arXiv subjects

Paul M. Goldbart

Publications and source records attributed to Paul M. Goldbart.

At least 55 records · Page 3Linked to original sources

arXiv2009

Two-step stabilization of orbital order and the dynamical frustration of spin in the model charge-transfer insulator KCuF3

We report a combined experimental and theoretical study of KCuF3, which offers - because of this material's relatively simple lattice structure and valence configuration (d9, i.e., one hole in the d-shell) - a particularly clear view of the essential role of the orbital degree of freedom in governing the dynamical coupling between the spin and lattice degrees of freedom. We present Raman and x-ray scattering evidence that the phase behaviour of KCuF3 is dominated above the Neel temperature (T_N = 40 K) by coupled orbital/lattice fluctuations that are likely associated with rotations of the CuF6 octahedra, and we show that these orbital fluctuations are interrupted by a static structural distortion that occurs just above T_N. A detailed model of the orbital and magnetic phases of KCuF3 reveals that these orbital fluctuations - and the related frustration of in-plane spin-order-are associated with the presence of nearly degenerate low-energy spin-orbital states that are highly susceptible to thermal fluctuations over a wide range of temperatures. A striking implication of these results is that the ground state of KCuF3 at ambient pressure lies near a quantum critical point associated with an orbital/spin liquid phase that is obscured by emergent Neel ordering of the spins; this exotic liquid phase might be accessible via pressure studies.

cond-mat.str-el↗

arXiv2009

Critical velocity of a clean one-dimensional superconductor

We revisit the problem of the critical velocity of a clean one-dimensional superconductor. {\changed At the level of mean-field theory}, we find that the zero-temperature value of the critical velocity--the uniform velocity of the superfluid condensate at which the superconducting state becomes unstable--is a factor of $\sqrt{2}$ smaller than the Landau critical velocity. This is in contrast to a prior finding, which held that the critical velocity is equal to the Landau critical velocity. The smaller value of the critical velocity, which our analysis yields, is the result of a pre-emptive Clogston-Chandrasekhar--like discontinuous phase transition, and is an analog of the threshold value of the uniform exchange-field of a superconductor, previously investigated by Sarma and by Maki and Tsuneto. We also consider the impact of nonzero temperature, study critical currents, and examine metastability and its limits in the temperature versus flow-velocity phase diagram. In addition, we comment on the effects of electron scattering by impurities.

cond-mat.supr-con↗

arXiv2009

Approaching multichannel Kondo physics using correlated bosons: Quantum phases and how to realize them

We discuss how multichannel Kondo physics can arise in the setting of a localized level coupled to several bosonic Tomonaga-Luttinger liquid leads. We propose one physical realization involving ultracold bosonic atoms coupled to an atomic quantum dot, and a second, based on superconducting nanowires coupled to a Cooper-pair box. The corresponding zero-temperature phase diagram is determined via an interplay between Kondo-type phenomena arising from the dot and the consequences of direct inter-lead hopping, which can suppress the Kondo effect. We demonstrate that the multichannel Kondo state is stable over a wide range of parameters. We establish the existence of two nontrivial phase transitions, involving a competition between Kondo screening at the dot and strong correlations either within or between the leads (which respectively promote local number- and phase-pinning). These transitions coalesce at a self-dual multicritical point.

cond-mat.mes-hall↗

arXiv2009

Stochastic dynamics of phase-slip trains and superconductive-resistive switching in current-biased nanowires

Superconducting nanowires fabricated via carbon-nanotube-templating can be used to realize and study quasi-one-dimensional superconductors. However, measurement of the linear resistance of these nanowires have been inconclusive in determining the low-temperature behavior of phase-slip fluctuations, both quantal and thermal. Thus, we are motivated to study the nonlinear current-voltage characteristics in current-biased nanowires and the stochastic dynamics of superconductive-resistive switching, as a way of probing phase-slip events. In particular, we address the question: Can a single phase-slip event occurring somewhere along the wire--during which the order-parameter fluctuates to zero--induce switching, via the local heating it causes? We explore this and related issues by constructing a stochastic model for the time-evolution of the temperature in a nanowire whose ends are maintained at a fixed temperature. We derive the corresponding master equation as tool for evaluating and analyzing the mean switching time at a given value of current. The model indicates that although, in general, several phase-slip events are necessary to induce switching via a thermal runaway, there is indeed a regime of temperatures and currents in which a single event is sufficient. We carry out a detailed comparison of the results of the model with experimental measurements of the distribution of switching currents, and provide an explanation for the counter-intuitive broadening of the distribution width that is observed upon lowering the temperature. Moreover, we identify a regime in which the experiments are probing individual phase-slip events, and thus offer a way for exploring the physics of nanoscale quantum tunneling of the superconducting order parameter.

