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Peter B. Littlewood

Publications and source records attributed to Peter B. Littlewood.

At least 19 recordsLinked to original sources

Critical scaling in one-dimensional non-reciprocal matter

Unveiling universal non-equilibrium scaling laws has been a central theme in modern statistical physics, with recent attention increasingly directed toward non-equilibrium phases that exhibit rich dynamical phenomena. A striking example arises in non-reciprocal systems, where asymmetric interactions between components lead to inherently dynamic phases and unconventional criticality near a critical exceptional point (CEP), where the criticality arises from the coalescence of collective modes with an existing Nambu-Goldstone mode. However, the scaling behavior that emerges in this system with full consideration of many-body effects and stochastic noise remains largely elusive. Here, we establish a dynamical scaling law in a generic one-dimensional (1D) stochastic non-reciprocal $O(2)$-symmetric system. Through large-scale simulations, we uncover a new non-equilibrium scaling in the vicinity of the CEP, distinct from any previously known equilibrium or non-equilibrium universality classes. We report an anomalously large roughening exponent $α_{\rm CEP}=1.35(5)$, which is to be compared with those of simple diffusion $α_{\rm EW}=1/2$. In regimes where the system breaks into domains with opposite chirality and spatiotemporal vortices inevitably emerge, we find that fluctuations are strongly suppressed, leading to a logarithmic scaling as a function of system size $L$ that manifests a short-range correlation. This work elucidates the beyond-mean-field dynamics of non-reciprocal matter, thereby shedding light on the exploration of criticality in non-reciprocal phase transition across diverse physical contexts, from active matter and driven quantum systems to biological pattern formation and non-Hermitian physics.

cond-mat.stat-mech↗

Spin-only dynamics of the multi-species nonreciprocal Dicke model

The Hepp-Lieb-Dicke model is ubiquitous in cavity quantum electrodynamics, describing spin-cavity coupling which does not conserve excitation number. Coupling the closed spin-cavity system to an environment realizes the open Dicke model, and by tuning the structure of the environment or the system-environment coupling, interesting spin-only models can be engineered. In this work, we focus on a variation of the multi-species open Dicke model which realizes mediated nonreciprocal interactions between the spin species and, consequently, a dynamical limit-cycle phase. In particular, we improve upon adiabatic elimination and, instead, employ a Redfield master equation in order to describe the effective dynamics of the spin-only system. We assess this approach at the mean-field level, comparing it both to adiabatic elimination and the full spin-cavity model, and find that the predictions are sensitive to the presence of single-particle incoherent decay. Additionally, we clarify the symmetries of the model and explore the dynamical limit-cycle phase in the case of explicit PT-symmetry breaking, finding a region of phase coexistence terminating at an codimension-two exceptional point. Lastly, we go beyond mean-field theory by exact numerical diagonalization of the master equation, appealing to permutation symmetry in order to increase the size of accessible systems. We find signatures of phase transitions even for small system sizes.

cond-mat.quant-gas↗

Theory of two-component superfluidity of microcavity polaritons

We develop a microscopic mean-field theory describing the coexistence of Bose-Einstein condensates of upper and lower polaritons (UP/LP) in a semiconductor microcavity. Incorporating interbranch scattering within a modified polariton Hamiltonian, we introduce a phenomenological population-split parameter $α$ that quantifies the relative LP/UP occupations. At zero detuning, the critical temperature becomes independent of $α$, converging to a single value that marks the balanced, resonant regime. Away from resonance, variations in $α$ lead to distinctive and experimentally resolvable changes in both the sound velocity $c_s$ and critical temperature $T_c$, relative to the single-component (LP-only) condensate limit. The system under study consists of excitons confined in a transition metal dichalcogenide (TMDC) monolayer, particularly WSe$_2$ embedded within a planar optical microcavity of GaAs where they strongly couple to cavity photons. Our analysis focuses on monolayer WSe$_2$ embdedded in a GaAs microcavity. We present results for GaAs/AlGaAs quantum wells embedded in a GaAs microcavity in the Appendix. While mean-field in scope, the framework provides analytic benchmarks and physical insight for future treatments that include dissipation and fluctuations in nonequilibrium polariton superfluids.

cond-mat.quant-gas↗

Phase Transitions in Nonreciprocal Driven-Dissipative Condensates

We investigate the influence of boundaries and spatial nonreciprocity on nonequilibrium driven-dissipative phase transitions. We focus on a one-dimensional lattice of nonlinear bosons described by a Lindblad master equation, where the interplay between coherent and incoherent dynamics generates nonreciprocal interactions between sites. Using a mean-field approach, we analyze the phase diagram under both periodic and open boundary conditions. For periodic boundaries, the system always forms a condensate at nonzero momentum and frequency, resulting in a time-dependent traveling wave pattern. In contrast, open boundaries reveal a far richer phase diagram, featuring multiple static and dynamical phases, as well as exotic phase transitions, including the spontaneous breaking of particle-hole symmetry associated with a critical exceptional point and phases with distinct bulk and edge behavior. Our model does not require post-selection and is experimentally realizable in platforms such as superconducting circuits.

