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Philip Walther

Publications and source records attributed to Philip Walther.

At least 73 records · Page 4Linked to original sources
arXiv2023

Controlling the Photon Number Coherence of Solid-state Quantum Light Sources for Quantum Cryptography

Quantum communication networks rely on quantum cryptographic protocols including quantum key distribution (QKD) using single photons. A critical element regarding the security of QKD protocols is the photon number coherence (PNC), i.e. the phase relation between the zero and one-photon Fock state, which critically depends on the excitation scheme. Thus, to obtain flying qubits with the desired properties, optimal pumping schemes for quantum emitters need to be selected. Semiconductor quantum dots generate on-demand single photons with high purity and indistinguishability. Exploiting two-photon excitation of a quantum dot combined with a stimulation pulse, we demonstrate the generation of high-quality single photons with a controllable degree of PNC. Our approach provides a viable route toward secure communication in quantum networks.

quant-ph↗
arXiv2023

Programmable multi-photon quantum interference in a single spatial mode

The interference of non-classical states of light enables quantum-enhanced applications reaching from metrology to computation. Most commonly, the polarisation or spatial location of single photons are used as addressable degrees-of-freedom for turning these applications into praxis. However, the scale-up for the processing of a large number of photons of such architectures is very resource demanding due to the rapidily increasing number of components, such as optical elements, photon sources and detectors. Here we demonstrate a resource-efficient architecture for multi-photon processing based on time-bin encoding in a single spatial mode. We employ an efficient quantum dot single-photon source, and a fast programmable time-bin interferometer, to observe the interference of up to 8 photons in 16 modes, all recorded only with one detector--thus considerably reducing the physical overhead previously needed for achieving equivalent tasks. Our results can form the basis for a future universal photonics quantum processor operating in a single spatial mode.

quant-ph↗
arXiv2023

Benchmarking the human brain against computational architectures

The human brain has inspired novel concepts complementary to classical and quantum computing architectures, such as artificial neural networks and neuromorphic computers, but it is not clear how their performances compare. Here we report a new methodological framework for benchmarking cognitive performance based on solving computational problems with increasing problem size. We determine computational efficiencies in experiments with human participants and benchmark these against complexity classes. We show that a neuromorphic architecture with limited field-of-view size and added noise provides a good approximation to our results. The benchmarking also suggests there is no quantum advantage on the scales of human capability compared to the neuromorphic model. Thus, the framework offers unique insights into the computational efficiency of the brain by considering it a black box.

q-bio.NC↗
arXiv2023

Semi-device-independent certification of indefinite causal order in a photonic quantum switch

We report an experimental certification of indefinite causal order that relies only on the characterization of the operations of a single party. We do so in the semi-device-independent scenario with the fewest possible assumptions of characterization of the parties' local operations in which indefinite causal order can be demonstrated with the quantum switch. To achieve this result, we introduce the concept of semi-device-independent causal inequalities and show that the correlations generated in a photonic quantum switch, in which all parties are able to collect local outcome statistics, achieve a violation of this inequality of 224 standard deviations. This result consists of the experimental demonstration of indefinite causal order with the fewest device-characterization assumptions to date.

quant-ph↗
arXiv2023

Single-active-element demultiplexed multi-photon source

Temporal-to-spatial demultiplexing routes non-simultaneous events of the same spatial mode to distinct output trajectories. This technique has now been widely adopted because it gives access to higher-number multi-photon states when exploiting solid-state quantum emitters. However, implementations so far have required an always-increasing number of active elements, rapidly facing resource constraints. Here, we propose and demonstrate a demultiplexing approach that utilizes only a single active element for routing to, in principle, an arbitrary number of outputs. We employ our device in combination with a high-efficiency quantum dot based single-photon source, and measure up to eight demultiplexed highly indistinguishable single photons. We discuss the practical limitations of our approach, and describe in which conditions it can be used to demultiplex, e.g., tens of outputs. Our results thus provides a path for the preparation of resource-efficient larger-scale multi-photon sources.

quant-ph↗
arXiv2023

Nonlinear quantum logic with colliding graphene plasmons

Graphene has emerged as a promising platform to bring nonlinear quantum optics to the nanoscale, where a large intrinsic optical nonlinearity enables long-lived and actively tunable plasmon polaritons to strongly interact. Here we theoretically study the collision between two counter-propagating plasmons in a graphene nanoribbon, where transversal subwavelength confinement endows propagating plasmons with %large effective masses a flat band dispersion that enhances their interaction. This scenario presents interesting possibilities towards the implementation of multi-mode polaritonic gates that circumvent limitations imposed by the Shapiro no-go theorem for photonic gates in nonlinear optical fibers. As a paradigmatic example we demonstrate the feasibility of a high fidelity conditional Pi phase shift (CZ), where the gate performance is fundamentally limited only by the single-plasmon lifetime. These results open new exciting avenues towards quantum information and many-body applications with strongly-interacting polaritons.

