arXiv subjects

Pavel E. Dolgirev

Publications and source records attributed to Pavel E. Dolgirev.

At least 37 records · Page 2Linked to original sources

arXiv2022

Efficient variational approach to the Fermi polaron problem in two dimensions, both in and out of equilibrium

We develop a non-Gaussian variational approach that enables us to study both equilibrium and far-from-equilibrium physics of the two-dimensional Fermi polaron. This method provides an unbiased analysis of the polaron-to-molecule phase transition without relying on truncations in the total number of particle-hole excitations. Our results -- which include the ground state energy and quasiparticle residue -- are in qualitative agreement with the known Monte Carlo calculations. The main advantage of the non-Gaussian states compared to conventional numerical methods is that they enable us to explore long-time polaron evolution and, in particular, study various spectral properties accessible to both solid-state and ultracold atom experiments. We design two types of radiofrequency spectroscopies to measure polaronic and molecular spectral functions. Depending on the parameter regime, we find that these spectral functions and fermionic density profiles near the impurity display either long-lived oscillations between the repulsive and attractive polaron branches or exhibit fast relaxational dynamics to the molecular state.

cond-mat.quant-gas↗

arXiv2022

Optically-induced Umklapp shift currents in striped cuprates

Motivated by recent experiments that observed low-frequency second-order optical responses in doped striped superconductors, here we investigate the nonlinear electrodynamics of systems exhibiting a charge density wave (CDW) order parameter. Due to the Bragg scattering off the CDW order, an incoming spatially homogeneous electric field in addition to zero momentum current generates Umklapp currents that are modulated in space at momenta of the reciprocal CDW lattice. In particular, here we predict and microscopically evaluate the Umklapp shift current, a finite momentum analog of the regular shift current which represents the second-order optical process that downconverts homogeneous AC electric field into low-frequency, zero momentum current. Specifically, we evaluate real-time response functions within mean-field theory via the Keldysh technique and use the Peierls substitution to compute observables at finite momenta in lattice models. We find that systems with certain lattice symmetries (such as inversion symmetry), where the regular shift current is disallowed, may give rise to the Umklapp one. We apply our framework to investigate lattice symmetries in layered materials with helical-like stripes and show that both types of shift currents provide insight into the nature of intertwined phases of matter. Finally, we discuss the relation of our findings to recent experiments in striped superconductors.

cond-mat.str-el↗

arXiv2022

Periodic dynamics in superconductors induced by an impulsive optical quench

A number of experiments have evidenced signatures of enhanced superconducting correlations after photoexcitation. Initially, these experiments were interpreted as resulting from quasi-static changes in the Hamiltonian parameters, for example, due to lattice deformations or melting of competing phases. Yet, several recent observations indicate that these conjectures are either incorrect or do not capture all the observed phenomena, which include reflectivity exceeding unity, large shifts of Josephson plasmon edges, and appearance of new peaks in terahertz reflectivity. These observations can be explained from the perspective of a Floquet theory involving a periodic drive of system parameters, but the origin of the underlying oscillations remains unclear. In this paper, we demonstrate that following incoherent photoexcitation, long-lived oscillations are generally expected in superconductors with low-energy Josephson plasmons, such as in cuprates or fullerene superconductor K$_3$C$_{60}$. These oscillations arise from the parametric generation of plasmon pairs due to pump-induced perturbation of the superconducting order parameter. We show that this bi-plasmon response can persist even above the transition temperature as long as strong superconducting fluctuations are present. Our analysis offers a robust framework to understand light-induced superconducting behavior, and the predicted bi-plasmon oscillations can be directly detected using available experimental techniques.

cond-mat.supr-con↗

arXiv2022

Characterizing two-dimensional superconductivity via nanoscale noise magnetometry with single-spin qubits

We propose nanoscale magnetometry via isolated single-spin qubits as a probe of superconductivity in two-dimensional materials. We characterize the magnetic field noise at the qubit location, arising from current and spin fluctuations in the sample and leading to measurable polarization decay of the qubit. We show that the noise due to transverse current fluctuations studied as a function of temperature and sample-probe distance can be used to extract useful information about the transition to a superconducting phase and the pairing symmetry of the superconductor. Surprisingly, at low temperatures, the dominant contribution to the magnetic noise arises from longitudinal current fluctuations and can be used to probe collective modes such as monolayer plasmons and bilayer Josephson plasmons. We also characterize the noise due to spin fluctuations, which allows probing the spin structure of the pairing wave function. Our results provide a non-invasive route to probe the rich physics of two-dimensional superconductors.

