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Paul Stevenson

Publications and source records attributed to Paul Stevenson.

At least 19 recordsLinked to original sources

Nanoscale imaging of ferromagnetic vortex dynamics with scanning NV magnetometry

The generation and manipulation of spin waves at the nanoscale via magnetic vortices are of considerable importance because of their broad applications across magnonic and quantum technologies. Previously, fixed nitrogen-vacancy (NV) centers in diamond have been used to locally characterize vortex dynamics, and scanning NV magnetometry (SNVM) has been used to image vortices' static stray fields. Here, we demonstrate SNVM imaging of both the static and microwave fields generated by vortices in mesoscopic permalloy structures with $\sim$50 nm spatial resolution, achieving excellent agreement with micromagnetic simulations, while revealing the effects of disorder. We further demonstrate a 40$\times$ microwave field enhancement near a vortex core and image the disorder-dependent, spatially varying, evanescent decay of these microwaves. Our ambient, tabletop technique surpasses diffraction-limited techniques' resolutions by at least 5$\times$, with far greater accessibility and throughput than synchrotron radiation-based techniques, offering new opportunities in the study and development of magnonic devices.

cond-mat.mes-hall

Fault-tolerant quantum algorithms for simulating atomic nuclei

To maximize the value of fault-tolerant quantum computers, it is essential to develop concrete applications beyond well-established domains such as chemistry and condensed-matter physics. Here we construct and compile quantum algorithms to simulate the structure of atomic nuclei -- a topic that has received relatively little attention from the quantum computing community despite its similarities to the electronic structure problem in chemistry -- via effective shell-model Hamiltonians and no-core-shell-model Hamiltonians with three-body interactions derived from chiral effective field theory. Furthermore, we provide quantum resource estimates, in terms of Toffoli gate and qubit counts, for these algorithms, which, to our knowledge, are the first such estimates for fault-tolerant quantum simulation of atomic nuclei. Notably, the estimates for $^{32}$Mg and $^{219}$At shell-model Hamiltonians are comparable to recent estimates of Femoco simulations, a standard benchmark in chemistry. For no-core-shell-model Hamiltonians suitable for light nuclei (up to $^{40}$Ca or so), we find that resource requirements are significantly higher, suggesting that more bespoke strategies are required to make such simulations practicable. Throughout this work, we draw upon the similarities between nuclear and electronic structure problems, while also highlighting challenges that are specific to the former. We hope this work will spur long-term collaborations between the nuclear and quantum computing community with the ultimate goal of realizing useful nuclear simulations on quantum computers.

quant-ph

Qubit-efficient variational algorithm for nuclear structure

In this work, we compare three qubit-mapping strategies to study the structure of the nuclear ground state within the shell model description employing the Variational Quantum Eigensolver (VQE) approach. Although the initial point for different mappings is a Hamiltonian matrix in many-body particle basis or Slater determinant (SD) basis, the structure of the trial wavefunction and resource counts are different for each mapping. These three mappings are tested for a mid $p$-shell nucleus $^{10}$B and compared the quantum resources required to find the ground state for each mapping. Further, we extend the qubit-efficient mapping to study the ground state of one more mid $p$-shell nucleus $^{12}$C. We run circuits up to 26-qubits representing their ground states on a noisy simulator (IBM's FakeFez backend) and quantum hardware ($ibm\_fez$). The best post-error mitigated results from the hardware for $^{10}$B ground state is obtained following SD to qubit mapping with a percent error of 0.21 \%. The percent errors for the same state following cSD and pnSD mapping are 3.37 and 8.88 \%, respectively. On the other hand, following the cSD mapping, the post-error mitigated ground state energy of $^{12}$C is 6.82 \% away from the exact result. We further evaluate the fidelity of the VQE wavefunctions obtained from hardware with respect to the shell model wavefunctions for the cSD mapping. This cSD mapping can be useful for scaling the VQE algorithm for complex nuclei across different mass regions in terms of qubit efficiency.

