arXiv subjects

Peng-Jun Liang

Publications and source records attributed to Peng-Jun Liang.

11 recordsLinked to original sources

arXiv2026

Heterogeneous entanglement between a trapped ion and a solid-state quantum memory

Hybrid quantum networks offer a promising architecture for scalable quantum information processing and a future quantum internet, as they can combine the complementary strengths of disparate physical platforms. While single-atom systems provide deterministic quantum logic gates, atomic ensembles enable large-capacity quantum storage. However, generating entanglement between such heterogeneous systems has remained an open challenge, primarily due to fundamental spectral mismatches and system complexity. Here, we demonstrate a hybrid quantum network that entangles a single trapped $\mathrm{^{171}Yb^{+}}$ ion and a quantum memory based on $\rm ^{153}Eu^{3+}\colon\!Y_2SiO_5$ crystal over a 75-m separation. Using polarization-maintaining quantum frequency conversion, we map spin-photon entanglement onto a hybrid entanglement between a single spin qubit and a collective excitation of the quantum memory. The resulting entangled state achieves a fidelity of $(89.21 \pm 2.23)\%$ and violates the CHSH-Bell inequality by 6 standard deviations ($S = 2.328 \pm 0.055$), confirming nonlocality between two heterogeneous nodes. This work establishes entanglement between a quantum processing module with a multiplexed quantum memory node, representing a key step toward a scalable, multifunctional quantum internet.

quant-ph↗

arXiv2025

Efficient integrated quantum memory for light

Scalable implementation of quantum networks and photonic processors require integrated photonic memories with high efficiency, yet current integrated systems have been limited to storage efficiencies below 27.8%. Here, we demonstrate highly efficient integrated quantum memories based on rare-earth-iondoped crystals coupled with impedance-matched microcavities, realized in two novel architectures: 200-micrometer-thin membranes of Eu3+:Y2SiO5 integrated with fiber-based microcavities, and waveguide-based cavities fabricated using femtosecond lasers. Our approach achieves reliable integrated quantum storage with record efficiencies of 80.3(7)% for weak coherent pulses and 69.8(1.6)% for telecom-heralded single photons, alongside the storage of 20 temporal modes with an average efficiency of 51.3(2)%. Moreover, the thin-membrane Eu3+:Y2SiO5 architecture enables spectrally tunable efficient quantum storage via variable strain, providing a flexible interface for quantum networks. By combining high efficiency, large multimode capacity, and tunability, our devices establish a versatile hardware foundation for scalable quantum repeaters and chip-scale photonic processors.

quant-ph↗

arXiv2025

Multichannel and high dimensional integrated photonic quantum memory

Integrated photonic quantum memories are essential components for scalable quantum networks and photonic information processors. However, prior implementations have been confined to single-channel operation, limiting their capacity to manipulate multiple photonic pulses and support high-dimensional information. In this work, we introduce an 11-channel integrated quantum memory based on laser-written waveguide arrays in $^{151}$Eu$^{3+}$:Y$_2$SiO$_5$ crystals. On-chip electrode arrays enable independent control over the readout times for each channel via Stark-shift-induced atomic interference. Our device achieves random-access quantum storage of three time-bin qubits with a fidelity exceeding 99%, as well as storage of five-dimensional path-encoded quantum states with a fidelity above 96%. This multichannel integrated storage device enables versatile applications through its random access capability and lays a solid foundation for the development of high-dimensional quantum networks in integrated architectures.

quant-ph↗

arXiv2025

A Metropolitan-scale Multiplexed Quantum Repeater with Bell Nonlocality

Quantum repeaters can overcome exponential photon loss in optical fibers, enabling heralded entanglement between distant quantum memories. The definitive benchmark for this entanglement is Bell nonlocality; however, recent metropolitan-scale demonstrations based on single-photon interference (SPI) schemes have been limited to generating low-quality entanglement, falling short of Bell nonlocality certification. Here, we introduce a multiplexed quantum repeater protocol based on time measurements (MQR-TM), successfully combining the high heralding rate of SPI schemes with the phase robustness of two-photon interference (TPI) schemes. This approach achieves heralded entanglement distribution between two solid-state quantum memories over a record 14.5~km separation, generating a Bell state with a fidelity of $78.6 \pm 2.0\%$. We observe a CHSH-Bell inequality violation by 3.7 standard deviations, marking the first certification of Bell nonlocality in metropolitan-scale quantum repeaters. Our architecture supports autonomous quantum node operation without fiber channel phase stabilization, offering a practical framework for scalable quantum-repeater networks.

