arXiv subjects

Philip J. Bustard

Publications and source records attributed to Philip J. Bustard.

At least 19 recordsLinked to original sources

arXiv2026

Simultaneous amplitude and phase spectroscopy using two-photon interference

Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin beams of light to reduce the noise sources inherent to absorption spectroscopy. However, measurements of the phase shift imparted by the chemical sample, which provides complementary information to the absorption, continue to be a challenge. Here, we propose and demonstrate a scheme using entangled photon pairs that can simultaneously measure both the absorption and phase shift of a sample with extremely low optical intensities and with relatively fast few-minute acquisition times. This method combines the previous use of intensity correlations with a broadband quantum interferometer utilizing two-photon interference to measure the complete linear optical response of the sample. Our work shows that precise measurements of absorption can also be made phase-sensitive using suitable choices of probe beam and detection scheme. This enables a new class of quantum spectroscopy schemes which measure absorption and phase with a single probe. Our technique is relevant to the characterization of a wide array of chemical and biological samples, such as quantum dots and organic fluorophores, and may be useful for spectroscopic measurements that are otherwise constrained in intensity.

quant-ph↗

arXiv2025

Ultrafast switching of telecom photon-number states

A crucial component of photonic quantum information processing platforms is the ability to modulate, route, convert, and switch quantum states of light noiselessly with low insertion loss. For instance, a high-speed, low-loss optical switch is crucial for scaling quantum photonic systems that rely on measurement-based feed-forward approaches. Such a device will also ideally be capable of operating on photon-number states, which can act as non-Gaussian resources. Here, we demonstrate ultrafast all-optical switching of heralded photon-number states, of up to 6 photons, using the optical Kerr effect in a single-mode fiber. A local birefringence is created by a high-intensity pump pulse at a center wavelength of 1030 nm which overlaps temporally with the 1550 nm photons in the fiber. A switching efficiency of $>$99 % is reached with a resolution of 2.3 ps, an insertion loss of $2.27\pm0.08$ dB, and a signal-to-noise ratio of 32,000.

quant-ph↗

arXiv2025

Broadband spectral manipulation of single photons using cross-phase modulation

Manipulating the frequency and bandwidth of light is crucial in classical and quantum applications including communication, spectroscopy, imaging, and signal processing. Such capabilities also offer potential for interfacing disparate quantum systems in quantum networking and for quantum information processing. We experimentally demonstrate deterministic, broadband frequency control of heralded telecom-band single photons via cross-phase modulation in a short length of single-mode fiber. An intense, ultrafast pump pulse imposes a transient, intensity-dependent refractive-index gradient which imparts a tunable phase shift on the single photons. We present absolute frequency shifts of up to $+6.46\pm0.01$\,THz and $-5.74\pm0.01$\,THz, and bandwidth manipulation ranging from a factor of $0.66\pm0.03$ to $8.4\pm0.3$ times that of the input. Spectral measurements are acquired with a time-of-flight spectrometer and superconducting nanowire detectors. Our scheme offers a compact and scalable route to spectral routing and bandwidth engineering for ultrafast quantum networking and quantum information processing.

quant-ph↗

arXiv2025

Imaging at the quantum limit with convolutional neural networks

Deep neural networks have been shown to achieve exceptional performance for computer vision tasks like image recognition, segmentation, and reconstruction or denoising. Here, we evaluate the ultimate performance limits of deep convolutional neural network models for image reconstruction, by comparing them against the standard quantum limit set by shot-noise and the Heisenberg limit on precision. We train U-Net models on images of natural objects illuminated with coherent states of light, and find that the average mean-squared error of the reconstructions can surpass the standard quantum limit, and in some cases reaches the Heisenberg limit. Further, we train models on well-parameterized images for which we can calculate the quantum Cramér-Rao bound to determine the minimum possible measurable variance of an estimated parameter for a given probe state. We find the mean-squared error of the model predictions reaches these bounds calculated for the parameters, across a variety of parameterized images. These results suggest that deep convolutional neural networks can learn to become the optimal estimators allowed by the laws of physics, performing parameter estimation and image reconstruction at the ultimate possible limits of precision for the case of classical illumination of the object.

