arXiv subjects

Peizhe Tang

Publications and source records attributed to Peizhe Tang.

At least 19 recordsLinked to original sources

arXiv2026

Coherent seeding and control of dynamical ferroelectricity by phonon anharmonicity

Optical control of quantum materials has progressed along two separate directions: creating non-equilibrium states inaccessible at equilibrium, and coherently controlling ultrafast dynamics with multi-pulse protocols. Ferroelectricity is especially attractive in this context because its order parameter, macroscopic polarization, directly links inversion-symmetry breaking to functional response. Yet light-induced ferroelectricity has so far been confined to quantum paraelectrics near the ferroelectric instability, where critical fluctuations obscure the formation of a homogeneous ferroelectric state and complicate its deterministic coherent control. Unifying these capabilities -- preparing a symmetry-broken state and then coherently steering its functionality -- remains a central challenge. Here we show that intense terahertz excitation of a soft phonon mode induces a ferroelectric state in centrosymmetric PbTe, a thermoelectric material with strong lattice anharmonicity but no ferroelectric transition at finite temperature. The light-induced symmetry-broken state can be realized up to about 100 K, without relying on local dipolar fluctuations. Experiment and theory together reveal that terahertz-driven anharmonic coupling between degenerate transverse optical phonons underlies this ferroelectric induction. Furthermore, we demonstrate coherent amplification and suppression of the induced polarization via a double-pulse-excitation protocol. These results establish terahertz-driven anharmonic mode coupling as a general strategy for controlling mode-mediated functionalities in quantum materials, opening a route to ultrafast information processing.

cond-mat.mtrl-sci↗

arXiv2026

Saturated and Anisotropic Magnetostriction in an Altermagnet

Magnetostriction, a fundamental phenomenon bridging magnetism and mechanics, has enabled a broad spectrum of applications. For almost two centuries, it has been mainly investigated for ferromagnets. Regarding the magnetostriction of antiferromagnets (AFMs), limitedly known examples for both conventional collinear AFMs and noncollinear AFMs predominantly exhibit non-saturating magnetic-field dependence. Herein, we report an easily saturated magnetostriction effect in a prototypical altermagnet - MnTe, which is an emerging class of collinear AFMs with special crystal symmetries. For high-quality MnTe single crystals, the magnetostriction saturates under a moderate field of ~0.7 T with an intriguing two-fold-symmetry anisotropy. First-principles calculations reveal that the saturated and anisotropic magnetostriction originates from symmetry-allowed coupling between elastic strain and its N\'eel order parameter. These findings break the traditional wisdom on antiferromagnetic magnetostriction.

cond-mat.mtrl-sci↗

arXiv2026

Occupation Dynamics of Floquet-Volkov States and Spectral Sum Rule

Time-periodic light fields can dress electronic states in quantum materials, forming Floquet states whose dynamic occupation determines transient material properties. Here by using time- and angle-resolved photoemission spectroscopy (TrARPES), we reveal the transient occupation of Floquet-Volkov states in two semiconductors, black phosphorus and MoSe$_2$. While the occupation of the light-induced sidebands, directly reflected by TrARPES spectral weight, strongly depends on the driving field, we find that the total spectral weight obtained by summing up all sidebands is conserved upon below-gap driving. Our work provides critical insights into the Floquet population dynamics, which are essential for light-field tailoring of transient material properties.

