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Peter Böni

Publications and source records attributed to Peter Böni.

At least 19 recordsLinked to original sources

Quantum interferometric probe of neutron--hidden neutron oscillations

The nature of dark matter remains an outstanding problem in particle physics and cosmology. Hidden-sector extensions of the Standard Model predict a neutral partner of the neutron, whose weak mixing with ordinary neutrons induces oscillations between visible and dark baryonic states. We show that macroscopic quantum interferometry provides a direct and experimentally accessible probe of this phenomenon. In particular, a Mach--Zehnder interferometer with very cold neutrons converts neutron--hidden neutron oscillations into measurable phase-dependent intensity modulations. By combining controlled phase shifts with tunable magnetic fields and material potentials, the setup enables a resonant exploration of the hidden-sector parameter space. We find that existing cold-neutron facilities can probe mixing amplitudes down to $ε_{nn'} \sim 10^{-14}\,\mathrm{eV}$ for mass splittings $δm \sim 10^{-9}\,\mathrm{eV}$, accessing a previously unexplored region of parameter space relevant to baryonic dark matter scenarios. These results establish neutron interferometry as a precision laboratory tool for testing hidden-sector physics.

hep-ph↗

Evolution of the spin dynamics during freezing in the spin-glass Fe$_{x}$Cr$_{1-x}$

In the iron--chromium system, Fe$_{x}$Cr$_{1-x}$, a wide dome of spin-glass behavior emerges when the ferromagnetism of iron is suppressed and the antiferromagnetism of chromium emerges as a function of increasing iron content $x$. As both, the high-temperature state and the characteristic cluster size vary as a function of $x$, different regimes of spin-glass behavior may be compared in a single, isostructural material system. Here, we report a study of the spin dynamics across the freezing process into the spin-glass state for different iron concentrations ($x = 0.145$, $0.175$, $0.21$) using Modulation of IntEnsity with Zero Effort (MIEZE) spectroscopy. In the parameter range studied, the relaxation process observed experimentally may be described well in terms of a stretched exponential. In the reentrant cluster-glass regime, $x = 0.145$, this behavior persists up to high temperatures. In comparison, in the superparamagnetic regime, $x = 0.175$ and $x = 0.21$, a single relaxation time at elevated temperatures is observed. For all samples studied, the spin relaxation exhibits a momentum dependence consistent with a power law, providing evidence of a dispersive character of the spin relaxation.

cond-mat.str-el↗

Nested mirror optics for neutron extraction, transport, and focusing

Neutron scattering is a well-established tool for the investigation of the static and dynamic properties of condensed matter systems over a wide range of spatial and temporal scales. Many studies of high interest, however, can only be performed on small samples and typically require elaborate environments for variation of parameters such as temperature, magnetic field and pressure. To improve the achievable signal-to-background ratio, focusing devices based on elliptic or parabolic neutron guides or Montel mirrors have been implemented. Here we report an experimental demonstration of a nested mirror optics (NMO), which overcomes some of the disadvantages of such devices. While even simpler than the original Wolter design, our compact assembly of elliptic mirrors images neutrons from a source to a target, minimizing geometric aberrations, gravitational effects and waviness-induced blurring. Experiments performed at MIRA at FRM-II demonstrate the expected focusing properties and a beam transport efficiency of 72 % for our first prototype. NMO seem particularly well-suited to i) extraction of neutrons from compact high-brilliance neutron moderators, ii) general neutron transport, and iii) focusing and polarizing neutrons. The phase space of the neutrons hitting a sample can be tailored on-line to the needed experimental resolution, resulting in small scattering backgrounds. As additional benefits, NMO situated far away from both the moderator and the sample are less susceptible to radiation damage and can easily be replaced. NMO enable a modular and physically transparent realization of beam lines for neutron physics similar to setups used in visible light optics.

physics.ins-det↗

A Design Study of a Compact Small-Angle Neutron Scattering Instrument

Nanoscale structure determination belongs to one of the crucial tasks in materials science. Small-angle neutron scattering (SANS) is a highly valuable tool to investigate nanostructures. Here, we explore the possibility of a compact SANS instrument to be installed at an individual accelerator based pulsed low-flux source, and discuss applications in structural characterization, education, and training. Monte Carlo simulations of a realistic setup demonstrate the feasibility of such an instrument, with an ideal measurement taking about 7 hours. The anticipated length-scale measurement range is 0.5 nm to 50 nm. The minimalistic design results in an easy to operate, low maintenance instrument, independent of the schedules of large-scale facilities. Size, cost, and maintenance are comparable to laboratory small-angle X-ray scattering (SAXS) instruments, which makes SANS affordable for individual research teams at universities and provides unique chances for education and training. The proposed setup creates the opportunity to measure ultraslow structural changes, at a fraction of the cost of existing SANS instruments, hence enables weekly or monthly repetition rates. The concept can be expanded to an entire suite of instruments, including wide-angle neutron scattering (WANS) and diffraction, neutron reflectometry (NR), neutron radiography, grating interferometry (GI), and prompt gamma activation analysis (PGAA).

