arXiv subjects

Patrick A. Lee

Publications and source records attributed to Patrick A. Lee.

At least 55 records · Page 3Linked to original sources

arXiv2021

Superconducting-like response in driven systems near the Mott transition

We point out that fractionalized bosonic charge excitations can explain the recently discovered photo-induced superconducting-like response in $κ\text{-(ET})_2\text{Cu}[\text{N(CN)}_2]\text{Br}$, an organic metal close to the Mott transition. The pump laser exerts a periodic drive on the fractionalized field, creating a non-equilibrium condensate, which gives a Drude peak much narrower than the equilibrium scattering rate, hence superconducting-like response. Our proposal illuminates new possibilities of detecting fractionalization and can be readily tested in spin liquid candidates and in cold atom systems.

cond-mat.str-el↗

arXiv2021

Quantum Oscillation of Thermally Activated Conductivity in a Monolayer WTe$_2$-like Excitonic Insulator

Recently, quantum oscillation of the resistance in insulating monolayer WTe$_2$ was reported. An explanation in terms of gap modulation in the hybridized Landau levels of an excitonic insulator was also proposed by one of us. However, the previous picture of gap modulation in the Landau levels spectrum was built on a pair of well nested electron and hole Fermi surfaces, while the monolayer WTe$_2$ has one hole and two electron Fermi pockets with relative anisotropy. Here we demonstrate that for system like monolayer WTe$_2$, the excitonic insulating state arising from the coupled one hole and two electron pockets possesses a finite region in interaction parameter space that shows gap modulation in a magnetic field. In this region, the thermally activated conductivity displays the $1/B$ periodic oscillation and it can further develop into discrete peaks at low temperature, in agreement with the experimental observation. We show that the relative anisotropy of the bands is a key parameter and the qunatum oscillations decrease rapidly if the anisotropy increases further than the realistic value for monolayer WTe$_2$.

cond-mat.mes-hall↗

arXiv2021

Photo-induced superconducting-like response in strongly correlated systems

We propose a novel mechanism for the photo-induced superconducting-like response recently reported in cuprates and other strongly correlated materials. This mechanism relies on quantum-fluctuating bosons consisting of electron pairs. With periodic drive, the electron pairs and vacancies of pairs form a coherent non-equilibrium condensate, different from conventional superconductors, yet showing superconducting-like response in some regimes even with dissipation. Unlike the case of driven fermionic bands which results in the familiar Floquet bands with hybridization gaps, for driven bosons the "gap" opens up in the momentum direction, resulting in a resonant region in momentum space where the eigenvalues are complex. We give a simple physical argument why this picture leads to a "perfect conductor" which exhibits superconducting-like frequency-dependent conductivity but no Meissner response. While our model is quite general, in the case of cuprates, quantum-fluctuating pair density wave in the pseudogap region may serve as the origin of the quantum-fluctuating electron pairs.

cond-mat.str-el↗

arXiv2021

Competition of Spinon Fermi Surface and Heavy Fermi Liquids states from the Periodic Anderson to the Hubbard model

We study a model of correlated electrons coupled by tunnelling to a layer of itinerant metallic electrons, which allows to interpolate from a frustrated limit favorable to spin liquid states to a Kondo-lattice limit favorable to interlayer coherent heavy metallic states. We study the competition of the spinon fermi surface state and the interlayer coherent heavy Kondo metal that appears with increasing tunnelling. Employing a slave rotor mean-field approach, we obtain a phase diagram and describe two regimes where the spin liquid state is destroyed by weak interlayer tunnelling, (i) the Kondo limit in which the correlated electrons can be viewed as localized spin moments and (ii) near the Mott metal-insulator-transition where the spinon Fermi surface transitions continuously into a Fermi liquid. We study the shape of LDOS spectra of the putative spin liquid layer in the heavy Fermi liquid phase and describe the temperature dependence of its width arising from quasiparticle interactions and disorder effects throughout this phase diagram, in an effort to understand recent STM experiments of the candidate spin liquid 1T-TaSe$_2$ residing on metallic 1H-TaSe$_2$. Comparison of the shape and temperature dependence of the theoretical and experimental LDOS suggest that this system is either close to the localized Kondo limit, or in an intermediate coupling regime where the Kondo coupling and the Heisenberg exchange interaction are comparable.

