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Philipp Pirro

Publications and source records attributed to Philipp Pirro.

At least 19 recordsLinked to original sources

Magneto-optical signal from $\mathrm{Co_2Mn}$-based Heusler thin films in MOKE and BLS

$\mathrm{Co_2Mn}$-based Heusler compounds offer a versatile, composition-tunable platform for magnonics and spintronics. Among them, the half-metallic $\mathrm{Co_2MnSi}$ is of particular interest for magnonics owing to its ultralow Gilbert damping, yet its weak magneto-optical response in the visible challenges optical probing such as Brillouin light scattering (BLS). We study the magneto-optical response of epitaxial $\mathrm{Co_2Mn}X$ films ($X = \{\mathrm{Al}_x\mathrm{Si}_{1-x}, \mathrm{Ga}_x\mathrm{Ge}_{1-x}, \mathrm{Sn}\}$) by magneto-optical Kerr effect (MOKE) spectroscopy and BLS. Angle-resolved MOKE resolves a significant, wavelength-dependent quadratic MOKE (QMOKE) only for $\mathrm{Co_2MnSi}$, whereas $\mathrm{Co_2MnAl}$, $\mathrm{Co_2MnGa}$ and $\mathrm{Co_2MnSn}$ respond dominantly linearly. Comparing BLS intensities of thermal magnons at two wavelengths, $\mathrm{Co_2MnSi}$ gives the weakest signal at 532 nm yet among the strongest at 457 nm, tracking the spectral dependence of its Kerr angle. These results emphasise the relation between the two magneto-optical techniques, guiding the choice of probing wavelength for $\mathrm{Co_2Mn}$-based Heusler compounds.

cond-mat.mes-hall

Resonant excitations via low frequency pumping in driven magnon systems

We analyse resonant excitations of ferromagnetic magnons via microwave pumping using Floquet theory. Special focus is put on driving frequencies that are below the corresponding magnon energy, which can be excited in large parameter regions via parametric resonances. We develop a theoretical framework that analytically predicts the regions of resonances and resonance thresholds in thin films of ferro- and ferri-magnetic materials like YIG as a function of damping, amplitude and frequency. Resonance regions are separated by exceptional points of the quasi-energies and the results are compared with micromagnetic simulations. The corresponding threshold amplitudes can be estimated from a characteristic powerlaw with damping, leading to the possibility of targeted exciatations at selected wavenumbers using low frequency drive.

cond-mat.mes-hall

Microscaled Tunable Magnonic RF Phase Shifters

Tunable, microscopic, and energy-efficient solutions for radio-frequency (RF) signal manipulation in the GHz regime are a key technology for efficient communication and sensing applications. Spin waves offer micrometer wavelengths at GHz frequencies, combined with strong magnetic-field tunability, making them inherently well-suited for tunable analog signal processing. Here, we demonstrate a novel concept: a micron-scale tunable RF phase shifter based on the wavelength shift of propagating spin waves. High energy efficiency is achieved by using the stray field of a micromagnet on a piezoelectrically actuated MEMS cantilever to locally induce this shift. The device shows a phase shift of more than 360{\deg} at a center frequency of 6.1 GHz using a phase-shifting area of less than 0.02mm$^2$. By changing the magnetic bias field, its functionality is experimentally confirmed over a range of center frequencies from 3 GHz to 8.2 GHz, and simulations show its applicability up to 14 GHz. A system-level characterization of an embedded device version demonstrates the qualification of magnonic phase shifters for highly integrated RF systems.

physics.app-ph

Integrated magnonic neural circuits based on nonlinear wave neurons

Artificial intelligence is driving intense interest in alternative computing hardware capable of neural information processing beyond conventional charge-based electronics. Among emerging approaches, wave-based computing promises highly parallel and energy-efficient operation, but scalable physical neural hardware has remained elusive because wave systems generally lack cascadable nonlinear neurons with signal regeneration and phase-robust operation. Here we demonstrate integrated magnonic neural circuits based on nonlinear threshold neurons realized in nanoscale yttrium iron garnet waveguides. The neurons perform weighted summation of multiple spin-wave inputs, while a pump-controlled nonlinear activation defines continuously tunable firing thresholds. Owing to deeply nonlinear spin-wave dynamics, the activated neurons emit self-normalized outputs whose intensities are largely independent of the input amplitudes, while nonlinear phase self-adjustment suppresses sensitivity to the relative input phases, enabling deterministic neuron-to-neuron cascading without external signal restoration. We experimentally realize programmable threshold neurons, reconfigurable weighted classification and deterministic cascading between sequential neuronal stages, and further demonstrate reconfigurable physical pattern recognition in a seven-neuron integrated magnonic circuit through experimental classification of the binary letter patterns 'HUST'. These results establish nonlinear magnons as a scalable platform for integrated neural hardware and position nonlinear wave dynamics as a general paradigm for physical neuromorphic computing.

