arXiv subjects
Publications and source records attributed to Paolo Longo.
We investigate the coupled-system dynamics of two-level quantum dots placed on a vibrating nanomechanical resonator. The ensemble of quantum dots exhibits superradiance features which are transferred to the mechanical degrees of freedom representing fast quantum dynamics and enhanced phonon emission in a nanomechanical setup, resembling of the superradiance effect.
Epitaxial strain, layer confinement and inversion symmetry breaking have emerged as powerful new approaches to control the electronic and atomic-scale structural properties in complex metal oxides. Nickelate heterostructures, based on RENiO$_3$, where RE is a trivalent rare-earth cation, have been shown to be relevant model systems since the orbital occupancy, degeneracy, and, consequently, the electronic/magnetic properties can be altered as a function of epitaxial strain, layer thickness and superlattice structure. One such recent example is the tri-component LaTiO$_3$-LaNiO$_3$-LaAlO$_3$ superlattice, which exhibits charge transfer and orbital polarization as the result of its interfacial dipole electric field. A crucial step towards control of these parameters for future electronic and magnetic device applications is to develop an understanding of both the magnitude and range of the octahedral network's response towards interfacial strain and electric fields. An approach that provides atomic-scale resolution and sensitivity towards the local octahedral distortions and orbital occupancy is therefore required. Here, we employ atomic-resolution imaging coupled with electron spectroscopies and first principles theory to examine the role of interfacial charge transfer and symmetry breaking in a tricomponent nickelate superlattice system. We find that nearly complete charge transfer occurs between the LaTiO$_3$ and LaNiO$_3$ layers, resulting in a Ni$^{2+}$ valence state. We further demonstrate that this charge transfer is highly localized with a range of about 1 unit cell, within the LaNiO$_3$ layers. The results presented here provide important feedback to synthesis efforts aimed at stabilizing new electronic phases that are not accessible by conventional bulk or epitaxial film approaches.
Cooperative phenomena arising due to the coupling of individual atoms via the radiation field are a cornerstone of modern quantum and optical physics. Recent experiments on x-ray quantum optics added a new twist to this line of research by exploiting superradiance in order to construct artificial quantum systems. However, so far, systematic approaches to deliberately design superradiance properties are lacking, impeding the desired implementation of more advanced quantum optical schemes. Here, we develop an analytical framework for the engineering of single-photon superradiance in extended media applicable across the entire electromagnetic spectrum, and show how it can be used to tailor the properties of an artificial quantum system. This "reverse engineering" of superradiance not only provides an avenue towards non-linear and quantum mechanical phenomena at x-ray energies, but also leads to a unified view on and a better understanding of superradiance across different physical systems.
The collective emission from a one-dimensional chain of interacting two-level atoms is investigated. We calculate the light scattered by dissipative few-excitation eigenstates in the far-field, and in particular focus on signatures of a lattice two-body bound state. We present analytical results for the angle-resolved, temporal decay of the scattered light intensity. Moreover, we find that the steady-state emission spectrum that emerges when the system is probed by a weak, incoherent driving field exhibits a distinct signature for the existence of a bound state, and allows to determine the momentum distribution of the two-body relative wavefunction. Intriguingly, our study does not rely on single-atom addressability and/or manipulation techniques.
We present a detailed analysis of the dynamics of photon transport in waveguiding systems in the presence of a two-level system. In these systems, quantum interference effects generate a strong effective optical nonlinearity on the few-photon level. We clarify the relevant physical mechanisms through an appropriate quantum many-body approach. Based on this, we demonstrate that a single-particle photon-atom bound state with an energy outside the band can be excited via multi-particle scattering processes. We further show that these trapping effects are robust and, therefore, will be useful for the control of photon entanglement in solid-state based quantum optical systems.