cond-mat.str-el↗

arXiv2020

Low temperature $T$-linear resistivity due to umklapp scattering from a critical mode

We consider the transport properties of a model of fermions scattered by a critical bosonic mode. The mode is overdamped and scattering is mainly in the forward direction. Such a mode appears at the quantum critical point for a electronic nematic phase transition, and in gauge theories for a U(1) spin liquid. It leads to a short fermion life-time, violating Landau's criterion for a Fermi liquid. In spite of this, transport can be described by a Boltzmann equation. We include momentum relaxation by umklapp scattering, supplemented by weak impurity scattering. We find that above a very low temperature which scales with $Δ_q^3$, where $Δ_q$ is the minimum umklapp scattering vector, the resistivity is linear in $T$ with a coefficient which is independent of the amount of disorder. We compare the relaxation time approximation with an exact numerical solution of the Boltzmann equation. Surprisingly we find that unlike the resistivity, the Hall Coefficient strongly deviates from the relaxation time approximation and shows a strong reduction with increasing temperature. We comment on possible comparisons with experiments on high $T_c$ Cuprates.

cond-mat.str-el↗

arXiv2020

Quantum oscillations in the activated conductivity in excitonic insulators: possible application to monolayer WTe2

A recent paper on the insulating state of monolayer WTe2 reported the observation of large oscillations in the conductivity that are periodic in 1/B, resembling quantum oscillations in metals. This remarkable observation has inspired suggestions of exotic physics such as spin-charge separation. We show that a rather more conventional but still nontrivial explanation in terms of gap modulation may be possible in a model of excitonic insulator subject to a magnetic field.

cond-mat.str-el↗

arXiv2020

Dynamic fingerprint of fractionalized excitations in single-crystalline Cu$_3$Zn(OH)$_6$FBr

Quantum spin liquid (QSL) represents a new class of condensed matter states characterized by the long-range many-body entanglement of topological orders. The most prominent feature of the elusive QSL state is the existence of fractionalized spin excitations. Subject to the strong quantum fluctuations, the spin-1/2 antiferromagnetic system on a kagome lattice is the promising candidate for hosting a QSL ground state, but the structurally ideal realization is rare. Here, we report Raman scattering on the single crystalline Cu$_3$Zn(OH)$_6$FBr, and confirm that the ideal kagome structure remains down to low temperatures without any lattice distortion by the angle-resolved polarized Raman responses and second-harmonic-generation measurements. Furthermore, at low temperatures the Raman scattering reveals a continuum of the spin excitations in Cu$_3$Zn(OH)$_6$FBr, in contrast to the sharp magnon peak in the ordered kagome antiferromagnet EuCu$_3$(OH)$_6$Cl$_3$. Such magnetic Raman continuum, in particular, the substantial low-energy one-pair spinon excitation serves as strong evidence for fractionalized spin excitations in Cu$_3$Zn(OH)$_6$FBr.

