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Pengcheng Ma

Publications and source records attributed to Pengcheng Ma.

8 recordsLinked to original sources

Cooperative concurrence of 4f and 3d flat bands in kagome heavy-fermion metal YbCr6Ge6

Flat-band (FB) systems originating from special lattice geometry like in kagome metals as well as localized orbitals in the materials such as heavy-fermion (HF) compounds have induced intensive interest due to their band topology and strong electron correlation effects, leading to emergent quantum states of matter. However, the question of how these two distinct FBs coexist and interact remains unsettled. Here, we report that YbCr6Ge6 hosting both Cr-kagome lattice and Yb-4f electrons exhibits HF behaviors and a robust antiferromagnetic ground state with transition temperature TN = 3 K, significantly higher than other similar kagome metals with Yb ions. Angle-resolved photoemission spectroscopy measurements reveal the coexistence of FBs originating from both Cr-kagome lattice and localized Yb-4f electrons near Fermi energy level EF. More importantly, the clear spectroscopic signatures of a hybridization of Yb-4f FB with kagome-lattice-derived conduction bands and the high density of states of Cr-kagome FB near EF provide the underlying microscopic mechanisms of HF behaviors and enhanced antiferromagnetism in YbCr6Ge6. Our findings demonstrate that the novel kagome HF metals can not only host the cooperative coexistence of two different types of FBs, but also provide a paradigm material platform to explore the exotic correlated topological quantum phenomena.

cond-mat.str-el

Coexistence of near-EF van Hove singularity and in-gap topological Dirac surface states in superconducting electrides

Superconducting electrides have attracted growing attention for their potential to achieve high superconducting transition temperatures (TC) under pressure. However, many known electrides are chemically reactive and unstable, making high-quality single-crystal growth, characterization, and measurements difficult, and most do not exhibit superconductivity at ambient pressure. In contrast, La3In stands out for its ambient-pressure superconductivity (TC ~ 9.4 K) and the availability of high-quality single crystals. Here, we investigate its low-energy electronic structure using angle-resolved photoemission spectroscopy and first-principles calculations. The bands near the Fermi energy are mainly derived from La 5d and In 5p orbitals. A saddle point is directly observed at the Brillouin zone (BZ) boundary, while a three-dimensional van Hove singularity crosses EF at the BZ corner. First-principles calculations further reveal topological Dirac surface states within the bulk energy gap above EF. The coexistence of a high density of states and in-gap topological surface states near EF suggests that La3In offers a promising platform for tuning superconductivity and exploring possible topological superconducting phases through doping or external pressure.

cond-mat.supr-con

Evidence for Anion-Free-Electron Duality and Enhanced Superconducting Role of Interstitial Anionic Electrons in Electrides

The discovery of superconducting electrides, characterized by interstitial anionic electrons (IAEs) residing in lattice cavities, has established a distinctive platform for investigating superconductors. Yet the superconducting origin and the fundamental role of IAEs in Cooper pairing formation remain poorly understood due to the challenges in directly observing IAEs. Here, combining angle-resolved photoemission spectroscopy (ARPES), transport measurements, and first-principles calculations, we certify that the IAEs in electride La3In (Tc = 9.4 K) exhibit a dual nature as both anions and free electrons. With the finite-depth potential well model, we trace that IAEs originate from electronic states near the Fermi level located above potential barriers, forming a Fermi sea susceptible to scattering by La-derived phonons, triggering superconductivity. ARPES combined with high-resolution XRD measurements on oxygen-treated samples directly reveals IAEs' spatial distribution and energy dispersion from interstitial sites with the consistent energy value predicted by our theory model. The concomitant diminution of free electrons upon oxygen treatment, leading to a marked reduction in superconductivity, further provides compelling experimental evidence that IAEs actively participate in electron-phonon coupling. Our findings resolve the long-standing ambiguity regarding the electronic nature of IAEs, elucidate their enhancing superconductivity in the phonon-mediated mechanism, and provide a foundation for exploring advanced electride-based superconductors.

cond-mat.supr-con

Interstitial anionic electrons involved superconductivity and T-linear resistivity behavior in electride La3In

Electrides are unique materials because of the existence of interstitial anionic electrons (IAEs). Due to these loosely bound IAEs and their strong interaction with the framework of cations, electrides can host superconductivity with rather high Tc, especially under high pressure, as predicted in theory. However, the experimental observations of superconductivity in electrides are very rare, let alone the detailed studies on intrinsic properties of single crystals. Here, we report the superconducting and normal-state properties of electride La3In single crystals. La3In shows a type-II superconductivity with Tc ~ 9.4 K and a T-linear resistivity in a wide temperature range. Experimental measurements and theoretical calculations suggest that the relatively high Tc could be ascribed to the high density of states around the Fermi level caused by short flat bands along R-M direction and the strong electron-phonon coupling, partially derived from the IAEs. Meanwhile, the T-linear resistivity may reflect the significant electronic correlation effect in this material. These findings will shed light on understanding the role of IAEs in superconductivity and open a promising way to explore high-temperature superconductors in electrides.

