arXiv subjects

Paul Indelicato

Publications and source records attributed to Paul Indelicato.

At least 19 recordsLinked to original sources

arXiv2026

Nuclear Charge Radius of $^9$Be from Muonic Atom Spectroscopy Using a Microcalorimeter

The $2p\to1s$ transition energy in muonic $^9$Be was measured using a metallic magnetic calorimeter, resulting in $E_{2p\to 1s}=33\,391.48(34)\,$eV. The result is 30 times more precise than the previous best measurement and enables the extraction of the corresponding nuclear charge radius $r_c($$^9$Be$)=2.5506(51)\,$fm. It is $2.4$ times more precise than the commonly used value based on electron scattering and differs from it by $2.3$ times the combined uncertainties. This measurement represents the first determination of a nuclear charge radius using muonic x-ray spectroscopy with microcalorimeters.

nucl-ex↗

arXiv2026

Theoretical ab initio Evolution of Satellite Intensity near Threshold for Cu K-shell transitions

In this work, we have investigated the evolution of satellite intensity near the ionization threshold for Cu K-shell transitions through theoretical methods. Employing standard state-of-the-art ab initio methods, we have calculated all Cu K-shell transitions and simulated the full K$α_1$ and K$α_2$ spectrum where all transition parameters, as well as shake probabilities were determined theoretically. Through these calculations we show that standard state-of-the-art ab initio methods achieve good agreement with experiment and enable us to simulate the intensity evolution near ionization thresholds within a good margin of error. Below-threshold satellite intensity was found to originate from resonant 1s$\rightarrow$3d and 1s$\rightarrow$4p excitations in Cu(I) and Cu(II) oxide phases respectively, which were included in our simulations.

physics.atom-ph↗

arXiv2026

Probing Nuclear Structure with Kaonic Atoms through E2 Resonance Mixing

Kaonic atoms provide a unique laboratory to investigate the interplay between atomic, nuclear, and strong-interaction physics. In heavy nuclei, atomic transitions can couple to low-lying collective nuclear excitations via the electric quadrupole interaction. When the energy difference between two kaonic atomic levels approaches that of a nuclear $2^+$ excitation, a resonant configuration mixing may occur, known as the E2 nuclear resonance effect. In this work, we investigate the conditions for E2 resonance in kaonic molybdenum isotopes. We describe the mixing using state-of-the-art Dirac-Fock calculations combined with updated nuclear structure inputs, including recent electric quadrupole transition strength values and excitation energies. We evaluate the sensitivity of the effect to key parameters, assess its observability in future experiments such as the EXKALIBUR program, and discuss its impact on cascade dynamics. Our results demonstrate the potential of kaonic atoms as a probe of nuclear structure, complementary to conventional nuclear spectroscopy.

nucl-ex↗

arXiv2026

Binding Energy of Muonic Beryllium: Perturbative versus All--Order Calculations

We compute the ground-state binding energy of muonic $^9$Be in two ways: first, the fully perturbative treatment of the nuclear-size effect often employed in light systems, and second, an approach that accounts for the finite-nuclear-size to all orders (and is inspired by calculations otherwise employed for heavy muonic ions). The results are compared term by term and show that both approaches agree to better than one part-per-million of the total energy. The objective of this work is twofold. The first is practical: to provide a parametrization that allows the extraction of the $^9$Be charge radius from recent and forthcoming experiments with high precision. The second is more conceptual: to act as a bridge between the community working on calculations for light systems and those focusing on heavy systems, demonstrating that the fully relativistic approach otherwise chosen for heavy systems can be enhanced to cover theoretical predictions for all charge numbers.

physics.atom-ph↗

arXiv2026

Shake-up and shake-off spectra in the electron capture decay of atomic $^7$Be

The most stringent laboratory-based experimental limits on the existence of sub-MeV sterile neutrinos are currently set by decay spectroscopy of radioactive $^7$Be embedded into superconducting sensors. The systematic uncertainties are dominated by the modeling of the electron shake-up and shake-off spectra that are not based on state-of-the-art atomic theory and do not include electron correlations or relativistic effects. We have used the multiconfiguration Dirac-Fock formalism to obtain correlated wavefunctions ab initio and compute all single and double shake processes in the electron capture decay of atomic $^7$Be. The simulations can explain some but not all of the observed spectral features, likely because the wave functions are modified by the Ta sensor material that the $^7$Be is embedded into. The new models also show that the L/K electron capture ratio of $^7$Be in Ta has previously been slightly underestimated revising the previous value of 0.070(7) to a new value of 0.0756(20).

