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Philip Walther

Publications and source records attributed to Philip Walther.

At least 19 recordsLinked to original sources

Experimental Quantum Key Distribution in an Indefinite Causal Order

In quantum physics the order in which different operations occur can be placed in superposition. The resulting processes have an indefinite causal order and are both of fundamental interest and can be viewed as a novel quantum resource that enables a variety of new protocols. Here we report an experimental implementation of one such protocol, where we perform BB84-like quantum cryptography by placing Alice and Bob's measurement-and-preparation operations in a photonic quantum SWITCH. By embedding Alice and Bob within the quantum SWITCH, the protocol achieves an average eavesdropper detection probability of $0.15 \pm 0.02$ per shared qubit, with eavesdropper detection performed through measurements of the control qubit rather than by comparing the key. Unlike the standard BB84 and related schemes, which detect eavesdropping by publicly revealing and discarding a fraction of the raw key, our approach requires no disclosure of key material: every retained qubit can, in principle, be tested for eavesdropping while remaining available for key generation. The experiment relies on a new measurement technique that allows the polarization of a photon to be measured inside the quantum SWITCH without destroying path coherence. Although the present implementation does not yet constitute a secure quantum key distribution protocol, owing to the post-selection required for measurements within the quantum SWITCH, it provides a proof of principle that indefinite causal order can be exploited to detect eavesdropping without sacrificing key bits.

quant-ph

Scaling native entanglement generation in layered semiconductors with quasi-phase matching

Efficient generation of entangled photons typically relies on spontaneous parametric down-conversion (SPDC) in phase-matched macroscopic nonlinear media. However, generating entanglement under phase-matching constraints requires additional bulk optics or interferometers. In contrast, ultrathin van der Waals semiconductors - such as transition metal dichalcogenides (TMDs) - exhibit strong enough optical nonlinearities for SPDC to be observed from subwavelength-thick media, thereby bypassing conventional phase-matching constraints. In this microscopic domain, the intrinsic crystal symmetry governs the nonlinear optical response, enabling the native generation of polarization-entangled photon pairs. However, generating these states efficiently has been fundamentally restricted by the material's coherence length ($L_c$), which limits the attainable conversion efficiency. Here, we investigate periodically-poled TMDs (PPTMDs) designed to scale up this interaction via quasi-phase matching. We demonstrate that mechanically flipping the sign of the nonlinearity at precise intervals of $L_c$ introduces quasi-phase matching, that scales the pair-production rate while preserving the pristine, symmetry-generated polarization entanglement, with fidelities exceeding 99%. Backed by a rigorous theoretical model, our work clarifies the interplay between crystal symmetry and propagation effects in thin nonlinear media, providing a new avenue for engineering quantum light in nanophotonic systems.

quant-ph

Realization of waveguide many-body quantum optics

Controlling light photon-by-photon is central to quantum optics. At a fundamental level, photon interactions are mediated by their coupling to atoms, and ultimate control requires deterministic light-matter interfacing of single photons to single atoms. Extending this paradigm to radiatively couple multiple individual atoms in a deterministic and scalable manner opens the arena of many-body quantum optics. Here, we realize such a setting by coherently coupling solid-state artificial atoms to a nanophotonic waveguide and demonstrate higher-order photon correlations that are controlled by the number of quantum emitters. We study the scaling of nonlinear photonic transport induced by emitter-photon scattering and demonstrate that adding a quantum emitter generates higher-order photon correlations. Specifically, we experimentally observe genuine three-photon correlations from a pair of collectively coupled emitters, while contributions from lower photon numbers are suppressed. In addition, we scale to three resonant quantum emitters coupled to the waveguide. These advancements demonstrate the onset of many-body quantum optics in waveguide quantum electrodynamics, enabling new photonic quantum simulators, the creation of many-body entangled states, and the exploration of novel quantum phase transitions.

quant-ph

Distribution of GHz sequential Time-bin Entanglement in a Metropolitan Fiber Network