cond-mat.supr-con↗

arXiv2009

Emergent superfluid crystals, frustration, and topologically defected states in multimode cavity QED

We propose that condensed matter phenomena involving the spontaneous emergence and dynamics of crystal lattices can be realized in the setting of ultracold Bose-condensed atoms coupled to multimode cavities. Previously, it was shown that in the case of a transversely pumped single-mode cavity, the atoms self-organize at either the even or the odd antinodes of the cavity mode, given sufficient pump intensity, and hence spontaneously break a discrete translational symmetry. Here, we demonstrate that in multimode cavities the self-organization brings the additional feature of continuous translational symmetry breaking, via a variant of Brazovskii's transition, thus paving the way for realizations of compliant lattices and associated phenomena, e.g., quantum melting, topological defects, frustration, glassiness, and even supersolidity; such phenomena are absent in ultracold atomic systems when the optical lattices are externally imposed. We apply a functional integral approach to this many-body cavity QED system, which enables us, inter alia, to calculate transition thresholds, explore fluctuations near this transition, and determine how such fluctuations are manifest in the light emitted from the cavity.

cond-mat.other↗

arXiv2008

Quantized vortices and superflow in arbitrary dimensions: Structure, energetics and dynamics

The structure and energetics of superflow around quantized vortices, and the motion inherited by these vortices from this superflow, are explored in the general setting of the superfluidity of helium-four in arbitrary dimensions. The vortices may be idealized as objects of co-dimension two, such as one-dimensional loops and two-dimensional closed surfaces, respectively, in the cases of three- and four-dimensional superfluidity. By using the analogy between vorticial superflow and Ampere-Maxwell magnetostatics, the equilibrium superflow containing any specified collection of vortices is constructed. The energy of the superflow is found to take on a simple form for vortices that are smooth and asymptotically large, compared with the vortex core size. The motion of vortices is analyzed in general, as well as for the special cases of hyper-spherical and weakly distorted hyper-planar vortices. In all dimensions, vortex motion reflects vortex geometry. In dimension four and higher, this includes not only extrinsic but also intrinsic aspects of the vortex shape, which enter via the first and second fundamental forms of classical geometry. For hyper-spherical vortices, which generalize the vortex rings of three dimensional superfluidity, the energy-momentum relation is determined. Simple scaling arguments recover the essential features of these results, up to numerical and logarithmic factors.

cond-mat.stat-mech↗

arXiv2008

Probing individual topological tunnelling events of a quantum field via their macroscopic consequences

Phase slips are topological fluctuation events that carry the superconducting order-parameter field between distinct current carrying states. Owing to these phase slips low-dimensional superconductors acquire electrical resistance. In quasi-one-dimensional nanowires it is well known that at higher temperatures phase slips occur via the process of thermal barrier-crossing by the order-parameter field. At low temperatures, the general expectation is that phase slips should proceed via quantum tunnelling events, which are known as quantum phase slips (QPS). Here we report strong evidence for individual quantum tunnelling events undergone by the superconducting order-parameter field in homogeneous nanowires.We accomplish this via measurements of the distribution of switching currents-the high-bias currents at which superconductivity gives way to resistive behaviour-whose width exhibits a rather counter-intuitive, monotonic increase with decreasing temperature. We outline a stochastic model of phase slip kinetics which relates the basic phase slip rates to switching rates. Comparison with this model indicates that the phase predominantly slips via thermal activation at high temperatures but at sufficiently low temperatures switching is caused by individual topological tunnelling events of the order-parameter field, i.e., QPS. Importantly, measurements on several wires show that quantum fluctuations tend to dominate over thermal fluctuations at larger temperatures in wires having larger critical currents. This fact provides strong supports the view that the anomalously high switching rates observed at low temperatures are indeed due to QPS, and not consequences of extraneous noise or hidden inhomogeneity of the wire.

cond-mat.supr-con↗

arXiv2008

Emergence of $h/e$-period oscillations in the critical temperature of small superconducting rings threaded by magnetic flux