physics.atom-ph↗

arXiv2026

All-Order Wichmann and Kroll Contribution in Heavy Electronic and Exotic Atoms

We present a theoretical study of the Wichmann and Kroll correction to the one-loop vacuum polarization (VP) to all-orders in $αZ$. We consider electronic, muonic, and antiprotonic atoms for a wide range of nuclear charge numbers and explicitly investigate the influence of finite nuclear size effects and different nuclear models. Moreover, we place special emphasis on circular Rydberg states in the exotic atoms as they have recently attracted interest as a tool to perform isolated tests of strong-field QED. We find that the higher-order vacuum polarization is strongly enhanced in exotic atoms and remains large enough in highly excited Rydberg states that an accurate treatment is crucial for the analysis of upcoming spectroscopy experiments like PAX. Moreover, our calculations show that the VP contribution to the Lamb shift in these exotic Rydberg states has almost no dependence on the structure of the nucleus.

physics.atom-ph↗

arXiv2025

EXKALIBUR: Towards a Kaonic Atoms Periodic Table to test Fundamental Interactions

Kaonic atoms, formed when a negatively charged kaon replaces an electron, provide a unique laboratory to test fundamental interactions at low energies. EXKALIBUR (EXtensive Kaonic Atoms research: from LIthium and Beryllium to URanium) is a program to perform systematic, high-precision X-ray spectroscopy of selected kaonic atoms across the periodic table at the DA$Φ$NE accelerator at the National Laboratory of Frascati (INFN-LNF). Here, we outline its detector-driven strategy: Silicon Drift Detectors for 10-40 keV transitions in light targets (Li, Be, B, O), CdZnTe detectors for 40-300 keV lines in intermediate-$Z$ systems (Mg, Al, Si, S), and a High-Purity Germanium detector for high-$Z$ atoms (Se, Zr, Ta, Mo, W, Pb), complemented by VOXES, a high-resolution crystal spectrometer for sub-eV studies. EXKALIBUR plans to (i) reduce the charged-kaon mass uncertainty below 10 keV, (ii) produce a database of nuclear shifts and widths to constrain multi-nucleon K$^{-}$-nucleus interaction models, and (iii) provide precision data for testing bound-state QED in strong fields. We summarize the planned measurements and expected sensitivities within DA$Φ$NE luminosities.

nucl-ex↗

arXiv2025

A Bayesian Approach for Strong Field QED Tests with He-like Ions

Detailed comparisons between theory and experiment for quantum electrodynamics (QED) effects in He-like ions have been performed in the literature to search for hints of new physics. Different frequentist statistical analyses of the existing atomic transition energy data have shown contradictory conclusions as to the presence of possible deviations from the theory predictions. We present here an approach using Bayesian statistics which allows to assign quantitative probabilities to the different deviation models from theory for He-like ions for $Z = 5$ to 92. Potential deviations beyond the standard model or higher order QED effects are modeled with $f(Z) \propto Z^k$ functions. Considering the currently available data, no significant difference between theory and experiment is found, and we show that recent experiments have reduced the possible deviations previously observed in the literature. Using past measurements and a weighted average on the different deviation models, we indicate the accuracy required for future measurements to investigated possible divergences.

physics.atom-ph↗

arXiv2025

Towards Precision Spectroscopy of Antiprotonic Atoms for Probing Strong-field QED

PAX (antiProtonic Atom X-ray spectroscopy) is a new experiment with the aim to test strong-field quantum electrodynamics (QED) effects by performing high-precision x-ray spectroscopy of antiprotonic atoms. By utilizing advanced microcalorimeter detection techniques and a low-energy antiproton beam provided by the ELENA ring at CERN, gaseous targets will be used for the creation of antiprotonic atoms, and the measurement of transitions between circular Rydberg states will be conducted with up to two orders of magnitude improved accuracy over previous studies using high-purity germanium detectors. Our approach eliminates the longstanding issue of nuclear uncertainties that have hindered prior studies using highly charged ions, thus enabling direct and purely QED-focused measurements. By precisely probing atomic systems with electric fields up to two orders of magnitude above the Schwinger limit, PAX will test vacuum polarization and second-order QED corrections, opening new frontiers in fundamental physics and uncovering potential pathways to physics beyond the Standard Model.

physics.atom-ph↗

arXiv2024

High-precision, reference-free measurements of 2p $\rightarrow$ 1s transitions in boron-like sulfur and argon

We have measured several 2p $\rightarrow$ 1s transition energies in core-excited boron-like ions of sulfur and argon. The measurements are reference-free, with an accuracy of a few parts per million. The x-rays were produced by the plasma of a an electron-cyclotron resonance ion source and were measured by a double-crystal x-ray spectrometer. The precision obtained for the measured 1s2s22p2 J -- 1s2 2s2 2p J ' lines is $\approx$4 ppm for sulfur and $\approx$2 ppm for argon. The line energies are compared to relativistic atomic structure calculations performed with the mdfgme multi-configuration Dirac-Fock code. This comparison is used for line identification and test the theoretical methods, which reach an agreement with experimental data up to 15 meV. The theoretical calculations have been extended to C+, Si9+, Cr19+ and Fe21+, which were the only B-like ions where such transitions were measured up to now.

