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Philip J. D. Crowley

Publications and source records attributed to Philip J. D. Crowley.

At least 19 recordsLinked to original sources

Universal non-power-law scaling from a chaotic renormalisation group in the Harper-Hofstadter model

Previous studies of incommensurate systems concluded that their critical scaling is sensitively dependent on the irrational, $α$, which determines the incommensuration. Contrary to this belief, in the canonical Harper-Hofstadter model, we show there is universal $α$-independent scaling for almost all $α$. This critical scaling is characterized by non-power-law time-length scaling $t \sim r^{ζ\log \log r}$. We demonstrate this in the superfluid fraction of a Bose gas, and the specific heat of a Fermi gas. This scaling is generic of a broad class of generalized Harper-Hofstadter models. The $α$-independent scaling emerges as the number theoretic properties of almost all irrational numbers are statistically identical (\emph{à la} Gauss-Kuzmin statistics). Consequently, we conjecture similar $α$-independent scaling applies in incommensurate models more generally.

cond-mat.stat-mech↗

Theory of Scalable Spin Squeezing with Disordered Quantum Dipoles

Spin squeezed entanglement enables metrological precision beyond the classical limit. Understood through the lens of continuous symmetry breaking, dipolar spin systems exhibit the remarkable ability to generate spin squeezing via their intrinsic quench dynamics. To date, this understanding has primarily focused on lattice spin systems; in practice however, dipolar spin systems$\unicode{x2014}$ranging from ultracold molecules to nuclear spin ensembles and solid-state color centers$\unicode{x2014}$often exhibit significant amounts of positional disorder. Here, we develop a theory for scalable spin squeezing in a two-dimensional randomly diluted lattice of quantum dipoles, which naturally realize a dipolar XXZ model. Via extensive quantum Monte Carlo simulations, we map out the phase diagram for finite-temperature XY order, and by extension scalable spin squeezing, as a function of both disorder and Ising anisotropy. As the disorder increases, we find that scalable spin squeezing survives only near the Heisenberg point. We show that this behavior is due to the presence of rare tightly-coupled dimers, which effectively heat the system post-quench. In the case of strongly-interacting nitrogen-vacancy centers in diamond, we demonstrate that an experimentally feasible strategy to decouple the problematic dimers from the dynamics is sufficient to enable scalable spin squeezing.

quant-ph↗

Persistent Fluctuating Superconductivity and Planckian Dissipation in Fe(Te,Se)

Increasingly intricate phase diagrams in new classes of superconductors host fascinating interactions between superconductivity, diverse quantum phases, and quantum critical dynamics. The native superfluids, however, often exhibit much lower density and much greater inhomogeneity than conventional superfluids. This may render the superconductivity susceptible to fluctuations that are ordinarily assumed to be frozen out far below the superconducting transition temperature $T_c$, calling into question the degree to which the superconducting state is fully coherent. In this work, we leverage terahertz spectroscopy to demonstrate strongly fluctuating superconductivity in topological compositions of the multiband iron-based superconductor Fe(Te,Se). These fluctuations are found to persist undiminished far below $T_c$ and converge upon the limit of Planckian dissipation above $T_c$. These results indicate that extended quantum fluctuations dominate the electrodynamics of both the superconducting and Planckian-dissipative precursor states of Fe(Te,Se), and demonstrate that the assumption of phase coherence must be rigorously validated in emerging classes of unconventional superconductors.

cond-mat.supr-con↗

Stability of sub-dimensional localization to electronic interactions

Sub-dimensional localization, also known as directional localization, arises when 2d electrons are subject to a periodic potential and incommensurate magnetic field which cause them to become exponentially localized along one crystal axis, while remaining extended in the orthogonal direction. We establish that sub-dimensional localization is robust to the presence of electronic interactions, which are known to generically destabilize single-particle localization. Consequently we predict that sub-dimensional localization may occur in moire materials, where it is manifest as a total absence of conductivity in the localized (transverse) direction, with finite conductivity in the extended (longitudinal) direction. We find the electrons form longitudinal charge density waves which are incommensurate with the moire potential, allowing them to slide and hence conduct in the longitudinal direction. The conductivity remains prohibited in the transverse direction due an emergent charge dipole moment conservation law.

