arXiv subjects

Patrick Talou

Publications and source records attributed to Patrick Talou.

12 recordsLinked to original sources

arXiv2025

Updating GEANIE $^{239}$Pu prompt $\gamma$-ray experimental data using modern Hauser-Feshbach fission fragment decay model

We calculate fission $\gamma$ rays for neutron-induced reactions on $^{239}$Pu with the Hauser-Feshbach fission fragment decay model. By applying the calculated fission $\gamma$ rays as a background contribution, the historical $^{239}$Pu(n,$x$n$\gamma$) reaction cross section data measured by the GEANIE (GErmanium Array for Neutron Induced Excitations) spectrometer are corrected. The correction also includes other (n,$x$n) reactions that have very similar energies to the $\gamma$ lines reported by GEANIE. In many cases, the original GEANIE data are strongly reduced and they become much closer to the statistical Hauser-Feshbach model predictions. The total inelastic scattering, (n,2n), and (n,3n) cross sections are inferred based on the corrected GEANIE data, and compared with available experimental data as well as the statistical model calculations. Expected $\gamma$-ray energy spectra for neutron-induced measurements on $^{239}$Pu are also discussed.

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arXiv2025

Deblurring fission fragment mass distributions

Measurements of fission fragment mass distributions provide valuable insights into the properties of fissioning systems and the dynamics of the fission process. Pre-neutron emission distributions, essential for fission fragment evaporation codes like \cgmf{}, are extracted from distributions that are always measured after neutron emission, as the time scale of the emission of prompt fission neutrons is too short for direct measurement before the emission. However, obtaining accurate pre-neutron emission distributions requires methods that eliminate the effects of mass resolution and detector efficiency. We propose a deblurring technique based on the Richardson-Lucy (RL) algorithm, commonly used in optics for image restoration, to correct for these experimental effects. The RL algorithm uses the measured mass distributions and a transfer matrix to perform iterative deconvolution. The advantage of this method over others is that it does not assume any predefined shape such as a sum of Gaussians, as in \cgmf{}, for the distributions. In this paper, we apply the algorithm to the fission fragment mass distributions measured in the spontaneous fission of $^{252}$Cf to extract pre-neutron emission fission fragment mass distributions. The results from deblurring are then used as inputs to \cgmf{}, and we compare the \cgmf{} results obtained using deblurring inputs with the default \cgmf{} results.

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arXiv2025

Time Evolution of Prompt Gamma-Ray Emission in $^{252}$Cf(sf) and $^{233,235}$U($n$,f) Reactions

We investigate the time evolution of prompt fission $\gamma$ emission due to the presence of ns to ms isomers in the fragments produced in the neutron-induced fission of $^{233,235}$U and in the spontaneous fission of $^{252}$Cf. Calculations performed with the CGMF fission event generator are compared with recent experimental data on $^{252}$Cf(sf) and $^{235}$U($n$,f) obtained with the DANCE+NEUANCE setup at the Los Alamos Neutron Science Center. Of particular interest are the average $\gamma$-ray energy spectrum as a function of time since scission, $\phi(\epsilon_\gamma,t)$, the increase of the average $\gamma$-ray multiplicity over time, $N_\gamma(t)$, and its evolution in time as a function of the fission fragment mass, $N_\gamma(A,t)$. The time evolution of isomeric ratios in post-neutron emission fission fragments can be defined and used to test and reveal some deficiencies in our knowledge of the low-lying levels of neutron-rich nuclei produced in fission reactions.

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arXiv2023

Solving one-dimensional penetration problem for fission channel in the statistical Hauser-Feshbach theory

We solve the Schr\"{o}dinger equation for an arbitrary one-dimensional potential energy to calculate the transmission coefficient in the fission channel of compound nucleus reactions. We incorporate the calculated transmission coefficients into the statistical Hauser-Feshbach model calculation for neutron-induced reactions on $^{235,238}$U and $^{239}$Pu. The one-dimensional model reproduces the evaluated fission cross section data reasonably well considering the limited number of model parameters involved. A resonance-like structure appears in the transmission coefficient for a double-humped fission barrier shape that includes an intermediate well, which is understood to be a quantum mechanical effect in the fission channel. The calculated fission cross sections for the neutron-induced reactions on $^{235,238}$U and $^{239}$Pu all exhibit a similar structure.