physics.atom-ph↗

arXiv2024

MMC Array to Study X-ray Transitions in Muonic Atoms

The QUARTET collaboration aims to significantly improve the precision of the absolute nuclear charge radii of light nuclei from Li to Ne by using an array of metallic magnetic calorimeters to perform high-precision X-ray spectroscopy of low-lying states in muonic atoms. A proof-of-principle measurement with lithium, beryllium and boron is planned for fall 2023 at the Paul Scherrer Institute. We discuss the performance achieved with the maXs-30 detector module to be used. To place the detector close to the target chamber where the muon beam will impact the material under study, we have developed a new dilution refrigerator sidearm. We further discuss the expected efficiency given the transparency of the X-ray windows and the quantum efficiency of the detector. The expected muonic X-ray rate combined with the high resolving power and detection efficiency of the detector suggest that QUARTET will be able to study the de-excitation of light muonic atoms at an unprecedented level, increasing the relative energy resolution by up to a factor of 20 compared to conventional detector techniques.

physics.ins-det↗

arXiv2024

Towards Precision Muonic X-Ray Measurements of Charge Radii of Light Nuclei

We propose an experiment to measure the nuclear charge radii of light elements with up to 20~times higher accuracy. These are essential both for understanding nuclear physics at low energies, and for experimental and theoretical applications in simple atomic systems. Such comparisons advance the understanding of bound-state quantum electrodynamics and are useful for searching for new physics beyond the Standard Model. The energy levels of muonic atoms are highly susceptible to nuclear structure, especially to the mean square charge radius. The radii of the lightest nuclei (with the atomic number, $Z=1,2$) have been determined with high accuracy using laser spectroscopy in muonic atoms, while those of medium mass and above were determined using X-ray spectroscopy with semiconductor detectors. In this communication, we present a new experiment, aiming to obtain precision measurements of the radii of light nuclei $3 \leq Z \leq 10$ using single-photon energy measurements with cryogenic microcalorimeters; a quantum-sensing technology capable of high efficiency with outstanding resolution for low-energy X-rays.

physics.atom-ph↗

arXiv2024

Penning-trap measurement of the $Q$-value of the electron capture in $^{163}\mathrm{Ho}$ for the determination of the electron neutrino mass

The investigation of the absolute scale of the effective neutrino mass remains challenging due to the exclusively weak interaction of neutrinos with all known particles in the standard model of particle physics. Currently, the most precise and least model-dependent upper limit on the electron antineutrino mass is set by the KATRIN experiment from the analysis of the tritium \b{eta}-decay. Another promising approach is the electron capture in $^{163}\mathrm{Ho}$, which is under investigation using microcalorimetry within the ECHo and HOLMES collab orations. An independently measured Q-value of this process is vital for the assessment of systematic uncertainties in the neutrino mass determination. Here, we report a direct, independent determination of this $Q$-value by measuring the free-space cyclotron frequency ratio of highly charged ions of $^{163}\mathrm{Ho}$ and $^{163}\mathrm{Dy}$ in the Penning trap experiment \textsc{Pentatrap}. Combining this ratio with atomic physics calculations of the electronic binding energies yields a $Q$-value of $2863.2(0.6)\,\mathrm{eV}/c^{2}$ - a more than 50-fold improvement over the state-of-the-art. This will enable the determination of the electron neutrino mass on a sub-eV level from the analysis of the electron capture in $^{163}\mathrm{Ho}$.

nucl-ex↗

arXiv2023

Observation of a low-lying metastable electronic state in highly charged lead by Penning-trap mass spectrometry

Highly charged ions (HCIs) offer many opportunities for next-generation clock research due to the vast landscape of available electronic transitions in different charge states. The development of XUV frequency combs has enabled the search for clock transitions based on shorter wavelengths in HCIs. However, without initial knowledge of the energy of the clock states, these narrow transitions are difficult to be probed by lasers. In this Letter, we provide experimental observation and theoretical calculation of a long-lived electronic state in Nb-like Pb$^{41+}$ which could be used as a clock state. With the mass spectrometer Pentatrap, the excitation energy of this metastable state is directly determined as a mass difference at an energy of 31.2(8) eV, corresponding to one of the most precise relative mass determinations to date with a fractional uncertainty of $4\times10^{-12}$. This experimental result agrees within 1 $σ$ with two partially different \textit{ab initio} multi-configuration Dirac-Hartree-Fock calculations of 31.68(13) eV and 31.76(35) eV, respectively. With a calculated lifetime of 26.5(5.3) days, the transition from this metastable state to the ground state bears a quality factor of $1.1\times10^{23}$ and allows for the construction of a HCI clock with a fractional frequency instability of $<10^{-19}/\sqrtτ$.