cond-mat.mes-hall↗

Observation of spin squeezing with contact interactions in one- and three-dimensional easy-plane magnets

Entanglement in a many-particle system can enable measurement sensitivities beyond that achievable by only classical correlations. For an ensemble of spins, all-to-all interactions are known to reshape the quantum projection noise, leading to a form of entanglement known as spin squeezing. Here, we demonstrate spin squeezing with strictly short-range contact interactions. In particular, working with ultracold lithium atoms in optical lattices, we utilize superexchange interactions to realize a nearest-neighbor anisotropic Heisenberg model. We investigate the resulting quench dynamics from an initial product state in both one and three dimensions. In 1D, we observe $1.9^{+0.7}_{-0.5}$ dB of spin squeezing in quantitative agreement with theory. However, in 3D, we observe a maximum of $2.0^{+0.7}_{-0.7}$ dB of squeezing, over an order of magnitude smaller than that expected. We demonstrate that this discrepancy arises from the presence of a finite density of holes; both the motion of the holes as well as direct coupling between spin and density qualitatively alter the spin dynamics. Our observations point to the importance of understanding the complex interplay between motional and spin degrees of freedom in quantum simulators.

quant-ph↗

Band structure engineering using a moiré polar substrate

Applying long wavelength periodic potentials on quantum materials has recently been demonstrated to be a promising pathway for engineering novel quantum phases of matter. Here, we utilize twisted bilayer boron nitride (BN) as a moiré substrate for band structure engineering. Small-angle-twisted bilayer BN is endowed with periodically arranged up and down polar domains, which imprints a periodic electrostatic potential on a target two-dimensional (2D) material placed on top. As a proof of concept, we use Bernal bilayer graphene as the target material. The resulting modulation of the band structure appears as superlattice resistance peaks, tunable by varying the twist angle, and Hofstadter butterfly physics under a magnetic field. Additionally, we demonstrate the tunability of the moiré potential by altering the dielectric thickness underneath the twisted BN. Finally, we find that near-60°-twisted bilayer BN provides a unique platform for studying the moiré structural effect without the contribution from electrostatic moiré potentials. Tunable moiré polar substrates may serve as versatile platforms to engineer the electronic, optical, and mechanical properties of 2D materials and van der Waals heterostructures.

cond-mat.mes-hall↗

Absence of disordered Thouless pumps at finite frequency

A Thouless pump is a slowly driven one-dimensional band insulator which pumps charge at a quantised rate. Previous work showed that pumping persists in weakly disordered chains, and separately in clean chains at finite drive frequency. We study the interplay of disorder and finite frequency, and show that the pump rate always decays to zero due to non-adiabatic transitions between the instantaneous eigenstates. However, the decay is slow, occurring on a time-scale that is exponentially large in the period of the drive. In the adiabatic limit, the band gap in the instantaneous spectrum closes at a critical disorder strength above which pumping ceases. We predict the scaling of the pump rate around this transition from a model of scattering between rare states near the band edges. Our predictions can be experimentally tested in ultracold atomic and photonic platforms.

cond-mat.dis-nn↗

Dimensional reduction from magnetic field in moiré superlattices

Moiré materials provide a highly tunable platform in which novel electronic phenomena can emerge. We study strained moiré materials in a uniform magnetic field and predict highly anisotropic electrical conductivity which switches easy-axis as magnetic field or strain is varied. The dramatic anisotropy reflects one-dimensional localization (dimensional reduction) of the electron wavefunctions along a crystal axis due to quantum interference effects. This can be understood in an effective one-dimensional quasiperiodic Aubry-André-like models, or in a complementary semiclassical picture. This phenomenon should be observable in strained moiré materials at realistic fields and low strain disorder, as well as unstrained systems with anisotropic Fermi surfaces.

cond-mat.mes-hall↗

Phenomenology of the Prethermal Many-Body Localized Regime

The dynamical phase diagram of interacting disordered systems has seen substantial revision over the past few years. Theory must now account for a large prethermal many-body localized (MBL) regime in which thermalization is extremely slow, but not completely arrested. We derive a quantitative description of these dynamics in short-ranged one-dimensional systems using a model of successive many-body resonances. The model explains the decay timescale of mean autocorrelators, the functional form of the decay - a stretched exponential - and relates the value of the stretch exponent to the broad distribution of resonance timescales. The Jacobi method of matrix diagonalization provides numerical access to this distribution, as well as a conceptual framework for our analysis. The resonance model correctly predicts the stretch exponents for several models in the literature. Successive resonances may also underlie slow thermalization in strongly disordered systems in higher dimensions, or with long-range interactions.