quant-ph↗
arXiv2023

Enhancing quantum cryptography with quantum dot single-photon sources

Quantum cryptography harnesses quantum light, in particular single photons, to provide security guarantees that cannot be reached by classical means. For each cryptographic task, the security feature of interest is directly related to the photons' non-classical properties. Quantum dot-based single-photon sources are remarkable candidates, as they can in principle emit deterministically, with high brightness and low multiphoton contribution. Here, we show that these sources provide additional security benefits, thanks to the tunability of coherence in the emitted photon-number states. We identify the optimal optical pumping scheme for the main quantum-cryptographic primitives, and benchmark their performance with respect to Poisson-distributed sources such as attenuated laser states and down-conversion sources. In particular, we elaborate on the advantage of using phonon-assisted and two-photon excitation rather than resonant excitation for quantum key distribution and other primitives. The presented results will guide future developments in solid-state and quantum information science for photon sources that are tailored to quantum communication tasks.

quant-ph↗
arXiv2022

A compiler for universal photonic quantum computers

Photons are a natural resource in quantum information, and the last decade showed significant progress in high-quality single photon generation and detection. Furthermore, photonic qubits are easy to manipulate and do not require particularly strongly sealed environments, making them an appealing platform for quantum computing. With the one-way model, the vision of a universal and large-scale quantum computer based on photonics becomes feasible. In one-way computing, the input state is not an initial product state, but a so-called cluster state. A series of measurements on the cluster state's individual qubits and their temporal order, together with a feed-forward procedure, determine the quantum circuit to be executed. We propose a pipeline to convert a QASM circuit into a graph representation named measurement-graph (m-graph), that can be directly translated to hardware instructions on an optical one-way quantum computer. In addition, we optimize the graph using ZX-Calculus before evaluating the execution on an experimental discrete variable photonic platform.

quant-ph↗
arXiv2022

Experimental Semi-quantum Key Distribution With Classical Users

Quantum key distribution, which allows two distant parties to share an unconditionally secure cryptographic key, promises to play an important role in the future of communication. For this reason such technique has attracted many theoretical and experimental efforts, thus becoming one of the most prominent quantum technologies of the last decades. The security of the key relies on quantum mechanics and therefore requires the users to be capable of performing quantum operations, such as state preparation or measurements in multiple bases. A natural question is whether and to what extent these requirements can be relaxed and the quantum capabilities of the users reduced. Here we demonstrate a novel quantum key distribution scheme, where users are fully classical. In our protocol, the quantum operations are performed by an untrusted third party acting as a server, which gives the users access to a superimposed single photon, and the key exchange is achieved via interaction-free measurements on the shared state. We also provide a full security proof of the protocol by computing the secret key rate in the realistic scenario of finite-resources, as well as practical experimental conditions of imperfect photon source and detectors. Our approach deepens the understanding of the fundamental principles underlying quantum key distribution and, at the same time, opens up new interesting possibilities for quantum cryptography networks

quant-ph↗
arXiv2022

Enhanced Photonic Maxwell's Demon with Correlated Baths

Maxwell's Demon is at the heart of the interrelation between quantum information processing and thermodynamics. In this thought experiment, a demon generates a temperature gradient between two thermal baths initially at equilibrium by gaining information at the single-particle level and applying classical feed-forward operations, allowing for the extraction of work. Here we implement a photonic version of Maxwell's Demon with active feed-forward in a fibre-based system using ultrafast optical switches. We experimentally show that, if correlations exist between the two thermal baths, the Demon can generate a temperature difference over an order of magnitude larger than without correlations, and so extract more work. Our work demonstrates the great potential of photonic experiments -- which provide a unique degree of control on the system -- to access new regimes in quantum thermodynamics.

quant-ph↗
arXiv2022

Experimental beating the standard quantum limit under non-markovian dephasing environment

Entanglement enhanced quantum metrology has been well investigated for beating the standard quantum limit (SQL). However, the metrological advantage of entangled states becomes much more elusive in the presence of noise. Under strictly Markovian dephasing noise, the uncorrelated and maximally entangled states achieve exactly the same measurement precision. However, it was predicted that in a non-Markovian dephasing channel, the entangled probes can recover their metrological advantage. Here, by using a highly controlled photonic system, we simulate a non-Markovian dephasing channel fulfill the quadratic decay behaviour. Under such a channel, we demonstrate the GHZ states can surpass the SQL in a scaling manner, up to six photons. Since the quadratic decay behavior is quite general for short time expansion in open quantum systems (also known as the quantum Zeno effect), our results suggest a universal and scalable method to beat the SQL in the real-word metrology tasks.

