arXiv subjects

Peter Reimann

Publications and source records attributed to Peter Reimann.

At least 55 records · Page 3Linked to original sources

arXiv2012

Dimer motion on a periodic substrate: Spontaneous symmetry breaking and absolute negative mobility

We consider two coupled particles moving along a periodic substrate potential with negligible inertia effects (overdamped limit). Even when the particles are identical and the substrate spatially symmetric, a sinusoidal external driving of appropriate amplitude and frequency may lead to spontaneous symmetry breaking in the form of a permanent directed motion of the dimer. Thermal noise restores ergodicity and thus zero net velocity, but entails arbitrarily fast diffusion of the dimer for sufficiently weak noise. Moreover, upon application of a static bias force, the dimer exhibits a motion opposite to that force (absolute negative mobility). The key requirement for all these effects is a non-convex interaction potential of the two particles.

cond-mat.stat-mech↗

arXiv2012

Equilibration of isolated macroscopic quantum systems

We investigate the equilibration of an isolated macroscopic quantum system in the sense that deviations from a steady state become unmeasurably small for the overwhelming majority of times within any sufficiently large time interval. The main requirements are that the initial state, possibly far from equilibrium, exhibits a macroscopic population of at most one energy level and that degeneracies of energy eigenvalues and of energy gaps (differences of energy eigenvalues) are not of exceedingly large multiplicities. Our approach closely follows and extends recent works by Short and Farrelly [2012 New J. Phys. 14 013063], in particular going beyond the realm of finite-dimensional systems and large effective dimensions.

cond-mat.stat-mech↗

arXiv2012

Particle sorting by a structured microfluidic ratchet device with tunable selectivity: Theory and Experiment

We theoretically predict and experimentally demonstrate that several different particle species can be separated from each other by means of a ratchet device, consisting of periodically arranged triangular (ratchet) shaped obstacles. We propose an explicit algorithm for suitably tailoring the externally applied, time-dependent voltage protocol so that one or several, arbitrarily selected particle species are forced to migrate oppositely to all the remaining species. As an example we present numerical simulations for a mixture of five species, labelled according to their increasing size, so that species 2 and 4 simultaneously move in one direction and species 1, 3, and 5 in the other. The selection of species to be separated from the others can be changed at any time by simply adapting the voltage protocol. This general theoretical concept to utilize one device for many different sorting tasks is experimentally confirmed for a mixture of three colloidal particle species.

cond-mat.stat-mech↗

arXiv2012

Hidden multiple bond effects in dynamic force spectroscopy

In dynamic force spectroscopy, a (bio-)molecular complex is subjected to a steadily increasing force until the chemical bond breaks. Repeating the same experiment many times results in a broad distribution of rupture forces, whose quantitative interpretation represents a formidable theoretical challenge. In this study we address the situation that more than a single molecular bond is involved in one experimental run, giving rise to multiple rupture events which are even more difficult to analyze and thus are usually eliminated as far as possible from the further evaluation of the experimental data. We develop and numerically solve a detailed model of a complete dynamic force spectroscopy experiment including a possible clustering of molecules on the substrate surface, the formation of bonds, their dissociation under load, and the post processing of the force extension curves. We show that the data, remaining after elimination of obvious multiple rupture events, may still contain a considerable number of "hidden" multiple bonds, which are experimentally indistinguishable from "true" single bonds, but which have considerable effects on the resulting rupture force statistics and its consistent theoretical interpretation.

physics.bio-ph↗

arXiv2012

Rolling and sliding of a nanorod between two planes: Tribological regimes and control of friction

The motion of a cylindrical crystalline nanoparticle sandwiched between two crystalline planes, one stationary and the other pulled at a constant velocity and pressed down by a normal load, is considered theoretically using a planar model. The results of our model calculations show that, depending on load and velocity, the nanoparticle can be either rolling or sliding. At sufficiently high normal loads, several sliding states characterized by different friction forces can coexist, corresponding to different orientations of the nanoparticle, and allowing one to have low or high friction at the same pulling velocity and normal load.

cond-mat.mes-hall↗

arXiv2012

Anisotropic diffusion in square lattice potentials: giant enhancement and control

The unbiased thermal diffusion of an overdamped Brownian particle in a square lattice potential is considered in the presence of an externally applied ac driving. The resulting diffusion matrix exhibits two orthogonal eigenvectors with eigenvalues $D_1>D_2>0$, indicating anisotropic diffusion along a "fast" and a "slow principal axis". For sufficiently small temperatures, $D_1$ may become arbitrarily large and at the same time $D_2$ arbitrarily small. The principal diffusion axis can be made to point into (almost) any direction by varying either the driving amplitude or the coupling of the particle to the potential, without changing any other property of the system or the driving.

cond-mat.stat-mech↗

arXiv2010

Giant transversal particle diffusion in a longitudinal magnetic ratchet

We study the transversal motion of paramagnetic particles on a uniaxial garnet film, exhibiting a longitudinal ratchet effect in the presence of an oscillating magnetic field. Without the field, the thermal diffusion coefficient obtained by video microscopy is $D_{0}\approx 3\times 10^{-4}$ $μm^2/s$. With the field, the transversal diffusion exhibits a giant enhancement by almost four decades and a pronounced maximum as a function of the driving frequency. We explain the experimental findings with a theoretical interpretation in terms of random disorder effects within the magnetic film.

cond-mat.stat-mech↗

arXiv2010

Exploiting lattice potentials for sorting chiral particles

Several ways are demonstrated of how periodic potentials can be exploited for sorting molecules or other small objects which only differ by their chirality. With the help of a static bias force, the two chiral partners can be made to move along orthogonal directions. Time-periodic external forces even lead to motion into exactly opposite directions.