cond-mat.dis-nn↗

Ergodicity breaking in rapidly rotating C60 fullerenes

Ergodicity, the central tenet of statistical mechanics, requires that an isolated system will explore all of its available phase space permitted by energetic and symmetry constraints. Mechanisms for violating ergodicity are of great interest for probing non-equilibrium matter and for protecting quantum coherence in complex systems. For decades, polyatomic molecules have served as an intriguing and challenging platform for probing ergodicity breaking in vibrational energy transport, particularly in the context of controlling chemical reactions. Here, we report the observation of rotational ergodicity breaking in an unprecedentedly large and symmetric molecule, 12C60. This is facilitated by the first ever observation of icosahedral ro-vibrational fine structure in any physical system, first predicted for 12C60 in 1986. The ergodicity breaking exhibits several surprising features: first, there are multiple transitions between ergodic and non-ergodic regimes as the total angular momentum is increased, and second, they occur well below the traditional vibrational ergodicity threshold. These peculiar dynamics result from the molecules' unique combination of symmetry, size, and rigidity, highlighting the potential of fullerenes to uncover emergent phenomena in mesoscopic quantum systems.

physics.atom-ph↗

Superconductivity and strong interactions in a tunable moiré quasiperiodic crystal

Electronic states in quasiperiodic crystals generally preclude a Bloch description, rendering them simultaneously fascinating and enigmatic. Owing to their complexity and relative scarcity, quasiperiodic crystals are underexplored relative to periodic and amorphous structures. Here, we introduce a new type of highly tunable quasiperiodic crystal easily assembled from periodic components. By twisting three layers of graphene with two different twist angles, we form two moiré patterns with incommensurate moiré unit cells. In contrast to many common quasiperiodic structures that are defined on the atomic scale, the quasiperiodicity in our system is defined on moiré length scales of several nanometers. This novel "moiré quasiperiodic crystal" allows us to tune the chemical potential and thus the electronic system between a periodic-like regime at low energies and a strongly quasiperiodic regime at higher energies, the latter hosting a large density of weakly dispersing states. Interestingly, in the quasiperiodic regime we observe superconductivity near a flavor-symmetry-breaking phase transition, the latter indicative of the important role electronic interactions play in that regime. The prevalence of interacting phenomena in future systems with in situ tunability is not only useful for the study of quasiperiodic systems, but it may also provide insights into electronic ordering in related periodic moiré crystals. We anticipate that extending this new platform to engineer quasiperiodic crystals by varying the number of layers and twist angles, and by using different two-dimensional components, will lead to a new family of quantum materials to investigate the properties of strongly interacting quasiperiodic crystals.

cond-mat.mes-hall↗

Coupled Layer Construction for Synthetic Hall Effects in Driven Systems

Quasiperiodically driven fermionic systems can support topological phases not realized in equilibrium. The fermions are localized in the bulk, but support quantized energy currents at the edge. These phases were discovered through an abstract classification, and few microscopic models exist. We develop a coupled layer construction for tight-binding models of these phases in $d\in\{1,2\}$ spatial dimensions, with any number of incommensurate drive frequencies $D$. The models exhibit quantized responses associated with synthetic two- and four-dimensional quantum Hall effects in the steady state. A numerical study of the phase diagram for $(d+D) = (1+2)$ shows: (i) robust topological and trivial phases separated by a sharp phase transition; (ii) charge diffusion and a half-integer energy current between the drives at the transition; and (iii) a long-lived topological energy current which remains present when weak interactions are introduced.

cond-mat.mes-hall↗

Moiré Landau fans and magic zeros

We study the energy spectrum of moiré systems under a uniform magnetic field. The superlattice potential generally broadens Landau levels into Chern bands with finite bandwidth. However, we find that these Chern bands become flat at a discrete set of magnetic fields which we dub "magic zeros". The flat band subspace is generally different from the Landau level subspace in the absence of the moiré superlattice. By developing a semiclassical quantization method and taking account of superlattice induced Bragg reflection, we prove that magic zeros arise from the simultaneous quantization of two distinct $k$-space orbits. The flat bands at magic zeros provide a new setting for exploring crystalline fractional quantum Hall physics.