cond-mat.mtrl-sci

Spin-polarization of the electric current in half-metallic Co$_2$MnSi Heusler thin films

Using propagating spin wave spectroscopy we measure the spin wave Doppler shift in patterned MgO/Co$_2$MnSi/MgO thin films and determine the degree of spin-polarization of the electric current. Our measurements reveal that the current is fully spin-polarized in the devices. This shows that the half-metallic character of the electron band structure translates into a fully spin polarized current flowing across the patterned films. Additionally, we measure a current-induced change of the spin-wave attenuation from which we estimate the non-adiabatic spin-transfer-torque parameter.

cond-mat.mtrl-sci

Spin-wave phase modulation using magnetic domain walls in dipolarly coupled structures for non-volatile magnonic computation

A controllable phase shifter is a key component for spin-wave-based logic and information processing devices. Here, we propose a domain-wall-position-controlled spin-wave phase shifter that exploits dipolar coupling between two closely spaced waveguides to enable continuous phase tuning over a range approaching 360degrees while keeping the spin-wave amplitude constant. Using micromagnetic simulations, we model a bias-free hybrid structure composed of a nanoscale waveguide magnetostatically coupled to a half-ring-shaped structure both made from bismuth-doped yttrium iron garnet with strong perpendicular magnetic anisotropy. Displacing a domain wall in the half-ring modulates the dispersion relation in the adjacent straight waveguide due to the changed magnetostatic interaction, providing a compact and dynamically reconfigurable phase-shifting mechanism. This approach offers precise and non-volatile control over spin-wave propagation and is compatible with energy-efficient magnonic logic architectures.

cond-mat.mes-hall

Epitaxial $\mathrm{Co_2MnSi}$ with intrinsic magnetocrystalline anisotropy as a route to bias-field-free nonlinear half-metal magnonics at the nanoscale

Half-metallic Heusler compounds like $\mathrm{Co_2MnSi}$ allow to bridge magnonic and spintronic functionality for hybrid unconventional computing approaches with sought-after properties like 100% spin polarization and associated low Gilbert damping $\alpha\leq 10^{-3}$. However, the desirable material parameters are inherently tied to the crystal lattice with a particularly critical dependence on structural order in $\mathrm{Co_2MnSi}$. To date, the successful fabrication of nanoscale devices with robust structural integrity remains yet a challenge, and consequently the impact of the material parameters on the resulting nonlinear spin-wave dynamics remains largely unexplored. Here, we report on a study of linear and nonlinear spin-wave dynamics in transversally magnetized $\mathrm{Co_2MnSi}$ waveguides with impeccable crystalline ordering. We show that epitaxial, $\mathrm{L2}_1$-ordered $\mathrm{Co_2MnSi}$ exhibits an intrinsic cubic anisotropy with first- and second-order contributions, stabilizing a magnetization alignment along the crystal $\langle110\rangle$ directions. We confirm the implication of an unaffected crystal structure resulting in preserved magnetic properties in the patterned structures. Herein, the persistent magnetocrystalline anisotropy reshapes the spin-wave dispersion which yields a first-order nonlinear instability suppression range extending over several GHz - even for vanishing bias fields. Moreover, the intrinsic magnetocrystalline anisotropy can be exploited to counteract shape demagnetization for a stabilized low bias field operation in the favourable Damon-Eshbach geometry with high group velocities and decay lengths. Together with the proven half-metallicity and ultralow Gilbert damping, this research establishes $\mathrm{Co_2MnSi}$ as a robust, scalable platform towards bias-field-free nonlinear half-metal magnonics.

cond-mat.mes-hall

Phase-dependent parametric amplification of propagating spin waves in YIG nanostructures enabled by local inhomogeneities

As magnonics evolves towards non-conventional computing, the development of phase-conserving and phase-sensitive amplification mechanisms becomes increasingly important. A particularly promising approach is non-adiabatic parametric amplification. In this work, the influence of local inhomogeneities on the parallel parametric amplification of spin waves in nano-scale Yttrium Iron Garnet waveguides is investigated. Micromagnetic simulations reveal that in larger pump regions, where only adiabatic amplification is expected, scattering centers provide additional linear momentum that enables non-adiabatic amplification of propagating spin waves. Importantly, the coherence of the process remains unaffected by the scattering and the generation of co-propagating spin waves enhance the effective amplification. Our simulations are confirmed by micro-focused Brillouin light scattering spectroscopy experiments, reproducing both the phase-dependent behavior and the characteristic features of the time-resolved dynamics. These findings demonstrate the flexibility of the parametric amplification process and provide a key mechanism for the development of large-scale spin-wave computing circuits.

