arXiv subjects

Pavlos G. Lagoudakis

Publications and source records attributed to Pavlos G. Lagoudakis.

At least 55 records · Page 3Linked to original sources

arXiv2020

Engineering spatial coherence in lattices of polariton condensates

Artificial lattices of coherently coupled macroscopic states are at the heart of applications ranging from solving hard combinatorial optimisation problems to simulating complex many-body physical systems. The size and complexity of the problems scales with the extent of coherence across the lattice. Although the fundamental limit of spatial coherence depends on the nature of the couplings and lattice parameters, it is usually engineering constrains that define the size of the system. Here, we engineer polariton condensate lattices with active control on the spatial arrangement and condensate density that result in near-diffraction limited emission, and spatial coherence that exceeds by nearly two orders of magnitude the size of each individual condensate. We utilise these advancements to unravel the dependence of spatial correlations between polariton condensates on the lattice geometry.

cond-mat.mes-hall↗

arXiv2020

Optical orientation, polarization pinning, and depolarization dynamics in optically confined polariton condensates

We investigate the optical orientation, polarization pinning, and depolarization of optically confined semiconductor exciton-polariton condensates. We perform a complete mapping of the condensate polarization as a function of incident nonresonant excitation polarization and power. We utilize a ring-shaped excitation pattern to generate an exciton-induced potential that spatially confines polariton condensates into a single mode. We observe that formation of circular polarization in the condensate persists even for a weakly cocircularly polarized pump. By varying the excitation ring diameter we realize a transition from the condensate polarization being pinned along the coordinate-dependent cavity-strain axes, to a regime of zero degree of condensate polarization. Analysis through the driven-dissipative stochastic Gross-Pitaevskii equation reveals that this depolarization stems from a competition between sample induced in-plane polarization splitting and the condensate-reservoir overlap. An increase in the role of the latter results in weakening of the condensate fixed-point phase space attractors, and enhanced random phase space walk and appearance of limit cycle trajectories, reducing the degree of time-integrated polarization.

cond-mat.mes-hall↗

arXiv2020

Coherence Revivals of a Spinor Polariton Condensate from Self-induced Larmor Precession

First order coherence measurements of a polariton condensate, reveal a regime where the condensate pseudo-spin precesses persistently within the driving optical pulse. Within a single 20 $μ$s optical pulse the condensate pseudo-spin performs over $10^5$ precessions with striking frequency stability. The condensate maintains its phase coherence even after a complete precession of the spin vector, making the observed state by a definition a spin coherent state. The emergence of the precession is traced to the polariton interactions that give rise to a self-induced out-of-plane magnetic field that in turn drives the spin dynamics. We find that the Larmor oscillation frequency scales with the condensate density, enabling external tuning of this effect by optical means. The stability of the system allows for the realization of integrated optical magnetometry devices with the use of materials with enhanced exciton $g$-factor and can facilitate spin squeezing effects and active coherent control on the Bloch sphere in polariton condensates.

cond-mat.mes-hall↗

arXiv2020

All-optical cascadable universal logic gate with sub-picosecond operation

Today, almost all information processing is performed using electronic logic circuits operating with up to several gigahertz frequency. All-optical logic, however, that holds the promise to allow up to three orders of magnitude higher speed [1] has not been able to provide a viable alternative because approaches that had been tried were either not scalable, not energy efficient or did not show a significant speed benefit. Whereas essential all-optical transistor functionalities have been already demonstrated across a range of platforms [2-4], using them to implement the complete Boolean logic gate set and in particular negation - switching off an optical signal with another optical signal - poses a major challenge [5]. Here, we realize a universal NOR logic gate by introducing the concept of non-ground-state dynamic exciton-polariton condensation in an organic semiconductor microcavity under non-resonant pulsed excitation. In the presence of either of the input signals inserted at opposite in-plane momenta, non-ground state dynamic condensation supersedes spontaneous ground-state condensation, resulting in a NOR-operator output signal within less than a picosecond. An additional optical transistor, fed by the output of the NOR gate, is then used to regenerate the output signal such that it is usable as input for cascading gates, a prerequisite for scale up. Our results constitute an essential step towards the realization of more complex logic optical circuitry that could boost future information processing applications.

