arXiv subjects

Pascale Senellart

Publications and source records attributed to Pascale Senellart.

At least 19 recordsLinked to original sources

arXiv2026

Spin-to-polarization mapping with a coherent quantum dot-cavity receiver

Coherent light-matter interfaces controllably modifying the state of a photon upon interaction with a stationary qubit are a key resource for implementing deterministic entangling gates for optical quantum technologies. This requires a one-to-one mapping between the state of the scattered photon and that of the embedded qubit. Here, we present an experimental signature of such a bijection by leveraging the spin-induced Kerr rotation present in a low-noise charged quantum dot-micropillar cavity device. Through time-resolved polarization measurements, we project the electron spin to one of its eigenstates with $95\pm2\%$ fidelity with a single reflected photon detection, and follow the subsequent spin relaxation through the detection of a second reflected photon. We demonstrate that, after a transient regime governed by the trion radiative lifetime, two orthogonal polarization states can be produced, each associated to a given spin eigenstate. While the current results are limited by a timescale competition between electron spin relaxation and trion radiative lifetime, they could be improved using hole spins displaying increased relaxation times. Our work paves the way towards deterministic logic gates exploiting this one-to-one mapping between a spin and the polarization of a scattered photon.

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arXiv2026

Industry-ready spin-photon interfaces for hybrid photonic quantum computing

Hybrid photonic quantum computers, combining stationary matter qubits and flying photonic qubits, offer an intrinsically networked and resource-efficient route to large-scale, error-corrected quantum computation. Their core components are cavity-coupled matter qubits that act as light--matter interfaces, enabling: high-efficiency on-demand single-photon generation, stable near-unity photon indistinguishability and spin--multi-photon entanglement. Semiconductor quantum dots in microcavities are a leading platform for realizing such devices. Yet reaching the performance, reproducibility and spin-coherence thresholds for large-scale error correction remains a major challenge requiring industrial fabrication and control. Here we report thousands of monolithic semiconductor quantum-dot devices fabricated using a III--V pilot production-line process compatible with large-scale deployment. Systematic control of source parameters yields state-of-the-art efficiency and supports a path to optical losses below fault-tolerance thresholds. Using field-quadrature state reconstruction as a stringent joint test of efficiency and indistinguishability, we observe near-unity photon quantum purity stable over tens of minutes and a record single-photon Wigner-function negativity. We further demonstrate seven-partite spin--multi-photon entanglement and spin coherence extendable to microsecond timescales in the low-magnetic-field regime. Finally, photons from distant sources are as indistinguishable as photons emitted successively by a single source. These results establish foundry-compatible III--V quantum dots as a scalable platform for hybrid photonic quantum computing.

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arXiv2026

Near-identical photons from distant quantum dot-cavity devices

Scalable optical quantum technologies require interference between large numbers of indistinguishable single-photons emitted by independent sources. Semiconductor quantum dots are known to be excellent on-demand sources of single-photons. They show record efficiency when inserted into optical cavities to control their spontaneous emission and generate trains of near identical photons over microsecond timescales. However, generating perfectly identical photons from distant cavity-based sources has remained a long-standing challenge. It requires precise matching of the emission wavelengths and emission dynamics, while simultaneously minimizing spectral noise across all time scales for distant emitters in uncorrelated environments. Here, we report on the nanofabrication of a large number of quantum dot-cavity sources with ultra-low spectral noise and wavelength dispersion. The high source efficiency and the use of two tuning mechanisms enable precise optimization of the spectral overlap between distant sources. With this approach, we demonstrate a two-photon indistinguishability of $88\pm1$ % between photons emitted from two distant sources. Remarkably, this value reaches the upper bound set by the intrinsic indistinguishability of photons emitted successively by each source. These results represent a key milestone for scaling photon-based quantum technologies.