As a function of the magnetic flux threading the object, the Little-Parks oscillation in the critical temperature of a large-radius, thin-walled superconducting ring or hollow cylinder has a period given by $h/2e$, due to the binding of electrons into Cooper pairs. On the other hand, the single-electron Aharonov-Bohm oscillation in the resistance or persistent current for a clean (i.e. ballistic) normal-state system having the same topological structure has a period given by $h/e$. A basic question is whether the Little-Parks oscillation changes its character, as the radius of the superconducting structure becomes smaller, and even comparable to the zero-temperature coherence length. We supplement the argument that the $h/e$ oscillations should also be exhibited via a microscopic analysis of this regime, formulated in terms of the Gor'kov approach of BCS theory. We see that as the radius of the ring becomes smaller, an oscillation of critical temperature in the period of $h/e$ emerges in addition to the usual Little-Parks dependence. We argue that in the clean limit there is a superconductor-normal transition, at nonzero flux, as the ring radius becomes sufficiently small, and that the transition can be either continuous or discontinuous, depending on the radius and the external flux. In the dirty limit, we argue that the transition is rendered continuous, which results in continuous quantum phase transitions tuned by flux and radius.

cond-mat.supr-con↗

arXiv2007

Local superfluid densities probed via current-induced superconducting phase gradients

We have developed a superconducting phase gradiometer consisting of two parallel DNA-templated nanowires connecting two thin-film leads. We have ramped the cross current flowing perpendicular to the nanowires, and observed oscillations in the lead-to-lead resistance due to cross-current-induced phase differences. By using this gradiometer we have measured the temperature and magnetic field dependence of the superfluid density and observed an amplification of phase gradients caused by elastic vortex displacements. We examine our data in light of Miller-Bardeen theory of dirty superconductors and a microscale version of Campbell's model of field penetration.

cond-mat.supr-con↗

arXiv2007

Inherent stochasticity of superconductive-resistive switching in nanowires

Hysteresis in the current-voltage characteristic in a superconducting nanowire reflects an underlying bistability. As the current is ramped up repeatedly, the state switches from a superconductive to a resistive one, doing so at random current values below the equilibrium critical current. Can a single phase-slip event somewhere along the wire--during which the order-parameter fluctuates to zero--induce such switching, via the local heating it causes? We address this and related issues by constructing a stochastic model for the time-evolution of the temperature in a nanowire whose ends are maintained at a fixed temperature. The model indicates that although, in general, several phase-slip events are necessary to induce switching, there is indeed a temperature- and current-range for which a single event is sufficient. It also indicates that the statistical distribution of switching currents initially broadens, as the temperature is reduced. Only at lower temperatures does this distribution show the narrowing with cooling naively expected for resistive fluctuations consisting of phase slips that are thermally activated.

cond-mat.supr-con↗

arXiv2006

Elastic heterogeneity of soft random solids

Spatial heterogeneity in the elastic properties of soft random solids is investigated via a two-pronged approach. First, a nonlocal phenomenological model for the elastic free energy is examined. This features a quenched random kernel, which induces randomness in the residual stress and Lame coefficients. Second, a semi-microscopic model network is explored using replica statistical mechanics. The Goldstone fluctuations of the semi-microscopic model are shown to reproduce the phenomenological model, and via this correspondence the statistical properties of the residual stress and Lame coefficients are inferred. Correlations involving the residual stress are found to be long-ranged and governed by a universal parameter that also gives the mean shear modulus.

cond-mat.dis-nn↗

arXiv2006

Thermal Fluctuations and Rubber Elasticity

The effects of thermal elastic fluctuations in rubber materials are examined. It is shown that, due to an interplay with the incompressibility constraint, these fluctuations qualitatively modify the large-deformation stress-strain relation, compared to that of classical rubber elasticity. To leading order, this mechanism provides a simple and generic explanation for the peak structure of Mooney-Rivlin stress-strain relation, and shows a good agreement with experiments. It also leads to the prediction of a phonon correlation function that depends on the external deformation.

cond-mat.soft↗

arXiv2006

Elasticity of highly cross-linked random networks

Starting from a microscopic model of randomly cross-linked particles with quenched disorder, we calculate the Laudau-Wilson free energy S for arbitrary cross-link densities. Considering pure shear deformations, S takes the form of the elastic energy of an isotropic amorphous solid state, from which the shear modulus can be identified. It is found to be an universal quantity, not depending on any microscopic length-scales of the model.

cond-mat.soft↗

arXiv2006

Phase-slip avalanches in the superflow of $^4$He through arrays of nanopores

Recent experiments by Sato et al. [1] have explored the dynamics of $^4$He superflow through an array of nanopores. These experiments have found that, as the temperature is lowered, phase-slippage in the pores changes its character, from synchronous to asynchronous. Inspired by these experiments, we construct a model to address the characteristics of phase-slippage in superflow through nanopore arrays. We focus on the low-temperature regime, in which the current-phase relation for a single pore is linear, and thermal fluctuations may be neglected. Our model incorporates two basic ingredients: (1) each pore has its own random value of critical velocity (due, e.g., to atomic-scale imperfections), and (2) an effective inter-pore coupling, mediated through the bulk superfluid. The inter-pore coupling tends to cause neighbours of a pore that has already phase-slipped also to phase-slip; this process may cascade, creating an avalanche of synchronously slipping phases. As the temperature is lowered, the distribution of critical velocities is expected to effectively broaden, owing to the reduction in the superfluid healing length, leading to a loss of synchronicity in phase-slippage. Furthermore, we find that competition between the strength of the disorder in the critical velocities and the strength of the inter-pore interaction leads to a phase transition between non-avalanching and avalanching regimes of phase-slippage. [1] Sato, Y., Hoskinson, E. Packard, R. E. cond-mat/0605660.