physics.ins-det↗

Phase Reconstruction of a Cu(001) Seed Layer from $\textit{in situ}$ Polarized Neutron Reflectometry Data using Fe Reference Layers

The reconstruction of the complex reflection coefficient obtained by in situ Polarized Neutron Reflectometry is presented. Using the reference layer method, with a magnetic Fe layer, the phase information of the underlying Cu(001) seed layer sample structure is successfully retrieved and its scattering length density is calculated and compared with results obtained from traditional fitting. Two different reference layer approaches for retrieving the phase information are compared.

cond-mat.mtrl-sci↗

Fermi-Surface Modeling of Light-Rare-Earth Hexaborides with 2D-ACAR Spectroscopy

Two dimensional angular correlation of the positron annihilation radiation (2D-ACAR) spectra are measured for $\mathrm{LaB}_6$ along high symmetry directions and compared with first principle calculations based on density functional theory (DFT). This allows the modeling of the Fermi surface in terms of ellipsoid electron pockets centered at $X$-points elongated along the $Σ$ axis (${Γ-M}$ direction). The obtained structure is in agreement with quantum oscillation measurements and previous band structure calculations. For the isostructural topologically not-trivial $\mathrm{SmB}_6$ the similar ellipsoids are connected through necks that have significantly smaller radii in the case of $\mathrm{LaB}_6$. A theoretical analysis of the 2D-ACAR spectra is also performed for $\mathrm{CeB}_6$ including the on-site repulsion $U$ correction to the local-density approximation (LDA+$U$) of the DFT. The similarities of 2D-ACAR spectra and the Fermi-surface projections of these two compounds allow to infer that both $\mathrm{LaB}_6$ and $\mathrm{CeB}_6$ are topologically trivial correlated metals.

cond-mat.mtrl-sci↗

MIEZE Neutron Spin-Echo Spectroscopy of Strongly Correlated Electron Systems

Recent progress in neutron spin-echo spectroscopy by means of longitudinal Modulation of IntEnsity with Zero Effort (MIEZE) is reviewed. Key technical characteristics are summarized which highlight that the parameter range accessible in momentum and energy, as well as its limitations, are extremely well understood and controlled. Typical experimental data comprising quasi-elastic and inelastic scattering are presented, featuring magneto-elastic coupling and crystal field excitations in Ho2Ti2O7, the skyrmion lattice to paramagnetic transition under applied magnetic field in MnSi, ferromagnetic criticality and spin waves in Fe. In addition bench marking studies of the molecular dynamics in H2O are reported. Taken together, the advantages of MIEZE spectroscopy in studies at small and intermediate momentum transfers comprise an exceptionally wide dynamic range of over seven orders of magnitude, the capability to perform straight forward studies on depolarizing samples or under depolarizing sample environments, as well as on incoherently scattering materials.

cond-mat.str-el↗

The longitudinal neutron resonant spin echo spectrometer RESEDA

The instrumental layout and technical realisation of the neutron resonant spin echo (NRSE) spectrometer RESEDA at the Heinz Maier-Leibnitz Zentrum (MLZ) in Garching, Germany, is presented. RESEDA is based on a longitudinal field configuration, boosting both dynamic range and maximum resolution of the spectrometer compared to the conventional transverse layout. The resonant neutron spin echo technique enables the realisation of two complementary implementations: A longitudinal NRSE (LNRSE) option comparable to the classical neutron spin echo (NSE) method for highest energy resolution and large momentum transfers as well as a Modulation of Intensity with Zero Effort (MIEZE) option for depolarising samples or sample environments such as high magnetic fields, and strong incoherent scattering samples. With their outstanding dynamic range, exceeding nominally seven orders of magnitude, both options cover new fields for ultra-high resolution neutron spectroscopy in hard and soft condensed matter systems. In this paper the concept of RESEDA as well as the technical realisation along with reference measurements are reported.