cs.LG↗

arXiv2025

Quantum enhanced beam tracking surpassing the Heisenberg uncertainty limit

Determining a beam's full trajectory requires tracking both its position and momentum (angular) information. However, the product of position and momentum uncertainty in a simultaneous measurement of the two parameters is bound by the Heisenberg uncertainty limit (HUL). In this work, we present a proof-of-principle demonstration of a quantum-enhanced beam tracking technique, leveraging the inherent position and momentum entanglement between photons produced via spontaneous parametric down-conversion (SPDC). We show that quantum entanglement can be exploited to achieve a beam tracking accuracy beyond the HUL in a simultaneous measurement. Moreover, with existing detection technologies, it is already possible to achieve near real-time beam tracking capabilities at the single-photon level. The technique also exhibits high resilience to background influences, with negligible reduction in tracking accuracy even when subjected to a disruptive beam that is significantly brighter than SPDC.

quant-ph↗

arXiv2025

Ultrafast all-optical modulation of spatially structured photons

Manipulating the structure of single photons in the ultrafast domain is enabling new quantum information processing technologies. At the picosecond timescale, quantum information can be processed before decoherence can occur. In this work, we study the capabilities of few-mode cross-phase modulation via the optical Kerr effect, using ultrafast pulses. We observe a significant modulation in the spatial mode of structured photons on timescales $\leq 1.3$~ps.

quant-ph↗

arXiv2025

Terahertz electro-optic modulation of single photons

The manipulation of visible and near-infrared light at the single-photon level plays a key role in quantum communication systems where information is encoded into photonic degrees of freedom. In practical implementations, it is important to achieve this manipulation with high speeds, low loss, and low noise. In this work, we propose the use of terahertz~(THz) electric fields as a pump source for electro-optic modulation of single photons in bulk media. We demonstrate spectral modulations of single photons in the form of frequency translation and bandwidth manipulations as the terahertz field imparts linear and quadratic phases on the photons at various time delays within 1~ps. Our results show frequency translations exceeding 500~GHz at multi-THz modulation speeds and loss levels of $\approx$1~dB, complementing the current state-of-the-art electro-optic modulation techniques limited to speeds up to 100~GHz. The proposed approach leverages recent developments in terahertz generation techniques, introducing new avenues to manipulate non-classical light in an unexplored regime for quantum photonics.

quant-ph↗

arXiv2024

Multiphoton interference in a single-spatial-mode quantum walk

Multiphoton interference is crucial to many photonic quantum technologies. In particular, interference forms the basis of optical quantum information processing platforms and can lead to significant computational advantages. It is therefore interesting to study the interference arising from various states of light in large interferometric networks. Here, we implement a quantum walk in a highly stable, low-loss, multiport interferometer with up to 24 ultrafast time bins. This time-bin interferometer comprises a sequence of birefringent crystals which produce pulses separated by 4.3\,ps, all along a single optical axis. Ultrafast Kerr gating in an optical fiber is employed to time-demultiplex the output from the quantum walk. We measure one-, two-, and three-photon interference arising from various input state combinations, including a heralded single-photon state, a thermal state, and an attenuated coherent state at one or more input ports. Our results demonstrate that ultrafast time bins are a promising platform to observe large-scale multiphoton interference.

quant-ph↗

arXiv2024

Programmable Photonic Quantum Circuits with Ultrafast Time-bin Encoding

We propose a quantum information processing platform that utilizes the ultrafast time-bin encoding of photons. This approach offers a pathway to scalability by leveraging the inherent phase stability of collinear temporal interferometric networks at the femtosecond-to-picosecond timescale. The proposed architecture encodes information in ultrafast temporal bins processed using optically induced nonlinearities and birefringent materials while keeping photons in a single spatial mode. We demonstrate the potential for scalable photonic quantum information processing through two independent experiments that showcase the platform's programmability and scalability, respectively. The scheme's programmability is demonstrated in the first experiment, where we successfully program 362 different unitary transformations in up to 8 dimensions in a temporal circuit. In the second experiment, we show the scalability of ultrafast time-bin encoding by building a passive optical network, with increasing circuit depth, of up to 36 optical modes. In each experiment, fidelities exceed 97\%, while the interferometric phase remains passively stable for several days.