quant-ph↗
arXiv2022

Demonstration of universal time-reversal for quantum processes

Although the laws of classical physics are deterministic, thermodynamics gives rise to an arrow of time through irreversible processes. In quantum mechanics the unitary nature of the time evolution makes it intrinsically reversible, however the question of how to revert an unknown time evolution nevertheless remains. Remarkably, there have been several recent demonstrations of protocols for reverting unknown unitaries in scenarios where even the interactions with the target system are unknown. The practical use of these universal rewinding protocols is limited by their probabilistic nature, raising the fundamental question of whether time-reversal could be performed deterministically. Here we show that quantum physics indeed allows for deterministic universal time-reversal by exploiting the non-commuting nature of quantum operators, and demonstrate a recursive protocol for two-level quantum systems with an arbitrarily high probability of success. Using a photonic platform we demonstrate our protocol, reverting the discrete time evolution of a polarization state with an average state fidelity of over 95%. Our protocol, requiring no knowledge of the quantum process to be rewound, is optimal in its running time, and brings quantum rewinding into a regime of practical relevance.

quant-ph↗
arXiv2022

High-harmonic generation enhancement with graphene heterostructures

We investigate high-harmonic generation in graphene heterostructures consisting of metallic nanoribbons separated from a graphene sheet by either a few-nanometer layer of aluminum oxide or an atomic monolayer of hexagonal boron nitride. The nanoribbons amplify the near-field at the graphene layer relative to the externally applied pumping, thus allowing us to observe third- and fifth-harmonic generation in the carbon monolayer at modest pump powers in the mid-infrared. We study the dependence of the nonlinear signals on the ribbon width and spacer thickness, as well as pump power and polarization, and demonstrate enhancement factors relative to bare graphene reaching 1600 and 4100 for third- and fifth-harmonic generation, respectively. Our work supports the use of graphene heterostructures to selectively enhance specific nonlinear processes of interest, an essential capability for the design of nanoscale nonlinear devices.

cond-mat.mes-hall↗
arXiv2022

Inferring work by quantum superposing forward and time-reversal evolutions

The study of thermodynamic fluctuations allows one to relate the free energy difference between two equilibrium states with the work done on a system through processes far from equilibrium. This finding plays a crucial role in the quantum regime, where the definition of work becomes non-trivial. Based on these relations, here we develop a simple interferometric method allowing a direct estimation of the work distribution and the average dissipative work during a driven thermodynamic process by superposing the forward and time-reversal evolutions of the process. We show that our scheme provides useful upper bounds on the average dissipative work even without full control over the thermodynamic process, and we propose methodological variations depending on the possible experimental limitations encountered. Finally, we exemplify its applicability by an experimental proposal for implementing our method on a quantum photonics system, on which the thermodynamic process is performed through polarization rotations induced by liquid crystals acting in a discrete temporal regime.

quant-ph↗
arXiv2022

A perspective on few-copy entanglement detection in experiments

Although the realization of useful quantum computers poses significant challenges, swift progress in emerging quantum technologies is making this goal realistically approachable. In this context, one of the essential resources is quantum entanglement, which allows for quantum computations outperforming their classical counterparts. However, the task of entanglement detection is not always straightforward for several reasons. One of the main challenges is that standardly-used methods rapidly become unfeasible when dealing with quantum states containing more than a few qubits. Typically, this is due to the fact that a vast amount of measurements is needed on many copies of the state. Generally, it is not unusual to deal with a very limited number of state copies in experimental settings - in fact, this may be the case for many large quantum systems. In this article, an overview is provided of a probabilistic approach that enables high-confidence genuine multipartite entanglement detection using an exceptionally low number of state copies. Additionally, a study is presented that shows that this protocol remains efficient also in the presence of noise, thus confirming the practicality of the method for near-term quantum devices and its suitability for complex experimental settings.

quant-ph↗
arXiv2021

Experimental entanglement of temporal order

The study of causal relations has recently been applied to the quantum realm, leading to the discovery that not all physical processes have a definite causal structure. While indefinite causal processes have previously been experimentally shown, these proofs relied on the quantum description of the experiments. Yet, the same experimental data could also be compatible with definite causal structures within different descriptions. Here, we present the first demonstration of indefinite temporal order outside of quantum formalism. We show that our experimental outcomes are incompatible with a class of generalised probabilistic theories satisfying the assumptions of locality and definite temporal order. To this end, we derive physical constraints (in the form of a Bell-like inequality) on experimental outcomes within such a class of theories. We then experimentally invalidate these theories by violating the inequality using entangled temporal order. This provides experimental evidence that there exist correlations in nature which are incompatible with the assumptions of locality and definite temporal order.

quant-ph↗