Efficient generation and high-quality distribution of entanglement is becoming increasingly more relevant in the field of quantum technologies, with important applications such as multiparty computation as well as quantum key distribution (QKD) on the rise. Quantum communication protocols based on entanglement offer an inherent quantum based randomness for key generation and provide in general higher security compared to prepare and measure implementations. Moreover, the future quantum internet will also be based on the distribution of entanglement for securely connecting quantum computers in a network. In this work we show the feasibility of using sequential time-bin entangled states for quantum key distribution in metropolitan networks using off-the-shelf components. The time-bin encoding ensures high fidelity distribution robust against random polarisation fluctuations occuring in optical fibers. Modulated laser pulses in the GHz frequency range are used to generate time-bin entangled photon pairs. The entangled photons are then sent over an about 30km long (9.5dB loss) fiber link within the Vienna fiber network, showing high degree of distributed entanglement with a measured 93\% quantum visibility.

quant-ph

Photon Number Coherence of a Quantum Dot-Cavity System Excited Using the SUPER Scheme

To fulfill the security requirements of quantum cryptography, photon number coherence (PNC) of single photon sources has recently become an important figure of merit. Quantum dots (QDs) embedded in photonic microcavities offer a mature source of single photons, of which many properties can be tuned by the use of different excitation protocols or parameters. We show that the Swing-UP of quantum EmitteR population (SUPER) scheme can significantly decrease the PNC of the emitted photon, compared to resonant excitation. The reason for this is a laser-induced Stark shift, which effectively decouples the QD from the cavity during the SUPER excitation. Our calculations account for environmental effects such as phonons and radiative losses.

quant-ph

Toward an Experimental Device-Independent Verification of Indefinite Causal Order

In classical physics, events follow a definite causal order: the past influences the future, but not the reverse. Quantum theory, however, permits superpositions of causal orders -- so-called indefinite causal orders -- which can provide operational advantages over classical scenarios. Verifying such phenomena has sparked significant interest, much like earlier efforts devoted to refuting local realism and confirming quantum entanglement. To date, demonstrations of indefinite causal order have all been based a process called the quantum switch and have relied on device-dependent or semi-device-independent protocols. Achieving a device-independent verification of indefinite causal order would imply that nature allows for correlations that do not respect causality, independent of any experimental assumptions or underlying theoretical description of the experiment. To this end, a recent theoretical development introduced a Bell-like inequality that allows for fully device-independent verification of indefinite causal order in a quantum switch. Here we implement this verification by experimentally violating this inequality. In particular, we measure a value of $1.8328 \pm 0.0045$, which is 18 standard deviations above the Definite Causal Order Bound of $1.75$. Our work presents the first implementation of a device-independent protocol to verify indefinite causal order, albeit in the presence of experimental loopholes. This represents an important step towards the device-independent verification of an indefinite causal order, and provides a context in which to identify loopholes specifically related to the verification of indefinite causal order.

quant-ph

Time-Delocalized Local Measurements in an Indefinite Causal Order

Processes with indefinite causal order (ICO), such as the quantum switch, are an emerging resource for quantum tasks and a fundamental test bed for studies of temporal correlations in quantum mechanics. A limitation of past photonic implementations of the quantum switch, however, is their inability to perform measurements inside the switch without either destroying the superposition of causal orders or delaying readout until the after the quantum switch. Measurements where the results are read out locally are needed for several applications of ICO, but also for a loophole-free verification of ICO. Here, we overcome past limitations by introducing a $\mathit{local}$ measurement scheme and coupling the photon in the switch to a $\mathit{time-delocalized}$ ancilla system. We experimentally realize this protocol using a photonic quantum switch with post-selected linear optical logic gates. Our method ensures that the measurement apparatus interacts with the system at two distinct times and yet yields a single outcome. We use a quantum eraser measurement to preserve the ICO, which we certify by measuring a causal witness and finding a negative value of $\mathcal{C}_W \approx -0.305 (1)$. Furthermore, by explicitly realizing a time-delocalized ancilla system, our protocol not only enables a new class of quantum switch protocols requiring local readout, but also provides a general method for path-coherence-preserving measurements with broad applications beyond ICO.

quant-ph

Quantum interferometry in external gravitational fields

Current models of quantum interference experiments in external gravitational fields lack a common framework: while matter-wave interferometers are commonly described using the Schrödinger equation with a Newtonian potential, gravitational effects in quantum optics are modeled using either post-Newtonian metrics or highly symmetric exact solutions to Einstein's field equations such as those of Schwarzschild and Kerr. To coherently describe both kinds of experiments, this paper develops a unified framework for modeling quantum interferometers in general stationary space-times. This model provides a rigorous description and coherent interpretation of the effects of classical gravity on quantum probes.