quant-ph↗

Optical probes of coherence in two dimensional Bose gases of polaritons

Due to their photonic components, exciton-polariton systems provide a convenient platform to study the coherence properties of weakly-interacting Bose gases. In particular, optical interferometry enables the measurement of the first-order coherence function which provides information about the intrinsic correlations of the system. In this paper, we derive a universal curve for the coherent fraction of a noninteracting, equilibrium, homogeneous, two-dimensional Bose gas, with density expressed in units of the observation area, and compare to recent experimental results. Although there is a sharp transition from normal to superfluid phases in the thermodynamic limit, the coherent fraction of the gas varies continuously across this transition due to the finite system size. We find that the theory agrees nearly perfectly with the experimental data in the low-density limit with no free parameters other than the effective temperature, highly constrained by the measurements. At higher density, the experiments are consistent with standard weakly-interacting Bose gas theory. By having a theory that treats both the optical diffraction and Bose coherence, we can clearly see the effect of the quantum statistics on the coherence.

cond-mat.quant-gas↗

Field Theory of Birhythmicity

Non-equilibrium dynamics are present in many aspects of our lives, ranging from microscopic physical systems to the functioning of the brain. What characterizes stochastic models of non-equilibrium processes is the breaking of the fluctuation-dissipation relations as well as the existence of non-static stable states, or phases. A prototypical example is a dynamical phase characterized by a limit cycle - the order parameter of finite magnitude rotating or oscillating at a fixed frequency. Consequently, birhythmicity, where two stable limit cycles coexist, is a natural extension of the simpler single limit cycle phase. Both the abundance of real systems exhibiting such states as well as their relevance for building our understanding of non-equilibrium phases and phase transitions are strong motivations to build and study models of such behavior. Field theoretic tools can be used to provide insights into either phase and the transition between them. In this work we explore a simple linear model of the single limit cycle phase with phase-amplitude coupling. We demonstrate how such non-equilibrium coupling affects the fluctuation spectrum of the theory. We then extend this model to include a continuous transition to a two-cycle phase. We give various results, such as an appearance of a critical exceptional point, the destruction of the transition, enhancement of noise for the phase and the presence of KPZ dynamics. Finally, we qualitatively demonstrate these results with numerics and discuss future directions.

cond-mat.stat-mech↗

Gaussian fluctuations of non-reciprocal systems

Non-reciprocal systems can be thought of as disobeying Newtons third law - an action does not cause an equal and opposite reaction. In recent years there has been a dramatic rise in interest towards such systems. On a fundamental level, they can be a basis of describing non-equilibrium and active states of matter, with applications ranging from physics to social sciences. However, often the first step to understanding complex nonlinear models is to linearize about the steady states. It is thus useful to develop a careful understanding of linear non-reciprocal systems, similar to our understanding of Gaussian systems in equilibrium statistical mechanics. In this work we explore simplest linear non-reciprocal models with noise and spatial extent. We describe their regions of stability and show how non-reciprocity can enhance the stability of a system. We demonstrate the appearance of exceptional and critical exceptional points with the respective enhancement of fluctuations for the latter. We show how strong non-reciprocity can lead to a finite-momentum instability. Finally, we comment how non-reciprocity can be a source of colored, $1/f$ type noise.

cond-mat.stat-mech↗

Exceptional points in nonlinear and stochastic dynamics

We study a class of bifurcations generically occurring in dynamical systems with non-mutual couplings ranging from models of coupled neurons to predator-prey systems and non-linear oscillators. In these bifurcations, extended attractors such as limit cycles, limit tori, and strange attractors merge and split in a similar way as fixed points in a pitchfork bifurcation. We show that this merging and splitting coincides with the coalescence of covariant Lyapunov vectors with vanishing Lyapunov exponents, generalizing the notion of exceptional points to non-linear dynamical systems. We distinguish two classes of bifurcations, corresponding respectively to continuous and discontinuous behaviors of the covariant Lyapunov vectors at the transition. We outline some physical consequences of generalized exceptional points on the dynamics of the system, including non-reciprocal responses, the destruction of isochrons, and enhanced sensitivity to noise. We illustrate our results with concrete examples from neuroscience, ecology, and physics. When applied to interpret existing experimental observations, our analysis suggests a simple explanation for the non-trivial phase delays observed in the population dynamics of plankton communities and the recently measured statistics of rotation reversals for a solid body immersed in a Rayleigh-Bénard convection cell.