cond-mat.supr-con↗

arXiv2022

Single-spin qubit magnetic spectroscopy of two dimensional superconductivity

A single-spin qubit placed near the surface of a conductor acquires an additional contribution to its $1/T_1$ relaxation rate due to magnetic noise created by electric current fluctuations in the material. We analyze this technique as a wireless probe of superconductivity in atomically thin two dimensional materials. At temperatures $T \lesssim T_c$, the dominant contribution to the qubit relaxation rate is due to transverse electric current fluctuations arising from quasiparticle excitations. We demonstrate that this method enables detection of metal-to-superconductor transitions, as well as investigation of the symmetry of the superconducting gap function, through the noise scaling with temperature. We show that scaling of the noise with sample-probe distance provides a window into the non-local quasi-static conductivity of superconductors, both clean and disordered. At low temperatures the quasiparticle fluctuations get suppressed, yet the noise can be substantial due to resonant contributions from collective longitudinal modes, such as plasmons in monolayers and Josephson plasmons in bilayers. Potential experimental implications are discussed.

cond-mat.supr-con↗

arXiv2021

Role of equilibrium fluctuations in light-induced order

Engineering novel states of matter with light is at the forefront of materials research. An intensely studied direction is to realize broken-symmetry phases that are "hidden" under equilibrium conditions but can be unleashed by an ultrashort laser pulse. Despite a plethora of experimental discoveries, the nature of these orders and how they transiently appear remain unclear. To this end, we investigate a nonequilibrium charge density wave (CDW) in rare-earth tritellurides, which is suppressed in equilibrium but emerges after photoexcitation. Using a pump-pump-probe protocol implemented in ultrafast electron diffraction, we demonstrate that the light-induced CDW consists solely of order parameter fluctuations, which bear striking similarities to critical fluctuations in equilibrium despite differences in the length scale. By calculating the dynamics of CDW fluctuations in a nonperturbative model, we further show that the strength of the light-induced order is governed by the amplitude of equilibrium fluctuations. These findings highlight photoinduced fluctuations as an important ingredient for the emergence of transient orders out of equilibrium. Our results further suggest that materials with strong fluctuations in equilibrium are promising platforms to host "hidden" orders after laser excitation.

cond-mat.mtrl-sci↗

arXiv2021

Emergence of a sharp quantum collective mode in a one-dimensional Fermi polaron

The Fermi-polaron problem of a mobile impurity interacting with fermionic medium emerges in various contexts, ranging from the foundations of Landau's Fermi-liquid theory to electron-exciton interaction in semiconductors, to unusual properties of high-temperature superconductors. While classically the medium provides only a dissipative environment to the impurity, quantum picture of polaronic dressing is more intricate and arises from the interplay of few- and many-body aspects of the problem. The conventional expectation for the dynamics of Fermi polarons is that it is dissipative in character, and any excess energy is rapidly emitted away from the impurity as particle-hole excitations. Here we report a strikingly different type of polaron dynamics in a one-dimensional system of the impurity interacting repulsively with the fermions. When the total momentum of the system equals the Fermi momentum, there emerges a sharp collective mode corresponding to long-lived oscillations of the polaronic cloud surrounding the impurity. This mode can be observed experimentally with ultracold atoms using Ramsey interferometry and radio-frequency spectroscopy.

cond-mat.quant-gas↗

arXiv2020

Non-Gaussian correlations imprinted by local dephasing in fermionic wires

We study the behavior of an extended fermionic wire coupled to a local stochastic field. Since the quantum jump operator is Hermitian and quadratic in fermionic operators, it renders the model soluble, allowing investigation of the properties of the non-equilibrium steady-state and the role of dissipation-induced fluctuations. We derive a closed set of equations of motion solely for the two-point correlator; on the other hand, we find, surprisingly, that the many-body state exhibits non-Gaussian correlations. Density-density correlation function demonstrates a crossover from a regime of weak dissipation characterized by moderate heating and stimulated fluctuations to a quantum Zeno regime ruled by strong dissipation, which tames quantum fluctuations. Instances of soluble dissipative impurities represent an experimentally viable platform to understand the interplay between dissipation and Hamiltonian dynamics in many-body quantum systems.