gr-qc

Quantum cryptography beyond key distribution: theory and experiment

Owing to its fundamental principles, quantum theory holds the promise to enhance the security of modern cryptography, from message encryption to anonymous communication, digital signatures, online banking, leader election, one-time passwords and delegated computation. While quantum key distribution (QKD) has already enabled secure key exchange over hundreds of kilometers, a myriad of other quantum-cryptographic primitives are being developed to secure future applications against quantum adversaries. This review surveys the theoretical and experimental developments in quantum cryptography beyond QKD over the decades, along with advances in secure quantum computation. It provides an intuitive classification of the main quantum primitives and their security levels, summarizes their possibilities and limits, and discusses their implementation with current photonic technology.

quant-ph

50-km fiber interferometer for testing gravitational signatures in quantum interference

Quantum mechanics and general relativity are the foundational pillars of modern physics, yet experimental tests that combine the two frameworks remain rare. Measuring optical phase shifts of massless photons in a gravitational potential provides a unique quantum platform to probe gravity beyond Newtonian descriptions, but laboratory-based interferometers have not yet reached the sensitivity needed to access this regime. Here, we report the realization of a 50-km table-top Mach-Zehnder fiber interferometer operating at the single-photon level, achieving a phase sensitivity of $4.42\times10^{-6}$ rad root-mean-square (RMS) within the frequency range of 0.01 Hz to 5 Hz. We demonstrate that this sensitivity is sufficient to resolve a phase-shift signal of $(6.18 \pm 0.44)\times10^{-5}$ rad RMS at 0.1 Hz, associated with a modulated gravity-induced signal. Our results establish a milestone for quantum sensing with large-scale optical interferometry, demonstrating the capability to detect gravitational redshifts in a local laboratory, thereby paving the way for testing quantum phenomena within general relativistic frameworks.

quant-ph

A scalable advantage in multi-photon quantum machine learning

Photons are promising candidates for quantum information technology due to their high robustness and long coherence time at room temperature. Inspired by the prosperous development of photonic computing techniques, recent research has turned attention to performing quantum machine learning on photonic platforms. Although photons possess a high-dimensional quantum feature space suitable for computation, a general understanding of how to harness it for learning tasks remains blank. Here, we establish both theoretically and experimentally a scalable advantage in quantum machine learning with multi-photon states. Firstly, we prove that the learning capacity of linear optical circuits scales polynomially with the photon number, enabling generalization from smaller training datasets and yielding lower test loss values. Moreover, we experimentally corroborate these findings through unitary learning and metric learning tasks, by performing online training on a fully programmable photonic integrated platform. Our work highlights the potential of photonic quantum machine learning and paves the way for achieving quantum enhancement in practical machine learning applications.

quant-ph

Testing Single Photon Entanglement using Self-Referential Measurements

Entanglement does not always require one particle per party. It was predicted some thirty years ago that a single photon traversing a beam splitter could violate a Bell inequality. Although initially debated, single-photon nonlocality was eventually demonstrated via homodyne measurements. Here, we present an alternate realisation that avoids the complexity of homodyne measurements and potential loopholes in their implementation. We violate a Bell inequality by performing joint measurements on two copies of the same single-photon entangled state, where one photon acts as a phase reference for the other, making it self-referential. We observe CHSH parameters of $2.71\pm 0.09$ and $2.23\pm 0.07$, depending on the joint measurements implemented. This offers a new perspective on single-photon nonlocality and a more accessible experimental route, potentially applicable to general mode-entangled states in diverse platforms.

quant-ph

Measuring space-time curvature using maximally path-entangled quantum states

Experiments at the interface of quantum field theory and general relativity would greatly benefit theoretical research towards their unification. The gravitational aspects of quantum experiments performed so far can be explained either within Newtonian gravity or by Einstein's equivalence principle. Here, we describe a way to measure components of the Riemann curvature tensor with maximally path-entangled quantum states of light. We show that the entanglement-induced increase in sensitivity also holds for gravitationally-induced phases in Mach-Zehnder interferometers. As a result, the height difference between the two interferometer arms necessary to rule out flat space-time by measuring gravity gradients can be significantly reduced.

