arXiv subjects

Patrick M. Ledingham

Publications and source records attributed to Patrick M. Ledingham.

16 recordsLinked to original sources

arXiv2026

A Fibre-Integrated SPDC Heralded Single-Photon Source Using Zn-Indiffused PPLN Ridge Waveguides at Telecom Wavelengths

We report a fibre-integrated heralded single-photon source based on a commercial Zn-indiffused MgO:PPLN ridge waveguide operated in Type-0 degenerate spontaneous parametric down-conversion (SPDC). The device emits a broadband spectrum spanning approximately 70 nm across the telecom C-and L-bands, with an absolute brightness of $9.1\times 10^{9}$ pairs/(s mW). After accounting for optical losses, we determine an internal heralding efficiency of 58(5)%. The source maintains high purity, exhibiting a coincidences-to-accidentals ratio exceeding $9\times 10^{4}$ and a heralded second-order correlation of $g_{\text{h}}^{(2)}(0) = (5.53 \pm 0.46)\times 10^{-4}$. Low multi-photon noise and broadband emission demonstrate the viability of such platforms for wavelength-multiplexed quantum networking.

quant-ph↗

arXiv2026

Dynamic rephasing in a telecom warm vapor quantum memory

The Off-Resonant Cascaded Absorption (ORCA) protocol in warm atomic vapors offers a scalable platform for high-bandwidth, low noise quantum memories, but its coherence time is fundamentally limited by Doppler-induced dephasing. We introduce and experimentally demonstrate a dynamic rephasing protocol that counteracts Doppler dephasing in a telecom-band ORCA quantum memory. By transferring the stored excitation to an auxiliary shelving state, we effectively reverse the accumulated Doppler phase and extend the storage time by a factor of 50 while preserving the memory's GHz bandwidth and low noise. Using this protocol, we then demonstrate on-demand storage and retrieval of four independent time-bin modes within a single warm vapor memory -- showing that Doppler dephasing can alternatively be harnessed for high-dimensional temporal mode processing. Our results establish rephasing in warm atomic vapors as a viable route toward high-bandwidth, temporally multiplexed quantum memories operating at room temperature.

quant-ph↗

arXiv2025

Single-Photon-Level Atomic Frequency Comb Storage in Room Temperature Alkali Vapour

We have demonstrated the coherent storage and retrieval of single-photon-level light using the atomic frequency comb protocol in a room temperature rubidium vapour. Velocity-selective optical pumping is used to prepare the comb within the $F=2$ hyperfine ground state of rubidium, with the spacing between peaks coinciding with half the $F = 2 - F =3$ hyperfine splitting of the $5^2$P$_{3/2}$ excited state. Weak coherent states of average photon number $\mu_\mathrm{in} = 0.083(5)$ are stored with pre-programmed recall time of $7.5\,$ns with an efficiency of $\eta_{\textrm{AFC}} = 6.59(5)\,\%$, while two temporally distinct modes have been stored and recalled with $\eta_{\textrm{AFC}} = 2.6(1)\,\%$, allowing for time-bin qubit storage. Finally, the efficiency is observed to be independent of the input pulse polarisation, paving the way for polarisation qubit storage.

quant-ph↗

arXiv2019

Raman Quantum Memory with Built-In Suppression of Four-wave Mixing Noise

Quantum memories are essential for large-scale quantum information networks. Along with high efficiency, storage lifetime and optical bandwidth, it is critical that the memory add negligible noise to the recalled signal. A common source of noise in optical quantum memories is spontaneous four-wave mixing. We develop and implement a technically simple scheme to suppress this noise mechanism by means of quantum interference. Using this scheme with a Raman memory in warm atomic vapour we demonstrate over an order of magnitude improvement in noise performance. Furthermore we demonstrate a method to quantify the remaining noise contributions and present a route to enable further noise suppression. Our scheme opens the way to quantum demonstrations using a broadband memory, significantly advancing the search for scalable quantum photonic networks.

quant-ph↗

arXiv2018

A two-way photonic interface for linking Sr+ transition at 422 nm to the telecommunications C-band

We report a single-stage bi-directional interface capable of linking Sr+ trapped ion qubits in a long-distance quantum network. Our interface converts photons between the Sr+ emission wavelength at 422 nm and the telecoms C-band to enable low-loss transmission over optical fiber. We have achieved both up- and down-conversion at the single photon level with efficiencies of 9.4% and 1.1% respectively. Furthermore we demonstrate noise levels that are low enough to allow for genuine quantum operation in the future.

quant-ph↗

arXiv2018

Experimental demonstration of quantum effects in the operation of microscopic heat engines