cond-mat.mes-hall↗

Mean field theory of failed thermalizing avalanches

We show that localization in quasiperiodically modulated, two-dimensional systems is stable to the presence of a finite density of ergodic grains. This contrasts with the case of randomly modulated systems, where such grains seed thermalizing avalanches. These results are obtained within a quantitatively accurate, self-consistent entanglement mean field theory which analytically describes two level systems connected to a central ergodic grain. The theory predicts the distribution of entanglement entropies of each two level system across eigenstates, and the late time values of dynamical observables. In addition to recovering the known phenomenology of avalanches, the theory reproduces exact diagonalization data, and predicts the spatial profile of the thermalized region when the avalanche fails.

cond-mat.dis-nn↗

Many-Body Localization with Quasiperiodic Driving

Sufficient disorder is believed to localize static and periodically-driven interacting chains. With quasiperiodic driving by $D$ incommensurate tones, the fate of this many-body localization (MBL) is unknown. We argue that randomly disordered MBL exists for $D=2$, but not for $D\geq 3$. Specifically, a putative two-tone driven MBL chain is neither destabilized by thermal avalanches seeded by rare thermal regions, nor by the proliferation of long-range many-body resonances. For $D\geq 3$, however, sufficiently large thermal regions have continuous local spectra and slowly thermalize the entire chain. En route, we generalize the eigenstate thermalization hypothesis to the quasiperiodically-driven setting, and verify its predictions numerically. Two-tone driving enables new topological orders with edge signatures; our results suggest that localization protects these orders indefinitely.

cond-mat.dis-nn↗

Error measurements for a quantum annealer using the one-dimensional Ising model with twisted boundaries

A finite length ferromagnetic chain with opposite spin polarisation imposed at its two ends is one of the simplest frustrated spin models. In the clean classical limit the domain wall inserted on account of the boundary conditions resides with equal probability on any one of the bonds, and the degeneracy is precisely equal to the number of bonds. If quantum mechanics is introduced via a transverse field, the domain wall will behave as a particle in a box, and prefer to be nearer the middle of the chain rather than the ends. A simple characteristic of a real quantum annealer is therefore which of these limits obtains in practice. Here we have used the ferromagnetic chain with antiparallel boundary spins to test a real flux qubit quantum annealer and discover that contrary to both expectations, the domain walls found are non-uniformly distributed on account of effective random longitudinal fields present notwithstanding tuning carried out to zero out such fields when the couplings between qubits are nominally zero. We present a simple derivation of the form of the distribution function for the domain walls, and show also how the effect we have discovered can be used to determine the strength of the effective random fields (noise) characterising the annealer. The noise measured in this fashion is smaller than what is seen during the single qubit tuning process, but nonetheless qualitatively affects the outcome of the simulation performed by the annealer.

quant-ph↗

Supercurrent induced resonant optical response

The optical conductivity encodes the current response to a time dependent electric field. We develop a theory of the optical conductivity $σ(ω)$ in presence of a dc supercurrent. Current induced optical response is prohibited by Galilean invariance from occurring in systems with a single parabolic band. However, we show that lattice effects give rise to a pronounced current dependent peak in $σ(ω)$ at the gap edge $ω= 2 Δ$, which diverges in the clean limit. We demonstrate this in a model of a multi-band superconductor. Our theory explains the recent observation of a current induced peak in the optical conductivity in NbN by Nakamura et al. (2019), and provides a new mechanism for direct activation of the Higgs mode with light.

cond-mat.supr-con↗

Boosting the Quantum State of a Cavity with Floquet Driving

The striking nonlinear effects exhibited by cavity QED systems make them a powerful tool in modern condensed matter and atomic physics. A recently discovered example is the quantized pumping of energy into a cavity by a strongly-coupled, periodically-driven spin. We uncover a remarkable feature of these energy pumps: they coherently translate, or boost, a quantum state of the cavity in the Fock basis. Current optical cavity and circuit QED experiments can realize the required Hamiltonian in a rotating frame. Boosting thus enables the preparation of highly-excited non-classical cavity states in near-term experiments.

quant-ph↗