arXiv subjects

Pengfei Lan

Publications and source records attributed to Pengfei Lan.

At least 19 recordsLinked to original sources

arXiv2026

6.2-GW tabletop attosecond light source

The generation of attosecond pulses (1 as=10-18 s) has enabled real-time observation and manipulation of coherent electron dynamics, yet their low peak power has hindered the development of advanced attosecond pump-probe spectroscopy and attosecond nonlinear metrology. Here we overcome this limitation by generating 1.64 uJ, 263 as isolated attosecond pulses with a peak power of 6.2 GW, the highest pulse energy and peak power reported for a tabletop isolated attosecond source. This is achieved by combining a 2.1 TW, few-cycle (8.3 fs) two-color synthesizer with a loose focusing geometry that enables macroscopic phase-matching. The synthesizer features a stabilized carrier-envelope phase and an actively synchronized relative time delay between the two-color channels, ensuring high stability and reproducibility. This robust tabletop attosecond source enables nonlinear effect experiments that were previously inaccessible with lower-power IAPs, establishing a foundation for advanced attosecond spectroscopy and nonlinear metrology.

physics.optics↗

arXiv2026

Quantum Trajectory Separation and Attosecond Mapping in Liquid High-Harmonic Generation

High-harmonic generation (HHG) from liquids offers a potential pathway to attosecond spectroscopy in chemically complex and disordered environments, yet fundamental questions remain open: whether liquid harmonic emission preserves well-defined attosecond synchronization, and whether harmonic emission can involve simultaneous contributions from multiple quantum trajectories with distinct excursion times despite strong disorder and scattering. Here, we address these issues experimentally by resolving the trajectory-dependent temporal structure of liquid HHG. By optimizing the laser focusing geometry, we achieve clear spatial discrimination of short- and long-trajectory contributions, providing direct evidence for the existence of multiple quantum trajectories in liquids. Using a phase-controlled two-color driving field, we independently retrieve the attochirp associated with each trajectory and demonstrate opposite energy-time correlations for short and long trajectories, establishing a trajectory-resolved energy-time mapping in liquid HHG. All observations are well reproduced by semiclassical recollision simulations. These results place liquid HHG on the same conceptual footing as gas- and solid-phase HHG and establish a robust foundation for attosecond-resolved spectroscopy of ultrafast electronic and chemical dynamics in liquid environments.

physics.optics↗

arXiv2025

Quantum Path Control in High-Order Harmonic Generation via Squeezed Lights

High-order harmonic generation (HHG), a robust tabletop source for producing attosecond pulses, has been extensively utilized in attosecond metrology. Traditionally, HHG driven by classical laser fields involves two typical quantum paths (short and long quantum paths) contributing to harmonic emission. Here, we demonstrate that these quantum paths in HHG can be selectively controlled using squeezed lights, a form of non-classical light. Our results indicate that the long (short) quantum path of HHG will be dramatically suppressed in the phase (amplitude)-squeezed fields. The time-frequency analysis reveals that this quantum path control stems from the quantum fluctuations in the squeezed light, which modify the phase matching of harmonic emission from different quantum states of the squeezed light. Such a quantum path selection can be achieved for the whole harmonic plateau, which has great potential to generate ultrashort isolated attosecond pulse with duration less than one atomic unit of time.

physics.optics↗

arXiv2025

Complete suppression of the non-dipole drift effect in high harmonic generation

In high harmonic generation (HHG), non-dipole effects become increasingly significant at long driving wavelengths, as the magnetic field leads to a lateral drift of the continuum electron, which disrupts the electron recollision and inhibits the harmonic emission. To address this problem, we revisit the dynamics of the continuum electrons under electromagnetic fields in the HHG process and show that the magnetic effect on the drift includes a fundamental-frequency and a double-frequency component. By adding an additional field to counteract the double-frequency effect caused by the magnetic field, we construct an effective linearly polarized field that recovers the recollision of all returning electrons to the parent ion. Consequently, the harmonic yield is restored and becomes the same as the result within the dipole approximation across the broad spectral range. This work provides a scheme that completely suppresses the non-dipole drift effect and fully compensates for the harmonic yield reduction, paving the way to efficiently generate coherent radiation in the range from extreme ultraviolet to soft x-ray and ultrashort pulses based on HHG.

