arXiv subjects

Paweł Wójcik

Publications and source records attributed to Paweł Wójcik.

At least 19 recordsLinked to original sources

arXiv2026

Strong-coupling multigap superconductivity in the Heusler compound ScAu$_2$Al

ScAu$_2$Al is the Heusler superconductor with the highest reported transition temperature, Tc, close to 5 K. Here, we combine high-resolution ac calorimetry and electrical-transport measurements with first-principles-based Eliashberg calculations. The large specific-heat jump, $ΔC/{γ_nT_c} =$ 2.2, well above the weak-coupling BCS value of 1.43, together with an electron-phonon coupling constant $λ = $1.1, establishes ScAu2Al as a strong-coupling superconductor. The electronic specific heat is described better by a two-gap α model, with $2Δ_S/k_BT_c = $ 4.1 and $2Δ_L/k_BT_c = $ 4.8, than by a single-gap model. The thermodynamic upper critical field follows a conventional WHH-like temperature dependence with $B_{c2}(0) = 0.18$ T, whereas the resistively determined critical field reaches values about three times larger and exhibits a pronounced positive curvature. We attribute the enhanced resistive field scale to superconductivity in disordered grain-boundary and interfacial regions. The experimental results are supported by calculations of the heat capacity and upper critical field within the Eliashberg formalism using Fermi-surface and electron-phonon parameters obtained from first-principles calculations

cond-mat.supr-con↗

arXiv2026

Topological superconductivity of a two-dimensional electron gas at the (001) LaAlO\textsubscript{3}/SrTiO\textsubscript{3} interface

We investigate the emergence of topological superconductivity and Majorana zero modes in the two-dimensional electron gas formed at the LaAlO$_3$/SrTiO$_3$ (001) interface. Using a realistic multiband tight binding model that incorporates the $t_{2g}$ orbital structure together with atomic and Rashba spin-orbit couplings, we determine the topological phase diagrams for both fully two-dimensional and quasi-one-dimensional geometries. In the two-dimensional limit, we show that a finite out-of-plane magnetic-field component is required to drive a topological phase transition. In this case, the critical field is strongly band dependent, and for higher-lying bands, it is controlled by the interplay of spin and orbital Zeeman effects, as well as atomic spin-orbit coupling. Although a purely in-plane field is insufficient to induce the topological transition in a full 2D system, we demonstrate that a lateral confinement relaxes this constraint. In this case, the character of the edge modes depends sensitively on the field orientation, with out-of-plane fields producing conventional counterpropagating chiral modes and transverse in-plane fields giving rise to co-propagating antichiral modes. Finally, Majorana zero modes in LAO/STO nanowires with varying widths are analyzed. We demonstrate that subbands predominantly composed of $d_{yz/xz}$ orbitals exhibit exceptionally long localization lengths, which may preclude the observation of Majorana bound states in nanowires of typical experimental dimensions.

cond-mat.mes-hall↗

arXiv2025

Interplay between altermagnetism and superconductivity in two dimensions: intertwined symmetries and singlet-triplet mixing

We study the interplay between altermagnetism and unconventional superconductivity for the case of two-dimensional square- and triangular-lattice systems. Our approach is based on an effective single particle Hamiltonian which mimics the alternating spin splitting characteristic for the $d$-$wave$ and $i$-$wave$ altermagnetic state. By supplementing the model with intersite pairing term we characterize the principal features of the coexistent altermagnetic-superconducting state as well as the possibility of inducing the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase. Our calculations show that the subtle interplay between the symmetries of the superconducting and altermagnetic order parameters as well as the shape/size of the Fermi surface lead to various types of anisotropic behaviors of the resultant non-zero momentum pairing, which has not been possible in the originally proposed FFLO state. Moreover, in the considered systems additional pairing symmetries appear leading to an exotic multi-component order parameter with singlet-triplet mixing. To interpret the obtained data we analyze the Cooper pair density in the momentum space and the corresponding Fermi wave vector mismatch resulting from the altermagnetic spin splitting. We discuss our result in the context of possible applications like, e.g., the superconducting diode.

cond-mat.supr-con↗

arXiv2025

Broad nonlocal spectrum in the Pb-InSb hybrid three terminals for potential realization of Kitaev chains

