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Peijie Sun

Publications and source records attributed to Peijie Sun.

At least 19 recordsLinked to original sources

SG-UMP: Sequence-Guided Universal Multimodal Prioritization Calculation Framework

Multimodal sequential recommendation (MSR) improves recommendation by incorporating heterogeneous information such as text, images, and user interactions. However, existing MSR methods often fail to capture user-level preference heterogeneity and dataset-level modality bias, limiting their adaptability across users and datasets. To address this issue, we propose \textbf{S}equence-\textbf{G}uided \textbf{U}niversal \textbf{M}ultimodal \textbf{P}rioritization Calculation Framework (\textbf{SG-UMP}), a plug-and-play plugin for enhancing multimodal information processing in MSR. SG-UMP includes a Module Combiner for flexible multimodal processing and a Module Router for dynamic module ordering, enabling adaptation to both user preferences and dataset characteristics. Experiments on four real-world datasets show that SG-UMP consistently improves recommendation performance across different backbones and multimodal settings. The code is available at https://github.com/esemsc-xz524/SG-UMP .

cs.IR

Giant magnetocaloric effect at low fields in triangular-lattice NdMgAl$_{11}$O$_{19}$

Magnetic refrigeration in the sub-Kelvin regime requires refrigerant materials to retain a large magnetic entropy at low temperatures by suppressing magnetic ordering. Quantum spin liquids (QSLs), which evade long-range magnetic ordering while retaining strong quantum fluctuations to the lowest temperatures, therefore provide a promising platform for realizing high-performance magnetic refrigerants. Here, we investigate the magnetic ground state and the magnetocaloric effect of the hexaaluminate, NdMgAl$_{11}$O$_{19}$, in which the Nd$^{3+}$ ions form a network of triangular lattices. Magnetic susceptibility and specific heat measurements indicate a magnetically dynamic state down to 50~mK, consistent with a QSL state. Specific heat measurements further reveal substantial magnetic entropy retained below 50~mK. Quasi-adiabatic demagnetization measurements demonstrate a superior cooling performance of NdMgAl$_{11}$O$_{19}$, which can be cooled to 113~mK from 1.9~K by only a small magnetic field change of 2~T. The outstanding refrigeration performance is attributed to the persistent spin fluctuations associated with the QSL-like ground state, together with a large effective \textit{g} factor and the smallness of the exchange interactions along the easy-axis direction. This study demonstrates that frustration, combined with strong spin-orbit coupling and crystal-electric-field effect in the rare earth magnets provides a promising design principle for next-generation cryogenic magnetic refrigerants.

cond-mat.str-el

Ising Supercriticality and Universal Magnetocalorics in Spiral Antiferromagnet Nd$_3$BWO$_9$

The celebrated analogy between the pressure-temperature phase diagram of a liquid-gas system and the field-temperature phase diagram of a ferromagnet has long been a cornerstone for understanding universality of phase transitions and critical phenomena. Here we extend this analogy to a highly frustrated antiferromagnet, the spiral Ising compound Nd$_3$BWO$_9$ with kagome layers. In its phase diagram, we identify a metamagnetic transition line with a critical endpoint (CEP) located at $μ_0H_{\mathrm{c}} \simeq 1.04$ T and $T_{\mathrm{c}} \simeq 0.3$ K. Above the CEP, an Ising supercritical regime emerges with crossover lines that follow a universal scaling law, as evidenced by the specific heat, magnetic susceptibility, and magnetocaloric measurements. Remarkably, we observe highly sensitive magnetic cooling near the emergent CEP, characterized by a divergent magnetic Grüneisen ratio $Γ_H \propto 1/t^{β+γ-1}$, with $β+ γ\simeq 1.563$ the sum of critical exponents of the 3D Ising universality class and $t \equiv (T-T_{\rm c})/T_{\rm c}$ the reduced temperature. Adiabatic demagnetization from 2 K and 4 T reaches a minimum temperature of 195 mK, via a self-cascading process that combines supercritical and topological cooling. Our findings open a new avenue for studying supercritical phenomena and magnetic refrigeration with the frustrated rare-earth compounds RE$_3$BWO$_9$ and, more broadly, in Ising-anisotropic antiferromagnets such as spin ices.

