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Partha P. Mukherjee

Publications and source records attributed to Partha P. Mukherjee.

4 recordsLinked to original sources

Ultra-broadband Mid to Long-wave Infrared Spintronic Poisson Bolometer

Infrared detectors have traditionally been divided into two fundamental classes, mid-wave (MWIR, 3-5 um) and long-wave (LWIR, 8-14 um). Integrating MWIR and LWIR within a single device is challenging due to distinct materials, cooling needs, and detection mechanisms, while such integration is critical for improved object recognition, temperature estimation, and environmental sensing. In this work, we demonstrate a Spintronic Poisson (SP) bolometer enabling room-temperature ultra-broadband sensing across 3-14 um. Unlike conventional bolometers that rely on continuous analog signals, the SP bolometer implements a Poisson-counting detection paradigm, encoding temperature in discrete stochastic events, which turns thermal noise from a limitation into the basis of the estimator itself. We fabricate the SP bolometer using a spintronic transduction layer integrated with a plasmonic nanoantenna array to enhance broadband infrared absorption. Using spintronic transduction, the device achieves the noise-equivalent temperature difference (NETD, thermal sensitivity metric) of 80-100 mK at 300 K, surpassing uncooled detectors and approaching cooled technologies. This work establishes a statistical detection paradigm for room-temperature infrared sensing with broad application potential.

physics.optics

Quantifying the unknown impact of segmentation uncertainty on image-based simulations

Image-based simulation, the use of 3D images to calculate physical quantities, fundamentally relies on image segmentation to create the computational geometry. However, this process introduces image segmentation uncertainty because there is a variety of different segmentation tools (both manual and machine-learning-based) that will each produce a unique and valid segmentation. First, we demonstrate that these variations propagate into the physics simulations, compromising the resulting physics quantities. Second, we propose a general framework for rapidly quantifying segmentation uncertainty. Through the creation and sampling of segmentation uncertainty probability maps, we systematically and objectively create uncertainty distributions of the physics quantities. We show that physics quantity uncertainty distributions can follow a Normal distribution, but, in more complicated physics simulations, the resulting uncertainty distribution can be both nonintuitive and surprisingly nontrivial. We also establish that simply bounding the uncertainty can fail in situations that are sensitive to image segmentation. While our work does not eliminate segmentation uncertainty, it makes visible the previously unrecognized range of uncertainty currently plaguing image-based simulation, enabling more credible simulations.

cs.CE

Modulating nano-inhomogeneity at electrode-solid electrolyte interfaces for dendrite-proof solid-state batteries and long-life memristors

The penetration of dendrites in ceramic lithium conductors severely constrains the development of solid-state batteries (SSBs) while its nanoscopic origin remain unelucidated. We develop an in-situ nanoscale electrochemical characterization technique to reveal the nanoscopic lithium dendrite growth kinetics and use it as a guiding tool to unlock the design of interfaces for dendrite-proof SSBs. Using Li7La3Zr2O12 (LLZO) as a model system, in-situ nanoscopic dendrite triggering measurements, ex-situ electro-mechanical characterizations, and finite element simulations are carried out which reveal the dominating role of Li+ flux detouring and nano-mechanical inhomogeneity on dendrite penetration. To mitigate such nano-inhomogeneity, an ionic-conductive homogenizing layer based on poly(propylene carbonate) is designed which in-situ reacts with lithium to form a highly conformal interphase at mild conditions. A high critical current density of 1.8mA cm-2 and a low interfacial resistance of 14Ω cm2 is achieved. Practical SSBs based on LiFePO4 cathodes show great cyclic stability without capacity decay over 300 cycles. Beyond this, highly reversible electrochemical dendrite healing behavior in LLZO is discovered using the nano-electrode, based on which a model memristor with a high on/off ratio of ~10^5 is demonstrated for >200 cycles. This work not only provides a novel tool to investigate and design interfaces in SSBs but offers also new opportunities for solid electrolytes beyond energy applications.

physics.app-ph

Mesoscale Elucidation of Biofilm Shear Behavior

Formation of bacterial colonies as biofilm on the surface/interface of various objects has the potential to impact not only human health and disease but also energy and environmental considerations. Biofilms can be regarded as soft materials, and comprehension of their shear response to external forces is a key element to the fundamental understanding. A mesoscale model has been presented in this article based on digitization of a biofilm microstructure. Its response under externally applied shear load is analyzed. Strain stiffening type behavior is readily observed under high strain loads due to the unfolding of chains within soft polymeric substrate. Sustained shear loading of the biofilm network results in strain localization along the diagonal direction. Rupture of the soft polymeric matrix can potentially reduce the intercellular interaction between the bacterial cells. Evolution of stiffness within the biofilm network under shear reveals two regions: a) initial increase in stiffness due to strain stiffening of polymer matrix, and b) eventual reduction in stiffness because of tear in polymeric substrate.

physics.flu-dyn