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Phila Rembold

Publications and source records attributed to Phila Rembold.

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Adaptive Reconstruction of Bosonic Quantum States

Bosonic quantum systems provide a hardware-efficient platform for quantum information processing but remain challenging to characterise due to their large Hilbert space and the high measurement cost of state tomography. Existing approaches estimate the fidelity with respect to a single target state, making them unsuitable for applications in which physically equivalent states differ by phase space translations, rotations, or other transformations. Here, we introduce an adaptive reconstruction technique that estimates the fidelity with respect to a family of bosonic states while reconstructing the underlying Wigner function from a small number of measurements. The method combines a physics-informed parametric model with Bayesian inference, bootstrap, and active learning to iteratively select the most informative phase space sampling points. We implement the approach on a circuit quantum electrodynamics platform and benchmark it on Schr\"odinger cat states with amplitudes $\alpha\in[1,3]$. The reconstruction yields reproducible fidelity estimates within a few minutes, remains robust to substantial displacements and rotations in phase space despite using a mismatched prior, and is sensitive to subtle state imperfections. We further compare the adaptive strategy with existing Wigner function sampling protocols experimentally, demonstrating the advantage of adaptive sampling for measurement-efficient fidelity estimation with respect to a family of cat states. Finally, we incorporate the reconstructed fidelity into the figure of merit used in a proof-of-principle closed-loop quantum optimal control experiment, demonstrating the applicability of the method to autonomous optimisation of bosonic quantum states.

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Genuine Multipartite Entanglement between Logical Qubits via Cross-Code Lattice Surgery

Universal quantum computers are expected to generate arbitrary complex quantum states of logical qubits encoded in many physical qubits. This capability hinges on a fault-tolerantly implemented universal gate set, which no single quantum error-correction code admits transversally but which becomes accessible by joining complementary codes via lattice surgery. Here we report on the experimental generation and certification of logical genuine multipartite entanglement in a trapped-ion quantum processor using a transversally implemented universal logical gate set. The gate set is accessed via lattice surgery across two different codes and comprises a Hadamard gate on a four-qubit surface code and a doubly controlled Pauli-$Z$ ($\overline{\mathrm{CCZ}}$) gate on an eight-qubit 3D colour code. To showcase this lattice-surgery toolbox, we generate both stabiliser (Greenberger-Horne-Zeilinger) and non-stabiliser ($|\overline{\mathrm{CCZ}}\rangle$) states of three logical qubits and verify their genuine multipartite entanglement--a form of correlation beyond statistical mixtures of bipartite entanglement across any bipartition. We further use these cross-code primitives to demonstrate arbitrary rotations of single logical qubits via a $\overline{\mathrm{CCZ}}$-based resource gadget accessing the full universal gate set through lattice surgery. Together, these demonstrations showcase the core building blocks of an architecture for fault-tolerant quantum computation and its ability to generate complex logical quantum states.

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Experimental Verification of Electron-Photon Entanglement

Entanglement, a key resource of emerging quantum technologies, describes correlations between particles that defy classical physics. It has been studied extensively on various platforms, but has remained elusive in electron microscopy. Transmission electron microscopes are well-established tools for materials characterisation with unparalleled spatial resolution. They provide control over the preparation and detection of high energy electrons, with largely unexploited potential in the study of many-body quantum correlations. Here, we demonstrate entanglement in electron-photon pairs generated via cathodoluminescence in a transmission electron microscope. Employing coincidence imaging techniques adapted from photonic quantum optics, we reconstruct both near- and far-field ``ghost'' images of periodic transmission masks. By measuring spatial and momentum correlations, we show a violation of the classical uncertainty bound: $\Delta x_-^2 \Delta k_+^2 = 0.502 \pm 0.047<1$. Hence, we demonstrate entanglement in position and momentum -- the continuous variables at the base of most imaging methods, bridging the fields of electron microscopy and quantum optics. Our work paves the way for exploring quantum correlations in free-electron systems and their application to quantum-enhanced imaging techniques on the nanoscale.

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State-Agnostic Approach to Certifying Electron-Photon Entanglement in Electron Microscopy

Transmission electron microscopes (TEMs) enable atomic-scale imaging and characterisation, driving advances across fields from materials science to biology. Quantum correlations, specifically entanglement, may provide a basis for novel hybrid sensing techniques to make TEMs compatible with sensitive samples prone to radiation damage. We present a protocol to certify entanglement between electrons and photons naturally arising from certain coherent cathodoluminescence (CL) processes. Using mutually unbiased bases in position and momentum, our method allows robust, state-agnostic entanglement verification and provides a lower bound on the entanglement of formation, enabling quantitative comparisons across platforms. Simulations under experiment-inspired conditions and preliminary experimental data highlight the feasibility of implementing this approach in modern TEM systems with optical specimen access. Our work integrates photonic quantum information techniques with electron microscopy. It establishes a foundation for entanglement-based imaging at the atomic scale, offering a potential pathway to reduce radiation exposure.