cond-mat.str-el↗

arXiv2020

A continuous metal-insulator transition driven by spin correlations

Metal-insulator transitions involve a mix of charge, spin, and structural degrees of freedom, and when strongly-correlated, can underlay the emergence of exotic quantum states. Mott insulators induced by the opening of a Coulomb gap are an important and well-recognized class of transitions, but insulators purely driven by spin correlations are much less common, as the reduced energy scale often invites competition from other degrees of freedom. Here we demonstrate a clean example of a spin-correlation-driven metal-insulator transition in the all-in-all-out pyrochlore antiferromagnet Cd2Os2O7, where the lattice symmetry is fully preserved by the antiferromagnetism. After the antisymmetric linear magnetoresistance from conductive, ferromagnetic domain walls is carefully removed experimentally, the Hall coefficient of the bulk reveals four Fermi surfaces, two of electron type and two of hole type, sequentially departing the Fermi level with decreasing temperature below the Néel temperature, T_N. Contrary to the common belief of concurrent magnetic and metal-insulator transitions in Cd2Os2O7, the charge gap of a continuous metal-insulator transition opens only at T~10K, well below T_N=227K. The insulating mechanism resolved by the Hall coefficient parallels the Slater picture, but without a folded Brillouin zone, and contrasts sharply with the behavior of Mott insulators and spin density waves, where the electronic gap opens above and at T_N, respectively.

cond-mat.str-el↗

arXiv2020

Imaging spinon density modulations in a 2D quantum spin liquid

Two-dimensional triangular-lattice antiferromagnets are predicted under some conditions to exhibit a quantum spin liquid ground state whose low-energy behavior is described by a spinon Fermi surface. Directly imaging the resulting spinons, however, is difficult due to their fractional, chargeless nature. Here we use scanning tunneling spectroscopy to image spinon density modulations arising from a spinon Fermi surface instability in single-layer 1T-TaSe$_2$, a two-dimensional Mott insulator. We first demonstrate the existence of localized spins arranged on a triangular lattice in single-layer 1T-TaSe$_2$ by contacting it to a metallic 1H-TaSe$_2$ layer and measuring the Kondo effect. Subsequent spectroscopic imaging of isolated, single-layer 1T-TaSe$_2$ reveals long-wavelength modulations at Hubbard band energies that reflect spinon density modulations. This allows direct experimental measurement of the spinon Fermi wavevector, in good agreement with theoretical predictions for a 2D quantum spin liquid. These results establish single-layer 1T-TaSe$_2$ as a new platform for studying novel two-dimensional quantum-spin-liquid phenomena.

cond-mat.str-el↗

arXiv2019

The Physics of Pair Density Waves

We review the physics of pair density wave (PDW) superconductors. We begin with a macroscopic description that emphasizes order induced by PDW states, such as charge density wave, and discuss related vestigial states that emerge as a consequence of partial meting of the PDW order. We review and critically discuss the mounting experimental evidence for such PDW order in the cuprate superconductors, the status of the theoretical microscopic description of such order, and the current debate on whether the PDW is a "mother order" or another competing order in the cuprates. In addition, we give an overview of the weak coupling version of PDW order, Fulde-Ferrell-Larkin-Ovchinnikov states, in the context of cold atom systems, unconventional superconductors, and non-centrosymmetric and Weyl materials.

cond-mat.supr-con↗

arXiv2019

Modeling the pseudogap metallic state in cuprates: quantum disordered pair density wave

We present a way to quantum-disorder a pair density wave, and propose it to be a candidate of the effective low-energy description of the pseudogap metal which may reveal itself in a sufficiently high magnetic field that suppresses the d-wave pairing. The ground state we construct is a small-pocket Fermi liquid with a bosonic Mott insulator in the density-wave-enlarged unit cell. At low energy, the charge density is mainly carried by charge 2e bosons, which develop a small insulating gap. As an intermediate step, we discuss the quantum disordering of a fully gapped superconductor and its excitation spectrum. In order to illustrate the concepts we introduce, we introduce a simplified 1D model which we solve numerically. We discuss a number of experimental consequences. The interplay between the electron and the small-gap boson results in a step function background in the electron spectral function which may be consistent with existing ARPES data. Optical excitation across the boson gap can explain the onset and the magnitude of the mid-infra-red absorption reported long ago.