nlin.CD↗

Coalescence of limit cycles in the presence of noise

Complex dynamical systems may exhibit multiple steady states, including time-periodic limit cycles, where the final trajectory depends on initial conditions. With tuning of parameters, limit cycles can proliferate or merge at an exceptional point. Here we ask how dynamics in the vicinity of such a bifurcation are influenced by noise. A pitchfork bifurcation can be used to induce bifurcation behavior. We model a limit cycle with the normal form of the Hopf oscillator, couple it to the pitchfork, and investigate the resulting dynamical system in the presence of noise. We show that the generating functional for the averages of the dynamical variables factorizes between the pitchfork and the oscillator. The statistical properties of the pitchfork in the presence of noise in its various regimes are investigated and a scaling theory is developed for the correlation and response functions. The analysis is done by perturbative calculations as well as numerical means. Finally, observables illustrating the coupling of a system with a limit cycle to a pitchfork are discussed and the phase-phase correlations are shown to exhibit non-diffusive behavior with universal scaling.

cond-mat.stat-mech↗

Dynamic crystallography reveals spontaneous anisotropy in cubic GeTe

Cubic energy materials such as thermoelectrics or hybrid perovskite materials are often understood to be highly disordered. In GeTe and related IV-VI compounds, this is thought to provide the low thermal conductivities needed for thermoelectric applications. Since conventional crystallography cannot distinguish between static disorder and atomic motions, we develop the energy-resolved variable-shutter pair distribution function technique. This collects structural snapshots with varying exposure times, on timescales relevant for atomic motions. In disagreement with previous interpretations, we find the time-averaged structure of GeTe to be crystalline at all temperatures, but with anisotropic anharmonic dynamics at higher temperatures that resemble static disorder at fast shutter speeds, with correlated ferroelectric fluctuations along the $<$100$>$c direction. We show that this anisotropy naturally emerges from a Ginzburg-Landau model that couples polarization fluctuations through long-range elastic interactions. By accessing time-dependent atomic correlations in energy materials, we resolve the long-standing disagreement between local and average structure probes, and show that spontaneous anisotropy is ubiquitous in cubic IV-VI materials.

cond-mat.mtrl-sci↗

Going Beyond the Cumulant Approximation II:Power Series Correction to Single Particle Green's Function in 1D Holstein Chain

Previously, we introduced a method for systematically correcting a quasiparticle green's function via a power series expansion. Here we present an ODE based formalisms of power series correction that goes beyond the cumulant approximation and implement it to 1D Holstein chain for a wide range of coupling strengths in a scalable and inexpensive fashion at both zero and finite temperature. We show that this first differential formalism of the power series is both qualitatively and quantitatively in excellent agreement with exact diagonalization results on 1D Holstein chain with dispersive bosons for a large range of electron-boson coupling strength. We investigate carrier mass growth rate and carrier energy displacement across a wide range of coupling strength. Finally, we present a heuristic argument which predicts most of the rich satellite structure without explicit calculation.

cond-mat.mtrl-sci↗

Quantum Melting in a Polariton Lattice

Inspired by the recent experimental observation of strongly coupled polaritons in a Moiré heterobilayer, we study a model of dipole-interacting excitons localized on sites of a lattice and coupled to planar cavity photons. We calculate the phase diagram of this system by computing fluctuations around the mean field and determining the stability of the excitation spectrum. We find that the transition from the normal state to a polariton condensate is intermediated by a series of ordered states at partial fillings of the exciton lattice, stabilized by the exciton interactions. In particular we predict a supersolid phase in which a polariton condensate coexists with spatial order.

cond-mat.str-el↗

Semi-metallicity and electron-hole liquid in two-dimensional C and BN based compounds

Insulating-metallic transition mediated by substitutional atoms is predicted in a series of two-dimensional carbon-based structures. Introducing Si atoms in selected sites of tetrahexcarbon [Carbon 137 (2018) 266] according to rational chemical rules, metallicity by trivial band inversion without band gap opening is induced. Additional substitution of remaining C atoms by BN dimers introduces no changes in the metallic properties. A series of isomorphous two-dimensional materials with isoelectronic structures derived by exchanging group IV elements exhibiting various band gaps is obtained. Dynamical stability is verified with phonon analysis and beyond the harmonic approximation with molecular dynamics up to room temperature. The semi-metallic compounds have well-nested pockets of carriers and are good candidates for the formation of an excitonic insulator.

cond-mat.mtrl-sci↗

Going Beyond the Cumulant Approximation: Power Series Correction to Single Particle Green's Function in Holstein System

