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Philip W. Phillips

Publications and source records attributed to Philip W. Phillips.

84 records · Page 5Linked to original sources

Non-Fermi Liquid behavior at the Orbital Ordering Quantum Critical Point in the Two-Orbital Model

The critical behavior of a two-orbital model with degenerate $d_{xz}$ and $d_{yz}$ orbitals is investigated by multidimensional bosonization. We find that the corresponding bosonic theory has an overdamped collective mode with dynamical exponent $z=3$, which appears to be a general feature of a two-orbital model and becomes the dominant fluctuation in the vicinity of the orbital-ordering quantum critical point. Since the very existence of this $z=3$ overdamped collective mode induces non-Fermi liquid behavior near the quantum critical point, we conclude that a two-orbital model generally has a sizable area in the phase diagram showing non-Fermi liquid behavior. Furthermore, we show that the bosonic theory resembles the continuous model near the d-wave Pomeranchuk instability, suggesting that orbital order in a two-orbital model is identical to nematic order in a continuous model. Our results can be applied to systems with degenerate $d_{xz}$ and $d_{yz}$ orbitals such as iron-based superconductors and bilayer strontium ruthenates Sr$_3$Ru$_2$O$_7$.

cond-mat.str-el↗

Absence of Luttinger's Theorem due to Zeros in the Single-Particle Green Function

We show exactly with an SU(N) interacting model that even if the ambiguity associated with the placement of the chemical potential, $μ$, for a T=0 gapped system is removed by using the unique value $μ(T\rightarrow 0)$, Luttinger's sum rule is violated even if the ground-state degeneracy is lifted by an infinitesimal hopping. The failure stems from the non-existence of the Luttinger-Ward functional for a system in which the self-energy diverges. Since it is the existence of the Luttinger-Ward functional that is the basis for Luttinger's theorem which relates the charge density to sign changes of the single-particle Green function, no such theorem exists. Experimental data on the cuprates are presented which show a systematic deviation from the Luttinger count, implying a breakdown of the electron quasiparticle picture in strongly correlated electron matter.

cond-mat.str-el↗

Tuning thermoelectric power factor by crystal-field and spin-orbit couplings in Kondo lattice materials

We study thermoelectric transport at low temperatures in correlated Kondo insulators, motivated by the recent observation of a high thermoelectric figure of merit(ZT) in $FeSb_2$ at $T \sim 10 K$. Even at room temperature, correlations have the potential to lead to high ZT, as in $YbAl_3$, one of the most widely used thermoelectric metals. At low temperature correlation effects are especially worthy of study because fixed band structures are unlikely to give rise to the very small energy gaps $E_g \sim 5 kT$ necessary for a weakly correlated material to function efficiently at low temperature. We explore the possibility of improving the thermoelectric properties of correlated Kondo insulators through tuning of crystal field and spin-orbit coupling and present a framework to design more efficient low-temperature thermoelectrics based on our results.

cond-mat.mtrl-sci↗

Non-Fermi Liquid due to Orbital Fluctuations in Iron Pnictide Superconductors

We study the influence of quantum fluctuations on the electron self energy in the normal state of iron-pnictide superconductors using a five orbital tight binding model with generalized Hubbard on-site interactions. Within a one-loop treatment, we find that an overdamped collective mode develops at low frequency in channels associated with quasi-1D $d_{xz}$ and $d_{yz}$ bands. When the critical point for the $C_4$ symmetry broken phase (structural phase transition) is approached, the overdamped collective modes soften, and acquire increased spectral weight, resulting in non-Fermi liquid behavior at the Fermi surface characterized by the frequency dependence of the imaginary part of electron self energy of the form $ω^λ$, $0<λ<1$. We argue that this non-Fermi liquid behavior is responsible for the recently observed zero-bias enhancement in the tunneling signal in quantum point contact spectroscopy. A key experimental test of this proposal is the absence of the non-Fermi liquid behaviour in the hole-doped materials. Our result suggests that quantum criticality plays an important role in understanding the normal state properties of iron-pnictide superconductors.