physics.optics↗

arXiv2025

Instantaneous optical selection rule for independent control of valley currents

We reveal an instantaneous optical valley selection rule that illuminates the coupling between the instantaneous optical chirality of the driving laser field and the chirality of valley systems. Building on this principle, we propose and demonstrate that a single chirality-separated optical field, in which oppositely signed instantaneous optical chiralities are separated within an optical cycle, enables independent manipulation of currents from K and K' valleys. Based on this scheme, we highlight two key example applications: (1) complete separation of currents from different valleys, yielding 100%-purity valley-polarized currents, and (2) generation of pure valley current with zero net charge flow. Our work offers a robust and highly controllable all-optical strategy for ultrafast engineering valley currents in the optical cycle timescale, paving a new avenue for valleytronics and quantum information technologies.

physics.optics↗

arXiv2025

Unveiling unique ultrafast nonlinearities in liquid-phase high-order harmonic generation

High-order harmonic generation (HHG) provides a powerful optical tool for probing ultrafast dynamics on the attosecond timescale. While its mechanisms in gases and solids are well-established, understanding nonlinear optical responses in liquids remains challenging. The absence of long-range order in liquids questions the applicability of the existing HHG models developed in other media. Through combined experimental and theoretical investigations, we identify unique characters of liquid-phase HHG -- spectral redshift and broadening, which are fundamentally distinct from both the gaseous and solid-state counterparts. Quantitative measurements and simulations of HHG in liquids illustrate a near linear dependence of harmonic redshift and broadening on the laser intensity, with the nonlinear response of water exceeding that of ethanol. The simulations reveal that these features arise from delocalized electronic states with energy loss in multiple scatterings and transient Stark shift during their transitions in laser fields. Meanwhile, we find that liquid polarity or hydrogen bond exerts decisive control over the transition dipole momentum distributions of delocalized states. Our findings establish a nonlinear spectral method for probing the internal network in liquids, paving the way for studying its role in chemical and biological processes.

physics.optics↗

arXiv2025

"Molecular waveplate" for the control of ultrashort pulses carrying orbital angular momentum

Ultrashort laser pulses carrying orbital angular momentum (OAM) have become essential tools in Atomic, Molecular, and Optical (AMO) studies, particularly for investigating strong-field light-matter interactions. However, controlling and generating ultrashort vortex pulses presents significant challenges, since their broad spectral content complicates manipulation with conventional optical elements, while the high peak power inherent in short-duration pulses risks damaging optical components. Here, we introduce a novel method for generating and controlling broadband ultrashort vortex beams by exploiting the non-adiabatic alignment of linear gas-phase molecules induced by vector beams. The interaction between the vector beam and the gas-phase molecules results in spatially varying polarizability, imparting a phase modulation to a probe laser. This process effectively creates a tunable ``molecular waveplate'' that adapts naturally to a broad spectral range. By leveraging this approach, we can generate ultrashort vortex pulses across a wide range of wavelengths. Under optimized gas pressure and interaction length conditions, this method allows for highly efficient conversion of circularly polarized light into the desired OAM pulse, thus enabling the generation of few-cycle, high-intensity vortex beams. This molecular waveplate, which overcomes the limitations imposed by conventional optical elements, opens up new possibilities for exploring strong-field physics, ultrafast science, and other applications that require high-intensity vortex beams.

physics.optics↗

arXiv2024

Attosecond All-Optical Retrieval of Valley Polarization via Circular Dichroism in Transient Absorption