Hybrid superconductor-semiconductor(SC-SM) nanowires remain one of the foremost platforms for engineering topological superconductivity and Majorana zero modes(MZMs) towards fault-tolerant topological qubits, especially with the rapid development of artificial Kitaev chains. In contrast to the widely used aluminum(Al)-based hybrids, lead(Pb) offers a bulk superconducting gap of ~1.4meV and a critical temperature of ~7.2K, giving rise to a proximity-induced gap that is roughly five times larger than that obtained with Al. Here we present the first three-terminal Pb-hybrid devices and perform nonlocal differential-conductance spectroscopy on this platform. The nonlocal measurement simultaneously resolves a dual-gap feature of the parent Pb gap and the large, hard, gate-tunable induced superconducting gap, distinguished by a switch between electron- and hole-like dissipation processes. Within the induced gap we observe several types of Andreev bound states(ABSs) that undergo singlet-doublet transitions. Moreover, by tuning gate voltages we achieve gate-controlled resonating sign reversals of the nonlocal conductance, identifying three distinct regimes that correspond to different configurations of quantum-dot(QD) resonances(single-resonance, double-resonance, and series-resonance). Finally, the coupling between ABSs and QDs also present and can be modulated from the weak- to strong-coupling limit, indicating the feasibility of realizing the artificial Kitaev chains. Crucially, the robust nonlocal signatures persist up to temperatures(~1K) far above the operating temperature of Al-based devices thanks to the unusually large induced gap, thereby widening the accessible parameter space greatly and underscoring the suitability of Pb-based hybrids for implementing warm temperature artificial Kitaev chains and the topological quantum devices protected by a substantially larger topological gap.

quant-ph↗

arXiv2025

Anisotropic, multiband, and strong-coupling superconductivity of the Pb0.64Bi0.36 alloy

This paper presents theoretical and experimental studies on the superconductivity of Pb${_{0.64}}$Bi$_{0.36}$ alloy, which is a prototype of strongly coupled superconductors and exhibits one of the strongest coupling under ambient pressure among the materials studied so far. The critical temperature, the specific heat in the superconducting state, and the magnetic critical fields are experimentally determined. Deviations from the single-gap s-wave BCS-like behavior are observed. The electronic structure, phonons and electron-phonon interactions are analyzed in relation to the metallic Pb, explaining why the Pb-Bi alloy exhibits such a large value of the electron-phonon coupling parameter $λ\simeq 2$. Superconductivity is studied using the isotropic Eliashberg formalism as well as the anisotropic density functional theory for superconductors. We find that while Pb is a two-gap superconductor with well-defined separate superconducting gaps, in the Pb-Bi alloy an overlapped three-gap-like structure is formed with a strong anisotropy. Furthermore, the chemical disorder, inherent to this alloy, leads to strong electron scattering, which is found to reduce the critical temperature.

cond-mat.supr-con↗

arXiv2025

Enhanced and modulable induced superconducting gap and effective Landé g-factor in Pb-InSb hybrid devices

The hybrid system of a conventional superconductor (SC) on a semiconductor (SM) nanowire with strong spin-orbit coupling (SOC) represents a promising platform for achieving topological superconductivity and Majorana zero modes (MZMs) towards topological quantum computation. While aluminum (Al)-based hybrid nanowire devices have been widely utilized, their limited superconducting gap and intrinsic weak SOC as well as small Landé g-factor may hinder future experimental advancements. In contrast, we demonstrate that lead (Pb)-based hybrid quantum devices exhibit a remarkably large and hard proximity-induced superconducting gap, exceeding that of Al by an order of magnitude. By exploiting electrostatic gating to modulate wavefunction distribution and SC-SM interfacial coupling, this gap can be continuously tuned from its maximum value (~1.4 meV, matching the bulk Pb gap) down to nearly zero while maintaining the hardness. Furthermore, magnetic-field-dependent measurements reveal a radial evolution of the gap structure with anti-crossing feature, indicative of strong SOC and huge effective g-factors up to 76. These findings underscore the superior functionality of Pb-based hybrid systems, significantly advancing their potential for realizing and stabilizing MZMs and the further scalable topological quantum architectures.

cond-mat.mes-hall↗

arXiv2024

InP/GaSb core-shell nanowires: a novel hole-based platform with strong spin-orbit coupling for full-shell hybrid devices