cond-mat.other

Ultrafast formation of a large dynamic magnetic soliton

Nonlinear magnetization dynamics offers a rich variety of phenomena ranging from bistability to chaos. Here, we report the ultrafast formation of a dynamic magnetic soliton in thin ferrimagnetic garnet films with perpendicular magnetic anisotropy, driven by the microwave magnetic field of a microstrip antenna. Using time-resolved Brillouin light scattering microscopy and scanning transmission X-ray microscopy, we directly track the build-up of the large-angle precession state. The observed soliton is distinct from other nonlinear magnetic excitations in two key aspects: (i) it forms inside the linear spin-wave frequency band, and (ii) it is exceptionally large, reaching tens of microns beyond the antenna. We explain the soliton formation by the self-limiting mechanism upon a positive nonlinear frequency shift and the spatial extent of the near-field of the antenna. At large distances from the drive, the soliton collapses and emits short-wavelength spin waves via almost instantaneous spatial wavenumber conversion. Time-resolved measurements further reveal a small finite delay during soliton formation, while coherent long-range oscillations appear essentially simultaneously over distances up to 40 micrometers. These results establish microwave-driven solitons as a robust nonlinear phenomenon in thin-film garnets and suggest opportunities for fast, nonlocal manipulation of magnetic states and for applications in novel computational schemes.

cond-mat.mes-hall

Nonlinear frequency shift and bistability of magnon-polarons

We investigate the nonlinear dynamics of strongly coupled surface acoustic waves (SAWs) and spin waves (SWs) in a magnetoacoustic resonator based on a YIG/ZnO heterostructure by combining microwave reflection measurements with microfocused Brillouin light scattering spectroscopy. In the linear regime, the electrical response reveals clear hybridization between standing SAW cavity modes and finite-wave-vector SWs, resulting in pronounced avoided crossings. At elevated drive powers, the hybrid system exhibits a strongly field-dependent nonlinear response characterized by a positive frequency shift of the driven SW mode. Using the vector Hamiltonian formalism for nonlinear spin-wave dynamics, we show that this shift is dominated by a cross-shift term. In our resonator geometry, this contribution becomes significant because the standing SAW cavity mode simultaneously excites counterpropagating SWs with wave vectors $+k$ and $-k$. For suitable field detuning, the nonlinear shift drives the SW mode into resonance with the SAW excitation, leading to a strong enhancement of the magnon population, broadband nonlinear scattering, and bistable foldover behavior. Beyond the foldover threshold, both the magnon and phonon responses stabilize. These results establish SAW-driven $k \neq 0$ magnon-phonon hybrids as a promising platform for nonlinear magnetoacoustics and wave-based information processing.

cond-mat.mes-hall

True random number generation through stochastic magnonic bistability

True random number generators (TRNGs) underpin modern cryptography, yet existing implementations face fundamental trade-offs between speed, scalability, and entropy quality. Here, we demonstrate that stochastic switching in the bistable regime of spin-wave dynamics provides a physical entropy source for high-quality random number generation. Our magnonic random number generator (mRNG), based on a lithography-patterned microstrip on yttrium iron garnet (YIG), exploits thermal fluctuations near the nonlinear bistable regime to generate random bitstreams that pass all 15 NIST SP 800-22 statistical tests at rates with 20 Mb/s. We implement a random-bit multiplier using synchronized mRNG units and demonstrate scalability to 200-nm-wide nanoscale waveguides, establishing spin-wave bistability as a viable physical entropy source for integrated random number generation.

cond-mat.mtrl-sci

Characterizing the Linearity of Magnonic Devices for Radio-Frequency Applications

Magnonic devices exhibit strong amplitude-dependent nonlinearities, which are detrimental to signal integrity in radio-frequency (RF) signal processing applications. They also limit the power that such magnonic devices may process. In this paper we use micromagnetic simulations to characterize the nonlinearity of magnonic RF devices by investigating their intermodulation distortion (specifically third-order intermodulation products, IP$_3$ ). The IP$_3$ is a commonly used metric for RF components in communication systems and allows direct comparison with state-of-the-art electrical counterparts.