cond-mat.str-el

Safety Anchor: Defending Harmful Fine-tuning via Geometric Bottlenecks

The safety alignment of Large Language Models (LLMs) remains vulnerable to Harmful Fine-tuning (HFT). While existing defenses impose constraints on parameters, gradients, or internal representations, we observe that they can be effectively circumvented under persistent HFT. Our analysis traces this failure to the inherent redundancy of the high-dimensional parameter space: attackers exploit optimization trajectories that are orthogonal to defense constraints to restore harmful capabilities while deceptively adhering to safety restrictions. To address this, we propose Safety Bottleneck Regularization (SBR). SBR shifts the defensive focus from the redundant parameter space to the unembedding layer, which serves as a geometric bottleneck. By anchoring the final hidden states of harmful queries to those of the safety-aligned model, SBR enables the model to maintain safe responses even under persistent HFT. Extensive experiments confirm SBR's effectiveness, demonstrating that utilizing just a single safety anchor is sufficient to reduce the Harmful Score to $<$10 while preserving competitive performance on benign downstream tasks.

cs.CR

Efficient photo-Nernst terahertz emission in single heavy-metal films

State-of-the-art metallic terahertz (THz) emitters rely predominantly on spintronic heterostructures, where heavy metals serve as passive spin-to-charge converters. Here, we demonstrate efficient THz radiation from standalone Pt nanofilms at cryogenic temperatures and under external magnetic fields. The governing mechanism is identified as the ultrafast photo-Nernst effect, wherein a transient thermal gradient drives a transverse charge current. The THz emission polarity is directly dictated by the sign of the Nernst coefficient, as verified by the phase reversal observed between Pt and W or Ta. Remarkably, both thickness scaling and alloying-induced suppression of thermal conductivity independently amplify the single-layer emission to levels comparable with benchmark spintronic bilayers. These findings redefine the established role of heavy metals from passive spin-sinks to active THz emitters, uncovering a universal emission paradigm applicable across diverse spintronic and quantum materials.

cond-mat.mes-hall

Observation of Kondo hybridization wave in UTe2

Condensed matter systems with strong electronic correlations often manifest a variety of intertwined ordered phases of charge, spin, orbital and other degrees of freedom. As a prototypical strongly correlated electronic system, the Kondo lattice provides fertile soil for many fascinating quantum states, including quantum criticality, unconventional superconductivity, hidden order and topological Kondo insulator/semimetal. The foundation of Kondo physics lies in the hybridization between localized moments and itinerant electrons. Generally, the evolution of Kondo hybridization is characterized as a broad crossover rather than a phase transition. Thus far, an ordered hybridization phase has not been observed. Here, we use scanning tunneling microscopy (STM) to identify a translational-symmetry-breaking order of Kondo hybridization wave(KHW) for the first time on the surface of the spin-triplet heavy-fermion superconductor UTe2. The unprecedented phase of KHW manifests as a periodically modulated Fano lattice, accompanied by a commensurate charge density wave (CDW) and a pronounced energy gap opening near the Fermi level. This KHW-imprinted CDW has an intriguing real-space texture of complementary occupation of the heavy f and conduction charges, thereby forming a Kondo superlattice. The KHW is coexistent with superconductivity in UTe2, which may provide valuable insight into its controversial spin-triplet pairing symmetry and the underlying mechanism. Our first experimental evidence for an ordered hybridization state potentially sheds new light on the strong correlation physics of Kondo lattice system.

cond-mat.str-el

Giant Magnetocaloric Effect in a High-Spin Shastry-Sutherland Dipolar Magnet

The Shastry-Sutherland lattice is a prototypical frustrated quantum magnet. It is notable for its exactly solvable dimer-singlet ground state and hosts a wealth of magnetic phenomena under external fields. Here, this work investigates the high-spin (S = 7/2) Eu-based magnet Eu2MgSi2O7 (EMSO) using low-temperature magnetothermal measurements and Monte Carlo simulations, revealing a giant magnetocaloric effect (MCE) in this Shastry-Sutherland compound. The entropy change peak value is found to be 55.0 J kg-1 K-1 under a field change of B = 0-4 T, approximately 1.5 times larger than the commercial Gd3Ga5O12 (GGG). Adiabatic demagnetization refrigeration achieves a lowest temperature of 151 mK, deeply into the sub-Kelvin regime. Furthermore, a distinctive cooling effect persists below about 1 T, a characteristic absent for conventional magnetic coolants. A dipolar Shastry-Sutherland model is introduced as a minimal model to describe this system; in particular, the experimentally revealed 1/3 magnetization pseudo-plateau can be ascribed to the presence of dipolar couplings between Eu2+ ions, further stabilized by the thermal fluctuations, explaining the persistent cooling effect. This work establishes EMSO as a novel platform for exploring the dipolar Shastry-Sutherland system and for sub-Kelvin adiabatic demagnetization refrigeration.