physics.atom-ph↗

arXiv2023

The helion charge radius from laser spectroscopy of muonic helium-3 ions

Hydrogen-like light muonic ions, in which one negative muon replaces all the electrons, are extremely sensitive probes of nuclear structure, because the large muon mass increases tremendously the wave function overlap with the nucleus. Using pulsed laser spectroscopy we have measured three 2S-2P transitions in the muonic helium-3 ion ($μ^3$He$^+$), an ion formed by a negative muon and bare helium-3 nucleus. This allowed us to extract the Lamb shift $E(2P_{1/2}-2S_{1/2})= 1258.598(48)^{\rm exp}(3)^{\rm theo}$ meV, the 2P fine structure splitting $E_{\rm FS}^{\rm exp} = 144.958(114)$ meV, and the 2S-hyperfine splitting (HFS) $E_{\rm HFS}^{\rm exp} = -166.495(104)^{\rm exp}(3)^{\rm theo}$ meV in $μ^3$He$^+$. Comparing these measurements to theory we determine the rms charge radius of the helion ($^3$He nucleus) to be $r_h$ = 1.97007(94) fm. This radius represents a benchmark for few nucleon theories and opens the way for precision tests in $^3$He atoms and $^3$He-ions. This radius is in good agreement with the value from elastic electron scattering, but a factor 15 more accurate. Combining our Lamb shift measurement with our earlier one in $μ^4$He$^+$ we obtain $r_h^2-r_α^2 = 1.0636(6)^{\rm exp}(30)^{\rm theo}$ fm$^2$ to be compared to results from the isotope shift measurements in regular He atoms, which are however affected by long-standing tensions. By comparing $E_{\rm HFS}^{\rm exp}$ with theory we also obtain the two-photon-exchange contribution (including higher orders) which is another important benchmark for ab-initio few-nucleon theories aiming at understanding the magnetic and current structure of light nuclei.

physics.atom-ph↗

arXiv2022

Absolute measurement of the relativistic magnetic dipole transition in He-like sulfur

We have made the first absolute, reference-free measurement of the 1s2s 3 S1 $\rightarrow$ 1s 2 1 S0 relativistic magnetic dipole transition in He-like sulfur. The highly-charged S ions were provided by an electron-cyclotron resonance ion source, and the x rays were analysed with a high-precision double crystal spectrometer. A transition energy of 2430.3685(97) eV was obtained, and is compared to most advanced bound state quantum electrodynamics calculations, providing an important test of two-electron QED effects and precision atomic structure methods in medium-Z species. Thanks to the extremely narrow natural linewidth of this transition, and to the large dispersion of the spectrometer at this energy, a complementary study was also performed evaluating the impact of different silicon crystal atomic form factor models in the transition energy analysis. We find no significant dependence on the model used to determine the transition energy.

physics.atom-ph↗

arXiv2022

Muonic-Atom Spectroscopy and Impact on Nuclear Structure and Precision QED Theory

Recent progress in laser and x-ray spectroscopy of muonic atoms offers promising long-term possibilities at the intersection of atomic, nuclear and particle physics. In muonic hydrogen, laser spectroscopy measurements will determine the ground-state hyperfine splitting (HFS) and additionally improve the Lamb shift by a factor of 5. Precision spectroscopy with cryogenic microcalorimeters has the potential to significantly improve the charge radii of the light nuclei in the $Z=3-8$ range. Complementary progress in precision should be achieved on the theory of nucleon- and nuclear-structure effects. The impact of this muonic-atom spectroscopy program will be amplified by the upcoming results from H and He$^+$ spectroscopy, simple molecules such as HD$^+$ and Penning trap measurements. In this broader context, one can test ab-initio nuclear theories, bound-state QED for two- or three-body systems, and determine fundamental constants, such as the Rydberg ($R_\infty$) and the fine-structure ($α$) constants.

nucl-th↗

arXiv2022

Absolute Energy Measurements with Superconducting Transition-Edge Sensors for Muonic X-ray Spectroscopy at 44 keV

Superconducting transition-edge sensor (TES) microcalorimeters have great utility in x-ray applications owing to their high energy resolution, good collecting efficiency and the feasibility of being multiplexed into large arrays. In this work, we develop hard x-ray TESs to measure the absolute energies of muonic-argon ($μ$-Ar) transition lines around 44 keV and 20 keV. TESs with sidecar absorbers of different heat capacities were fabricated and characterized for their energy resolution and calibration uncertainty. We achieved ~ 1 eV absolute energy measurement accuracy at 44 keV, and < 12 eV energy resolution at 17.5 keV.

physics.ins-det↗