We propose a scheme for retrieving the ultrafast valley polarization (VP) dynamics in two-dimensional hexagonal materials via attosecond circular dichroism (CD) transient absorption spectroscopy. This approach builds on the CD transition between the first and higher conduction bands induced by the circularly polarized probe pulses. The population imbalance at nonequivalent valleys in the first conduction band is proportionally mapped onto the difference in absorption coefficients of two probe pulses with opposite helicities, supporting an unprecedented quantitative retrieval of the corresponding VP dynamics with subfemtosecond time resolution. We theoretically demonstrate the scheme for h-BN and MoS2 through ab initio calculations, achieving an accurate retrieval of the VP dynamics, particularly the transient VP switching processes, with a time resolution of 250 as.

physics.optics↗

arXiv2024

Helicity-selected near-circularly polarized attosecond pulses generated from mixed He-Ne gases

We present and theoretically demonstrate a method for generating helicity-selected near-circularly polarized attosecond pulses in mixed He-Ne gases using bichromatic counter-rotating circularly polarized (BCCP) fields. High-order harmonics driven by BCCP fields exhibit circular polarization for individual orders in the frequency domain, but adjacent orders have opposite helicities. By utilizing the He-Ne mixture, we select only one helical component of the harmonics, resulting in the generation of highly elliptically polarized attosecond pulses in the time domain. Our analyses based on the quantum-orbit theory and the strong field approximation further clarify that the polarization of attosecond pulses is governed by the interference mechanism of high-order harmonics emitted by He and Ne. This combination of BCCP fields and an atomic mixture which requires no alignment in experiments, significantly simplifies the generation of elliptically polarized harmonics dominated by one helical component, thereby paving the way for an efficient and robust method to generate bright attosecond pulses with large ellipticity.

physics.optics↗

arXiv2024

High-purity valley-polarized currents induced by bichromatic optical fields in two-dimensional materials

Producing currents predominantly from a single valley, namely valley-polarized currents, at optical-cycle timescales is an important aspect of the petahertz valleytronics, yet it remains less developed. This work exhibits the feasibility of achieving this goal using bichromatic optical fields, which allow for the precise control of sub-cycle electron dynamics. The combined effect of the helical and asymmetric waveforms of the optical fields leads to highly asymmetric excitation at different valleys and displacement of the excited electrons concurrently, thereby inducing valley-polarized currents with high valley purity, on the sub-optical-cycle timescale. Inherently, the purity of the currents built up from the optical approach remains high even for materials with short decoherence time. Moreover, the direction of the currents can be precisely controlled by adjusting the relative phase of the bichromatic components. Our work offers a promising avenue for generating and modulating high-purity valley-polarized currents at the femtosecond timescale, facilitating the development of petahertz valleytronics.

physics.optics↗

arXiv2024

Octave-spanning supercontinuum coherent soft X-ray for producing a single-cycle soft X-ray pulse

This study demonstrates the potential to generate a soft X-ray single-cycle attosecond pulse using a single-cycle mid-infrared pulse from the advanced dual-chirped optical parametric amplification. Supercontinuum high harmonic (HH) spectrum was generated in argon (80 eV - 160 eV) and neon (150 eV - 270 eV). The experimental spectra reasonably agree with those calculated by the strong-field approximation model and Maxwell's equations. In addition, simulation results indicate that the dispersion of HHs in argon can be compensated using a 207-nm Zr filter to obtain 40 as pulses (1.1 cycles at 118 eV). For neon, a 278-nm Sn filter can compensate for dispersion of HH and create 23 as pulses (1.1 cycles at 206 eV). This soft X-ray single-cycle attosecond pulse is expected to be highly valuable for ultrafast science and applications in quantum information science.

physics.optics↗

arXiv2023

Efficient spectral broadening and few-cycle pulse generation with multiple thin water films