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arXiv2022

Consideration of memory of spin and parity in the fissioning compound nucleus by applying the Hauser-Feshbach fission fragment decay model to photonuclear reactions

Prompt and $\beta$-delayed fission observables, such as the average number of prompt and delayed neutrons, the independent and cumulative fission product yields, and the prompt $\gamma$-ray energy spectra for the photonuclear reactions on $^{235,238}$U and $^{239}$Pu are calculated with the Hauser-Feshbach Fission Fragment Decay (HF$^3$D) model and compared with available experimental data. In the analysis of neutron-induced fission reactions to the case of photo-induced fission, an excellent reproduction of the delayed neutron yields supports a traditional assumption that the photo-fission might be similar to the neutron-induced fission at the same excitation energies regardless of the spin and parity of the fissioning systems.

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arXiv2022

Correlations between energy and $\gamma$-ray emission in $^{239}\mathrm{Pu}(n,\mathrm{f})$

We study $\gamma$-ray emission following $^{239}\mathrm{Pu}(n,\mathrm{f})$ over an incident neutron energy range of $2 < E_i < 40$ MeV. We present the first experimental evidence for positive correlations between the total angular momentum generated in fission and the excitation energy of the compound nucleus prior to fission. The $\gamma$-ray multiplicity increases linearly with incident energy below the 2\textsuperscript{nd}-chance fission threshold with a slope of $0.085 \pm 0.010$ MeV$^{-1}$. This linear trend appears to hold for the average excitation energy of the compound nucleus between $9 < \langle E_x \rangle < 19$ MeV. Most of the multiplicity increase comes from an enhancement around a $\gamma$-ray energy of 0.7 MeV, which we interpret as stretched quadrupole $\gamma$ rays that indicate an increase in total fission-fragment angular momentum with excitation energy.

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arXiv2021

Structure in the Event-by-Event Energy-Dependent Neutron-Gamma Multiplicity Correlations in $^{252}\text{Cf}$(sf)

The emission of neutrons and gamma rays by fission fragments reveal important information about the properties of fragments immediately following scission. The initial fragment properties, correlations between fragments, and emission competition give rise to correlations in neutron-gamma emission. Neutron-gamma correlations are important in nonproliferation applications because the characterization of fissionable samples relies on the identification of signatures in the measured radiation. Furthermore, recent theoretical and experimental advances have proposed to explain the mechanism of angular momentum generation in fission. In this paper, we present a novel analysis method of neutrons and gamma rays emitted by fission fragments that allows us to discern structure in the observed correlations. We have analyzed data collected on \ce{^{252}Cf}(sf) at the Chi-Nu array at the Los Alamos Neutron Science Center. Through our analysis of the energy-differential neutron-gamma multiplicity covariance, we have observed enhanced neutron-gamma correlations, corresponding to rotational band gamma-ray transitions, at gamma-ray energies of $0.7$ and $1.2$ MeV. To shed light on the origin of this structure, we compare the experimental data with the predictions of three model calculations. The origin of the observed correlation structure is understood in terms of a positive spin-energy correlation in the generation of angular momentum in fission.

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arXiv2021

Influence of non-statistical properties in nuclear structure on emission of prompt fission neutrons

The Hauser-Feshbach Fission Fragment Decay (HF$^3$D) model is extended to calculate the prompt fission neutron spectrum (PFNS) for the thermal neutron induced fission on $^{235}$U, where the evaporated neutrons from all possible fission fragment pairs are aggregated. By studying model parameter sensitivities on the calculated PFNS, as well as non-statistical behavior of low-lying discrete level spin distribution, we conclude that discrepancies between the aggregation calculation and the experimental PFNS seen at higher neutron emission energies can be attributed to both the primary fission fragment yield distribution and the possible high spin states that are not predicted by the statistical theory of nuclear structure.

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arXiv2019

Event-by-Event Multiplicity Correlations in $^{252}$Cf(sf)

Excited nuclear fragments are emitted during nuclear fission. The de-excitation of these fission fragments takes place as sequential emission of neutrons followed by photons. A correlation between neutron and photon multiplicities accompanying fission is thus expected. Fission event generators based on established statistical nuclear physics models predict a negative event-by-event correlation in neutron-photon multiplicity. A survey of published experimental results of an event-by-event covariance between the neutron and photon multiplicities emitted following the spontaneous fission of $^{252}$Cf is presented. Analytic unfolding expressions are developed in this work to determine the bias introduced by background sources, particle misclassification, pulse pileup, and inelastic photon production. The published experimental data are re-analyzed using these unfolding techniques and are found to be in qualitative agreement with the predictions of model-based calculations. In particular, we have concluded that there exists a significant event-by-event neutron-photon emission competition following the spontaneous fission of $^{252}$Cf.