cond-mat.mtrl-sci↗

arXiv2026

Multiple Layer-Selective Polar Charge Density Waves in ${\rm{EuTe}}_{4}$

${\rm{EuTe}}_{4}$ is a polar charge density wave (CDW) material, with giant thermal hysteresis and non-volatile state switching under electric and optical fields, attracting great attention in recent years. However, the in-depth understanding of these anomalous phenomena remains elusive. Herein, via first-principles calculations, we reveal that the polar CDW state in ${\rm{EuTe}}_{4}$ hosts a novel layer-selective nature, wherein multiple energetically close CDW configurations coexist and exhibit low interconversion energy barriers. Monte Carlo simulations indicate that the giant thermal hysteresis in ${\rm{EuTe}}_{4}$ originates from a phase transition mainly driven by the change of configurational entropy, around which the material hosts a metastable CDW state characterized by diverse local polar configurations breaking the out-of-plane translational symmetry. The configurational composition of this metastable CDW state can be effectively controlled by electric and optical fields, thereby enabling non-volatile state switching. Our theoretical findings align well with recent experimental observations in ${\rm{EuTe}}_{4}$ and pave the way for exploring the emerging phenomena and applications of polar CDW in multilayered systems.

cond-mat.mtrl-sci↗

arXiv2025

Lattice-decoupled rotatable stripe-like charge order within the strange metal phase of 2M-WS2

In quantum materials, charge orders typically stabilize in specific crystallographic orientations, though their formation mechanisms may vary. Here, using low-temperature scanning tunneling microscopy (STM), we discover a lattice-decoupled rotatable stripe-like charge order coexisting with superconductivity in 2M-WS2. The charge order manifests five distinct orientations across different sample regions, yet maintains an identical wavelength. This directional decoupling from host lattice challenges existing paradigms. First-principles calculations of phonon spectra and nesting function fail to explain the ordering mechanism. Intriguingly, the transition temperature of the charge orders exhibits spatial variations (21-46 K), coinciding with the temperature range of the recently reported strange metal phase in this material. This correlation suggests that the interplay between strong electronic correlations and electron-phonon coupling must be critically evaluated to elucidate the emergence of this unconventional charge order.

cond-mat.supr-con↗

arXiv2025

Multiple Photon Field-induced Topological States in Bulk HgTe

Strong light-matter interactions can be exploited to modify properties of quantum materials both in and out of thermal equilibrium. Recent studies suggest electromagnetic fields in photonic structures can hybridize with condensed matter systems, resulting in photon field-dressed collective quantum states such as charge density waves, superconductivity, and ferroelectricity. Here, we show that photon fields in photonic structures, including optical cavities and waveguides, induce emergent topological phases in solids through polarization-mediated symmetry-breaking mechanisms. Using state-of-the-art quantum electrodynamic density functional theory (QEDFT) calculations, we demonstrate that strong light-matter coupling can reconfigure both the electronic and ionic structures of HgTe, driving the system into Weyl, nodal-line, or topological insulator phases. These phases depend on the relative orientation of the sample in the photonic structures, as well as the coupling strength. Unlike previously reported laser-driven phenomena with ultrashort lifetimes, the photon field-induced symmetry breaking arises from steady-state photon-matter hybridization, enabling multiple robust topological states to emerge. Our study demonstrates that vacuum fluctuations in photonic structures can be used to engineer material properties and realize rich topological phenomena in quantum materials on demand.

cond-mat.mtrl-sci↗

arXiv2025

Topological surface states in {\gamma}-PtBi$_2$ evidenced by scanning tunneling microscopy

For the application of topological materials, the specific location of their topological surface states with respect to the Fermi level are important. {\gamma}-PtBi2 has been demonstrated to be a Weyl semimetal possessing superconducting Fermi arcs by photoemission spectroscopy. However, the evidence of its topological surface states is lacking by scanning tunneling microscopy (STM), which should be rather sensitive to detect the surface states. Here, we show multiple STM evidences for the existence of topological surface states in {\gamma}-PtBi2. We observe not only the step-edge and screw dislocation induced quasiparticle interference fringes, originating from the electron scatterings between the Fermi arcs of {\gamma}-PtBi2, but also the back-scattering prohibition related to the spin-flip process, which is the direct evidence for the topological nature of the surface states. Moreover, we demonstrate that the topological surface states are precisely located over a narrow energy range near the Fermi level, within which sharply enhanced intensity and slow spatial decay of quasiparticle interference are observed.