High-energy, few-cycle laser pulses are essential for numerous applications in the fields of ultrafast optics and strong-field physics, due to their ultrafast temporal resolution and high peak intensity. In this work, different from the traditional hollow-core fibers and multiple thin solid plates, we represent the first demonstration of the octave-spanning supercontinuum broadening by utilizing multiple ultrathin liquid films (MTLFs) as the nonlinear media. The continuum covers a range from 380 to 1050 nm, corresponding to a Fourier transform limit pulse width of 2.5 fs, when 35 fs Ti:sapphire laser pulse is applied on the MTLFs. The output pulses are compressed to 3.9 fs by employing chirped mirrors. Furthermore, a continuous high-order harmonic spectrum up to the 33rd order is realized by subjecting the compressed laser pulses to interact with Kr gas. The utilization of flowing water films eliminates permanent optical damage and enables wider and stronger spectrum broadening. Therefore, this MTLFs scheme provides new solutions for the generation of highly efficient femtosecond supercontinuum and nonlinear pulse compression, with potential applications in the fields of strong-field physics and attosecond science.

physics.optics↗

arXiv2023

High Harmonic Generation in Solids: Particle and Wave Perspectives

High harmonic generation (HHG) from gas phase atoms (or molecules) has opened up a new frontier in ultrafast optics, where attosecond time resolution and Angstrom spatial resolution are accessible. The fundamental physical pictures of HHG are always explained by the laser-induced recollision of particle-like electron motion, which lay the foundation of attosecond spectroscopy. In recent years, HHG has also been observed in solids. One can expect the extension of attosecond spectroscopy to the condensed matter if a description capable of resolving ultrafast dynamics is provided. Thus, a large number of theoretical studies have been proposed to understand the underlying physics of HHG. Here, we revisit the recollision picture in solid HHG and show some challenges of current methods with particle perspective, and present the recently developed wave perspective Huygens-Fresnel picture in understanding dynamical systems within the ambit of strong-field physics.

physics.optics↗

arXiv2022

DPIVE: A Regionalized Location Obfuscation Scheme with Personalized Privacy Levels

The popularity of cyber-physical systems is fueling the rapid growth of location-based services. This poses the risk of location privacy disclosure. Effective privacy preservation is foremost for various mobile applications. Recently, geo-indistinguishability and expected inference error are proposed for limiting location leakages. In this paper, we argue that personalization means regionalization for geo-indistinguishability, and we propose a regionalized location obfuscation mechanism called DPIVE with personalized utility sensitivities. This substantially corrects the differential and distortion privacy problem of PIVE framework proposed by Yu et al. on NDSS 2017. We develop DPIVE with two phases. In Phase I, we determine disjoint sets by partitioning all possible positions such that different locations in the same set share the Protection Location Set (PLS). In Phase II, we construct a probability distribution matrix in which the rows corresponding to the same PLS have their own sensitivity of utility (PLS diameter). Moreover, by designing QK-means algorithm for more search space in 2-D space, we improve DPIVE with refined location partition and present fine-grained personalization, enabling each location to have its own privacy level endowed with a customized privacy budget. Experiments with two public datasets demonstrate that our mechanisms have the superior performance, typically on skewed locations.

cs.CR↗

arXiv2022

All-optical spatio-temporal metrology for isolated attosecond pulses

Characterizing an isolated attosecond pulse (IAP) is essential for its potential applications. A complete characterization of an IAP ultimately requires the determination of its electric field in both time and space domains. However, previous methods, like the widely-used RABBITT and attosecond streaking, only measure the temporal profile of the attosecond pulse. Here we demonstrate an all-optical method for the measurement of the space-time properties of an IAP. By introducing a non-collinear perturbing pulse to the driving field, the process of IAP generation is modified both spatially and temporally, manifesting as a spatial and a frequency modulation in the harmonic spectrum. By using a FROG-like retrieval method, the spatio-spectral phases of the harmonic spectrum are faithfully extracted from the induced spatio-spectral modulations, which allows a thoroughgoing characterization of the IAP in both time and space. With this method, the spatio-temporal structures of the IAP generated in a two-color driving field in both the near- and far-field are fully reconstructed, from which a weak spatio-temporal coupling in the IAP generation is revealed. Our approach overcomes the limitation in the temporal measurement in conventional in situ scheme, providing a reliable and holistic metrology for IAP characterization.