cond-mat.quant-gas↗

arXiv2020

Self-similar dynamics of order parameter fluctuations in pump-probe experiments

Upon excitation by a laser pulse, broken-symmetry phases of a wide variety of solids demonstrate similar order parameter dynamics characterized by a dramatic slowing down of relaxation for stronger pump fluences. Motivated by this recurrent phenomenology, we develop a simple non-perturbative effective model of dynamics of collective bosonic excitations in pump-probe experiments. We find that as the system recovers after photoexcitation, it shows universal prethermalized dynamics manifesting a power-law, as opposed to exponential, relaxation, explaining the slowing down of the recovery process. For strong quenches, long-wavelength over-populated transverse modes dominate the long-time dynamics; their distribution function exhibits universal scaling in time and space, whose universal exponents can be computed analytically. Our model offers a unifying description of order parameter fluctuations in a regime far from equilibrium, and our predictions can be tested with available time-resolved techniques.

cond-mat.other↗

arXiv2020

Amplitude dynamics of charge density wave in LaTe$_3$: theoretical description of pump-probe experiments

We formulate a dynamical model to describe a photo-induced charge density wave (CDW) quench transition and apply it to recent multi-probe experiments on LaTe$_3$ [A. Zong et al., Nat. Phys. 15, 27 (2019)]. Our approach relies on coupled time-dependent Ginzburg-Landau equations tracking two order parameters that represent the modulations of the electronic density and the ionic positions. We aim at describing the amplitude of the order parameters under the assumption that they are homogeneous in space. This description is supplemented by a three-temperature model, which treats separately the electronic temperature, temperature of the lattice phonons with stronger couplings to the electronic subsystem, and temperature of all other phonons. The broad scope of available data for LaTe$_3$ and similar materials as well as the synergy between different time-resolved spectroscopies allow us to extract model parameters. The resulting calculations are in good agreement with ultra-fast electron diffraction experiments, reproducing qualitative and quantitative features of the CDW amplitude evolution during the initial few picoseconds after photoexcitation.

cond-mat.mes-hall↗

arXiv2019

Phase-sensitive thermoelectricity and long-range Josephson effect supported by thermal gradient

We demonstrate that thermoelectric signal as well as dc Josephson current may be severely enhanced in multi-terminal superconducting hybrid nanostructures exposed to a temperature gradient. At temperatures $T$ strongly exceeding the Thouless energy of our device both the supercurrent and the thermo-induced voltage are dominated by the contribution from non-equilibrium low energy quasiparticles and are predicted to decay slowly (algebraically rather than exponentially) with increasing $T$. We also predict a non-trivial current-phase relation and a transition to a $π$-junction state controlled by both the temperature gradient and the system topology. All these features are simultaneously observable in the same experiment.

cond-mat.mes-hall↗

arXiv2019

Phase coherent electron transport in asymmetric cross-like Andreev interferometers

We present a detailed theoretical description of quantum coherent electron transport in voltage-biased cross-like Andreev interferometers. Making use of the charge conjugation symmetry encoded in the quasiclassical formalism, we elucidate a crucial role played by geometric and electron-hole asymmetries in these structures. We argue that a non-vanishing Aharonov-Bohm-like contribution to the current $I_S$ flowing in the superconducting contour may develop only in geometrically asymmetric interferometers making their behavior qualitatively different from that of symmetric devices. The current $I_N$ in the normal contour -- along with $I_S$ -- is found to be sensitive to phase-coherent effects thereby also acquiring a $2π$-periodic dependence on the Josephson phase. In asymmetric structures this current develops an odd-in-phase contribution originating from electron-hole asymmetry. We demonstrate that both phase dependent currents $I_S$ and $I_N$ can be controlled and manipulated by tuning the applied voltage, temperature and system topology, thus rendering Andreev interferometers particularly important for future applications in modern electronics.

cond-mat.supr-con↗

arXiv2019

Light-Induced Charge Density Wave in LaTe$_3$

When electrons in a solid are excited with light, they can alter the free energy landscape and access phases of matter that are beyond reach in thermal equilibrium. This accessibility becomes of vast importance in the presence of phase competition, when one state of matter is preferred over another by only a small energy scale that, in principle, is surmountable by light. Here, we study a layered compound, LaTe$_3$, where a small in-plane (a-c plane) lattice anisotropy results in a unidirectional charge density wave (CDW) along the c-axis. Using ultrafast electron diffraction, we find that after photoexcitation, the CDW along the c-axis is weakened and subsequently, a different competing CDW along the a-axis emerges. The timescales characterizing the relaxation of this new CDW and the reestablishment of the original CDW are nearly identical, which points towards a strong competition between the two orders. The new density wave represents a transient non-equilibrium phase of matter with no equilibrium counterpart, and this study thus provides a framework for unleashing similar states of matter that are "trapped" under equilibrium conditions.