cond-mat.supr-con↗

arXiv2025

Floquet-Volkov interference in a semiconductor

Intense light-field can dress both Bloch electrons inside crystals and photo-emitted free electrons in the vacuum, dubbed as Floquet and Volkov states respectively. These quantum states can further interfere coherently, modulating light-field dressed states. Here, we report experimental evidence of the Floquet-Volkov interference in a semiconductor - black phosphorus. A highly asymmetric modulation of the spectral weight is observed for the Floquet-Volkov states, and such asymmetry can be further controlled by rotating the pump polarization. Our work reveals the quantum interference between different light-field dressed electronic states, providing insights for material engineering on the ultrafast timescale.

cond-mat.mes-hall↗

arXiv2025

Floquet optical selection rules in black phosphorus

Optical selection rules endorsed by symmetry are crucial for understanding the optical properties of quantum materials and the associated ultrafast spectral phenomena. Here, we introduce momentum-resolved Floquet optical selection rules using group theory to elucidate the pump-probe photoemission spectral distributions of monolayer black phosphorus (BP), which are governed by the symmetries of both the material and the lasers. Using time-dependent density functional theory (TDDFT), we further investigate the dynamical evolution of Floquet(-Volkov) states in the photoemission spectra of monolayer BP, revealing their spectral weights at specific momenta for each sideband. These observations are comprehensively explained by the proposed Floquet optical selection rules. Our framework not only clarifies experimental photoemission spectra but also uncovers unexplored characteristics under different pump-probe configurations. Our results are expected to deepen the understanding of light-induced ultrafast spectra in BP and can be extended to other Floquet systems.

cond-mat.mtrl-sci↗

arXiv2024

Laser-Controlled Nonlinear Hall Effect in Tellurium Solids via Nonlinear Phononics

A Terahertz (THz) laser with strong strength could excite more than one phonons and induce a transient lattice distortion termed as nonlinear phononics. This process allows dynamic control of various physical properties, including topological properties. Here, using first-principles calculations and dynamical simulations, we demonstrate that THz laser excitation can modulate the electronic structure and the signal of nonlinear Hall effect in elemental solid tellurium (Te). By strongly exciting the chiral phonon mode, we observe a non-equilibrium steady state characterized by lattice distortion along the breathing vibrational mode. This leads to a transition of Te from a direct to an indirect semiconductor. In addition, the energy dispersion around the Weyl point is deformed, leading to variations in the local Berry curvature dipole. As a result, the nonlinear Hall-like current in Te can be modulated with electron doping where the sign of current could be reversed under a strong THz laser field. Our results may stimulate further research on coupled quasiparticles in solids and the manipulation of their topological transport properties using THz lasers.

cond-mat.mtrl-sci↗

arXiv2024

Correlated topological flat bands in rhombohedral graphite

Flat bands and nontrivial topological physics are two important topics of condensed matter physics. With a unique stacking configuration analogous to the Su-Schrieffer-Heeger (SSH) model, rhombohedral graphite (RG) is a potential candidate for realizing both flat bands and nontrivial topological physics. Here we report experimental evidence of topological flat bands (TFBs) on the surface of bulk RG, which are topologically protected by bulk helical Dirac nodal lines via the bulk-boundary correspondence. Moreover, upon {\it in situ} electron doping, the surface TFBs show a splitting with exotic doping evolution, with an order-of-magnitude increase in the bandwidth of the lower split band, and pinning of the upper band near the Fermi level. These experimental observations together with Hartree-Fock calculations suggest that correlation effects are important in this system. Our results demonstrate RG as a new platform for investigating the rich interplay between nontrivial band topology, correlation effects, and interaction-driven symmetry-broken states.