physics.optics↗

arXiv2022

Fingerprint of the Interbond Electron Hopping in Second-Order Harmonic Generation

We experimentally explore the fingerprint of the microscopic electron dynamics in second-order harmonic generation (SHG). It is shown that the interbond electron hopping induces a novel source of nonlinear polarization and plays an important role even when the driving laser intensity is 2 orders of magnitude lower than the characteristic atomic field. Our model predicts anomalous anisotropic structures of the SHG yield contributed by the interbond electron hopping, which is identified in our experiments with ZnO crystals. Moreover, a generalized second-order susceptibility with an explicit form is proposed, which provides a unified description in both the weak and strong field regimes. Our work reveals the nonlinear responses of materials at the electron scale and extends the nonlinear optics to a previously unexplored regime, where the nonlinearity related to the interbond electron hopping becomes dominant. It paves the way for realizing controllable nonlinearity on an ultrafast time scale.

physics.optics↗

arXiv2021

A custom-tailored multi-TW optical electric field for gigawatt soft-x-ray isolated attosecond pulses

The bottleneck for an attosecond science experiment is concluded to be the lack of a high-peak-power isolated attosecond pulse source. Therefore, currently, generating an intense attosecond pulse would be one of the highest priority goals. In this paper, we review a TW-class parallel three-channel waveform synthesizer for generating a gigawatt-scale soft-x-ray isolated attosecond pulse (IAP) using high-order harmonics generation (HHG). Simultaneously, using several stabilization methods, namely, the low-repetition-rate laser carrier-envelope phase stabilization, Mach-Zehnder interferometer, balanced optical cross-correlator, and beam-pointing stabilizer, we demonstrate a stable 50-mJ three-channel optical-waveform synthesizer with a peak power at the multi-TW level. This optical-waveform synthesizer is capable of creating a stable intense optical field for generating an intense continuum harmonic beam thanks to the successful stabilization of all the parameters. Furthermore, the precision control of shot-to-shot reproducible synthesized waveforms is achieved. Through the HHG process employing a loose-focusing geometry, an intense shot-to-shot stable supercontinuum (50-70 eV) is generated in an argon gas cell. This continuum spectrum supports an IAP with a transform-limited duration of 170 as and a submicrojoule pulse energy, which allows the generation of a GW-scale IAP. Another supercontinuum in the soft-x-ray region with higher photon energy of approximately 100-130 eV is also generated in neon gas from the synthesizer. The transform-limited pulse duration is 106 as. According to this work, the enhancement of HHG output through optimized waveform synthesis is experimentally proved. The high-energy multicycle pulse with 10-Hz repetition rate is proved to have the same controllability for optimized waveform synthesis for HHG as few- or subcycle pulses from a 1-kHz laser.

physics.optics↗

arXiv2020

Strong field induced electron density tide in high harmonic generation from solids

In strong laser fields, the electron density in solids can show up tidal motions caused by the laser ``pulling'' on the electrons, which forms an electron density tide (EDT). However, the strong field processes in solids are always explained by the single-active-electron (SAE) model and the fluctuation of background electrons is neglected previously. Here, we demonstrate the strong field induced EDT effect and propose a model for revealing its role in high harmoinc generation (HHG) from solids. We show that the EDT effect induces an additional polarization current beyond the SAE approximation. It gives a new mechanism for HHG and leads to new anisotropic structures, which are experimentally observed with MgO. Our experiment indicates that the EDT effect becomes more obvious with increasing the laser intensity. Our work establishes the bridge between the HHG and the microscopic EDT in solids induced by the strong laser field, which paves the way to probe the ultrafast electron dynamics.

physics.optics↗