quant-ph↗

arXiv2024

Photonic quantum walk with ultrafast time-bin encoding

The quantum walk (QW) has proven to be a valuable testbed for fundamental inquiries in quantum technology applications such as quantum simulation and quantum search algorithms. Many benefits have been found by exploring implementations of QWs in various physical systems, including photonic platforms. Here, we propose a novel platform to perform quantum walks using an ultrafast time-bin encoding (UTBE) scheme. This platform supports the scalability of quantum walks to a large number of steps while retaining a significant degree of programmability. More importantly, ultrafast time bins are encoded at the picosecond time scale, far away from mechanical fluctuations. This enables the scalability of our platform to many modes while preserving excellent interferometric phase stability over extremely long periods of time without requiring active phase stabilization. Our 18-step QW is shown to preserve interferometric phase stability over a period of 50 hours, with an overall walk fidelity maintained above $95\%$

quant-ph↗

arXiv2024

3D-2D Neural Nets for Phase Retrieval in Noisy Interferometric Imaging

In recent years, neural networks have been used to solve phase retrieval problems in imaging with superior accuracy and speed than traditional techniques, especially in the presence of noise. However, in the context of interferometric imaging, phase noise has been largely unaddressed by existing neural network architectures. Such noise arises naturally in an interferometer due to mechanical instabilities or atmospheric turbulence, limiting measurement acquisition times and posing a challenge in scenarios with limited light intensity, such as remote sensing. Here, we introduce a 3D-2D Phase Retrieval U-Net (PRUNe) that takes noisy and randomly phase-shifted interferograms as inputs, and outputs a single 2D phase image. A 3D downsampling convolutional encoder captures correlations within and between frames to produce a 2D latent space, which is upsampled by a 2D decoder into a phase image. We test our model against a state-of-the-art singular value decomposition algorithm and find PRUNe reconstructions consistently show more accurate and smooth reconstructions, with a x2.5 - 4 lower mean squared error at multiple signal-to-noise ratios for interferograms with low (< 1 photon/pixel) and high (~100 photons/pixel) signal intensity. Our model presents a faster and more accurate approach to perform phase retrieval in extremely low light intensity interferometry in presence of phase noise, and will find application in other multi-frame noisy imaging techniques.

physics.optics↗

arXiv2024

Toward deterministic sources: Photon generation in a fiber-cavity quantum memory

We demonstrate the generation of photons within a fiber-cavity quantum memory, followed by later on-demand readout. Signal photons are generated by spontaneous four-wave mixing in a fiber cavity comprising a birefringent fiber with dichroic reflective end facets. The detection of the partner herald photon indicates the creation of the stored signal photon. After a delay, the signal photon is switched out of resonance with the fiber cavity by intracavity frequency translation using Bragg scattering four-wave mixing, driven by ancillary control pulses. We measure sub-Poissonian statistics in the output signal mode, with $g^{(2)}_{AC}=0.54(1)$ in the first readout bin and a readout frequency translation efficiency of $\approx$80%. The 1/e memory lifetime is $\approx$67 cavity cycles, or 1.68$μ$s. In an alternate fiber cavity, we show a strategy for noise reduction and measure $g^{(2)}_{AC}=0.068(10)$ after one cavity cycle.

quant-ph↗

arXiv2023

Ultrafast Measurement of Energy-Time Entanglement with an Optical Kerr Shutter

Recent experimental progress in quantum optics has enabled measurement of single photons on ultrafast timescales, beyond the resolution limit of single photon detectors. The energy-time degree of freedom has emerged as a promising avenue for quantum technologies, as entanglement between the frequency and temporal properties of two photons can be fully explored and utilized. Here, we implement optical Kerr shutters in single mode fibers to map out the sub-picosecond correlations of energy-time entangled photon pairs. These measurements, in addition to joint spectral measurements of the photon pair state, are used to verify entanglement by means of the violation of a time-bandwidth inequality.