nucl-th

Low $T$-count preparation of nuclear eigenstates with tensor networks

We present an efficient protocol leveraging classical computation to support Initial State Preparation for strongly correlated fermionic systems, a critical bottleneck for fault-tolerant quantum simulation. Focusing on nuclear shell model eigenstates, we first demonstrate that the Density Matrix Renormalization Group algorithm can efficiently approximate target states as Matrix Product States, capitalizing on the favourable entanglement structure of these fermionic systems. These high-fidelity approximations are then leveraged as a classical resource in a variational circuit optimization scheme to compile shallow quantum circuits. We establish concrete resource estimates by decomposing the resulting circuits into the industry-standard Clifford$+T$ gateset, exploring the benefits of specialized $U3$ synthesis techniques. For all nuclear systems tested, on up to 76 qubit Hamiltonians, we consistently find low $T$-count circuits preparing the nuclear eigenstates to high fidelity with $\sim 2\times 10^4$ total $T$ gates. This low number gives confidence these eigenstates can be prepared on early fault-tolerant quantum computers. Our work establishes a viable path toward practical ground state preparation for nuclear structure and other fermionic applications.

quant-ph

The role of the surface energy in nuclear octupole excitations

Octupole excitations of atomic nuclei can be viewed as fluctuations around an equilibrium shape. These fluctuations in turn can be seen as probes of nuclear matter properties to the extent that the shape changes explore changes in compression, surface to volume ratio, or isospin overlap. In the present work we use a series of Skyrme interactions, which were fitted to provide a systematic range of surface energies, to explore the surface energy dependence of octupole excitations in $^{208}$Pb. We find a strong positive linear corelation between the surface energy of a Skyrme interaction and its prediction of the first $3^-$ octupole excitation energy.

nucl-th

Topological textures and emergent altermagnetic signatures in ultrathin BiFeO3

Magnetoelectric multiferroics, materials with intrinsically coupled electric polarization and magnetic order, promise ultralow-power switching, nonvolatile memory, and energy-efficient signal transduction. Yet practical deployment demands ultrathin films down to the atomic limit, where both orders typically degrade. Maintaining both order parameters at the thinnest scales in complex oxides remains a tremendous challenge, as uncompensated bound charge drives nanoscale depolarization in most ferroelectrics, while off-stoichiometry, reduced anisotropy, and charge transfer can produce magnetic dead layers in ultrathin oxides at substrate interfaces. Here, we realize a multiferroic phase of BiFeO3 that not only sustains both order parameters at room temperature with no dead layer but also exhibits signatures of emergent altermagnetism in the four-unit-cell, ultrathin limit. First-principles calculations, spin symmetry analysis, atomic-resolution imaging, and angle-resolved magnetic imaging reveal that short-circuit electrostatic boundary conditions, together with epitaxial strain, drive a continuous second-order, thickness-driven phase transition that enables the formation of multiferroic topological textures. Moreover, the imposed boundary conditions stabilize a d-wave altermagnetic time-reversal symmetry breaking, with corresponding signatures observed in magnetic circular dichroism. Collectively, these results establish a pathway to stabilize unconventional multiferroicity at device-relevant thicknesses, reframing scaling limits for oxide electronics.

cond-mat.mtrl-sci

Single-step Quantum Simulation of Two Nucleons

Quantum computing offers a scalable approach to solving the nuclear shell model, a highly complex and exponentially scaled many-body problem. This work presents a numerical simulation of the subspace search variational quantum eigensolver (SSVQE) combined with an adaptive derivative-assembles pseudo-trotter (ADAPT) ansatz to obtain the low-lying states of any nuclear system in a single optimization run. As an example, we apply this method in this work to a trivial identical nucleon system, two nucleons in the $0p_{3/2}$ orbital, mapped to 4 qubits depicting m-scheme single-particle states including a surface delta effective interaction using the Jordan-Wigner transformation. The ADAPT-SSVQE algorithm, by utilizing a symmetry-preserving double-excitation ADAPT operator pool, uniquely optimizes a weighted energy sum, forcing the simultaneous convergence of two lowest states within the total angular momentum $M_J=0$ subspace. We demonstrate the accuracy of the method by benchmarking against the exact diagonalization, confirming its potential for probing nuclear structure and pairing phenomena on current and near-future quantum devices without requiring multi-step procedure for excited states.