cond-mat.str-el↗

Pomeranchuk Instability in a non-Fermi Liquid from Holography

The Pomeranchuk instability, in which an isotropic Fermi surface distorts and becomes anisotropic due to strong interactions, is a possible mechanism for the growing number of experimental systems which display transport properties that differ along the $x$ and $y$ axes. We show here that the gauge-gravity duality can be used to describe such an instability in fermionic systems. Our holographic model consists of fermions in a background which describes the causal propagation of a massive neutral spin-two field in an asymptotically AdS spacetime. The Fermi surfaces in the boundary theory distort spontaneously and become anisotropic once the neutral massive spin-two field develops a normalizable mode in the bulk. Analysis of the fermionic correlators reveals that the low-lying fermionic excitations are non-Fermi liquid-like both before and after the Fermi surface shape distortion. Further, the spectral weight along the Fermi surface is angularly dependent and can be made to vanish along certain directions.

hep-th↗

Impact of Dynamic Orbital Correlations on Magnetic Excitations in the Normal State of Iron-Based Superconductors

We show here that orbital degrees of freedom produce a distinct signature in the magnetic excitation spectrum of iron-based superconductors above the magnetic ordering temperature. Because $d_{xz}$ and $d_{yz}$ orbitals are strongly connected with the Fermi surface topology, the nature of magnetic excitations can be modified significantly due to the presence of either static or fluctuating orbital correlations. Within a five-orbital itinerant model, we show that static orbital order generally leads to an enhancement of commensurate magnetic excitations even when the original Fermi surface lacks nesting at $(π,0)$ or $(0,π)$. When long-range orbital order is absent, Gaussian fluctuations beyond the standard random-phase approximation (RPA) capture the effects of fluctuating orbital correlations on the magnetic excitations. We find that commensurate magnetic excitations can also be enhanced if the orbital correlations are strong. Our results offer a natural explanation for the incommensurate-to-commensurate transformation observed in a recent neutron scattering measurement (Z. Xu, et. al., arXiv:1201.4404), and we propose that this unusual transformation is an important signature to distinguish orbital from spin physics in the normal state of the pnictides. Implications for the magnetic and superconducting states are discussed.

cond-mat.str-el↗

Spectral Weight Transfer in Multi-Orbital Mott Systems

We develop here a general formalism for multi-orbital Mott systems which can be used to understand dynamical and static spectral weight transfer. We find that the spectral weight transferred from the high energy scales is greatly increased as a result of the multi-orbital structure. As a consequence certainly dynamically generated symmetries obtain at lower values of doping than in the single-band Hubbard model. For example, in the atomic limit, the particle-hole symmetric condition in the lower band shifts from the one-band result of $x=1/3$ to $x=1/(2n_o+1)$, where $n_o$ is the number of orbitals with an unpaired spin. Transport properties computed from effective low-energy theories which forbid double occupancy of bare electrons, such as the multi-orbital t-J generalization, should all be be sensitive to this particle-hole symmetric condition. Away from the atomic limit, the dynamical contributions increase the transferred spectral weight. Consequently, any phenomena which are sensitive to an emergent particle-hole symmetry should obtain at $x<(1/(2n_o+1)$.

cond-mat.str-el↗

Neutral Order Parameters in Metallic Criticality in d=2+1 from a Hairy Electron Star

We use holography to study the spontaneous condensation of a neutral order parameter in a (2+1)-dimensional field theory at zero-temperature and finite density, dual to the electron star background of Hartnoll and Tavanfar. An appealing feature of this field theory is the emergence of an IR Lifshitz fixed-point with a finite dynamical critical exponent $z$, which is due to the strong interaction between critical bosonic degrees of freedom and a finite density of fermions (metallic quantum criticality). We show that under some circumstances the electron star background develops a neutral scalar hair whose holographic interpretation is that the boundary field theory undergoes a quantum phase transition, with a Berezinski-Kosterlitz-Thouless character, to a phase with a neutral order parameter. Including the backreaction of the bulk neutral scalar on the background, we argue that the two phases across the quantum critical point have different $z$, a novelty that exists in certain quantum phase transitions in condensed matter systems. We also analyze the system at finite temperature and find that the phase transition becomes, as expected, second-order. Embedding the neutral scalar into a higher form, a variety of interesting phases could potentially be realized for the boundary field theory. Examples which are of particular interest to condensed matter physics include an antiferromagnetic phase where a vector condenses and break the spin symmetry, a quadrupole nematic phase which involves the condensation of a symmetric traceless tensor breaking rotational symmetry, or different phases of a system with competing order parameters.

