arXiv subjects

Pardis Sahafi

Publications and source records attributed to Pardis Sahafi.

6 recordsLinked to original sources

arXiv2026

Long-Lived Mechanically-Detected Molecular Spins for Quantum Sensing

Quantum sensors based on individual spins provide unprecedented access to local magnetic fields in condensed matter, chemistry, and biology, with solid-state defect spins emerging as the leading platform. However, their molecular-sensing capabilities are limited by confinement to a host lattice, which prevents placement in close proximity to a target molecule. Molecular spins offer an alternative, enabling chemical tunability and flexible positioning relative to the target system. Here we present a nanoscale sensing platform that combines molecular electron spins, ultrasensitive mechanical readout, and Hamiltonian engineering. Using a modified XYXY dipolar decoupling sequence, we suppress electron-electron dipolar interactions across a broad distribution of control fields, extending coherence times to $\sim 400~\mu$s in an attoliter-scale droplet containing $\sim$100 trityl-OX063 radicals. Leveraging this sequence, we demonstrate frequency-selective detection of nanotesla-scale AC fields and perform sensing and spectroscopy of small, local nuclear-spin ensembles. Collectively, these results establish SQUINT (Spin-based QUantum Integrated Nanomechanical Transduction) as a framework for quantum sensing that affords molecular-level control over sensor properties and enables direct integration into complex molecular targets.

quant-ph↗

arXiv2024

Magnetically-controlled Vortex Dynamics in a Ferromagnetic Superconductor

Ferromagnetic superconductors are exceptionally rare because the strong ferromagnetic exchange field usually destroys singlet superconductivity. EuFe$_2$(As$_{1-x}$P$_x$)$_2$, an iron-based superconductor with a maximum critical temperature of 25 K, uniquely exhibits full coexistence with ferromagnetic order below $T_\mathrm{FM}$ $\simeq$ $19$ K. The interplay leads to narrowing of ferromagnetic domains at higher temperatures and spontaneous nucleation of vortices/antivortices at lower temperatures. Here we demonstrate how the underlying magnetic structure controls the superconducting vortex dynamics in applied magnetic fields. Just below $T_\mathrm{FM}$ we observe a pronounced peak in the creep activation energy, and magnetic force microscopy measurements reveal the presence of very closely-spaced ($w\ll \lambda$) vortex clusters. We attribute these observations to the formation of vortex polarons for which we present a theoretical description. In contrast, we link strong magnetic irreversibility at low temperatures to a critical current governed by giant flux creep over an activation barrier for vortex-antivortex annihilation near domain walls. Our work suggests new routes for the magnetic enhancement of vortex pinning with important applications in high-current conductors.

cond-mat.supr-con↗

arXiv2024

Large-Enhancement Nanoscale Dynamic Nuclear Polarization Near a Silicon Nanowire Surface

Dynamic nuclear polarization (DNP) has revolutionized the field of NMR spectroscopy, expanding its reach and capabilities to investigate diverse materials, biomolecules, and complex dynamic processes. Bringing high-efficiency DNP to the nanometer scale would open new avenues for studying nanoscale nuclear spin ensembles, such as single biomolecules, virus particles, and condensed matter systems. Combining pulsed DNP with nanoscale force-detected magnetic resonance measurements, we demonstrated a 100-fold enhancement in the Boltzmann polarization of proton spins in nanoscale sugar droplets at 6 K and 0.33 T. Crucially, this enhancement corresponds to a factor of 200 reduction in the averaging time compared to measurements that rely on the detection of statistical fluctuations in nanoscale nuclear spin ensembles. These results significantly advance the capabilities of force-detected magnetic resonance detection as a practical tool for nanoscale imaging.

cond-mat.mes-hall↗

arXiv2022

Nanometer-Scale Nuclear Magnetic Resonance Diffraction with Sub-\AA ngstrom Precision

Achieving atomic resolution is the ultimate limit of magnetic resonance imaging (MRI), and attaining this capability offers enormous technological and scientific opportunities, from drug development to understanding the dynamics in interacting quantum systems. In this work, we present a new approach to nanoMRI utilizing nuclear magnetic resonance diffraction (NMRd) -- a method that extends NMR imaging to probe the structure of periodic spin systems. The realization of NMRd on the atomic scale would create a powerful new methodology for materials characterization utilizing the spectroscopic capabilities of NMR. We describe two experiments that realize NMRd measurement of $^{31}$P spins in an indium-phosphide (InP) nanowire with sub-\r{A}ngstrom precision. In the first experiment, we encode a nanometer-scale spatial modulation of the $z$-axis magnetization by periodically inverting the $^{31}$P spins, and detect the period and position of the modulation with a precision of $<0.8$ \r{A}. In the second experiment, we demonstrate an interferometric technique, utilizing NMRd, for detecting an \r{A}ngstrom-scale displacement of the InP sample with a precision of 0.07 \r{A}. The diffraction-based techniques developed in this work represent new measurement modalities in NMR for probing the structure and dynamics of spins on sub-\r{A}ngstrom length scales, and demonstrate the feasibility of crystallographic MRI measurements.

cond-mat.mes-hall↗

arXiv2020

Numerical Engineering of Robust Adiabatic Operations

Adiabatic operations are powerful tools for robust quantum control in numerous fields of physics, chemistry and quantum information science. The inherent robustness due to adiabaticity can, however, be impaired in applications requiring short evolution times. We present a single versatile gradient-based optimization protocol that combines adiabatic control with effective Hamiltonian engineering in order to design adiabatic operations tailored to the specific imperfections and resources of an experimental setup. The practicality of the protocol is demonstrated by engineering a fast, 2.3 Rabi cycle-long adiabatic inversion pulse for magnetic resonance with built-in robustness to Rabi field inhomogeneities and resonance offsets. The performance and robustness of the pulse is validated in a nanoscale force-detected magnetic resonance experiment on a solid-state sample, indicating an ensemble-averaged inversion accuracy of $\sim 99.997\%$. We further showcase the utility of our protocol by providing examples of adiabatic pulses robust to spin-spin interactions, parameter-selective operations and operations connecting arbitrary states, each motivated by experiments.

quant-ph↗

arXiv2019

Ultra-low dissipation patterned silicon nanowire arrays for scanning probe microscopy

In recent years, self-assembled semiconductor nanowires have been successfully used as ultra-sensitive cantilevers in a number of unique scanning probe microscopy (SPM) settings. We describe the fabrication of ultra-low dissipation patterned silicon nanowire (SiNW) arrays optimized for scanning probe applications. Our fabrication process produces, with high yield, ultra-high aspect ratio vertical SiNWs that exhibit exceptional force sensitivity. The highest sensitivity SiNWs have thermomechanical-noise limited force sensitivity of $9.7\pm0.4~\text{aN}/\sqrt{\text{Hz}}$ at room temperature and $500\pm20~\text{zN}/\sqrt{\text{Hz}}$ at 4 K. To facilitate their use in SPM, the SiNWs are patterned within $7~\mu\text{m}$ from the edge of the substrate, allowing convenient optical access for displacement detection.

physics.app-ph↗