cond-mat.stat-mech↗

arXiv2010

Canonical thermalization

For quantum systems that are weakly coupled to a much 'bigger' environment, thermalization of possibly far from equilibrium initial ensembles is demonstrated: for sufficiently large times, the ensemble is for all practical purposes indistinguishable from a canonical density operator under conditions that are satisfied under many, if not all, experimentally realistic conditions.

cond-mat.stat-mech↗

arXiv2009

Suppression of thermally activated escape by heating

The problem of thermally activated escape over a potential barrier is solved by means of path integrals for one-dimensional reaction dynamics with very general time dependences. For a suitably chosen but still quite simple static potential landscape, the net escape rate may be substantially reduced by temporally increasing the temperature above its unperturbed constant level.

cond-mat.stat-mech↗

arXiv2008

Foundation of Statistical Mechanics under experimentally realistic conditions

We demonstrate the equilibration of isolated macroscopic quantum systems, prepared in non-equilibrium mixed states with significant population of many energy levels, and observed by instruments with a reasonably bound working range compared to the resolution limit. Both properties are fulfilled under many, if not all, experimentally realistic conditions. At equilibrium, the predictions and limitations of Statistical Mechanics are recovered.

cond-mat.stat-mech↗

arXiv2008

Weak disorder strongly improves the selective enhancement of diffusion in a tilted periodic potential

The diffusion of an overdamped Brownian particle in a tilted periodic potential is known to exhibit a pronounced enhancement over the free thermal diffusion within a small interval of tilt-values. Here we show that weak disorder in the form of small, time-independent deviations from a strictly spatially periodic potential may further boost this diffusion peak by orders of magnitude. Our general theoretical predictions are in excellent agreement with experimental observations.

cond-mat.stat-mech↗

arXiv2008

Typicality of pure states randomly sampled according to the Gaussian adjusted projected measure

Consider a mixed quantum mechanical state, describing a statistical ensemble in terms of an arbitrary density operator $ρ$ of low purity, $\trρ^2\ll 1$, and yielding the ensemble averaged expectation value $\tr(ρA)$ for any observable $A$. Assuming that the given statistical ensemble $ρ$ is generated by randomly sampling pure states $|ψ>$ according to the corresponding so-called Gaussian adjusted projected measure $[$Goldstein et al., J. Stat. Phys. 125, 1197 (2006)$]$, the expectation value $<ψ|A|ψ>$ is shown to be extremely close to the ensemble average $\tr(ρA)$ for the overwhelming majority of pure states $|ψ>$ and any experimentally realistic observable $A$. In particular, such a `typicality' property holds whenever the Hilbert space $\hr$ of the system contains a high dimensional subspace $\hr_+\subset\hr$ with the property that all $|ψ>\in\hr_+$ are realized with equal probability and all other $|ψ> \in\hr$ are excluded.

cond-mat.stat-mech↗

arXiv2008

Single-molecule force spectroscopy: Practical limitations beyond Bell's model

Single-molecule force spectroscopy experiments, as well as a number of other physical systems, are governed by thermally activated transitions out of a metastable state under the action of a steadily increasing external force. The main observable in such experiments is the distribution of the forces, at which the escape events occur. The challenge in interpreting the experimental data is to relate them to the microscopic system properties. We work out a maximum likelihood approach and show that it is the optimal method to tackle this problem. When fitting actual experimental data it is unavoidable to assume some functional form for the force-dependent escape rate. We consider a quite general and common such functional form and demonstrate by means of data from a realistic computer experiment that the maximum number of fit parameters that can be determined reliably is three. They are related to the force-free escape rate and the position and height of the activation barrier. Furthermore, the results for the first two of these fit parameters show little dependence on the assumption about the manner in which the barrier decreases with the applied force, while the last one, the barrier height in the absence of force, depends strongly on this assumption.

cond-mat.soft↗

arXiv2007

Typicality for Generalized Microcanonical Ensembles

For a macroscopic, isolated quantum system in an unknown pure state, the expectation value of any given observable is shown to hardly deviate from the ensemble average with extremely high probability under generic equilibrium and nonequilibrium conditions. Special care is devoted to the uncontrollable microscopic details of the system state. For a subsystem weakly coupled to a large heat bath, the canonical ensemble is recovered under much more general and realistic assumptions than those implicit in the usual microcanonical description of the composite system at equilibrium.

cond-mat.stat-mech↗

arXiv2007

The Brownian gyrator: a minimal heat engine on the nano-scale

A Brownian particle moving in the vicinity of a generic potential minimum under the influence of dissipation and thermal noise from two different heat baths is shown to act as a minimal heat engine, generating a systematic torque onto the physical object at the origin of the potential and an opposite torque onto the medium generating the dissipation.

cond-mat.stat-mech↗

arXiv2004

Temperature Anisotropy in a Driven Granular Gas

When smooth granular material is fluidized by vertically shaking a container, we find that the temperature in the direction of energy input always exceeds the temperature in the other directions. An analytical model is presented which shows how the anisotropy can be traced back to the inelasticity of the interparticle collisions and the collisions with the wall. The model compares very well with molecular dynamics simulations. It is concluded that any non-isotropic driving of a granular gas in a steady state necessarily causes anisotropy of the granular temperature.

cond-mat.stat-mech↗

arXiv2004

Paradoxical non-linear response of a Brownian particle

We consider a Brownian particle in a ``meandering'' periodic potential when the ambient temperature is a periodically or stochastically varying function of time. Though far from equilibrium, the linear response of the particle to an external static force is exactly the same as in the equilibrium case, i.e. for constant temperature. Even more surprising is the non-linear response: the particle slows down and then even starts to move in the direction opposite to the applied force.

cond-mat.stat-mech↗