physics.ins-det↗

Polarized inelastic neutron scattering of non-reciprocal spin waves in MnSi

We report spin-polarized inelastic neutron scattering of the dynamical structure factor of the conical magnetic helix in the cubic chiral magnet MnSi. We find that the spectral weight of spin-flip scattering processes is concentrated on single branches for wavevector transfer parallel to the helix axis as inferred from well-defined peaks in the neutron spectra. In contrast, for wavevector transfers perpendicular to the helix the spectral weight is distributed among different branches of the magnon band structure as reflected in broader features of the spectra. Taking into account the effects of instrumental resolution, our experimental results are in excellent quantitative agreement with parameter-free theoretical predictions. Whereas the dispersion of the spin waves in MnSi appears to be approximately reciprocal at low energies and small applied fields, the associated spin-resolved spectral weight displays a pronounced non-reciprocity that implies a distinct non-reciprocal response in the limit of vanishing uniform magnetization at zero magnetic field.

cond-mat.str-el↗

Indications for Dzyaloshinskii-Moriya Interaction at the Pd/Fe Interface Studied by \textit{In Situ} Polarized Neutron Reflectometry

Using \textit{in situ} polarized neutron reflectometry, the depth resolved evolution of the magnetism and structure in a Pd/Fe/Pd trilayer thin-film is measured during growth. The initial film structure of Pd/Fe shows a small proximity induced magnetism in the underlayer and a magnetization in the Fe layer of $\approx1.6$\,$μ_{\text{B}}$ per Fe atom, less than the expected bulk value of $2.2$\,$μ_{\text{B}}$. Deposition of the Pd capping layer initially follows an island-like growth mode with subsequent coalescence. With increasing Pd deposition the Fe moment and the proximity-induced magnetism in the Pd capping layer decrease. After final deposition of the Pd capping layer, the magnetic profile is structurally and magnetically symmetric across the Fe layer, with magnetism induced in Pd up to 0.92 \,nm from the interface. Throughout the Pd deposition the Pd/Fe/Pd trilayer structure is becoming increasingly symmetric, a fact which points to a Dzyaloshinskii-Moriya interaction as a likely cause of the observed magnetic behavior.

cond-mat.mtrl-sci↗

Non-reciprocal magnons in non-centrosymmetric MnSi

Using two cold-neutron triple-axis spectrometers we have succeeded in fully mapping out the field-dependent evolution of the non-reciprocal magnon dispersion relations in all magnetic phases of MnSi. The non-reciprocal nature of the dispersion manifests itself in a full asymmetry (non-reciprocity) of the dynamical structure factor $S(q, E, μ_0 H_{int})$ with respect to flipping either the direction of the applied magnetic field $μ_0 H_{int}$, the reduced momentum transfer $q$, or the energy transfer $E$.

cond-mat.str-el↗

Field dependence of non-reciprocal magnons in chiral MnSi

Spin waves in chiral magnetic materials are strongly influenced by the Dzyaloshinskii-Moriya interaction resulting in intriguing phenomena like non-reciprocal magnon propagation and magnetochiral dichroism. Here, we study the non-reciprocal magnon spectrum of the archetypical chiral magnet MnSi and its evolution as a function of magnetic field covering the field-polarized and conical helix phase. Using inelastic neutron scattering, the magnon energies and their spectral weights are determined quantitatively after deconvolution with the instrumental resolution. In the field-polarized phase the imaginary part of the dynamical susceptibility $χ''(\varepsilon, {\bf q})$ is shown to be asymmetric with respect to wavevectors ${\bf q}$ longitudinal to the applied magnetic field ${\bf H}$, which is a hallmark of chiral magnetism. In the helimagnetic phase, $χ''(\varepsilon, {\bf q})$ becomes increasingly symmetric with decreasing ${\bf H}$ due to the formation of helimagnon bands and the activation of additional spinflip and non-spinflip scattering channels. The neutron spectra are in excellent quantitative agreement with the low-energy theory of cubic chiral magnets with a single fitting parameter being the damping rate of spin waves.

cond-mat.str-el↗

Design and realization of a sputter deposition system for the \textit{in situ-} and \textit{in operando-}use in polarized neutron reflectometry experiments

We report on the realization of a sputter deposition system for the in situ- and in operando-use in polarized neutron reflectometry experiments. Starting with the scientific requirements, which define the general design considerations, the external limitations and boundaries imposed by the available space at a neutron beamline and by the neutron and vacuum compatibility of the used materials, are assessed. The relevant aspects are then accounted for in the realization of our highly mobile deposition system, which was designed with a focus on a quick and simple installation and removability at the beamline. Apart from the general design, the in-vacuum components, the auxiliary equipment and the remote control via a computer, as well as relevant safety aspects are presented in detail.

physics.ins-det↗

Application of a Portable $^3$He-Based Polarization Insert at a Time-of-Flight Neutron Reflectometer