physics.optics↗

arXiv2020

Time-Delay Polaritonics

Non-linearity and finite signal propagation speeds are omnipresent in nature, technologies, and real-world problems, where efficient ways of describing and predicting the effects of these elements are in high demand. Advances in engineering condensed matter systems, such as lattices of trapped condensates, have enabled studies on non-linear effects in many-body systems where exchange of particles between lattice nodes is effectively instantaneous. Here, we demonstrate a regime of macroscopic matter-wave systems, in which ballistically expanding condensates of microcavity exciton-polaritons act as picosecond, microscale non-linear oscillators subject to time-delayed interaction. The ease of optical control and readout of polariton condensates enables us to explore the phase space of two interacting condensates up to macroscopic distances highlighting its potential in extended configurations. We demonstrate deterministic tuning of the coupled-condensate system between fixed point and limit cycle regimes, which is fully reproduced by time-delayed coupled equations of motion similar to the Lang-Kobayashi equation.

cond-mat.mes-hall↗

arXiv2020

Synchronization in optically-trapped polariton Stuart-Landau networks

We demonstrate tunable dissipative interactions between optically trapped exciton-polariton condensates. We apply annular shaped nonresonant optical beams to both generate and confine each condensate to their respective traps, pinning their natural frequencies. Coupling between condensates is realized through the finite escape rate of coherent polaritons from the traps leading to robust phase locking with neighboring condensates. The coupling is controlled by adjusting the polariton propagation distance between neighbors. This permits us to map out regimes of both strong and weak dissipative coupling, with the former characterized by clear in-phase and anti-phase synchronization of the condensates. With robust single-energy occupation governed by dissipative coupling of optically-trapped polariton condensates, we present a system which offers a potential optical platform for the optimization of randomly connected $XY$ Hamiltonians.

cond-mat.mes-hall↗

arXiv2019

Giant increase of temporal coherence in optically trapped polariton condensate

Coherent bosonic ensembles offer the promise of harnessing quantum effects in photonic and quantum circuits. In the dynamic equilibrium regime, the application of polariton condensates is hindered by exciton-polariton scattering induced de-coherence in the presence of a dark exciton reservoir. By spatially separating the condensate from the reservoir, we drive the system into the weak interaction regime, where the ensemble coherence time exceeds the individual particle lifetime by nearly three orders of magnitude. The observed nanosecond coherence provides an upper limit for polariton self-interactions. In contrast to conventional photon lasers, we observe an increased contribution from the super-Poissonian component of the condensate to the overall particle number fluctuations. Coupled with the recent emergence of a quantum regime in polaritonics, coherence times extended to several nanoseconds favour the realization of quantum information protocols.

cond-mat.quant-gas↗

arXiv2019

High-energy optical transitions and optical constants of CH$_3$NH$_3$PbI$_3$ measured by spectroscopic ellipsometry and spectrophotometry

Optoelectronics based on metal halide perovskites (MHPs) have shown substantial promise, following more than a decade of research. For prime routes of commercialization such as tandem solar cells, optical modeling is essential for engineering device architectures, which requires accurate optical data for the materials utilized. Additionally, a comprehensive understanding of the fundamental material properties is vital for simulating the operation of devices for design purposes. In this article, we use variable angle spectroscopic ellipsometry (SE) to determine the optical constants of CH$_3$NH$_3$PbI$_3$ (MAPbI$_3$) thin films over a photon energy range of 0.73 to 6.45 eV. We successfully model the ellipsometric data using six Tauc-Lorentz oscillators for three different incident angles. Following this, we use critical-point analysis of the complex dielectric constant to identify the well-known transitions at 1.58, 2.49, 3.36 eV, but also additional transitions at 4.63 and 5.88 eV, which are observed in both SE and spectrophotometry measurements. This work provides important information relating to optical transitions and band structure of MAPbI$_3$, which can assist in the development of potential applications of the material.