cond-mat.str-el↗

arXiv2019

Consideration of Thermal Hall Effect in Undoped Cuprates

A recent observation of thermal Hall effect of magnetic origin in underdoped cuprates calls for critical re-examination of low-energy magnetic dynamics in undoped antiferromagnetic compound on square lattice, where traditional, renormalized spin-wave theory was believed to work well. Using Holstein-Primakoff boson formalism, we find that magnon-based theories can lead to finite Berry curvature in the magnon band once the Dzyaloshinskii-Moriya spin interaction is taken into account explicitly, but fail to produce non-zero thermal Hall conductivity. Assuming accidental doping by impurities and magnon scattering off of such impurity sites fails to predict skew scattering at the level of Born approximation. Local formation of skyrmion defects is also found incapable of generating magnon thermal Hall effect. Turning to spinon-based scenario, we write down a simple model by adding spin-dependent diagonal hopping to the well-known π-flux model of spinons. The resulting two-band model has Chern number in the band structure, and generates thermal Hall conductivity whose magnetic field and temperature dependences mimic closely the observed thermal Hall signals. In disclaimer, there is no firm microscopic basis of this model and we do not claim to have found an explanation of the data, but given the unexpected nature of the experimental observation, it is hoped this work could serve as a first step towards reaching some level of understanding.

cond-mat.str-el↗

arXiv2019

Pair Density Wave in the Doped $t$-$J$ Model with Ring Exchange on a Triangular Lattice

In our previous work [arXiv:1803.00999, Phys. Rev. Lett. 121, 046401 (2018)], we found a quantum spin liquid phase with a spinon Fermi surface in the two dimensional spin-1/2 Heisenberg model with four-spin ring exchange on a triangular lattice. In this work we dope the spinon Fermi surface phase by studying the $t$-$J$ model with four-spin ring exchange. We perform density matrix renormalization group calculations on four-leg cylinders of a triangular lattice and find that the dominant pair correlation function is that of a pair density wave; i.e., it is oscillatory while decaying with distance with a power law. The doping dependence of the period is studied. This is the first example where pair density wave is the dominant pairing in a generic strongly interacting system where the pair density wave cannot be explained as a composite order and no special symmetry is required.

cond-mat.str-el↗

arXiv2019

Comment on "Superconductivity at low density near a ferroelectric quantum critical point: Doped SrTiO3"

Wölfle and Balatsky Phys. Rev. B 98, 104505 (2018) have proposed a microscopic pairing mechanism for doped SrTiO$_3$ (STO) based on the ${\textit gradient}$ coupling of electronic density to the soft TO phonon mode. Since this coupling to TO phonons is usually weak, this conclusion is surprising, especially for a low density superconductor such as STO, where the density of states is small. A crucial step in the argument made by Wölfle and Balatsky is that the displacement vector of the TO mode is not strictly perpendicular to the momentum vector, making a deformation coupling possible. We show that they have made a mistake in computing the eigenvector and have grossly overestimated this lack of orthogonality. When corrected, the coupling is negligible. We also use transport data to put upper bounds on the coupling constant which are much smaller than the estimate by Wölfle and Balatsky. Finally, we also object to their use of the Eliashberg equation when the phonon frequency is larger than the Fermi energy.

cond-mat.supr-con↗

arXiv2019

Odd-parity linear magnetoresistance and the planar Hall effect

The phenomena of odd-parity magnetoresistance and the planar Hall effect are deeply entwined with ferromagnetism. The intrinsic magnetization of the ordered state permits these unusual and rarely observed manifestations of Onsager's theorem when time reversal symmetry is broken at zero applied field. Here we study two classes of ferromagnetic materials, rare-earth magnets with high intrinsic coercivity and antiferromagnetic pyrochlores with strongly-pinned ferromagnetic layers at domain walls, which both exhibit odd-parity magnetoresistive behavior. The peculiar angular variation of the response with respect to the relative alignments of the magnetization, magnetic field, and current reveal the two underlying microscopic mechanisms: spin-polarization-dependent scattering of a Zeeman-shifted Fermi surface and magnetoresistance driven by the anomalous velocity physics usually associated with the anomalous Hall effect.

