering experiments at very forward angles. Combined with total photoabsorption data at higher excitation energy, this enables an extraction of the electric dipole polarizability $α_\mathrm{D}$($^{40}$Ca) = 1.92(17) fm$^3$. Together with the measured $α_{\rm D}$ in $^{48}$Ca, it provides a stringent test of modern theoretical approaches, including coupled cluster calculations with chiral effective field theory interactions and state-of-the art energy density functionals. The emerging picture is that for this medium-mass region dipole polarizabilities are well described theoretically, with important constraints for the neutron skin in $^{48}$Ca and related equation of state quantities.

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Isoscalar giant monopole strength in $^{58}$Ni, $^{90}$Zr, $^{120}$Sn and $^{208}$Pb

Inelastic $α$-particle scattering at energies of a few hundred MeV and very-forward scattering angles including $0^\circ$ has been established as a tool for the study of the isoscalar giant monopole (IS0) strength distributions in nuclei. An independent investigation of the IS0 strength in nuclei across a wide mass range was performed using the $0^\circ$ facility at iThemba Laboratory for Accelerator Based Sciences (iThemba LABS), South Africa, to understand differences observed between IS0 strength distributions in previous experiments performed at the Texas A\&M University (TAMU) Cyclotron Institute, USA and the Research Center for Nuclear Physics (RCNP), Japan. The isoscalar giant monopole resonance (ISGMR) was excited in $^{58}$Ni, $^{90}$Zr, $^{120}$Sn and $^{208}$Pb using $α$-particle inelastic scattering with $196$ MeV $α$ beam and scattering angles $θ_{\text{Lab}} = 0^\circ$ and $4^\circ$. The K$600$ magnetic spectrometer at iThemba LABS was used to detect and momentum analyze the inelastically scattered $α$ particles. The IS0 strength distributions in the nuclei studied were deduced with the difference-of-spectra (DoS) technique including a correction factor for the $4^\circ$ data based on the decomposition of $L > 0$ cross sections in previous experiments. IS0 strength distributions for $^{58}$Ni, $^{90}$Zr, $^{120}$Sn and $^{208}$Pb are extracted in the excitation-energy region $E_{\rm x} = 9 - 25$ MeV.Using correction factors extracted from the RCNP experiments, there is a fair agreement with their published IS0 results. Good agreement for IS0 strength in $^{58}$Ni is also obtained with correction factors deduced from the TAMU results, while marked differences are found for $^{90}$Zr and $^{208}$Pb.

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Nuclear level densities and $γ$-ray strength functions in $^{120,124}$Sn isotopes: impact of Porter-Thomas fluctuations

Nuclear level densities (NLDs) and $γ$-ray strength functions (GSFs) of $^{120,124}$Sn have been extracted with the Oslo method from proton-$γ$ coincidences in the ($p,p^{\prime}γ)$ reaction. The functional forms of the GSFs and NLDs have been further constrained with the Shape method by studying primary $γ$-transitions to the ground and first excited states.The NLDs demonstrate good agreement with the NLDs of $^{116,118,122}$Sn isotopes measured previously. Moreover, the extracted partial NLD of 1$^{-}$ levels in $^{124}$Sn is shown to be in fair agreement with those deduced from spectra of relativistic Coulomb excitation in forward-angle inelastic proton scattering. The experimental NLDs have been applied to estimate the magnitude of the Porter-Thomas (PT) fluctuations. Within the PT fluctuations, we conclude that the GSFs for both isotopes can be considered to be independent of initial and final excitation energies, in accordance with the generalized Brink-Axel hypothesis. Particularly large fluctuations observed in the Shape-method GSFs present a considerable contribution to the uncertainty of the method, and may be one of the reasons for deviations from the Oslo-method strength at low $γ$-ray energies and low values of the NLD (below $\approx1\cdot10^{3}-2\cdot10^{3}$ MeV$^{-1}$).

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PANDORA project: photo-nuclear reactions below $A=60$

Photo-nuclear reactions of light nuclei below a mass of $A=60$ are studied experimentally and theoretically by the PANDORA (Photo-Absorption of Nuclei and Decay Observation for Reactions in Astrophysics) project. Two experimental methods, virtual-photon excitation by proton scattering and real-photo absorption by a high-brilliance gamma-ray beam produced by laser Compton scattering, will be applied to measure the photo-absorption cross sections and the decay branching ratio of each decay channel as a function of the photon energy. Several nuclear models, e.g. anti-symmetrized molecular dynamics, mean-field type models, a large-scale shell model, and ab initio models, will be employed to predict the photo-nuclear reactions. The uncertainty in the model predictions will be evaluated from the discrepancies between the model predictions and the experimental data. The data and the predictions will be implemented in a general reaction calculation code TALYS . The results will be applied to the simulation of the photo-disintegration process of ultra-high-energy cosmic rays in inter-galactic propagation.

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