physics.app-ph↗

arXiv2019

Optical control of synchronous phases in a programmable polariton cell

We demonstrate deterministic control of the nearest and next-nearest neighbor coupling in the unit cell of a square lattice of microcavity exciton-polariton condensates. We tune the coupling in a continuous and reversible manner by optically imprinting potential barriers of variable height, in the form of spatially localized incoherent exciton reservoirs that modify the particle flow between condensates. By controlling the couplings in a $2\times2$ polariton cluster, we realize ferromagnetic, anti-ferromagnetic and paired ferromagnetic phases. Our approach paves the way towards simulating complex condensed matter phases through precise control of the individual couplings in networks of optical nonlinear oscillators.

cond-mat.mes-hall↗

arXiv2019

On the origin of blueshifts in organic polariton condensates

We report on the origin of energy-shifts in organic polariton condensates. The localised nature of Frenkel excitons in molecular semiconductors precludes interparticle Coulomb exchange interactions -the latter being the dominant mechanism for blueshifts in inorganic semiconductor microcavities that bear Wannier-Mott excitons. We examine the contribution of optically induced change of the intracavity non-linear refractive index, gain induced frequency-pulling and quenching of the Rabi splitting, as well as the role of polariton-exciton and polariton-polariton scattering in the energy-shift of the polariton mode at condensation threshold in strongly coupled molecular dye microcavities. We conclude that blueshifts in organic polariton condensates arise from the interplay of the saturation of molecular optical transitions and intermolecular energy migration. Our model predicts the commonly observed step-wise increase of both the emission energy and degree of linear polarisation at polariton condensation threshold.

cond-mat.mes-hall↗

arXiv2018

Generation of Anti-Stokes Fluorescence in a Strongly Coupled Organic Semiconductor Microcavity

We explore the generation of anti-Stokes fluorescence from strongly coupled organic dye microcavities following resonant ground-state excitation. We observe polariton emission along the lower polariton branch, with our results indicating that this process involves a return to the exciton reservoir and the absorption of thermal energy from molecules in a vibrationally excited ground-state. We speculate that the generation of a population of "hot" polaritons is enhanced by the fact that the cavity supresses the emission of Stokes-shifted fluorescence, as it is located energetically below the cut-off frequency of the cavity.

cond-mat.mes-hall↗

arXiv2017

Matter wave coupling of spatially separated and unequally pumped polariton condensates

Spatial quantum coherence between two separated driven-dissipative polariton condensates created non-resonantly and with a different occupation is studied. We identify the regions where the condensates remain coherent with the phase difference continuously changing with the pumping imbalance and the regions where each condensate acquires its own chemical potential with phase differences exhibiting time-dependent oscillations. We show that in the mutual coherence limit the coupling consists of two competing contributions: a symmetric Heisenberg exchange and the Dzyloshinskii-Moriya asymmetric interactions that enable a continuous tuning of the phase relation across the dyad and derive analytic expressions for these types of interactions. The introduction of non-equal pumping increases the complexity of the type of the problems that can be solved by polariton condensates arranged in a graph configuration. If equally pumped polaritons condensates arrange their phases to solve the constrained quadratic minimisation problem with a real symmetric matrix, the non-equally pumped condensates solve that problem for a general Hermitian matrix.

cond-mat.mes-hall↗

arXiv2017

Exotic states of matter with polariton chains

We consider linear periodic chains of exciton-polariton condensates formed by pumping polaritons non-resonantly into a linear network. To the leading order, such a sequence of condensates establishes relative phases as to minimize a classical one-dimensional XY Hamiltonian with nearest and next to nearest neighbors. We show that the low energy states of polaritonic linear chains demonstrate various classical regimes: ferromagnetic, antiferromagnetic and frustrated spiral phases, where quantum or thermal fluctuations are expected to give rise to a spin liquid state. At the same time nonlinear interactions at higher pumping intensities bring about phase chaos and novel exotic phases.

cond-mat.mes-hall↗

arXiv2017

A Polariton Graph Simulator

We discuss polariton graphs as a new platform for simulating the classical XY and Kuramoto models. Polariton condensates can be imprinted into any two-dimensional graph by spatial modulation of the pumping laser. Polariton simulators have the potential to reach the global minimum of the XY Hamiltonian in a bottom-up approach by gradually increasing excitation density to the threshold or to study large-scale synchronisation phenomena and dynamical phase transitions when operating above the threshold. We consider the modelling of polariton graphs using the complex Ginzburg-Landau model and derive analytical solutions for a single condensate, the XY model, two-mode model and the Kuramoto model establishing the relationships between them.