cond-mat.supr-con↗

arXiv2005

Universal point contact resistance between thin-film superconductors

A system comprising two superconducting thin films connected by a point contact is considered. The contact resistance is calculated as a function of temperature and film geometry, and is found to vanish rapidly with temperature, according to a universal, nearly activated form, becoming strictly zero only at zero temperature. At the lowest temperatures, the activation barrier is set primarily by the superfluid stiffness in the films, and displays only a weak (i.e., logarithmic) temperature dependence. The Josephson effect is thus destroyed, albeit only weakly, as a consequence of the power-law-correlated superconducting fluctuations present in the films below the Berezinskii-Kosterlitz-Thouless transition temperature. The behavior of the resistance is discussed, both in various limiting regimes and as it crosses over between these regimes. Details are presented of a minimal model of the films and the contact, and of the calculation of the resistance. A formulation in terms of quantum phase-slip events is employed, which is natural and effective in the limit of a good contact. However, it is also shown to be effective even when the contact is poor and is, indeed, indispensable, as the system always behaves as if it were in the good-contact limit at low enough temperature. A simple mechanical analogy is introduced to provide some heuristic understanding of the nearly-activated temperature dependence of the resistance. Prospects for experimental tests of the predicted behavior are discussed, and numerical estimates relevant to anticipated experimental settings are provided.

cond-mat.supr-con↗

arXiv2005

Enhancing superconductivity: Magnetic impurities and their quenching by magnetic fields

Magnetic fields and magnetic impurities are each known to suppress superconductivity. However, as the field quenches (i.e. polarizes) the impurities, rich consequences, including field-enhanced superconductivity, can emerge when both effects are present. For the case of superconducting wires and thin films, this field-spin interplay is investigated via the Eilenberger-Usadel scheme. Non-monotonic dependence of the critical current on the field (and therefore field-enhanced superconductivity) is found to be possible, even in parameter regimes in which the critical temperature decreases monotonically with increasing field. The present work complements that of Kharitonov and Feigel'man, which predicts non-monotonic behavior of the critical temperature.

cond-mat.supr-con↗

arXiv2005

Glassy correlations and microstructures in randomly crosslinked homopolymer blends

We consider a microscopic model of a polymer blend that is prone to phase separation. Permanent crosslinks are introduced between randomly chosen pairs of monomers, drawn from the Deam-Edwards distribution. Thereby, not only density but also concentration fluctuations of the melt are quenched-in in the gel state, which emerges upon sufficient crosslinking. We derive a Landau expansion in terms of the order parameters for gelation and phase separation, and analyze it on the mean-field level, including Gaussian fluctuations. The mixed gel is characterized by thermal as well as time-persistent (glassy) concentration fluctuations. Whereas the former are independent of the preparation state, the latter reflect the concentration fluctuations at the instant of crosslinking, provided the mesh size is smaller than the correlation length of phase separation. The mixed gel becomes unstable to microphase separation upon lowering the temperature in the gel phase. Whereas the length scale of microphase separation is given by the mesh size, at least close to the transition, the emergent microstructure depends on the composition and compressibility of the melt. Hexagonal structures, as well as lamellae or random structures with a unique wavelength, can be energetically favorable.

cond-mat.soft↗

arXiv2005

Squeezing superfluid from a stone: Coupling superfluidity and elasticity in a supersolid

In this work we start from the assumption that normal solid to supersolid (NS-SS) phase transition is continuous, and develop a phenomenological Landau theory of the transition in which superfluidity is coupled to the elasticity of the crystalline $^4$He lattice. We find that the elasticity does not affect the universal properties of the superfluid transition, so that in an unstressed crystal the well-known $λ$-anomaly in the heat capacity of the superfluid transition should also appear at the NS-SS transition. We also find that the onset of supersolidity leads to anomalies in the elastic constants near the transition; conversely, inhomogeneous strains in the lattice can induce local variations of the superfluid transition temperature, leading to a broadened transition.

cond-mat.soft↗