cond-mat.str-el↗

arXiv2018

Three-dimensional quantum Hall effect and metal-insulator transition in ZrTe5

Symmetry, dimensionality, and interaction are crucial ingredients for phase transitions and quantum states of matter. As a prominent example, the integer quantum Hall effect (QHE) represents a topological phase generally regarded as characteristic for two-dimensional (2D) electronic systems, and its many aspects can be understood without invoking electron-electron interaction. The intriguing possibility of generalizing QHE to three-dimensional (3D) systems was proposed decades ago, yet it remains elusive experimentally. Here, we report clear experimental evidence for the 3D QHE observed in bulk ZrTe5 crystals. Owing to the extremely high sample quality, the extreme quantum limit with only the lowest Landau level occupied can be achieved by an applied magnetic field as low as 1.5 T. Remarkably, in this regime, we observe a dissipationless longitudinal resistivity rho_xx=0 accompanied with a well-developed Hall resistivity plateau rho_xy=(1\pm0.1) h/e^2 (λ_(F,z)/2), where λ_(F,z) is the Fermi wavelength along the field direction (z axis). This striking result strongly suggests a Fermi surface instability driven by the enhanced interaction effects in the extreme quantum limit. In addition, with further increasing magnetic field, both rho_xx and rho_xy increase dramatically and display an interesting metal-insulator transition, representing another magnetic field driven quantum phase transition. Our findings not only unambiguously reveal a novel quantum state of matter resulting from an intricate interplay among dimensionality, interaction, and symmetry breaking, but also provide a promising platform for further exploration of more exotic quantum phases and transitions in 3D systems.

cond-mat.mtrl-sci↗

arXiv2018

Proposal to measure the pair field correlator of a fluctuating pair density wave

I propose a method to directly measure the space and time dependence of the pair field correlator of a pair density wave. The method is based on two separate ideas. First, we adopt the solenoid insertion method of Kapon et al (2017) to provide the momentum in a tunnel junction. Second, we suggest the use of optimal or over-doped Bi-2201 films as a tunneling electrode with a known charge ordering wave-vector which can match the expected pair density wave wave-vectors we wish to study. The method is applicable to both fluctuating and ordered states. Potential applications are to the proposed stripe pair density wave order in LBCO and the possible pair density wave fluctuations at finite temperature or in high magnetic field in underdoped YBCO as well as other members of the Cuprate family.

cond-mat.str-el↗

arXiv2018

Scaling and data collapse from local moments in frustrated disordered quantum spin systems

Recently measurements on various spin-1/2 quantum magnets such as H$_3$LiIr$_2$O$_6$, LiZn$_2$Mo$_3$O$_8$, ZnCu$_3$(OH)$_6$Cl$_2$ and 1T-TaS$_2$ -- all described by magnetic frustration and quenched disorder but with no other common relation -- nevertheless showed apparently universal scaling features at low temperature. In particular the heat capacity C[H,T] in temperature T and magnetic field H exhibits T/H data collapse reminiscent of scaling near a critical point. Here we propose a theory for this scaling collapse based on an emergent random-singlet regime extended to include spin-orbit coupling and antisymmetric Dzyaloshinskii-Moriya (DM) interactions. We derive the scaling $C[H,T]/T \sim H^{-γ} F_q[T/H]$ with $F_q[x] = x^{q}$ at small $x$, with $q \in$ (0,1,2) an integer exponent whose value depends on spatial symmetries. The agreement with experiments indicates that a fraction of spins form random valence bonds and that these are surrounded by a quantum paramagnetic phase. We also discuss distinct scaling for magnetization with a $q$-dependent subdominant term enforced by Maxwell's relations.

cond-mat.str-el↗