quant-ph↗

arXiv2023

Stark tuning of telecom single-photon emitters based on a single Er$^{3+}$

The implementation of scalable quantum networks requires photons at the telecom band and long-lived spin coherence. The single Er$^{3+}$ in solid-state hosts is an important candidate that fulfills these critical requirements simultaneously. However, to entangle distant Er$^{3+}$ ions through photonic connections, the emission frequency of individual Er$^{3+}$ in solid-state matrix must be the same, which is challenging because the emission frequency of Er$^{3+}$ depends on its local environment. Herein, we propose and experimentally demonstrate the Stark tuning of the emission frequency of a single Er$^{3+}$ in a Y$_2$SiO$_5$ crystal by employing electrodes interfaced with a silicon photonic crystal cavity. We obtain a Stark shift of 182.9 $\pm$ 0.8 MHz which is approximately 27 times of the optical emission linewidth, demonstrating the promising applications in tuning the emission frequency of independent Er$^{3+}$ into the same spectral channels. Our results provide a useful solution for construction of scalable quantum networks based on single Er$^{3+}$ and a universal tool for tuning emission of individual rare-earth ions.

quant-ph↗

arXiv2021

Heralded entanglement distribution between two absorptive quantum memories

Owing to the inevitable loss in communication channels, the distance of entanglement distribution is limited to approximately 100 kilometres on the ground. Quantum repeaters can circumvent this problem by using quantum memory and entanglement swapping. As the elementary link of a quantum repeater, the heralded distribution of two-party entanglement between two remote nodes has only been realized with built-in-type quantum memories. These schemes suffer from the trade-off between multiplexing capacity and deterministic properties and hence hinder the development of efficient quantum repeaters. Quantum repeaters based on absorptive quantum memories can overcome such limitations because they separate the quantum memories and the quantum light sources. Here we present an experimental demonstration of heralded entanglement between absorptive quantum memories. We build two nodes separated by 3.5 metres, each containing a polarization-entangled photon-pair source and a solid-state quantum memory with bandwidth up to 1 gigahertz. A joint Bell-state measurement in the middle station heralds the successful distribution of maximally entangled states between the two quantum memories with a fidelity of 80.4 $\pm$ 2.2 per cent ($\pm$1 standard deviation). The quantum nodes and channels demonstrated here can serve as an elementary link of a quantum repeater. Moreover, the wideband absorptive quantum memories used in the nodes are compatible with deterministic entanglement sources and can simultaneously support multiplexing, which paves the way for the construction of practical solid-state quantum repeaters and high-speed quantum networks.

quant-ph↗

arXiv2020

Hyperfine Structure and Coherent Dynamics of Rare Earth Spins Explored with Electron-Nuclear Double Resonance at Sub-Kelvin Temperatures

An experimental platform of ultralow-temperature pulsed ENDOR (electron-nuclear double resonance) spectroscopy is constructed for the bulk materials. Coherent property of the coupled electron and nuclear spins of the rare-earth (RE) dopants in a crystal (143Nd3+:Y2SiO5) is investigated from 100 mK to 6 K. At the lowest working temperatures, two-pulse-echo coherence time exceeding 2 ms and 40 ms are achieved for the electron and nuclear spins, while the electronic Zeeman and hyperfine population lifetimes are more than 15 s and 10 min. With the aid of the near-unity electron spin polarization at 100 mK, the complete hyperfine level structure with 16 energy levels is measured using ENDOR technique without the assistance of the reconstructed spin Hamiltonian. These results demonstrate the suitability of the deeply cooled paramagnetic RE-doped solids for memory components aimed for quantum communication and quantum computation. The developed experimental platform is expected to be a powerful tool for paramagnetic materials from various research fields.