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arXiv2018

$^{235}$U(n, f) Independent Fission Product Yield and Isomeric Ratio Calculated with the Statistical Hauser-Feshbach Theory

We have developed a Hauser-Feshbach fission fragment decay model, HF$^3$D, which can be applied to the statistical decay of more than 500 primary fission fragment pairs (1,000 nuclides) produced by the neutron induced fission of $^{235}$U. The fission fragment yield $Y(A)$ and the total kinetic energy TKE are model inputs, and we estimate them from available experimental data for the $^{235}$U(n$\rm_{th}$,f) system. The model parameters in the statistical decay calculation are adjusted to reproduce some fission observables, such as the neutron emission multiplicity $\overline{\nu}$, its distribution $P(\nu)$, and the mass dependence $\overline\nu(A)$. The calculated fission product yield and isomeric ratio are compared with experimental data. We show that the calculated independent fission product yield $Y_I(A)$ at the thermal energy reproduces the experimental data well, while the calculated isomeric ratios tend to be lower than the Madland-England model prediction. The model is extended to higher incident neutron energies up to the second chance fission threshold. We demonstrate for the first time that most of the isomeric ratios stay constant, although the production of isomeric state itself changes as the incident energy increases.

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arXiv2017

Hauser-Feshbach fission fragment de-excitation with calculated macroscopic-microscopic mass yields

The Hauser-Feshbach statistical model is applied to the de-excitation of primary fission fragments using input mass yields calculated with macroscopic-microscopic models of the potential energy surface. We test the sensitivity of the prompt fission observables to the input mass yields for two important reactions, $^{235}$U$(n_\mathrm{th},f)$ and $^{239}$Pu$(n_\mathrm{th},f)$, for which good experimental data exist. General traits of the mass yields, such as the location of the peaks and their widths, can impact both the prompt neutron and $\gamma$-ray multiplicities, as well as their spectra. Specifically, we use several mass yields to determine a linear correlation between the calculated prompt neutron multiplicity $\bar{\nu}$ and the average heavy-fragment mass $\langle A_h\rangle$ of the input mass yields $\partial\bar{\nu}/\partial\langle A_h\rangle = \pm 0.1\,n/f/\mathrm{u}$. The mass peak width influences the correlation between the total kinetic energy of the fission fragments and the total number of prompt neutrons emitted $\bar{\nu}_T(\mathrm{TKE})$. Typical biases on prompt particle observables from using calculated mass yields instead of experimental ones are: $\delta \bar{\nu} = 4\%$ for the average prompt neutron multiplicity, $\delta \bar{M}_\gamma = 1\%$ for the average prompt $\gamma$-ray multiplicity, $\delta \bar{\epsilon}_n^\mathrm{LAB} = 1\%$ for the average outgoing neutron energy, $\delta \bar{\epsilon}_\gamma = 1\%$ for the average $\gamma$-ray energy, and $\delta \langle\mathrm{TKE}\rangle = 0.4\%$ for the average total kinetic energy of the fission fragments.

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arXiv2017

Revisiting the role of the $(n,\gamma f)$ process in the low-energy fission of $^{235}$U and $^{239}$Pu

The $(n,\gamma f)$ process is reviewed in light of modern nuclear reaction calculations in both slow and fast neutron-induced fission reactions on $^{235}$U and $^{239}$Pu. Observed fluctuations of the average prompt fission neutron multiplicity and average total $\gamma$-ray energy below 100 eV incident neutron energy are interpreted in this framework. The surprisingly large contribution of the M1 transitions to the pre-fission $\gamma$-ray spectrum of $^{239}$Pu is explained by the dominant fission probabilities of 0$^+$ and $2^+$ transition states, which can only be accessed from compound nucleus states formed by the interaction of $s$-wave neutrons with the target nucleus in its ground state, and decaying through M1 transitions. The impact of an additional low-lying M1 scissors mode in the photon strength function is analyzed. We review experimental evidence for fission fragment mass and kinetic energy fluctuations in the resonance region and their importance in the interpretation of experimental data on prompt neutron data in this region. Finally, calculations are extended to the fast energy range where $(n,\gamma f)$ corrections can account for up to 3\% of the total fission cross section and about 20\% of the capture cross section.

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