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The Role of Bases in Quantum Optimal Control

Quantum Optimal Control (QOC) supports the advance of quantum technologies by tackling its problems at the pulse level: Numerical approaches iteratively work towards a given target by parametrising the applied time-dependent fields with a finite set of variables. The effectiveness of the resulting optimisation depends on the complexity of the problem and the number of variables. We consider different parametrisations in terms of basis functions, asking whether the choice of the applied basis affects the quality of the optimisation. Furthermore, we consider strategies to choose the most suitable basis. For the comparison, we test three different randomisable bases - introducing the sinc and sigmoid bases as alternatives to the Fourier basis - on QOC problems of varying complexity. For each problem, the basis-specific convergence rates result in a unique ranking. Especially for expensive evaluations, e.g., in closed-loop, a potential speed-up by a factor of up to 10 may be crucial for the optimisation's feasibility. We conclude that a problem-dependent basis choice is an influential factor for QOC efficiency and provide advice for its approach.

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QuOCS: The Quantum Optimal Control Suite

Quantum optimal control includes the family of pulse-shaping algorithms that aim to unlock the full potential of a variety of quantum technologies. Our Quantum Optimal Control Suite (QuOCS) unites experimental focus and model-based approaches in a unified framework. The easy usage and installation of QuOCS and the availability of various combinable optimization strategies is designed to improve the performance of many quantum technology platforms, such as color defects in diamond, superconducting qubits, atom- or ion-based quantum computers. It can also be applied to the study of more general phenomena in physics. In this paper, we describe the software and the main toolbox of gradient-free and gradient-based algorithms. We then show how the user can connect it to their experiment. In addition, we provide illustrative examples where our optimization suite solves typical quantum optimal control problems, in both open- and closed-loop settings. Integration into existing experimental control software is already provided for the experiment control software Qudi [J. M. Binder et al., SoftwareX, 6, 85-90, (2017)], and further extensions are investigated and highly encouraged. QuOCS is available from GitHub, under Apache License 2.0, and can be found on the PyPI repository.

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Macroscopic Hyperpolarization Enhanced with Quantum Optimal Control

Hyperpolarization of nuclear spins enhances nuclear magnetic resonance signals, which play a key role for imaging and spectroscopy in the natural and life sciences. This signal amplification unlocks previously inaccessible techniques, such as metabolic imaging of cancer cells. In this work, electron spins from the photoexcited triplet state of pentacene-doped naphthalene crystals are used to polarize surrounding protons. As existing strategies are rendered less effective by experimental constraints, they are replaced with optimal control pulses designed with RedCRAB. In contrast to previous optimal control approaches, which consider an average single nucleus, this closed-loop optimization is macroscopic. A 28% improvement in signal and 15% faster polarization rate is observed. Additionally, a strategy called Autonomously-optimized Repeated Linear Sweep (ARISE) is introduced to efficiently tailor existing hyperpolarization sequences in the presence of experimental uncertainty to enhance their performance. ARISE is expected to be broadly applicable in many experimental settings.

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Robust Magnetometry with Single NV Centers via Two-step Optimization

Shallow Nitrogen-Vacancy (NV) centers are promising candidates for high-precision sensing applications; these defects, when positioned a few nanometers below the surface, provide an atomic-scale resolution along with substantial sensitivity. However, the dangling bonds and impurities on the diamond surface result in a complex environment which reduces the sensitivity and is unique to each shallow NV center. To avoid the environment's detrimental effect, we apply feedback-based quantum optimal control. We first show how a direct search can improve the initialization/readout process. In a second step, we optimize microwave pulses for pulsed Optically Detected Magnetic Resonance (ODMR) and Ramsey measurements. Throughout the sensitivity optimizations, we focus on robustness against errors in the control field amplitude. This feature not only protects the protocols' sensitivity from drifts but also enlarges the sensing volume. The resulting ODMR measurements produce sensitivities below 1$\mu$T\,Hz$^{-\frac{1}{2}}$ for an 83\% decrease in control power, increasing the robustness by approximately one third. The optimized Ramsey measurements produce sensitivities below 100\,nT\,Hz$^{-\frac{1}{2}}$ giving a two-fold sensitivity improvement. Being on par with typical sensitivities obtained via single NV magnetometry, the complementing robustness of the presented optimization strategy may provide an advantage for other NV-based applications.

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Introduction to Quantum Optimal Control for Quantum Sensing with Nitrogen-Vacancy Centers in Diamond

Diamond based quantum technology is a fast emerging field with both scientific and technological importance. With the growing knowledge and experience concerning diamond based quantum systems, comes an increased demand for performance. Quantum optimal control (QOC) provides a direct solution to a number of existing challenges as well as a basis for proposed future applications. Together with a swift review of QOC strategies, quantum sensing and other relevant quantum technology applications of nitrogen-vacancy (NV) centers in diamond, we give the necessary background to summarize recent advancements in the field of QOC assisted quantum applications with NV centers in diamond.

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Generation and manipulation of Schrödinger cat states in Rydberg atom arrays

Quantum entanglement involving coherent superpositions of macroscopically distinct states is among the most striking features of quantum theory, but its realization is challenging, since such states are extremely fragile. Using a programmable quantum simulator based on neutral atom arrays with interactions mediated by Rydberg states, we demonstrate the deterministic generation of 'Schrödinger cat' states of the Greenberger-Horne-Zeilinger (GHZ) type with up to 20 qubits. Our approach is based on engineering the energy spectrum and using optimal control of the many-body system. We further demonstrate entanglement manipulation by using GHZ states to distribute entanglement to distant sites in the array, establishing important ingredients for quantum information processing and quantum metrology.

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