cond-mat.str-el↗

arXiv2024

Chiral Floquet Engineering on Topological Fermions in Chiral Crystals

The interplay of chiralities in light and quantum matter provides an opportunity to design and manipulate chirality-dependent properties in quantum materials. Herein we report the chirality-dependent Floquet engineering on topological fermions with the high Chern number in chiral crystal CoSi via circularly polarized light (CPL) pumping. Intense light pumping does not compromise the gapless nature of topological fermions in CoSi, but displaces the crossing points in momentum space along the direction of light propagation. The Floquet chirality index is proposed to signify the interplay between the chiralities of topological fermion, crystal, and incident light, which determines the amplitudes and directions of light-induced momentum shifts. Regarding the time-reversal symmetry breaking induced by the CPL pumping, momentum shifts of topological fermions result in the birth of transient anomalous Hall signals in non-magnetic CoSi within an ultrafast time scale, which Mid-infrared (IR) pumping and terahertz (THz) Kerr or Faraday probe spectroscopy could experimentally detect. Our findings provide insights into exploring novel applications in optoelectronic devices by leveraging the degree of freedom of chirality in the non-equilibrium regime.

physics.optics↗

arXiv2024

Symmetry-driven anisotropic coupling effect in antiferromagnetic topological insulator: Mechanism for high-Chern-number quantum anomalous Hall state

Antiferromagnetic (AFM) topological insulators (TIs), which host magnetically gapped Dirac-cone surface states and exhibit many exotic physical phenomena, have attracted great attention. Here, we find that the coupled surface states can be intertwined to give birth to a set of $2n$ unique new Dirac cones, dubbed intertwined Dirac cones, through the anisotropic coupling enforced by crystalline $n$-fold ($n=2, 3, 4, 6$) rotation symmetry $C_{nz}$ in the presence of a $PT$-symmetry breaking potential, for example, an electric field. Interestingly, we also find that the warping effect further drives the intertwined Dirac-cone state into a quantum anomalous Hall phase with a high Chern number ($C=n$). Then, based on first-principles calculations, we have explicitly demonstrated six intertwined Dirac cones and a Chern insulating phase with a high Chern number ($C=3$) in MnBi$_2$Te$_4$$/$(Bi$_2$Te$_3$)$_{\mathrm{m}}/$MnBi$_2$Te$_4$ heterostructures, as well as the $C=2$ and $C=4$ phases in HgS and $α$-Ag$_2$Te films, respectively. This work discovers the intertwined Dirac-cone state in AFM TI thin films, which reveals a mechanism for designing the quantum anomalous Hall state with a high Chern number and also paves a way for studying highly tunable high-Chen-number flat bands of twistronics.

cond-mat.mes-hall↗

arXiv2024

Strain and twist angle driven electronic structure evolution in twisted bilayer graphene

In twisted bilayer graphene (TBG) devices, local strains frequently coexist and intertwine with the twist-angle-dependent moir\'e superlattice, significantly influencing the electronic properties of TBG, yet their combined effects remain incompletely understood. Here, using low-temperature scanning tunneling microscopy, we study a TBG device exhibiting both a continuous twist-angle gradient from 0.35{\deg} to 1.30{\deg} and spatially varying strain fields, spanning the first (1.1{\deg}), second (0.5{\deg}) and third (0.3{\deg}) magic angles. We visualize the evolution of flat and remote bands in energy and real space with atomic resolution. Near the first magic angle, we discover an anomalous spectral weight transfer between the two flat band peaks, signifying the role of strain and electronic correlations, as further evidenced by an unusual spatial dispersion of these peaks within a moir\'e unit cell. In contrast, remote band peak energy offers a strain-insensitive indicator of the local twist angle. Structural analysis further reveals non-negligible shear strain across the sample. All observations are quantitatively reproduced by a continuum model that incorporates heterostrain and a self-consistent Hartree potential, revealing the critical but unexplored role of shear strain in shaping the low-energy electronic landscape of TBG.