nucl-th

From Classical to Quantum Machine Learning: Different Approaches in Fission Barrier Height Estimation

The fission barrier energy is a fundamental property of nuclear structure that governs the stability of nuclei against fission, directly affecting their spontaneous fission half-lives and the formation of superheavy elements. However, because it can only be measured indirectly, it also enables the emergence of alternative, complementary, fast, and accurate prediction tools for traditional theoretical models. In this study, we examine the use of classical, hybrid, and quantum support vector regression (SVR) approaches to estimate fission barrier heights, starting from fundamental nuclear properties and their derived additional properties. For this purpose, eight different SVR-based approaches are considered: (i) Classical SVR, (ii) Enhanced Classical SVR with polynomial and trigonometric feature extensions, (iii) Quantum-Inspired SVR, (iv) Hybrid SVR, (v) Enhanced Hybrid SVR, (vi) Quantum Core SVR, (vii) Fixed-Parameter Quantum Feature Map SVR, and (viii) Pure Quantum SVR. The models were trained and tested on a dataset of 317 isotopes in the Z (atomic number) range of 98-126, encompassing the actinide and superheavy regions. The model performance was evaluated in terms of R2, RMSE, MAE, and training-test R2 gap. The results show that the hybrid model achieves the best overall performance. However, while quantum-enhanced approaches are still limited by circuit depth and optimization precision, they achieve competitive accuracy comparable to classical results. Considering future developments in quantum hardware and algorithms, quantum approaches are expected to achieve considerable improvements. The findings suggest that quantum machine learning can supplement classical approaches and offer a promising path toward more accurate and efficient nuclear property predictions.

nucl-th

Efficient Radiofrequency Sensing with Fluorescence Encoding

Optically-active spin qubits have emerged as powerful quantum sensors capable of nanoscale magnetometry, yet conventional coherent sensing approaches are ultimately limited by the coherence time of the sensor, typically precluding detection in the sub-MHz regime. We present a broadly applicable fluorescence-encoding method that circumvents coherence-time constraints by transducing time-varying magnetic fields directly into modulated fluorescence signals. Using nitrogen-vacancy centers in diamond as a model system, we demonstrate shot-noise-limited sensitivity for AC magnetic fields spanning near-DC to MHz frequencies, with detection bandwidth tunable via optical excitation power. The technique captures complete spectral information in a single measurement, eliminating the need for point-by-point frequency scanning, and allows phase-sensitive multi-frequency detection with Hz-level resolution. This approach transforms quantum sensors into atomic-scale spectrum analyzers, with immediate applications for low-frequency RF communication, zero-field NMR, and bioelectronic sensing. Our approach is broadly applicable to the expanding class of optically-active spin qubits, including molecular systems and fluorescent proteins, opening new sensing regimes previously inaccessible to coherent techniques

quant-ph

A low-circuit-depth quantum computing approach to the nuclear shell model

In this work, we introduce a new qubit mapping strategy for the Variational Quantum Eigensolver (VQE) applied to nuclear shell model calculations, where each Slater determinant (SD) is mapped to a qubit, rather than assigning qubits to individual single-particle states. While this approach may increase the total number of qubits required in some cases, it enables the construction of simpler quantum circuits that are more compatible with current noisy intermediate-scale quantum (NISQ) devices. We apply this method to seven nuclei: Four lithium isotopes $^{6-9}$Li from the \textit{p}-shell, $^{18}$F from the \textit{sd}-shell, and two heavier nuclei ($^{210}$Po, and $^{210}$Pb). We run circuits representing their ground states on a noisy simulator (IBM's \textit{FakeFez} backend) and quantum hardware ($ibm\_pittsburgh$). For heavier nuclei, we demonstrate the feasibility of simulating $^{210}$Po and $^{210}$Pb as 22- and 29-qubit systems, respectively. Additionally, we employ Zero-Noise Extrapolation (ZNE) via two-qubit gate folding to mitigate errors in both simulated and hardware-executed results. Post-mitigation, the best results show less than 4 \% deviation from shell model predictions across all nuclei studied. This SD-based qubit mapping proves particularly effective for lighter nuclei and two-nucleon systems, offering a promising route for near-term quantum simulations in nuclear physics.