quant-ph↗

arXiv2023

Measuring ultrafast time-bin qudits

Time-bin qudits have emerged as a promising encoding platform in many quantum photonic applications. However, the requirement for efficient single-shot measurement of time-bin qudits instead of reconstructive detection has restricted their widespread use in experiments. Here, we propose an efficient method to measure arbitrary superposition states of time-bin qudits and confirm it up to dimension 4. This method is based on encoding time bins at the picosecond time scale, also known as ultrafast time bins. By doing so, we enable the use of robust and phase-stable single spatial mode temporal interferometers to measure time-bin qudit in different measurement bases.

quant-ph↗

arXiv2022

Toward a Quantum Memory in a Fiber Cavity Controlled by Intracavity Frequency Translation

We propose a quantum memory protocol based on trapping photons in a fiber-integrated cavity, comprised of a birefringent fiber with dichroic reflective end facets. Photons are switched into resonance with the fiber cavity by intracavity Bragg-scattering frequency translation, driven by ancillary control pulses. After the storage delay, photons are switched out of resonance with the cavity, again by intracavity frequency translation. We demonstrate storage of quantum-level THz-bandwidth coherent states for a lifetime up to 16 cavity round trips, or 200ns, and a maximum overall efficiency of 73%.

quant-ph↗

arXiv2021

Quantum communication with ultrafast time-bin qubits

The photonic temporal degree of freedom is one of the most promising platforms for quantum communication over fiber networks and free-space channels. In particular, time-bin states of photons are robust to environmental disturbances, support high-rate communication, and can be used in high-dimensional schemes. However, the detection of photonic time-bin states remains a challenging task, particularly for the case of photons that are in a superposition of different time-bins. Here, we experimentally demonstrate the feasibility of picosecond time-bin states of light, known as ultrafast time-bins, for applications in quantum communications. With the ability to measure time-bin superpositions with excellent phase stability, we enable the use of temporal states in efficient quantum key distribution protocols such as the BB84 protocol.

quant-ph↗

arXiv2021

Achieving ultimate noise tolerance in quantum communication

At the fundamental level, quantum communication is ultimately limited by noise. For instance, quantum signals cannot be amplified without the introduction of noise in the amplified states. Furthermore, photon loss reduces the signal-to-noise ratio, accentuating the effect of noise. Thus, most of the efforts in quantum communications have been directed towards overcoming noise to achieve longer communication distances, larger secret key rates, or to operate in noisier environmental conditions. Here, we propose and experimentally demonstrate a platform for quantum communication based on ultrafast optical techniques. In particular, our scheme enables the experimental realization of high-rates and quantum signal filtering approaching a single spectro-temporal mode, resulting in a dramatic reduction in channel noise. By experimentally realizing a 1-ps optically induced temporal gate, we show that ultrafast time filtering can result in an improvement in noise tolerance by a factor of up to 1200 compared to a 2-ns electronic filter enabling daytime quantum key distribution or quantum communication in bright fibers.

quant-ph↗

arXiv2017

Time-bin to Polarization Conversion of Ultrafast Photonic Qubits

The encoding of quantum information in photonic time-bin qubits is apt for long distance quantum communication schemes. In practice, due to technical constraints such as detector response time, or the speed with which co-polarized time-bins can be switched, other encodings, e.g. polarization, are often preferred for operations like state detection. Here, we present the conversion of qubits between polarization and time-bin encodings using a method that is based on an ultrafast optical Kerr shutter and attain efficiencies of 97% and an average fidelity of 0.827+/-0.003 with shutter speeds near 1 ps. Our demonstration delineates an essential requirement for the development of hybrid and high-rate optical quantum networks.

quant-ph↗