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arXiv2026

An Energetic Constraint for Qubit-Qubit Entanglement

We analyze qubit-qubit entanglement from an energetic perspective and reveal an energetic trade-off between quantum coherence and entanglement. We decompose each qubit internal energy into a coherent and an incoherent component. The qubits' coherent energies are maximal if the qubit-qubit state is pure and separable. They decrease as qubit-qubit entanglement builds up under locally-energy-preserving processes. This yields a ``coherent energy deficit'' that we show is proportional to a well-known measure of entanglement, the square concurrence. In general, a qubit-qubit state can always be represented as a mixture of pure states. Then, the coherent energy deficit splits into a quantum component, corresponding to the average square concurrence of the pure states, and a classical one reflecting the mixedness of the joint state. Minimizing the quantum deficit over the possible pure state decompositions yields the square concurrence of the mixture. Our findings bring out new figures of merit to optimize and secure entanglement generation and distribution under energetic constraints.

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arXiv2025

Benchmarking quantum key distribution by mixing single photons and laser light

Quantum key distribution is a key application of quantum mechanics, shaping the future of privacy and secure communications. Many protocols require single photons, often approximated by strongly attenuated laser pulses. Here, we harness the emission of a quantum dot embedded in a micropillar and explore a hybrid approach where the information is encoded on a mixture of single photons and laser pulses. We derive a phenomenological analysis of the configuration where both sources of light are mixed incoherently to perform the BB84 protocol, showing nearly perfect matching between theory and experiment. This provides a flexible technology compensating limited collected brightnesses of single-photon sources as well as a thorough investigation of single-photon statistics advantage scenarios over Poisson-distributed statistics. Explicitly, our model highlights an efficiency threshold for unconditional advantage of single photons over laser along with insights on the interplay between single-photon purity and collected brightness in the performances of BB84.

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arXiv2025

Measurement-induced back-action in a QD-based coherent spin-photon interface

Polarization-encoded spin-photon interfaces constitute promising candidates for the development of stationary nodes used as photon receivers, for quantum communication and distributed quantum computing. Here we introduce a time-resolved tomography approach which allows observing the dynamics of an electron spin, in a semiconductor quantum dot, mapped onto the dynamics of the polarization state of reflected photons. Through a single tomography experiment, we infer all the relevant spin dynamics timescales, including precession, decoherence and relaxation times. We also demonstrate and quantify the measurement back-action induced, on the embedded spin qubit, by the detection of a single reflected photon. We show that the induced population and coherence of the spin state can be tuned by the chosen polarization basis of the measurement. The control of the photon-induced back-action on the embedded spin qubit constitutes a crucial requirement for the use of spin-photon interfaces as quantum receivers.

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arXiv2025

Monitoring the generation of photonic linear cluster states with partial measurements

Quantum states of light with many entangled photons are key resources for photonic quantum computing and quantum communication. In this work, we exploit a highly resource-efficient generation scheme based on a linear optical circuit embedding a fibered delay loop acting as a quantum memory. The single photons are generated with a bright single-photon source based on a semiconductor quantum dot, allowing to perform the entangling scheme up to 6 photons. We demonstrate $2$, $3$, $4$ and $6$-photon entanglement generation at respective rates of $6$kHz, $120$Hz, $2.2$Hz, and $2$mHz, corresponding to an average scaling ratio of $46$. We introduce a method for real-time control of entanglement generation based on partially post-selected measurements. The visibility of such measurements carries faithful information to monitor the entanglement process, an important feature for the practical implementation of photonic measurement-based quantum computation.

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arXiv2025

Optimizing the quantum interference between single photons and local oscillator with photon correlations

The quantum interference between a coherent state and a single photon is an important tool in continuous variable optical quantum technologies to characterize and engineer non-Gaussian quantum states. Semiconductor quantum dots, which have recently emerged as a key platform for efficient single-photon generation, could become interesting assets in this context. An essential parameter for interfering single photons and classical fields is the mean wavepacket overlap between both fields. Here, we report on two homodyne photon-correlation techniques enabling the precise measurement of the overlap between a single photon generated by a quantum dot-cavity device and pulsed laser light. The different statistics of interfering fields lead to specific signatures of the quantum interference on the photon correlations at the output of the interfering beam splitter. We compare the behavior of maximized overlap, measuring either the Hong-Ou-Mandel visibility between both outputs or the photon bunching at a single output. Through careful tailoring of the laser light in various degrees of freedom, we maximize the overlap to $76\,\%$, with limitations primarily due to mismatched spectral and temporal profiles and low-frequency charge noise in the single-photon source.