nucl-th

Low-energy domain wall racetracks with multiferroic topologies

Conventional racetrack memories move information by pushing magnetic domain walls or other spin textures with spin-polarized currents, but the accompanying Joule heating inflates their energy budget and can hamper scaling. Here we present a voltage-controlled, magnetoelectric racetrack in which transverse electric fields translate coupled ferroelectric-antiferromagnetic walls along BiFeO3 nanostrips at room temperature. Because no charge traverses the track, the switching dissipates orders of magnitude less energy than the most efficient spin-torque devices with more favourable scaling, making the scheme significantly more attractive at the nanoscale. We further uncover noncollinear topological magnetoelectric textures that emerge at domain walls in BiFeO3, where the nature of these topologies influences their stability upon translation. Among these are polar bi-merons and polar vertices magnetoelectrically coupled with magnetic cycloid disclinations and previously unobserved, topological magnetic cycloid twist topologies. We observe domain wall velocities of at least kilometres per second - matching or surpassing the fastest ferrimagnetic and antiferromagnetic racetracks and approaching the acoustic-phonon limit of BiFeO3 - while preserving these topologies over tens of micrometres. The resulting high velocity, low-energy racetrack delivers nanosecond access times without the thermal overhead of current-driven schemes, charting a path toward dense, ultralow-power racetrack devices which rely on spin texture translation.

cond-mat.mtrl-sci

Quantum Dynamical Microscopic Approach to Stellar Carbon Burning

The process of carbon burning is vital to understanding late stage stellar evolution of massive stars and the conditions of certain supernovae. Carbon burning is a complex problem, involving quantum tunnelling and nuclear molecular states. Quantum dynamical calculations of carbon burning are presented, combining the time-dependent wave-packet method and the density-constrained time-dependent Hartree-Fock (DC-TDHF) approach. By limiting the contribution of triaxial molecular configurations to fusion, we demonstrate that the DC-TDHF interaction potential successfully explains the appearance of some resonant structures in the sub-barrier fusion cross-section. This result shows the critical role of nucleon-nucleon interactions in the 12C + 12C fusion resonances observed at astrophysical energies.

nucl-th

Signatures of Non-Abelian Kitaev quantum spin liquids in noise magnetormetry

Identification of isolated Majorana zero modes (MZMs) is a key step towards the realization of fault-tolerant topological quantum computation. Here we show how the $T_1$-based noise magnetormetry of a nitrogen-vacancy (NV) center qubit can reveal the unique signatures of Majorana fermions attached to vacancies in a non-Abelian Kitaev quantum spin liquid (KQSL). The $1/T_1$ of the NV center is found to be increased significantly when the working frequency of the NV center matches the energy difference between a MZM and a low-energy hybridized mode involving dangling Majorana fermions adjacent to vacancies. In experiments, this energy difference can be tuned by an external Zeeman field. Because of the large excitation gap of flipping a local $Z_2$ gauge field, the $1/T_1$ spectrum is robust against other fluctuations in KQSLs. Our study presents a promising pathway for identifying the non-Abelian phase in Kitaev materials.

cond-mat.str-el

Flux channeling induced nano-confinement and enhancement of microwaves imaged by Rabi oscillation mapping

With rapid advances in qubit technologies, techniques for localizing, modulating, and measuring RF fields and their impact on qubit performance are of the utmost importance. Here, we demonstrate that flux-channeling from a permalloy nanowire can be used to achieve localized spatial modulation of an RF field and that the modulated field can be mapped with high resolution using the Rabi oscillations of an NV center. Rabi maps reveal ~100 mm wavelength microwaves concentrated in sub-300 nm-scale regions with up to ~16$\times$ power enhancement. This modulation is robust over a 20 dBm power range and has no adverse impact on NV $T_2$ coherence time. Micromagnetic simulations confirm that the modulated field results from the nanowire's stray field through its constructive/destructive interference with the incident RF field. Our findings provide a new pathway for controlling qubits, amplifying RF signals, and mapping local fields in various on-chip RF technologies.