cond-mat.supr-con

Statistical evaluation of 571 GaAs quantum point contact transistors showing the 0.7 anomaly in quantized conductance using millikelvin cryogenic on-chip multiplexing

The mass production and the practical number of cryogenic quantum devices producible in a single chip are limited to the number of electrical contact pads and wiring of the cryostat or dilution refrigerator. It is, therefore, beneficial to contrast the measurements of hundreds of devices fabricated in a single chip in one cooldown process to promote the scalability, integrability, reliability, and reproducibility of quantum devices and to save evaluation time, cost and energy. Here, we use a cryogenic on-chip multiplexer architecture and investigate the statistics of the 0.7 anomaly observed on the first three plateaus of the quantized conductance of semiconductor quantum point contact (QPC) transistors. Our single chips contain 256 split gate field effect QPC transistors (QFET) each, with two 16-branch multiplexed source-drain and gate pads, allowing individual transistors to be selected, addressed and controlled through an electrostatic gate voltage process. A total of 1280 quantum transistors with nano-scale dimensions are patterned in 5 different chips of GaAs heterostructures. From the measurements of 571 functioning QPCs taken at temperatures T= 1.4 K and T= 40 mK, it is found that the spontaneous polarisation model and Kondo effect do not fit our results. Furthermore, some of the features in our data largely agreed with van Hove model with short-range interactions. Our approach provides further insight into the quantum mechanical properties and microscopic origin of the 0.7 anomaly in QPCs, paving the way for the development of semiconducting quantum circuits and integrated cryogenic electronics, for scalable quantum logic control, readout, synthesis, and processing applications.

quant-ph

Quantized conductance in split gate superconducting quantum point contacts with InGaAs semiconducting two-dimensional electron systems

Quantum point contact or QPC -- a constriction in a semiconducting two-dimensional (2D) electron system with a quantized conductance -- has been found as the building block of novel spintronic, and topological electronic circuits. They can also be used as readout electronic, charge sensor or switch in quantum nanocircuits. A short and impurity-free constriction with superconducting contacts is a Cooper pairs QPC analogue known as superconducting quantum point contact (SQPC). The technological development of such quantum devices has been prolonged due to the challenges of maintaining their geometrical requirement and near-unity superconductor-semiconductor interface transparency. Here, we develop advanced nanofabrication, material and device engineering techniques and report on an innovative realisation of nanoscale SQPC arrays with split gate technology in semiconducting 2D electron systems, exploiting the special gate tunability of the quantum wells, and report the first experimental observation of conductance quantization in hybrid InGaAs-Nb SQPCs. We observe reproducible quantized conductance at zero magnetic fields in multiple quantum nanodevices fabricated in a single chip and systematically investigate the quantum transport of SQPCs at low and high magnetic fields for their potential applications in quantum metrology, for extremely accurate voltage standards, and fault-tolerant quantum technologies.

quant-ph

Experimental evidence for topological phases in the magnetoconductance of 2DEG-based hybrid junctions

While the application of out-of-plane magnetic fields was, so far, believed to be detrimental for the formation of Majorana phases in artificially engineered hybrid superconducting-semiconducting junctions, several recent theoretical studies have found it indeed useful in establishing such topological phases 1-5. Majorana phases emerge as quantized plateaus in the magnetoconductance of the hybrid junctions based on two-dimensional electron gases (2DEG) under fully out-of-plane magnetic fields. The large transverse Rashba spin-orbit interaction in 2DEG, together with a strong magneto-orbital effect, yield topological phase transitions to nontrivial phases hosting Majorana modes. Such Majorana modes are formed at the ends of 2DEG-based wires with a hybrid superconductor-semiconductor integrity. Here, we report on the experimental observation of such topological phases in Josephson junctions, based on In0.75Ga0.25As 2DEG, by sweeping out-of-plane magnetic fields of as small as 0 < B(mT) < 100 and probing the conductance to highlight the characteristic quantized magnetoconductance plateaus. Our approaches towards (i) creation and detection of topological phases in small out-of-plane magnetic fields, and (ii) integration of an array of topological Josephson junctions on a single chip pave the ways for the development of scalable quantum integrated circuits for their potential applications in fault-tolerant quantum processing and computing.

cond-mat.mes-hall