Full-shell hybrid nanowires (NWs), structures comprising a superconductor shell that encapsulates a semiconductor (SM) core, have attracted considerable attention in the search for Majorana zero modes (MZMs). However, the predicted Rashba spin-orbit coupling (SOC) in the SM is too small to achieve substantial topological minigaps. In addition, the SM wavefunction spreads all across the section of the nanowire, leading typically to a finite background of trivial subgap states with which MZMs may coexist. To overcome both problems, we explore the advantages of utilizing core-shell hole-band NWs as the SM part of a full-shell hybrid, with an insulating core and an active SM shell. In particular, we consider InP/GaSb core-shell NWs, which allow to exploit the unique characteristics of the III-V compound SM valence bands. We demonstrate that they exhibit a robust hole SOC that emerges from the combination of the intrinsic spin-orbit interaction of the SM active shell and the confinement effects of the nanostructure, thus depending mainly on SM and geometrical parameters. In other words, the SOC is intrinsic and does not rely on red electric fields, which are non-tunable in a full-shell hybrid geometry. As a result, core-shell SM hole-band NWs are found to be a promising candidate to explore Majorana physics in full-hell hybrid devices, addressing several challenges in the field.

cond-mat.mes-hall↗

arXiv2024

Versatile Method of Engineering the Band Alignment and the Electron Wavefunction Hybridization of Hybrid Quantum Devices

With the development of quantum technology, hybrid devices that combine superconductors (S) and semiconductors (Sm) have attracted great attention due to the possibility of engineering structures that benefit from the integration of the properties of both materials. However, until now, none of the experiments have reported good control of band alignment at the interface, which determines the strength of S-Sm coupling and the proximitized superconducting gap. Here, we fabricate hybrid devices in a generic way with argon milling to modify the interface while maintaining its high quality. First, after the milling the atomically connected S-Sm interfaces appear, resulting in a large induced gap, as well as the ballistic transport revealed by the multiple Andreev reflections and quantized above-gap conductance plateaus. Second, by comparing transport measurement with Schrödinger-Poisson (SP) calculations, we demonstrate that argon milling is capable of varying the band bending strength in the semiconducting wire as the electrons tend to accumulate on the etched surface for longer milling time. Finally, we perform nonlocal measurements on advanced devices to demonstrate the coexistence and tunability of crossed Andreev reflection (CAR) and elastic co-tunneling (ECT) -- key ingredients for building the prototype setup for realization of Kitaev chain and quantum entanglement probing. Such a versatile method, compatible with the standard fabrication process and accompanied by the well-controlled modification of the interface, will definitely boost the creation of more sophisticated hybrid devices for exploring physics in solid-state systems.

cond-mat.mes-hall↗

arXiv2024

Variational Monte-Carlo Approach for Hubbard Model Applied to Twisted Bilayer WSe$_2$ at Half-Filling

We consider an effective Hubbard model with spin- and direction-dependent complex hoppings $t$, applied to twisted homobilayer WSe$_2$ using a variational Monte Carlo approach. The electronic correlations are taken into account by applying the Gutzwiller on-site correlator as well as long-range Jastrow correlators subjected to noninteracting part being of Pfaffian form. Our analysis shows the emergence of Mott insulating state at critical value of Hubbard interaction $U_{c1}\approx 6.5|t|\div7|t|$ estimated by extrapolating the density-density equal-time two-particle Green's functions. The signatures of an intermediate insulating phase between $U_{c1}$ and $U_{c2}\approx9.5|t|\div10|t|$ are also discussed. Furthermore, we report the formation of the $120^{\circ}$ in-plane Néel state indicated by the detailed analysis of the spin-spin correlation functions. As shown, switching between antiferromagnetic phases characterized by opposite chirality could be experimentally realized by the change of perpendicular electric field. In proper range of electric fields also a transition to in-plane ferromagnetic state appears.

cond-mat.str-el↗

arXiv2023

Honeycomb anti-dot artificial lattice as a prototypical correlated Dirac fermions system

We study theoretically the electronic properties of the artificial quantum dot honeycomb lattice defined in a two-dimensional electron gas, focusing on the possibility of achieving a regime in which electronic correlations play a dominant role. At first we establish a non-interacting model compatible with recently studied experimentally devices. According to the values of the obtained electron-electron interaction integrals, we postulate that the inclusion of inherent electron-gas self-screening is indispensable to reconstruct the experimental observations. Applying the Thomas-Fermi type of screening, we show that the radius of the anti-dot is crucial to achieve a correlated state in which phenomena like antiferromagentic ordering and interaction-induced insulating state appear. We estimate the conditions for which the electronically correlated state in an artificial honeycomb lattice can be realized.