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arXiv2025

Optical and magnetic response by design in GaAs quantum dots

Quantum networking technologies use spin qubits and their interface to single photons as core components of a network node. This necessitates the ability to co-design the magnetic- and optical-dipole response of a quantum system. These properties are notoriously difficult to design in many solid-state systems, where spin-orbit coupling and the crystalline environment for each qubit create inhomogeneity of electronic g-factors and optically active states. Here, we show that GaAs quantum dots (QDs) obtained via the quasi-strain-free local droplet etching epitaxy growth method provide spin and optical properties predictable from assuming the highest possible QD symmetry. Our measurements of electron and hole g-tensors and of transition dipole moment orientations for charged excitons agree with our predictions from a multiband k.p simulation constrained only by a single atomic-force-microscopy reconstruction of QD morphology. This agreement is verified across multiple wavelength-specific growth runs at different facilities within the range of 730 nm to 790 nm for the exciton emission. Remarkably, our measurements and simulations track the in-plane electron g-factors through a zero-crossing from -0.1 to 0.3 and linear optical dipole moment orientations fully determined by an external magnetic field. The robustness of our results demonstrates the capability to design - prior to growth - the properties of a spin qubit and its tunable optical interface best adapted to a target magnetic and photonic environment with direct application for high-quality spin-photon entanglement.

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arXiv2024

Indistinguishability of remote quantum dot-cavity single-photon sources

Generating identical photons from remote emitter-based bright single-photon sources is an important step for scaling up optical quantum technologies. Here, we study the Hong-Ou-Mandel interference of photons emitted from remote sources based on semiconductor quantum dots. We make use of a deterministic fabrication technique to position the quantum dots in a spectrally resonant micropillar cavity and fine tune their operation wavelength electrically. Doing so, we can match four pairs of sources between five distinct sources, study them under various excitation schemes and measure their degree of indistinguishability. We demonstrate remote indistinguishabiltiy between 44$\pm$1% and 69$\pm$1% depending on the pair of sources and excitation conditions, record values for quantum dots in cavities. The relative contribution of pure dephasing and spectral diffusion is then analysed, revealing that the remaining distinguishability is mostly due to low frequency noise

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arXiv2024

Minimizing resource overhead in fusion-based quantum computation using hybrid spin-photon devices

We present three schemes for constructing a (2,2)-Shor-encoded 6-ring photonic resource state for fusion-based quantum computing, each relying on a different type of photon source. We benchmark these architectures by analyzing their ability to achieve the loss tolerance threshold for fusion-based quantum computation using the target resource state. More precisely, we estimate their minimum hardware requirements for fault-tolerant quantum computation in terms of the number of photon sources to achieve on-demand generation of resource states with a desired generation period. Notably, we find that a group of 12 deterministic single-photon sources containing a single matter qubit degree of freedom can produce the target resource state near-deterministically by exploiting entangling gates that are repeated until success. The approach is fully modular, eliminates the need for lossy large-scale multiplexing, and reduces the overhead for resource-state generation by several orders of magnitude compared to architectures using heralded single-photon sources and probabilistic linear-optical entangling gates. Our work shows that the use of deterministic single-photon sources embedding a qubit substantially shortens the path toward fault-tolerant photonic quantum computation.