cond-mat.mtrl-sci↗

arXiv2019

Dynamical slowing down in an ultrafast photo-induced phase transition

Complex systems, which consist of a large number of interacting constituents, often exhibit universal behavior near a phase transition. A slowdown of certain dynamical observables is one such recurring feature found in a vast array of contexts. This phenomenon, known as critical slowing down, is well studied mostly in thermodynamic phase transitions. However, it is less understood in highly nonequilibrium settings, where the time it takes to traverse the phase boundary becomes comparable to the timescale of dynamical fluctuations. Using transient optical spectroscopy and femtosecond electron diffraction, we studied a photo-induced transition of a model charge-density-wave (CDW) compound, LaTe$_3$. We observed that it takes the longest time to suppress the order parameter at the threshold photoexcitation density, where the CDW transiently vanishes. This finding can be quantitatively captured by generalizing the time-dependent Landau theory to a system far from equilibrium. The experimental observation and theoretical understanding of dynamical slowing down may offer insight into other general principles behind nonequilibrium phase transitions in many-body systems.

cond-mat.str-el↗

arXiv2018

Topology-controlled thermopower oscillations in multiterminal Andreev interferometers

We theoretically investigate coherent oscillations of the thermopower $\mathcal{S}$ as a function of the magnetic flux $Φ$ in six-terminal Andreev interferometers. We demonstrate that the thermopower behavior is determined by a number of contributions originating from the Josephson-like and Aharonov-Bohm-like effects as well as from electron-hole asymmetry. The relative weight of these contributions depends on the relation between temperature, voltage bias and an effective Thouless energy of our setup. We particularly emphasize the role of the system topology that may have a dramatic impact on the behavior of $\mathcal{S}(Φ)$.

cond-mat.mes-hall↗

arXiv2018

Interplay between Josephson and Aharonov-Bohm effects in Andreev interferometers

Proximity induced quantum coherence of electrons in multi-terminal voltage-driven hybrid normal-superconducting nanostructures may result in a non-trivial interplay between topology-dependent Josephson and Aharonov-Bohm effects. We elucidate a trade-off between stimulation of the voltage-dependent Josephson current due to non-equilibrium effects and quantum dephasing of quasiparticles causing reduction of both Josephson and Aharonov-Bohm currents. We also predict phase-shifted quantum coherent oscillations of the induced electrostatic potential as a function of the externally applied magnetic flux. Our results may be employed for engineering superconducting nanocircuits with controlled quantum properties.

cond-mat.mes-hall↗

arXiv2018

Disentangling amplitude and phase dynamics of a charge density wave in a photo-induced phase transition

Upon excitation with an intense ultrafast laser pulse, a symmetry-broken ground state can undergo a non-equilibrium phase transition through pathways dissimilar from those in thermal equilibrium. Determining the mechanism underlying these photo-induced phase transitions (PIPTs) has been a long-standing issue in the study of condensed matter systems. To this end, we investigate the light-induced melting of a unidirectional charge density wave (CDW) material, LaTe$_3$. Using a suite of time-resolved probes, we independently track the amplitude and phase dynamics of the CDW. We find that a quick ($\sim\,$1$\,$ps) recovery of the CDW amplitude is followed by a slower reestablishment of phase coherence. This longer timescale is dictated by the presence of topological defects: long-range order (LRO) is inhibited and is only restored when the defects annihilate. Our results provide a framework for understanding other PIPTs by identifying the generation of defects as a governing mechanism.

cond-mat.mtrl-sci↗

arXiv2018

Current-phase relation and flux-dependent thermoelectricity in Andreev interferometers

We predict a novel $(I_0,ϕ_0)$-junction state of multi-terminal Andreev interferometers that emerges from an interplay between long-range quantum coherence and non-equilibrium effects. Under non-zero bias $V$ the current-phase relation $I_S(ϕ)$ resembles that of a $ϕ_0$-junction differing from the latter due to a non-zero average $I_0(V) = \left< I_S(ϕ)\right>_ϕ$. The flux-dependent thermopower ${\mathcal S}(Φ)$ of the system exhibits features similar to those of a $(I_0,ϕ_0)$-junction and in certain limits it can reduce to either odd or even function of $Φ$ in the agreement with a number of experimental observations.

cond-mat.supr-con↗