cond-mat.mtrl-sci

PRISM: Personalized Recommendation via Information Synergy Module

Multimodal sequential recommendation (MSR) leverages diverse item modalities to improve recommendation accuracy, while achieving effective and adaptive fusion remains challenging. Existing MSR models often overlook synergistic information that emerges only through modality combinations. Moreover, they typically assume a fixed importance for different modality interactions across users. To address these limitations, we propose \textbf{P}ersonalized \textbf{R}ecommend-ation via \textbf{I}nformation \textbf{S}ynergy \textbf{M}odule (PRISM), a plug-and-play framework for sequential recommendation (SR). PRISM explicitly decomposes multimodal information into unique, redundant, and synergistic components through an Interaction Expert Layer and dynamically weights them via an Adaptive Fusion Layer guided by user preferences. This information-theoretic design enables fine-grained disentanglement and personalized fusion of multimodal signals. Extensive experiments on four datasets and three SR backbones demonstrate its effectiveness and versatility. The code is available at https://github.com/YutongLi2024/PRISM.

cs.IR

Differentiated Directional Intervention A Framework for Evading LLM Safety Alignment

Safety alignment instills in Large Language Models (LLMs) a critical capacity to refuse malicious requests. Prior works have modeled this refusal mechanism as a single linear direction in the activation space. We posit that this is an oversimplification that conflates two functionally distinct neural processes: the detection of harm and the execution of a refusal. In this work, we deconstruct this single representation into a Harm Detection Direction and a Refusal Execution Direction. Leveraging this fine-grained model, we introduce Differentiated Bi-Directional Intervention (DBDI), a new white-box framework that precisely neutralizes the safety alignment at critical layer. DBDI applies adaptive projection nullification to the refusal execution direction while suppressing the harm detection direction via direct steering. Extensive experiments demonstrate that DBDI outperforms prominent jailbreaking methods, achieving up to a 97.88\% attack success rate on models such as Llama-2. By providing a more granular and mechanistic framework, our work offers a new direction for the in-depth understanding of LLM safety alignment.

cs.CR

Quantum fluctuations associated with first-order magnetic transition in a frustrated kagome lattice antiferromagnet

Intense quantum fluctuations arising from geometrical frustrations in kagome-lattice magnets provide a feasible approach to exotic quantum states. Here, we document an unexpected isosymmetric first-order magnetic transition in the recently synthesized frustrated kagome-lattice antiferromagnet Nd3ScBi5, which is characterized by significant latent heat and a pronounced magnetocaloric effect, as well as discontinuous Raman shifts and negligible hysteresis. Employing the magnetocaloric effect as a detection method, in conjunction with systematical field-dependent physical properties, we uncover a distinctive 1/2 magnetization plateau phase with significant quantum fluctuations. Our study unveils Nd3ScBi5 as a prototypical model with an emerging phase of enhanced quantum fluctuations triggered by first-order magnetic transitions.

cond-mat.str-el

Speech Recognition Model Improves Text-to-Speech Synthesis using Fine-Grained Reward

Recent advances in text-to-speech (TTS) have enabled models to clone arbitrary unseen speakers and synthesize high-quality, natural-sounding speech. However, evaluation methods lag behind: typical mean opinion score (MOS) estimators perform regression over entire utterances, while failures usually occur in a few problematic words. We observe that encoder-decoder ASR models (e.g., Whisper) surface word-level mismatches between speech and text via cross-attention, providing a fine-grained reward signal. Building on this, we introduce Word-level TTS Alignment by ASR-driven Attentive Reward (W3AR). Without explicit reward annotations, W3AR uses attention from a pre-trained ASR model to drive finer-grained alignment and optimization of sequences predicted by a TTS model. Experiments show that W3AR improves the quality of existing TTS systems and strengthens zero-shot robustness on unseen speakers. More broadly, our results suggest a simple recipe for generative modeling: understanding models can act as evaluators, delivering informative, fine-grained feedback for optimization.

