arXiv subjects

Peter Karlsen

Publications and source records attributed to Peter Karlsen.

4 recordsLinked to original sources

arXiv2020

Total internal reflection based super-resolution imaging for sub-IR frequencies

For measurements designed to accurately determine layer thickness, there is a natural trade-off between sensitivity to optical thickness and lateral resolution due to the angular ray distribution required for a focused beam. We demonstrate a near-field imaging approach that enables both sub-wavelength lateral resolution and optical thickness sensitivity. We illuminate a sample in a total internal reflection geometry, with a photo-activated spatial modulator in the near-field, which allows optical thickness images to be computationally reconstructed in a few seconds. We demonstrate our approach at 140 GHz (wavelength 2.15 mm), where images are normally severely limited in spatial resolution, and demonstrate mapping of optical thickness variation in inhomogeneous biological tissues.

physics.app-ph↗

arXiv2019

Approximations used in the analysis of signals in pump-probe spectroscopy

In pump-probe spectroscopy, one often needs to analyse the transmission or reflection of electromagnetic waves through optically pumped media. Here, it is common practice to approximate the analysis in order to extract non-equilibrium values for the optical constants of the media. Concentrating on optical pump-THz probe spectroscopy, and using the transfer matrix approach, we present a general method for evaluating the applicability of the most common approximations. Somewhat surprisingly, we find that these approximations are truly valid only in extreme cases where the optical thickness of the sample is several orders of magnitude smaller or larger than the probe wavelength.

physics.optics↗

arXiv2018

Sign inversion in the terahertz photoconductivity of single-walled carbon nanotube films

In recent years, there have been conflicting reports regarding the ultrafast photoconductive response of films of single walled carbon nanotubes (CNTs), which apparently exhibit photoconductivities that can differ even in sign. Here, we observe explicitly that the THz photoconductivity of CNT films is a highly variable quantity which correlates with the length of the CNTs, while the chirality distribution has little influence. Moreover, by comparing the photo-induced change in THz conductivity with heat-induced changes, we show that both occur primarily due to heat-generated modification of the Drude electron relaxation rate, resulting in a broadening of the plasmonic resonance present in finite-length metallic and doped semiconducting CNTs. This clarifies the nature of the photo-response of CNT films and demonstrates the need to carefully consider the geometry of the CNTs, specifically the length, when considering them for application in optoelectronic devices.

cond-mat.mes-hall↗

arXiv2017

Influence of nanotube length and density on the plasmonic terahertz response of single-walled carbon nanotubes

We measure the conductivity spectra of thin films comprising bundled single-walled carbon nanotubes (CNTs) of different average lengths in the frequency range 0.3-1000 THz and temperature interval 10-530 K. The observed temperature-induced changes in the terahertz conductivity spectra are shown to depend strongly on the average CNT length, with a conductivity around 1 THz that increases/decreases as the temperature increases for short/long tubes. This behaviour originates from the temperature dependence of the electron scattering rate, which we obtain from Drude fits of the measured conductivity in the range 0.3-2 THz for 10 $μ$m length CNTs. This increasing scattering rate with temperature results in a subsequent broadening of the observed THz conductivity peak at higher temperatures and a shift to lower frequencies for increasing CNT length. Finally, we show that the change in conductivity with temperature depends not only on tube length, but also varies with tube density. We record the effective conductivities of composite films comprising mixtures of WS$_2$ nanotubes and CNTs vs CNT density for frequencies in the range 0.3-1 THz, finding that the conductivity increases/decreases for low/high density films as the temperature increases. This effect arises due to the density dependence of the effective length of conducting pathways in the composite films, which again leads to a shift and temperature dependent broadening of the THz conductivity peak.

cond-mat.mes-hall↗