cond-mat.str-el↗

arXiv2022

Pressure effects on the electronic structure, phonons, and superconductivity of noncentrosymmetric ThCoC2

The electronic structure, phonons, electron-phonon coupling, and superconductivity are theoretically studied in noncentrosymmetric superconductor ThCoC$_2$ as a function of pressure, in the pressure range 0 - 20 GPa. We found that the electronic band splitting induced by the spin-orbit coupling is enhanced under pressure. In spite of the overall stiffening of the crystal lattice, the electron-phonon coupling constant $λ$ increases with pressure, from 0.583 at 0 GPa to 0.652 at 20 GPa. If the isotropic Eliashberg electron-phonon coupling theory is used to simulate the effect on the critical temperature $T_c$, such an increase in $λ$ results in a substantial increase of $T_c$ from 2.5~K at 0 GPa to 4~K at 20 GPa. This shows that examining the effect of pressure offers a chance to resolve the pairing mechanism in ThCoC$_2$.

cond-mat.supr-con↗

arXiv2022

An orthogonality relation in complex normed spaces based on norm derivatives

Let $X$ be a complex normed space. Based on the right norm derivative $ρ_{_{+}}$, we define a mapping $ρ_{_{\infty}}$ by \begin{equation*} ρ_{_{\infty}}(x,y) = \frac1π\int_0^{2π}e^{iθ}ρ_{_{+}}(x,e^{iθ}y)dθ\quad(x,y\in X). \end{equation*} The mapping $ρ_{_{\infty}}$ has a good response to some geometrical properties of $X$. For instance, we prove that $ρ_{_{\infty}}(x,y)=ρ_{_{\infty}}(y,x)$ for all $x, y \in X$ if and only if $X$ is an inner product space. In addition, we define a $ρ_{_{\infty}}$-orthogonality in $X$ and show that a linear mapping preserving $ρ_{_{\infty}}$-orthogonality has to be a scalar multiple of an isometry. A number of challenging problems in the geometry of complex normed spaces are also discussed.

math.FA↗

arXiv2022

On non-linear mappings preserving the semi-inner product

We say that a smooth normed space $X$ has a property (SL), if every mapping $f:X \to X$ preserving the semi-inner product on $X$ is linear. It is well known that every Hilbert space has the property (SL) and the same is true for every finite-dimensional smooth normed space. In this paper, we establish several new results concerning the property (SL). We give a simple example of a smooth and strictly convex Banach space which is isomorphic to the space $\ell_p$, but without the property (SL). Moreover, we provide a characterization of the property (SL) in the class of reflexive smooth Banach spaces in terms of subspaces of quotient spaces. As a consequence, we prove that the space $\ell_p$ have the property (SL) for every $1 < p < \infty$. Finally, using a variant of the Gowers-Maurey space, we construct an infinite-dimensional uniformly smooth Banach space $X$ such that every smooth Banach space isomorphic to $X$ has the property (SL).

math.FA↗

arXiv2021

Electronic structure, electron-phonon coupling and superconductivity in noncentrosymmetric ThCoC2 from ab initio calculations

Superconductors without inversion symmetry in their crystal structure are known to exhibit unconventional properties. Recently, based on the measured temperature dependence of the magnetic field penetration depth, superconductivity in noncentrosymmetric $\mathrm{ThCoC_2}$ was proposed to be a nodal $d$-wave and mediated by the spin fluctuations. Moreover, a non-BCS behavior of the temperature dependence of the electronic specific heat and the magnetic upper critical field were reported. In this work, the electronic structure, phonons and electron-phonon coupling are studied in $\mathrm{ThCoC_2}$ on the basis of \textit{ab initio} computations. The effect of the spin-orbit coupling on the electronic structure and electron-phonon interaction is analyzed, and a large splitting of the electronic band structure is found. The calculated electron-phonon coupling constant $λ= 0.59$ remains in decent agreement with the experimental estimates, suggesting that the electron-phonon interaction is strong enough to explain superconductivity with $T_c \simeq 2.5$~K. Nevertheless, we show that the conventional isotropic Eliashberg formalism is unable to describe the thermodynamic properties of the superconducting state, as calculated temperature dependence of the electronic specific heat and magnetic penetration depth deviate from experiments, which is likely driven by the strong spin-orbit coupling and inversion symmetry breaking. In addition, to shed more light on the pairing mechanism, we propose to measure the carbon isotope effect, as our calculations based on the electron-phonon coupling predict the observation of the isotope effect with an exponent $α\simeq 0.15$.