gr-qc

Quantum Communication with Quantum Dots Beyond Telecom Wavelengths via Hollow-Core Fibers

Quantum dot single-photon sources are promising for quantum communication. Yet, the most advanced devices operate near 900 nm, where standard single-mode fibers experience significant losses. We address this by employing a hollow-core fiber engineered for low-loss transmission at quantum dot wavelengths, with measured loss of 0.65 dB/km and potentially as low as 0.12 dB/km near 934 nm. The fiber also supports strong classical signals at 1550 nm without adding Raman noise. Using this platform, we transmit all four BB84 polarization states from an InAs quantum dot over 340 m with 0.1% QBER, preserving single-photon purity and indistinguishability even in the presence of a strong classical signal. These results highlight how tailored transmission media enable quantum networks beyond the limits of standard telecom fibers.

quant-ph

Atomically thin silver films for enhanced nanoscale nonlinear optics

The inherently weak nonlinear optical response of bulk materials remains a fundamental limitation in advancing photonic technologies. Nanophotonics addresses this challenge by tailoring the size and morphology of nanostructures to manipulate the optical near field, thus modulating the nonlinear response. Here, we explore a complementary strategy based on engineering the electronic band structure in the mesoscopic regime to enhance optical nonlinearities. Specifically, we demonstrate an increase in second-harmonic generation (SHG) from crystalline silver films as their thickness is reduced down to just a few atomic monolayers. Operating at the boundary between bulk and two-dimensional systems, these ultra-thin films exhibit a pronounced enhancement of SHG with decreasing thickness. This enhancement stems from quantum confinement effects that modify the interaction between electronic states and incident light, which we explain based on quantum-mechanical calculation. Our atomically-thin crystalline silver films provide a new means to overcome the small interaction volumes inherent to nanophotonic platforms, enabling efficient nanoscale nonlinear optics with potential applications in photonics, sensing, and quantum technologies.

physics.optics

Performance of Practical Quantum Oblivious Key Distribution

Motivated by the applications of secure multiparty computation as a privacy-protecting data analysis tool, and identifying oblivious transfer as one of its main practical enablers, we propose a practical realization of randomized quantum oblivious transfer. By using only symmetric cryptography primitives to implement commitments, we construct computationally-secure randomized oblivious transfer without the need for public-key cryptography or assumptions imposing limitations on the adversarial devices. We show that the protocol is secure under an indistinguishability-based notion of security and demonstrate an experimental implementation to test its real-world performance. Its security and performance are then compared to both quantum and classical alternatives, showing potential advantages over existing solutions based on the noisy storage model and public-key cryptography.

quant-ph

Purifying photon indistinguishability through quantum interference

Indistinguishability between photons is a key requirement for scalable photonic quantum technologies. We experimentally demonstrate that partly distinguishable single photons can be purified to reach near-unity indistinguishability by the process of quantum interference with ancillary photons followed by heralded detection of a subset of them. We report on the indistinguishability of the purified photons by interfering two purified photons and show improvements in the photon indistinguishability of $2.774(3)$\% in the low-noise regime, and as high as $10.2(5)$ \% in the high-noise regime.

quant-ph

Demonstration of Hardware Efficient Photonic Variational Quantum Algorithm

Quantum computing has brought a paradigm change in computer science, where non-classical technologies have promised to outperform their classical counterpart. Such an advantage was only demonstrated for tasks without practical applications, still out of reach for the state-of-art quantum technologies. In this context, a promising strategy to find practical use of quantum computers is to exploit hybrid quantum-classical models, where a quantum device estimates a hard-to-compute quantity, while a classical optimizer trains the parameters of the model. In this work, we demonstrate that single photons and linear optical networks are sufficient for implementing Variational Quantum Algorithms, when the problem specification, or ansatz, is tailored to this specific platform. We show this by a proof-of-principle demonstration of a variational approach to tackle an instance of a factorization task, whose solution is encoded in the ground state of a suitable Hamiltonian. This work which combines Variational Quantum Algorithms with hardware efficient ansatzes for linear-optics networks showcases a promising pathway towards practical applications for photonic quantum platforms.

quant-ph