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arXiv2024

Efficient fiber-pigtailed source of indistinguishable single photons

Semiconductor quantum dots in microcavities are an excellent platform for the efficient generation of indistinguishable single photons. However, their use in a wide range of quantum technologies requires their controlled fabrication and integration in compact closed-cycle cryocoolers, with a key challenge being the efficient and stable extraction of the single photons into a single-mode fiber. Here we report on a novel method for fiber-pigtailing of deterministically fabricated single-photon sources. Our technique allows for nanometer-scale alignment accuracy between the source and a fiber, alignment that persists all the way from room temperature to 2.4 K. We demonstrate high performance of the device under near-resonant optical excitation with g$^{(2)}$(0) = 1.3 %, a photon indistinguishability of 97.5 % and a fibered brightness of 20.8 %. We show that the indistinguishability and single-photon rate are stable for over ten hours of continuous operation in a single cooldown. We further confirm that the device performance is not degraded by nine successive cooldown-warmup cycles.

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arXiv2024

Spin Noise Spectroscopy of a Single Spin using Single Detected Photons

Spin noise spectroscopy has become a widespread technique to extract information on spin dynamics in atomic and solid-state systems, in a potentially non-invasive way, through the optical probing of spin fluctuations. Here we experimentally demonstrate a new approach in spin noise spectroscopy, based on the detection of single photons. Due to the large spin-dependent polarization rotations provided by a deterministically-coupled quantum dot-micropillar device, giant spin noise signals induced by a single-hole spin are extracted in the form of photon-photon cross-correlations. Ultimately, such a technique can be extended to an ultrafast regime probing mechanisms down to few tens of picoseconds.

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arXiv2023

A general-purpose single-photon-based quantum computing platform

Quantum computing aims at exploiting quantum phenomena to efficiently perform computations that are unfeasible even for the most powerful classical supercomputers. Among the promising technological approaches, photonic quantum computing offers the advantages of low decoherence, information processing with modest cryogenic requirements, and native integration with classical and quantum networks. To date, quantum computing demonstrations with light have implemented specific tasks with specialized hardware, notably Gaussian Boson Sampling which permitted quantum computational advantage to be reached. Here we report a first user-ready general-purpose quantum computing prototype based on single photons. The device comprises a high-efficiency quantum-dot single-photon source feeding a universal linear optical network on a reconfigurable chip for which hardware errors are compensated by a machine-learned transpilation process. Our full software stack allows remote control of the device to perform computations via logic gates or direct photonic operations. For gate-based computation we benchmark one-, two- and three-qubit gates with state-of-the art fidelities of $99.6\pm0.1 \%$, $93.8\pm0.6 \%$ and $86\pm1.2 \%$ respectively. We also implement a variational quantum eigensolver, which we use to calculate the energy levels of the hydrogen molecule with high accuracy. For photon native computation, we implement a classifier algorithm using a $3$-photon-based quantum neural network and report a first $6$-photon Boson Sampling demonstration on a universal reconfigurable integrated circuit. Finally, we report on a first heralded 3-photon entanglement generation, a key milestone toward measurement-based quantum computing.

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arXiv2023

Perceval: A Software Platform for Discrete Variable Photonic Quantum Computing

We introduce Perceval, an open-source software platform for simulating and interfacing with discrete-variable photonic quantum computers, and describe its main features and components. Its Python front-end allows photonic circuits to be composed from basic photonic building blocks like photon sources, beam splitters, phase-shifters and detectors. A variety of computational back-ends are available and optimised for different use-cases. These use state-of-the-art simulation techniques covering both weak simulation, or sampling, and strong simulation. We give examples of Perceval in action by reproducing a variety of photonic experiments and simulating photonic implementations of a range of quantum algorithms, from Grover's and Shor's to examples of quantum machine learning. Perceval is intended to be a useful toolkit for experimentalists wishing to easily model, design, simulate, or optimise a discrete-variable photonic experiment, for theoreticians wishing to design algorithms and applications for discrete-variable photonic quantum computing platforms, and for application designers wishing to evaluate algorithms on available state-of-the-art photonic quantum computers.