cond-mat.supr-con↗

arXiv2021

Strong-coupling superconductivity of SrIr2 and SrRh2: Phonon engineering of metallic Ir and Rh

Experimental and theoretical studies on superconductivity in SrIr$_2$ and SrRh$_2$ Laves phases are presented. The measured resistivity, heat capacity, and magnetic susceptibility confirm the superconductivity of these compounds with $T_c$ = 6.07 K and 5.41 K, respectively. Electronic structure calculations show that the Fermi surface is mostly contributed by 5$d$ (4$d$) electrons of Ir (Rh), with Sr atoms playing the role of electron donors. The effect of the spin-orbit coupling is analyzed and found to be important in both materials. Lattice dynamics and electron-phonon coupling (EPC) are studied and the strong electron-phonon interaction is found, contributed mostly by the low-frequency Ir and Rh vibrations. The enhancement of EPC when compared to weakly-coupled metallic Ir and Rh is explained by the strong modifications in the propagation of phonons in the network of Ir (Rh) tetrahedrons, which are the building blocks of the Laves phase, and originate from the metallic fcc structures of elemental iridium and rhodium.

cond-mat.supr-con↗

arXiv2019

Symmetry-Breaking Topological Insulators in the $\mathbb{Z}_2$ Bose-Hubbard Model

In this work, we study a one-dimensional model of interacting bosons coupled to a dynamical $\mathbb{Z}_2$ field, the $\mathbb{Z}_2$ Bose-Hubbard model, and analyze the interplay between spontaneous symmetry breaking and topological symmetry protection. In a previous work, we showed how this model exhibits a spontaneous breaking of the translational symmetry through a bosonic Peierls transition. Here we find how, at half filling, the resulting phase also displays topological features that coexist with the presence of long-range order and yields a topological bond order wave. Using both analytical and numerical methods, we describe the properties of this phase, showing that it cannot be adiabatically connected to a bosonic topological phase with vanishing Hubbard interactions, and thus constitutes an instance of an interaction-induced symmetry-breaking topological insulator.

cond-mat.quant-gas↗

arXiv2019

Interactions of benzene, naphthalene, and azulene with alkali-metal and alkaline-earth-metal atoms for ultracold studies

We consider collisional properties of polyatomic aromatic hydrocarbon molecules immersed into ultracold atomic gases and investigate intermolecular interactions of exemplary benzene, naphthalene, and azulene with alkali-metal (Li, Na, K, Rb, Cs) and alkaline-earth-metal (Mg, Ca, Sr, Ba) atoms. We apply the state-of-the-art \textit{ab initio} techniques to compute the potential energy surfaces (PESs). We use the coupled cluster method restricted to single, double, and noniterative triple excitations to reproduce the correlation energy and the small-core energy-consistent pseudopotentials to model the scalar relativistic effects in heavier metal atoms. We also report the leading long-range isotropic and anisotropic dispersion and induction interaction coefficients. The PESs are characterized in detail and the nature of intermolecular interactions is analyzed and benchmarked using symmetry-adapted perturbation theory. The full three-dimensional PESs are provided for selected systems within the atom-bond pairwise additive representation and can be employed in scattering calculations. Presented study of the electronic structure is the first step towards the evaluation of prospects for sympathetic cooling of polyatomic aromatic molecules with ultracold atoms. We suggest azulene, an isomer of naphthalene which possesses a significant permanent electric dipole moment and optical transitions in the visible range, as a promising candidate for electric field manipulation and buffer-gas or sympathetic cooling.

physics.chem-ph↗

arXiv2018

Approximately angle preserving mappings

In this paper, we present some characterizations of linear mappings, which preserve vectors at a specific angle. We introduce the concept of $(\varepsilon, c)$-angle preserving mappings for $|c|<1$ and $0\leq \varepsilon < 1 + |c|$. In addition, we define $\widehat{\varepsilon}\,(T, c)$ as the ``smallest'' number $\varepsilon$ for which $T$ is $(\varepsilon, c)$-angle preserving mapping. We state some properties of the function $\widehat{\varepsilon}\,(., c)$, and then propose an exact formula for $\widehat{\varepsilon}\,(T, c)$ in terms of the norm $\|T\|$ and the minimum modulus $[T]$ of $T$. Finally, we characterize the approximately angle preserving mappings.

math.FA↗