In the context of a single electron two orbital Holstein system coupled to dispersionless bosons, we develop a general method to correct single particle Green's function using a power series correction(PSC) scheme. We then outline the derivations of various flavors of cumulant approximation through the PSC scheme and explain the assumptions and approximations behind them. Finally, we compute and compare PSC spectral function with cumulant and exact diagonalized spectral functions and elucidate three regimes of this problem - two that cumulant explains and one where cumulant fails. We find that the exact and the PSC spectral functions match within spectral broadening across all three regimes.

cond-mat.str-el↗

Exploring Metastable States in UO$_2$ using Hybrid Functionals and Dynamical Mean Field Theory

A detailed exploration of the $f$-atomic orbital occupancy space for UO$_2$ is performed using a first principles approach based on density functional theory (DFT), employing a full hybrid functional within a systematic basis set. Specifically, the PBE0 functional is combined with an occupancy biasing scheme implemented in a wavelet-based algorithm which is adapted to large supercells. The results are compared with previous DFT+U calculations reported in the literature, while dynamical mean field theory (DMFT) is also performed to provide a further base for comparison. This work shows that the computational complexity of the energy landscape of a correlated $f$-electron oxide is much richer than has previously been demonstrated. The resulting calculations provide evidence of the existence of multiple previously unexplored metastable electronic states of UO$_2$, including those with energies which are lower than previously reported ground states.

cond-mat.str-el↗

Non-reciprocal phase transitions

Out of equilibrium, the lack of reciprocity is the rule rather than the exception. Non-reciprocal interactions occur, for instance, in networks of neurons, directional growth of interfaces, and synthetic active materials. While wave propagation in non-reciprocal media has recently been under intense study, less is known about the consequences of non-reciprocity on the collective behavior of many-body systems. Here, we show that non-reciprocity leads to time-dependent phases where spontaneously broken symmetries are dynamically restored. The resulting phase transitions are controlled by spectral singularities called exceptional points. We describe the emergence of these phases using insights from bifurcation theory and non-Hermitian quantum mechanics. Our approach captures non-reciprocal generalizations of three archetypal classes of self-organization out of equilibrium: synchronization, flocking and pattern formation. Collective phenomena in these non-reciprocal systems range from active time-(quasi)crystals to exceptional-point enforced pattern-formation and hysteresis. Our work paves the way towards a general theory of critical phenomena in non-reciprocal matter.

cond-mat.soft↗

Critical fluctuations at a many-body exceptional point

Critical phenomena arise ubiquitously in various context of physics, from condensed matter, high energy physics, cosmology, to biological systems, and consist of slow and long-distance fluctuations near a phase transition or critical point. Usually, these phenomena are associated with the softening of a massive mode. Here we show that a novel, non-Hermitian-induced mechanism of critical phenomena that do not fall into this class can arise in the steady state of generic driven-dissipative many-body systems with coupled binary order parameters such as exciton-polariton condensates and driven-dissipative Bose-Einstein condensates in a double-well potential. The criticality of this ``critical exceptional point'' is attributed to the coalescence of the collective eigenmodes that convert all the thermal-and-dissipative-noise activated fluctuations to the Goldstone mode, leading to anomalously giant phase fluctuations that diverge at spatial dimensions $d\le 4$. Our dynamic renormalization group analysis shows that this gives rise to a strong-coupling fixed point at dimensions as high as $d<8$ associated with a new universality class beyond the classification by Hohenberg and Halperin, indicating how anomalously strong the many-body corrections are at this point. We find that this anomalous enhancement of many-body correlation is due to the appearance of a sound mode at the critical exceptional point despite the system's dissipative character.

cond-mat.stat-mech↗

Superconductivity in the dilute single band limit in reduced Strontium Titanate

We report on superconductivity in single crystals of SrTiO$_{3-δ}$ with carrier densities $\textit{n} < 1.4 \times10^{18}cm^{-3}$, where only a single band is occupied. For all samples in this regime, the resistive transition occurs at $T_{c} \approx 65 \pm 25 \ mK$. We observe a zero resistance state for $\textit{n}$ as low as $1.03 \times10^{17}cm^{-3}$, and a partial resistive transition for $\textit{n} = 3.85 \times10^{16}cm^{-3}$. We observe low critical current densities, relatively high and isotropic upper critical fields, and an absence of diamagnetic screening in these samples. Our findings suggest an inhomogeneous superconducting state, embedded within a homogeneous high-mobility 3-dimensional electron gas. $T_{c}$ does not vary appreciably when $\textit{n}$ changes by more than an order of magnitude, inconsistent with conventional superconductivity.

cond-mat.supr-con↗