The heat engine, a machine that extracts useful work from thermal sources, is one of the basic theoretical constructs and fundamental applications of classical thermodynamics. The classical description of a heat engine does not include coherence in its microscopic degrees of freedom. By contrast, a quantum heat engine might possess coherence between its internal states. Although the Carnot efficiency cannot be surpassed, and coherence can be performance degrading in certain conditions, it was recently predicted that even when using only thermal resources, internal coherence can enable a quantum heat engine to produce more power than any classical heat engine using the same resources. Such a power boost therefore constitutes a quantum thermodynamic signature. It has also been shown that the presence of coherence results in the thermodynamic equivalence of different quantum heat engine types, an effect with no classical counterpart. Microscopic heat machines have been recently implemented with trapped ions, and proposals for heat machines using superconducting circuits and optomechanics have been made. When operated with standard thermal baths, however, the machines implemented so far have not demonstrated any inherently quantum feature in their thermodynamic quantities. Here we implement two types of quantum heat engines by use of an ensemble of nitrogen-vacancy centres in diamond, and experimentally demonstrate both the coherence power boost and the equivalence of different heat-engine types. This constitutes the first observation of quantum thermodynamic signatures in heat machines.

quant-ph↗

arXiv2017

Quantum correlations between single telecom photons and a multimode on-demand solid state quantum memory

Quantum correlations between long lived quantum memories and telecom photons that can propagate with low loss in optical fibers are an essential resource for the realization of large scale quantum information networks. Significant progress has been realized in this direction with atomic and solid state systems. Here, we demonstrate quantum correlations between a telecom photon and a multimode on-demand solid state quantum memory. This is achieved by mapping a correlated single photon onto a spin collective excitation in a Pr$^{3+}$:Y$_2$SiO$_5$ crystal for a controllable time. The stored single photons are generated by cavity enhanced spontaneous parametric down conversion (SPDC) and heralded by their partner photons at telecom wavelength. These results represent the first demonstration of a multimode on-demand solid state quantum memory for external quantum states of light. They provide an important resource for quantum repeaters and pave the way for the implementation of quantum information networks with distant solid-state quantum nodes.

quant-ph↗

arXiv2015

Ultrahigh and persistent optical depths of caesium in Kagomé-type hollow-core photonic crystal fibres

Alkali-filled hollow-core fibres are a promising medium for investigating light-matter interactions, especially at the single-photon level, due to the tight confinement of light and high optical depths achievable by light-induced atomic desorption. However, until now these large optical depths could only be generated for seconds at most once per day, severely limiting the practicality of the technology. Here we report the generation of highest observed transient ($>10^5$ for up to a minute) and highest observed persistent ($>2000$ for hours) optical depths of alkali vapours in a light-guiding geometry to date, using a caesium-filled Kagomé-type hollow-core photonic crystal fibre. Our results pave the way to light-matter interaction experiments in confined geometries requiring long operation times and large atomic number densities, such as generation of single-photon-level nonlinearities and development of single photon quantum memories.

physics.atom-ph↗

arXiv2015

A solid state spin-wave quantum memory for time-bin qubits

We demonstrate the first solid-state spin-wave optical quantum memory with on-demand read-out. Using the full atomic frequency comb scheme in a \PrYSO crystal, we store weak coherent pulses at the single-photon level with a signal to noise ratio $> 10$. Narrow-band spectral filtering based on spectral hole burning in a second \PrYSO crystal is used to filter out the excess noise created by control pulses to reach an unconditional noise level of $(2.0 \pm 0.3) \times10^{-3}$ photons per pulse. We also report spin-wave storage of photonic time-bin qubits with conditional fidelities higher than a measure and prepare strategy, demonstrating that the spin-wave memory operates in the quantum regime. This makes our device the first demonstration of a quantum memory for time-bin qubits, with on demand read-out of the stored quantum information. These results represent an important step for the use of solid-state quantum memories in scalable quantum networks.