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arXiv2022

Controlling photon polarisation with a single quantum dot spin

In the framework of optical quantum computing and communications, a major objective consists in building receiving nodes that implement conditional operations on incoming photons, using the interaction with a single stationary qubit. In particular, the quest for scalable nodes motivated the development of cavity-enhanced spin-photon interfaces with solid-state emitters. An important challenge remains, however, to produce a stable, controllable, spin-dependant photon state, in a deterministic way. Here we use a pillar-based high-Q cavity, embedding a singly-charged semiconductor quantum dot, to demonstrate the control of giant polarisation rotations induced by a single electron spin. A complete tomography approach is used to deduce the output polarisation Stokes vector, conditioned by a single spin state. We experimentally demonstrate rotation amplitudes such as $\pm \fracπ{2}$ and $π$ in the Poincaré sphere, as required for applications based on spin-polarisation mapping and spin-mediated photon-photon gates. In agreement with our modeling, we observe that the environmental noise does not limit the amplitude of the spin-induced rotation, yet slightly degrades the polarisation purity of the output states. We find that the polarisation state of the reflected photons can be manipulated in most of the Poincaré sphere, through controlled spin-induced rotations, thanks to moderate cavity birefringence and limited noise. This control allows the operation of spin-photon interfaces in various configurations, including at zero or low magnetic fields, which ensures compatibility with key protocols for photonic cluster state generation.

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arXiv2022

High-fidelity generation of four-photon GHZ states on-chip

Mutually entangled multi-photon states are at the heart of all-optical quantum technologies. While impressive progresses have been reported in the generation of such quantum light states using free space apparatus, high-fidelity high-rate on-chip entanglement generation is crucial for future scalability. In this work, we use a bright quantum-dot based single-photon source to demonstrate the high fidelity generation of 4-photon Greenberg-Horne-Zeilinger (GHZ) states with a low-loss reconfigurable glass photonic circuit. We reconstruct the density matrix of the generated states using full quantum-state tomography reaching an experimental fidelity to the target $|{\text{GHZ}_4}\rangle$ of $\mathcal{F}_{\text{GHZ}_4} (86.0\pm0.4)\,\%$, and a purity of $\mathcal{P}_{\text{GHZ}_4}=(76.3\pm0.6)\,\%$. The entanglement of the generated states is certified with a semi device-independent approach through the violation of a Bell-like inequality by more than 39 standard deviations. Finally, we carry out a four-partite quantum secret sharing protocol on-chip where a regulator shares with three interlocutors a sifted key with up to 1978 bits, achieving a qubit-error rate of $10.87\,\%$. These results establish that the quantum-dot technology combined with glass photonic circuitry for entanglement generation on chip offers a viable path for intermediate scale quantum computation and communication.

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arXiv2022

Orbital angular momentum based intra- and inter- particle entangled states generated via a quantum dot source

Engineering single-photon states endowed with Orbital Angular Momentum (OAM) is a powerful tool for quantum information photonic implementations. Indeed, thanks to its unbounded nature, OAM is suitable to encode qudits allowing a single carrier to transport a large amount of information. Nowadays, most of the experimental platforms use nonlinear crystals to generate single photons through Spontaneous Parametric Down Conversion processes, even if this kind of approach is intrinsically probabilistic leading to scalability issues for increasing number of qudits. Semiconductors Quantum Dots (QDs) have been used to get over these limitations being able to produce on demand pure and indistinguishable single-photon states, although only recently they were exploited to create OAM modes. Our work employs a bright QD single-photon source to generate a complete set of quantum states for information processing with OAM endowed photons. We first study the hybrid intra-particle entanglement between the OAM and the polarization degree of freedom of a single-photon. We certify the preparation of such a type of qudit states by means of the Hong-Ou-Mandel effect visibility which furnishes the pairwise overlap between consecutive OAM-encoded photons. Then, we investigate the hybrid inter-particle entanglement, by exploiting a probabilistic two qudit OAM-based entangling gate. The performances of our entanglement generation approach are assessed performing high dimensional quantum state tomography and violating Bell inequalities. Our results pave the way toward the use of deterministic sources (QDs) for the on demand generation of photonic quantum states in high dimensional Hilbert spaces.

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