The suitability of a transportable 3He-spin filter as temporary broadband polarizer for a Time-of-Flight neutron reflectometer is demonstrated. A simple two-wavelength method for characterisation of a 3He-spin filter is proposed, which can be applied even if the absolute transmittance of the 3He-spin filter cannot be accurately determined. We demonstrate the data treatment procedure for extracting the spin-up and spin-down neutron reflectivity from measurements obtained with a time dependent 3He polarization. The extraction of a very weak magnetic signal from reflectivity data, measured on the in-situ grown magnetic heterostructure Fe1 nm/Cu20 nm/Sisubstrate in an externally applied magnetic field of 30mT is presented and compared to similar measurements on the growth stage Cu20 nm/Sisubstrate of the very same sample, which does not yet contain any magnetic material.

physics.ins-det↗

In-situ Polarized Neutron Reflectometry: Epitaxial Thin Film Growth of Fe on Cu(001) by DC Magnetron Sputtering

The step-wise growth of epitaxial Fe on Cu(001)/Si(001), investigated by in-situ polarized neutron reflectometry is presented. A sputter deposition system was integrated into the neutron reflectometer AMOR at the Swiss neutron spallation source SINQ, which enables the analysis of the microstructure and magnetic moments during all deposition steps of the Fe layer. We report on the progressive evolution of the accessible parameters describing the microstructure and the magnetic properties of the Fe film, which reproduce known features and extend our knowledge on the behavior of ultrathin iron films.

cond-mat.mtrl-sci↗

Dipolar effects on the critical fluctuations in Fe: Investigation by MIEZE

Iron is one of the archetypical ferromagnets to study the critical fluctuations at a continuous phase transition thus serving as a model system for the application of scaling theory. We report a comprehensive study of the critical dynamics at the transition from the ferro- to the paramagnetic phase in Fe, employing the high-resolution neutron spin echo technique MIEZE. The results show that the dipolar interactions lead to an additional damping of the critical spin fluctuations at small momentum transfers $\bf q$. The results agree essentially with scaling theory if the dipolar interactions are taken into account by means of the mode-coupling equations. However, in contrast to expectations, the dipolar wavenumber $q_D$ that plays a central role in the scaling function $f(κ/q,q_D/κ)$ becomes temperature dependent. In the limit of small $\bf q$ the critical exponent $z$ crosses over from 2.5 to 2.0.

cond-mat.str-el↗

RESPECT: Neutron Resonance Spin-Echo Spectrometer for Extreme Studies

We propose the design of a Resonance SPin-echo spECtrometer for exTreme studies, RESPECT, that is ideally suited for the exploration of non-dispersive processes such as diffusion, crystallization, slow dynamics, tunneling processes, crystal electric field excitations, and spin fluctuations. It is a variant of the conventional neutron spin-echo technique (NSE) by i) replacing the long precession coils by pairs of longitudinal neutron spin-echo coils combined with RF-spin flippers and ii) by stabilizing the neutron polarization with small longitudinal guide fields that can in addition be used as field subtraction coils thus allowing to adjust the field integrals over a range of 8 orders of magnitude. Therefore, the dynamic range of RESPECT can in principle be varied over 8 orders of magnitude in time, if neutrons with the required energy are made available. Similarly as for existing NSE-spectrometers, spin echo times of up to approximately 1 microsecond can be reached if the divergence and the correction elements are properly adjusted. Thanks to the optional use of neutron guides and the fact that the currents for the correction coils are much smaller than in standard NSE, intensity gains of at least one order of magnitude are expected , making the concept of RESPECT also competitive for operation at medium flux neutron sources. RESPECT can also be operated in a MIEZE configuration allowing the investigation of relaxation processes in depolarizing environments as they occur when magnetic fields are applied at the sample position, i.e. for the investigation of the dynamics of flux lines in superconductors, magnetic fluctuations in ferromagnetic materials, and samples containing hydrogen.

physics.ins-det↗

Neutron depolarization imaging of the hydrostatic pressure dependence of inhomogeneous ferromagnets

The investigation of fragile and potentially inhomogeneous forms of ferromagnetic order under extreme conditions, such as low temperatures and high pressures, is of central interest for areas such as geophysics, correlated electron systems, as well as the optimization of materials synthesis for applications where particular material properties are required. We report neutron depolarization imaging measurements on the weak ferromagnet Ni$_3$Al under pressures up to 10kbar using a Cu:Be clamp cell. Using a polychromatic neutron beam with wavelengths $λ\geq$ 4Åin combination with $^3$He neutron spin filter cells as polarizer and analyzer we were able to track differences of the pressure response in inhomogeneous samples by virtue of high resolution neutron depolarization imaging. This provides spatially resolved and non-destructive access to the pressure dependence of the magnetic properties of inhomogeneous ferromagnetic materials.

cond-mat.str-el↗