quant-ph↗

arXiv2014

Storage of up-converted telecom photons in a doped crystal

We report on an experiment that demonstrates the frequency up-conversion of telecommunication wavelength single-photon-level pulses to be resonant with a $\mathrm{Pr}^{3+}$:$\mathrm{Y}_2\mathrm{Si}\mathrm{O}_5$ crystal. We convert the telecom photons at $1570\,\mathrm{nm}$ to $606\,\mathrm{nm}$ using a periodically-poled potassium titanyl phosphate nonlinear waveguide. The maximum device efficiency (which includes all optical loss) is inferred to be $η_{\mathrm{dev}}^{\mathrm{max}} = 22 \pm 1\,%$ (internal efficiency $η_{\mathrm{int}} = 75\pm8\,%$) with a signal to noise ratio exceeding 1 for single-photon-level pulses with durations of up to 560$\,$ns. The converted light is then stored in the crystal using the atomic frequency comb scheme with storage and retrieval efficiencies exceeding $η_{\mathrm{AFC}} = 20\,%$ for predetermined storage times of up to $5\,μ\mathrm{s}$. The retrieved light is time delayed from the noisy conversion process allowing us to measure a signal to noise ratio exceeding 100 with telecom single-photon-level inputs. These results represent the first demonstration of single-photon-level optical storage interfaced with frequency up-conversion.

quant-ph↗

arXiv2013

Coherent Storage of Temporally Multimode Light Using a Spin-Wave Atomic Frequency Comb Memory

We report on coherent and multi-temporal mode storage of light using the full atomic frequency comb memory scheme. The scheme involves the transfer of optical atomic excitations in Pr3+:Y2SiO5 to spin-waves in the hyperfine levels using strong single-frequency transfer pulses. Using this scheme, a total of 5 temporal modes are stored and recalled on-demand from the memory. The coherence of the storage and retrieval is characterized using a time-bin interference measurement resulting in visibilities higher than 80%, independent of the storage time. This coherent and multimode spin-wave memory is promising as a quantum memory for light.

quant-ph↗

arXiv2012

Experimental realization of light with time separated correlations by rephasing amplified spontaneous emission

Amplified spontaneous emission is a common noise source in active optical systems, it is generally seen as being an incoherent process. Here we excite an ensemble of rare earth ion dopants in a solid with a π-pulse, resulting in amplified spontaneous emission. The application of a second π-pulse leads to a coherent echo of the amplified spontaneous emission that is correlated in both amplitude and phase. For small optical thicknesses, we see evidence that the amplified spontaneous emission and its echo are entangled.

quant-ph↗

arXiv2012

Quantum Storage of a Photonic Polarization Qubit in a Solid

We report on the quantum storage and retrieval of photonic polarization quantum bits onto and out of a solid state storage device. The qubits are implemented with weak coherent states at the single photon level, and are stored for 500 ns in a praseodymium doped crystal with a storage and retrieval efficiency of 10%, using the atomic frequency comb scheme. We characterize the storage by using quantum state tomography, and find that the average conditional fidelity of the retrieved qubits exceeds 95% for a mean photon number mu=0.4. This is significantly higher than a classical benchmark, taking into account the Poissonian statistics and finite memory efficiency, which proves that our device functions as a quantum storage device for polarization qubits, even if tested with weak coherent states. These results extend the storage capabilities of solid state quantum memories to polarization encoding, which is widely used in quantum information science.

quant-ph↗

arXiv2011

Photon echo without a free induction decay in a double-Lambda system

We have characterized a novel photon-echo pulse sequence for a double-$Λ$ type energy level system where the input and rephasing transitions are different to the applied $π$-pulses. We show that despite having imperfect $π$-pulses (associated with large coherent emission due to free induction decay), the noise added is only 0.019$\pm$0.001 relative to the shot noise in the spectral mode of the echo. Using this echo pulse sequence in the `rephased amplified spontaneous emission' (RASE) scheme \cite{Ledingham2010} will allow for generation of entangled photon pairs that are in different frequency, temporal, and potentially spatial modes to any bright driving fields. The coherence and efficiency properties of this sequence were characterized in a Pr:YSO crystal.

quant-ph↗

arXiv2010

Hybrid optical and electronic laser locking using spectral hole burning

We report on a narrow linewidth laser diode system that is stabilized using both optical and electronic feedback to a spectral hole in cryogenic Tm:YAG. The laser system exhibits very low phase noise. The spectrum of the beat signal between two lasers, over millisecond timescales, is either Fourier limited or limited by the -111dBc/Hz noise floor. The resulting laser is well suited to quantum optics and sensing applications involving rare earth ion dopants.

physics.optics↗

arXiv2009

Non-classical photon streams using rephased amplified spontaneous emission

We present a fully quantum mechanical treatment of optically rephased photon echoes. These echoes exhibit noise due to amplified spontaneous emission, however this noise can be seen as a consequence of the entanglement between the atoms and the output light. With a rephasing pulse one can get an "echo" of the amplified spontaneous emission, leading to light with nonclassical correlations at points separated in time, which is of interest in the context of building wide bandwidth quantum repeaters. We also suggest a wideband version of DLCZ protocol based on the same ideas.

quant-ph↗