hep-th↗

Dynamically Generated Gap from Holography: Mottness from a Black Hole

In the fermionic sector of top-down approaches to holographic systems, one generically finds that the fermions are coupled to gravity and gauge fields in a variety of ways, beyond minimal coupling. In this paper, we take one such interaction -- a Pauli, or dipole, interaction -- and study its effects on fermion correlators. We find that this interaction modifies the fermion spectral density in a remarkable way. As we change the strength of the interaction, we find that spectral weight is transferred between bands, and beyond a critical value, a hard gap emerges in the fermion density of states. A possible interpretation of this bulk interaction then is that it drives the dynamical formation of a (Mott) gap, in the absence of continuous symmetry breaking.

hep-th↗

Dynamical Gap and Cuprate-like Physics from Holography

We study the properties of fermion correlators in a boundary theory dual to the Reissner-Nordström AdS_{d+1} background in the presence of a bulk dipole (Pauli) interaction term with strength p. We show that by simply changing the value of the parameter p we can tune continuously from a Fermi liquid (small p), to a marginal Fermi liquid behavior at a critical value of p, to a generic non-Fermi liquid at intermediate values of p, and finally to a Mott insulator at large values of the bulk Pauli coupling. As all of these phases are seen in the cuprate phase diagram, the holographic model we study has the key elements of the strong coupling physics typified by Mott systems. In addition, we extend our analysis to finite temperature and show that the Mott gap closes. Of particular interest is that it closes when the ratio of the gap to the critical temperature is of the order of ten. This behavior is very much similar to that observed in the classic Mott insulator VO_2. We then analyze the non-analyticities of the boundary theory fermion correlators for generic values of frequency and momentum by calculating the quasi-normal modes of the bulk fermions. Not surprisingly, we find no evidence for the dipole interaction inducing an instability in the boundary theory. Finally, we briefly consider the introduction of superconducting condensates, and find that in that case, the fermion gap is driven by scalar-fermion couplings rather than by the Pauli coupling.

hep-th↗

Universality of liquid-gas Mott transitions at finite temperatures

We explain in a consistent manner the set of seemingly conflicting experiments on the finite temperature Mott critical point, and demonstrate that the Mott transition is in the Ising universality class. We show that, even though the thermodynamic behavior of the system near such critical point is described by an Ising order parameter, the global conductivity can depend on other singular observables and, in particular, on the energy density. Finally, we show that in the presence of weak disorder the dimensionality of the system has crucial effects on the size of the critical region that is probed experimentally.

cond-mat.str-el↗

Much Ado about Zeros: The Luttinger Surface and Mottness

We prove that the Mott insulating state is characterized by a divergence of the electron self energy at well-defined values of momenta in the first Brillouin zone. When particle-hole symmetry is present, the divergence obtains at the momenta of the Fermi surface for the corresponding non-interacting system. Such a divergence gives rise to a surface of zeros (the Luttinger surface) of the single-particle Green function and offers a single unifying principle of Mottness from which pseudogap phenomena, spectral weight transfer, and broad spectral features emerge in doped Mott insulators. We also show that only when particle-hole symmetry is present does the volume of the zero surface equal the particle density. We identify that the general breakdown of Luttinger's theorem in a Mott insulator arises from the breakdown of a perturbative expansion for the self energy in the single-particle Green function around the non-interacting limit. A modified version of Luttinger's theorem is derived for special cases.

cond-mat.str-el↗