eess.AS

HADSF: Aspect Aware Semantic Control for Explainable Recommendation

Recent advances in large language models (LLMs) promise more effective information extraction for review-based recommender systems, yet current methods still (i) mine free-form reviews without scope control, producing redundant and noisy representations, (ii) lack principled metrics that link LLM hallucination to downstream effectiveness, and (iii) leave the cost-quality trade-off across model scales largely unexplored. We address these gaps with the Hyper-Adaptive Dual-Stage Semantic Framework (HADSF), a two-stage approach that first induces a compact, corpus-level aspect vocabulary via adaptive selection and then performs vocabulary-guided, explicitly constrained extraction of structured aspect-opinion triples. To assess the fidelity of the resulting representations, we introduce Aspect Drift Rate (ADR) and Opinion Fidelity Rate (OFR) and empirically uncover a nonmonotonic relationship between hallucination severity and rating prediction error. Experiments on approximately 3 million reviews across LLMs spanning 1.5B-70B parameters show that, when integrated into standard rating predictors, HADSF yields consistent reductions in prediction error and enables smaller models to achieve competitive performance in representative deployment scenarios. We release code, data pipelines, and metric implementations to support reproducible research on hallucination-aware, LLM-enhanced explainable recommendation. Code is available at https://github.com/niez233/HADSF

cs.LG

Realization of large magnetocaloric effect in the Kagome antiferromagnet Gd3BWO9 for Sub-Kelvin cryogenic refrigeration

Rare-earth (RE) based frustrated magnets have attracted great attention as excellent candidates for magnetic refrigeration at sub-Kelvin temperatures, while the experimental identification on systems exhibiting both large volumetric cooling capacity and reduced working temperatures far below 1 K remain to be a challenge. Here, through the ultra-low temperature magnetism and thermodynamic characterizations, we unveil the large magnetocaloric effect (MCE) realized at sub-Kelvin temperatures in the frustrated Kagome antiferromagnet Gd3BWO9 with TN~1.0 K. The isothermal magnetization curves indicate the existence of field (B) induced anisotropic magnetic phase diagrams, where four distinct magnetic phases for B // c-axis and five magnetic phases for B // ab-plane are identified at T< TN. The analysis of magnetic entropy S(B, T) data and direct adiabatic demagnetization tests reveal a remarkable cooling performance at sub-Kelvin temperatures featured by a large volumetric entropy density 502.2 mJ/K/cm3 and a low attainable minimal temperature Tmin~168 mK from the initial cooling condition of 2 K and 6 T, surpassing most of Gd-based refrigerants previously documented in temperature ranges of 0.25-4 K. The realized Tmin~168 mK far below TN ~ 1.0 K in Gd3BWO9 is related to the combined effects of magnetic frustration and criticality-enhanced MCE, which together leave a substantial magnetic entropy at reduced temperatures by enhancing spin fluctuations.

cond-mat.str-el

Anomalous Nernst Effect and Its Implications for Time-Reversal Symmetry Breaking in Kagome Metal ScV6Sn6

The nonmagnetic kagome metal ScV6Sn6 displays an unconventional charge order (CO) accompanied by signatures of an anomalous Hall effect, hidden magnetism, and multiple lattice instabilities. In this study, we report the observation of unconventional anomalous thermoelectric properties. Notably, unexpected anomalous transverse Nernst signals reach a peak value of ~4 μV/K near the TCDW ~92 K in ScV6Sn6, and these signals persist in the charge-ordered state as the temperature decreases to 10 K. Furthermore, both thermopower and thermal conductivity exhibit significant changes under magnetic fields, even in the nonmagnetic ground state. These observations strongly suggest the emergence of time-reversal symmetry breaking in ScV6Sn6, as supported by muon spin relaxation (μSR) measurements. While hidden magnetism represents the most plausible origin, alternative mechanisms involving orbital currents and chiral charge order remain possible.

cond-mat.str-el

Universal Magnetocaloric Effect near Quantum Critical Point of Magnon Bose-Einstein Condensation

Bose-Einstein condensation (BEC), a macroscopic quantum phenomenon arising from phase coherence and bosonic statistics, has been realized in quantum magnets. Here, we report the observation of a universal magnetocaloric effect (MCE) near a BEC quantum critical point (QCP) in copper sulfate crystal ($CuSO_4 \cdot 5H_2O$). By conducting magnetocaloric and nuclear magnetic resonance measurements, we uncover a field-driven BEC QCP, evidenced by the universal scaling law $T_c \propto (B_c - B)^{2/3}$ and the perfect data collapse of the magnetic Grüneisen ratio. Thermal excitation triggers a dimensional crossover to a 1D quantum-critical regime, where the MCE scaling strictly matches the universality class of 1D Fermi gases. Notably, the quantum-critical MCE enables cooling down to 12.8 mK without helium-3, with very fast thermal relaxation rate that is critical for high cooling power. This work demonstrates the universal MCE in magnon BEC systems, using a common copper sulfate compound as a paradigmatic example, and paves the way for next-generation sub-Kelvin cooling.