cond-mat.mes-hall

Epitaxial Strain Tuning of Er3+ in Ferroelectric Thin Films

Er3+ color centers are promising candidates for quantum science and technology due to their long electron and nuclear spin coherence times, as well as their desirable emission wavelength. By selecting host materials with suitable, controllable properties, we introduce new parameters that can be used to tailor the Er3+ emission spectrum. PbTiO3 is a well-studied ferroelectric material with known methods of engineering different domain configurations through epitaxial strain. By distorting the structure of Er3+-doped PbTiO3 thin films, we can manipulate the crystal fields around the Er3+ dopant. This is resolved through changes in the Er3+ resonant fluorescence spectra, tying the optical properties of the defect directly to the domain configurations of the ferroelectic matrix. Additionally, we are able to resolve a second set of peaks for films with in-plane ferroelectric polarization. We hypothesize these results to be due to either the Er3+ substituting different sites of the PbTiO3 crystal, differences in charges between the Er3+ dopant and the original substituent ion, or selection rules. Systematically studying the relationship between the Er3+ emission and the epitaxial strain of the ferroelectric matrix lays the pathway for future optical studies of spin manipulation by altering ferroelectric order parameters

cond-mat.mtrl-sci

Morphogenesis of Spin Cycloids in a Non-collinear Antiferromagnet

Pattern formation in spin systems with continuous-rotational symmetry (CRS) provides a powerful platform to study emergent complex magnetic phases and topological defects in condensed-matter physics. However, its understanding and correlation with unconventional magnetic order along with high-resolution nanoscale imaging is challenging. Here, we employ scanning NV magnetometry to unveil the morphogenesis of spin cycloids at both the local and global scales within a single ferroelectric domain of (111)-oriented BiFeO$_3$ (which is a non-collinear antiferromagnet), resulting in formation of a glassy labyrinthine pattern. We find that the domains of locally oriented cycloids are interconnected by an array of topological defects and exhibit isotropic energy landscape predicted by first-principles calculations. We propose that the CRS of spin-cycloid propagation directions within the (111) drives the formation of the labyrinthine pattern and the associated topological defects such as antiferromagnetic skyrmions. Unexpectedly, reversing the as-grown ferroelectric polarization from [$\bar{1}$$\bar{1}$$\bar{1}$] to [111] induces a magnetic phase transition, destroying the labyrinthine pattern and producing a deterministic non-volatile non cycloidal, uniformly magnetized state. These findings highlight that (111)-oriented BiFeO$_3$ is not only important for studying the fascinating subject of pattern formation but could also be utilized as an ideal platform for integrating novel topological defects in the field of antiferromagnetic spintronics.

cond-mat.mtrl-sci

A Quantum Diophantine Equation Solution Finder

Diophantine equations are multivariate equations, usually polynomial, in which only integer solutions are admitted. A brute force method for finding solutions would be to systematically substitute possible integer solutions and check for equality. Grover's algorithm is a quantum search algorithm which can find marked indices in a list very efficiently. By treating the indices as the integer variables in the diophantine equation, Grover's algorithm can be used to find solutions in brute force way more efficiently than classical methods. We present an example for the simplest possible diophantine equation.

math.NT

Selective temperature sensing in nanodiamonds using dressed states

Temperature sensing at the nanoscale is a significant experimental challenge. Here, we report an approach using dressed states to make a leading quantum sensor (the nitrogen vacancy (NV) center in diamond) selectively sensitive to temperature, even in the presence of normally-confounding magnetic fields. Using an experimentally straightforward approach, we are able to suppress the magnetic sensitivity of the NV center by a factor of seven while retaining full temperature sensitivity and narrowing the NV center linewidth. These results demonstrate the power of engineering the sensor Hamiltonian using external control fields to enable sensing with improved specificity to target signals.

cond-mat.mes-hall