cond-mat.other↗

arXiv2017

Simulating the spectral gap with polariton graphs

We recently proposed polariton graphs as a novel platform for solving hard optimization problems that can be mapped into the $XY$ model. Here, we elucidate a relationship between the energy spectrum of the $XY$ Hamiltonian and the total number of condensed polariton particles. Using as a test-bed the hexagonal unit lattice we show that the lower energy states of the $XY$ Hamiltonian are faithfully reproduced by mean-field numerical simulations utilising the Ginzburg--Landau equation coupled to an exciton reservoir. Our study paves the way to simulating the spectral gap of the XY model using polariton graphs.

cond-mat.other↗

arXiv2016

Realizing the $XY$ Hamiltonian in polariton simulators

Several platforms are currently being explored for simulating physical systems whose complexity increases faster than polynomially with the number of particles or degrees of freedom in the system. Defects and vacancies in semiconductors or dielectric materials, magnetic impurities embedded in solid helium \cite{lemeshko13}, atoms in optical lattices, photons, trapped ions and superconducting q-bits are among the candidates for predicting the behaviour of spin glasses, spin-liquids, and classical magnetism among other phenomena with practical technological applications. Here we investigate the potential of polariton graphs as an efficient simulator for finding the global minimum of the $XY$ Hamiltonian. By imprinting polariton condensate lattices of bespoke geometries we show that we can simulate a large variety of systems undergoing the U(1) symmetry breaking transitions. We realise various magnetic phases, such as ferromagnetic, anti-ferromagnetic, and frustrated spin configurations on unit cells of various lattices: square, triangular, linear and a disordered graph. Our results provide a route to study unconventional superfluids, spin-liquids, Berezinskii-Kosterlitz-Thouless phase transition, classical magnetism among the many systems that are described by the $XY$ Hamiltonian.

cond-mat.mes-hall↗

arXiv2016

Plasmon enhanced optical tweezers with gold-coated black silicon

Plasmonic optical tweezers are a ubiquitous tool for the precise manipulation of nanoparticles and biomolecules at low photon flux, while femtosecond-laser optical tweezers can probe the nonlinear optical properties of the trapped species with applications in biological diagnostics. In order to adopt plasmonic optical tweezers in real-world applications, it is essential to develop large-scale fabrication processes without compromising the trapping efficiency. Here, we develop a novel platform for continuous wave (CW) and femtosecond plasmonic optical tweezers, based on gold-coated black silicon. In contrast with traditional lithographic methods, the fabrication method relies on simple, single-step, maskless tabletop laser processing of silicon in water that facilitates scalability. Gold-coated black silicon supports repeatable trapping efficiencies comparable to the highest ones reported to date. From a more fundamental aspect, a plasmon-mediated efficiency enhancement is a resonant effect, and therefore, dependent on the wavelength of the trapping beam. Surprisingly, a wavelength characterization of plasmon-enhanced trapping efficiencies has evaded the literature. Here, we exploit the repeatability of the recorded trapping efficiency, offered by the gold-coated black silicon platform, and perform a wavelength-dependent characterization of the trapping process, revealing the resonant character of the trapping efficiency maxima. Gold-coated black silicon is a promising platform for large-scale parallel trapping applications that will broaden the range of optical manipulation in nanoengineering, biology, and the study of collective biophotonic effects.

physics.optics↗

arXiv2015

Near-field enhanced optical tweezers utilizing femtosecond-laser nanostructured substrates

We present experimental evidence of plasmonic-enhanced optical tweezers, of polystyrene beads in deionized water in the vicinity of metal-coated nanostructures. The optical tweezers operate with a continuous wave (CW) near-infrared laser. We employ a Cu/Au bilayer that significantly improves dissipation of heat generated by the trapping laser beam and avoid de-trapping from heat convection currents. We investigate the improvement of the optical trapping force, the effective trapping quality factor, and observe an exponential distance dependence of the trapping force from the nanostructures, expected from the evanescent plasmon field.

physics.optics↗