quant-ph↗

arXiv2019

Strict experimental test of macroscopic realism in a light-matter-interfaced system

Macroscopic realism is a classical worldview that a macroscopic system is always determinately in one of the two or more macroscopically distinguishable states available to it, and so is never in a superposition of these states. The question of whether there is a fundamental limitation on the possibility to observe quantum phenomena at the macroscopic scale remains unclear. Here we implement a strict and simple protocol to test macroscopic realism in a light-matter interfaced system. We create a micro-macro entanglement with two macroscopically distinguishable solid-state components and rule out those theories which would deny coherent superpositions of up to 76 atomic excitations shared by 10^10 ions in two separated solids. These results provide a general method to enhance the size of superposition states of atoms by utilizing quantum memory techniques and to push the envelope of macroscopicity at higher levels.

quant-ph↗

arXiv2018

Multiplexed storage and real-time manipulation based on a multiple-degree-of-freedom quantum memory

The faithful storage and coherent manipulation of quantum states with matter-systems enable the construction of large-scale quantum networks based on quantum repeater. To achieve useful communication rates, highly multimode quantum memories will be required to construct a multiplexed quantum repeater. Here, we present the first demonstration of the on-demand storage of orbital-angular-momentum states with weak coherent pulses at the single-photon-level in a rare-earth-ion doped crystal. Through the combination of this spatial degree-of-freedom with temporal and spectral degrees of freedom, we create a multiple-degree-of-freedom memory with high multimode capacity. This device can serve as a quantum mode converter with high fidelity, which is the fundamental requirements for the construction of a multiplexed quantum repeater. This device further enables essentially arbitrary spectral and temporal manipulations of spatial-qutrit-encoded photonic pulses in real-time. Therefore, the developed quantum memory can serve as a building block for scalable photonic quantum information processing architectures.

quant-ph↗

arXiv2018

Probing the collective dynamics of nuclear spin bath in a rare-earth ion doped crystal

Probing collective spin dynamics is a current challenge in the field of magnetic resonance spectroscopy and has important applications in material analysis and quantum information protocols. Recently, the rare-earth ion doped crystals are an attractive candidate for making long-lived quantum memory. Further enhancement of its performance would benefit from the direct knowledge on the dynamics of nuclear-spin bath in the crystal. Here we detect the collective dynamics of nuclear-spin bath located around the rare-earth ions in a crystal using dynamical decoupling spectroscopy method. From the measured spectrum, we analyze the configuration of the spin bath and characterize the flip-flop time between two correlated nuclear spins in a long time scale ($\sim $1s). Furthermore, we experimentally demonstrate that the rare-earth ions can serve as a magnetic quantum sensor for external magnetic field. These results suggest that the rare-earth ion is a useful probe for complex spin dynamics in solids and enable quantum sensing in the low-frequency regime, revealing promising possibilities for applications in diverse fields.

quant-ph↗

arXiv2018

A Raman-Heterodyne Study of the Hyperfine Interaction of the Optically-Excited State $^5$D$_0$ of Eu$^{3+}$:Y$_2$SiO$_5$

The spin coherence time of $^{151}$Eu$^{3+}$ which substitutes the yttrium at site 1 in Y$_2$SiO$_5$ crystal has been extended to 6 hours in a recent work [\textit{Nature} \textbf{517}, 177 (2015)]. To make this long-lived spin coherence useful for optical quantum memory applications, we experimentally characterize the hyperfine interaction of the optically-excited state $^5$D$_0$ using Raman-heterodyne-detected nuclear magnetic resonance. The effective spin Hamiltonians for excited and ground state are fitted based on the experimental spectra obtained in 200 magnetic fields with various orientations. To show the correctness of the fitted parameters and potential application in quantum memory protocols, we also characterize the ground-state hyperfine interaction and predict the critical magnetic field which produces the 6-hour-long coherence time. The complete energy level structure for both the $^7$F$_0$ ground state and $^5$D$_0$ excited state at the critical magnetic field are obtained. These results enable the design of quantum memory protocols and the optimization of optical pumping strategy for realization of photonic quantum memory with hour-long lifetime.

quant-ph↗