cond-mat.mes-hall↗

arXiv2024

Ultrafast Carrier Relaxation Dynamics in a Nodal-Line Semimetal PtSn$_4$

Topological Dirac nodal-line semimetals host topologically nontrivial electronic structure with nodal-line crossings around the Fermi level, which could affect the photocarrier dynamics and lead to novel relaxation mechanisms. Herein, by using time- and angle-resolved photoemission spectroscopy, we reveal the previously-inaccessible linear dispersions of the bulk conduction bands above the Fermi level in a Dirac nodal-line semimetal PtSn$_4$, as well as the momentum and temporal evolution of the gapless nodal lines. A surprisingly ultrafast relaxation dynamics within a few hundred femtoseconds is revealed for photoexcited carriers in the nodal line. Theoretical calculations suggest that such ultrafast carrier relaxation is attributed to the multichannel scatterings among the complex metallic bands of PtSn$_4$ via electron-phonon coupling. In addition, a unique dynamic relaxation mechanism contributed by the highly anisotropic Dirac nodal-line electronic structure is also identified. Our work provides a comprehensive understanding of the ultrafast carrier dynamics in a Dirac nodal-line semimetal.

cond-mat.mes-hall↗

arXiv2023

Light-induced ideal Weyl semimetal in HgTe via nonlinear phononics

Interactions between light and matter allow the realization of out-of-equilibrium states in quantum solids. In particular, nonlinear phononics is one of the efficient approaches to realizing the stationary electronic state in non-equilibrium. Herein, by using extended $ab~initio$ molecular dynamics, we identify that long-lived light-driven quasi-stationary geometry could stabilize the topological nature in the material family of HgTe compounds. We show that coherent excitation of the infrared-active phonon mode results in a distortion of the atomic geometry with a lifetime of several picoseconds. We show that four Weyl points are located exactly at the Fermi level in this non-equilibrium geometry, making it an ideal long-lived metastable Weyl semimetal. We propose that such a metastable topological phase can be identified by photoelectron spectroscopy of the Fermi arc surface states or ultrafast pump-probe transport measurements of the nonlinear Hall effect.

cond-mat.mtrl-sci↗

arXiv2023

Floquet engineering of black phosphorus upon below-gap pumping

Time-periodic light field can dress the electronic states and lead to light-induced emergent properties in quantum materials. While below-gap pumping is regarded favorable for Floquet engineering, so far direct experimental evidence of momentum-resolved band renormalization still remains missing. Here, we report experimental evidence of light-induced band renormalization in black phosphorus by pumping at photon energy of 160 meV which is far below the band gap, and the distinction between below-gap pumping and near-resonance pumping is revealed. Our work demonstrates light-induced band engineering upon below-gap pumping, and provides insights for extending Floquet engineering to more quantum materials.

cond-mat.mes-hall↗

arXiv2023

Stripe charge order driven manipulation of Majorana bound states in 2M-WS2 topological superconductor

Majorana bound states (MBSs) are building blocks for topological quantum computing. They can be generated via the combination of electronic topology and superconductivity. To achieve logic operations via Majorana braiding, positional control of the MBS must be established. To this end, exotic co-existing phases or collective modes in an intrinsic topological superconductor can provide a tuning knob to manipulate the MBS. Here we report the observation of a striped surface charge order coexisting with superconductivity and its controllable tuning of the MBS in the topological superconductor 2M-WS2 using low-temperature scanning tunneling microscopy. By applying an out-of-plane magnetic field, we observe that MBS is absent in vortices in the region with strong stripe order. This is in contrast to adjacent underlaying layers without charge order where vortex-bound MBSs are observed. Via theoretical simulations, we show that the surface stripe order does not destroy the bulk topology, but it can effectively modify the spatial distribution of MBS, i.e., it pushes them downward away from the 2M-WS2 surface. Our findings demonstrate that the interplay of charge order and topological superconductivity can be used to manipulate the positions of the MBS, and to explore of new states of matter.

cond-mat.supr-con↗