cond-mat.str-el

Giant Magnetocaloric Effect in Spin Supersolid Candidate Na$_2$BaCo(PO$_4$)$_2$

Supersolid, an exotic quantum state of matter that consists of particles forming an incompressible solid structure while simultaneously showing superfluidity of zero viscosity [1], is one of the long-standing pursuits in fundamental research [2, 3]. Although the initial report of $^4$He supersolid turned out to be an artifact [4], this intriguing quantum matter has inspired enthusiastic investigations into ultracold quantum gases [5-8]. Nevertheless, the realization of supersolidity in condensed matter remains elusive. Here we find evidence for a quantum magnetic analogue of supersolid -- the spin supersolid -- in the recently synthesized triangular-lattice antiferromagnet Na$_2$BaCo(PO$_4$)$_2$ [9]. Notably, a giant magnetocaloric effect related to the spin supersolidity is observed in the demagnetization cooling process, manifesting itself as two prominent valley-like regimes, with the lowest temperature attaining below 100 mK. Not only is there an experimentally determined series of critical fields but the demagnetization cooling profile also shows excellent agreement with the theoretical simulations with an easy-axis Heisenberg model. Neutron diffractions also successfully locate the proposed spin supersolid phases by revealing the coexistence of three-sublattice spin solid order and interlayer incommensurability indicative of the spin superfluidity. Thus, our results indicate a strong entropic effect of the spin supersolid phase in a frustrated quantum magnet and open up a viable and promising avenue for applications in sub-Kelvin refrigeration, especially in the context of persistent concerns about helium shortages [10, 11].

cond-mat.str-el

Quantum Next-Generation Reservoir Computing and Its Quantum Optical Implementation

Quantum reservoir computing (QRC) exploits the information-processing capabilities of quantum systems to tackle time-series forecasting tasks, which is expected to be superior to their classical counterparts. By far, many QRC schemes have been theoretically proposed. However, most of these schemes involves long-time evolution of quantum systems or networks with quantum gates. This poses a challenge for practical implementation of these schemes, as precise manipulation of quantum systems is crucial, and this level of control is currently hard to achieve with the existing state of quantum technology. Here, we propose a different way of QRC scheme, which is friendly to experimental realization. It implements the quantum version of nonlinear vector autoregression, extracting linear and nonlinear features of quantum data by measurements. Thus, the evolution of complex networks of quantum gates can be avoided. Compared to other QRC schemes, our proposal also achieves an advance by effectively reducing the necessary training data for reliable predictions in time-series forecasting tasks. Furthermore, we experimentally verify our proposal by performing the forecasting tasks, and the observation matches well with the theorectial ones. Our work opens up a new way toward complex tasks to be solved by using the QRC, which can herald the next generation of the QRC.

quant-ph

Strong superconducting pairing strength and pseudogap features in a putative multiphase heavy-fermion superconductor CeRh2As2 by soft point-contact spectroscopy

CeRh2As2 is a newly discovered candidate of multiphase heavy-fermion superconductor (Tc=0.3 K) with intriguing physical properties. Here, we employ soft point-contact spectroscopy to investigate its energy gap behaviors in both the normal and superconducting states. The differential conductance below Tc reveals an estimated superconducting energy gap of 2ΔSC=0.24 meV and thus an extremely strong superconducting pairing strength 2ΔSC/kBTc=8.8, which is comparable to those of cuprates and iron-based high-Tc superconductors as well as infinite-layer nickelates. Above Tc, a well-defined pseudogap feature is manifested as a V-shaped dip in the differential conductance spanning an energy scale of 2Δg=0.95-3.0 meV. The pseudogap feature persists to the highest characteristic temperature of Tg=8-9 K and is gradually suppressed by magnetic field of Bg=9.0T regardless of its direction relative to the crystallographic axes. The observation of pseudogap features prior to the superconducting phase transition enriches the phase diagram of CeRh2As2 and provides a novel platform to study the interplay of unconventional superconductivity and pseudogap phenomena.

cond-mat.supr-con