cond-mat.other

Integrated magnonic chip using cascaded logic

The transistor transformed not only electronics but everyday life, and the integrated circuit - now simply the "chip" - made computation scalable and ubiquitous. Magnonics has long promised a parallel path to low-energy information processing by using spin waves instead of charge. Progress, however, has been limited by two fundamental obstacles: intrinsic attenuation of spin waves and the requirement for precisely normalised output intensity and input phase to ensure reliable logic operation - conditions that are difficult to maintain in large-scale circuits owing to inevitable imperfections. Here, we report an integrated magnonic circuit that overcomes both limitations through engineered nonlinearity in nanoscale yttrium iron garnet waveguides. Nonlinear self-adjustment of the spin wave phase renders logic operation insensitive to the relative phases of the inputs, while a deeply nonlinear, threshold-activated self-normalised excitation restores and standardises the output intensity. Using space-resolved micro-focused Brillouin light scattering, we demonstrate reconfigurable AND, OR and three-input majority gates and realise deterministic cascading across sequential stages, establishing a scalable on-chip logic primitive. The architecture operates with gigahertz frequencies, supports dynamic threshold control for functional reconfiguration, and is compatible with scalable integration, making it attractive for adaptive and neuromorphic computing. By resolving phase-independent operation and signal restoration at the level of device physics, this work advances magnonics from isolated proof-of-concept devices towards integrated magnonic chips that can complement advanced CMOS in energy-constrained computing tasks.

cond-mat.mtrl-sci

Spin-wave emission with current-controlled frequency by a PMA-based spin-Hall oscillator

Spin-torque and spin-Hall oscillators (SHOs) have emerged as promising candidates for building blocks in neuromorphic computing due to their ability to synchronize mutually, a process that can be mediated by propagating spin waves. We demonstrate a SHO that takes advantage of a low-damping magnetic garnet with dominant perpendicular magnetic anisotropy (PMA), namely gallium-substituted yttrium-iron-garnet (Ga:YIG). In-plane magnetized Ga:YIG allows for the operation at a high efficiency level while also enabling resonant spin-wave emission. A nonlinear self-localization of the excitation is avoided by exploiting the positive nonlinear frequency shift, which facilitates a current-controlled frequency of the emitted spin waves. Via micro-focused Brillouin light scattering spectroscopy, we investigate the properties of the local auto-oscillation and its spin-wave emission. Multiple modes are excited and compete internally, with two propagating modes detected up to distances larger than 10 $\mu$m. Their frequencies combine to an extended frequency bandwidth of approximately 1.6 GHz. The experimentally observed two-mode system and its transition to a single mode at higher currents are reproduced via micromagnetic simulations, which account for spatial variation of the PMA arising due to the microstructures on Ga:YIG. Our results propose a promising platform for hosting SHOs, interconnected via propagating spin waves with particular relevance to neuromorphic computing.

cond-mat.mtrl-sci

Ultrafast propagation of magnon-polaritons

The manipulation of magnetization lies at the heart of spintronic and magnonic technologies, with the ultimate performance of such systems limited by the velocity at which magnetic excitations can propagate. Here, we demonstrate ultrafast propagation of magnon-polaritons-hybrid quasiparticles arising from the coupling between spin waves and electromagnetic fields in thin pure, bismuth-, and gallium substituted yttrium iron garnet (YIG, Bi:YIG and Ga:YIG) films. Using time- and phase-resolved Brillouin light scattering microscopy and time-resolved scanning transmission microscopy, we show that magnon-polaritons can propagate faster than 100 km/s, nearly three orders of magnitude more than conventional spin waves, and can be observed at distances exceeding 40 micrometers in 20 nm thick films. Analytical modeling based on retarded Maxwell equations and Polder tensor formalism confirms the hybridized nature of the excitations and captures the nontrivial dispersion and attenuation profiles. Notably, the magnon-polaritons maintain high initial magnetization amplitudes and long decay lengths, enabling ultrafast manipulation of the magnetization far away from the excitation source. We show, that they can move domain walls or stabilize nonlinear magnetization processes. The unprecedentedly high propagation velocities make magnon-polaritons promising candidates for high-speed information transfer in future spin-based computing architectures, potentially overcoming long-standing group delay bottlenecks in magnonic logic circuits.

physics.app-ph

Modelling spin-wave interference with electromagnetic leakage in micron-scaled spin-wave transducers

Utilization of spin-wave transducers for radio-frequency signal processing provides significant potential due to intrinsic tunability, scalability and nonlinearity. However, such components can exhibit passband ripples diminishing their operation and functionality. Here, we experimentally identify the electromagnetic crosstalk (EM) as a major source of passband ripples and provide a simple analytic model to predict the impact on device operation. The results are in good agreement with the experimental observation. In addition, we test multiple transducer geometries to identify operational regimes and minimize the EM impact. Finally, the effect of nonlinear device operation on the passband ripples is addressed, which is of relevance for the exploitation of the spin-waves intrinsic nonlinear traits.

physics.app-ph

An all-magnonic neuron with tunable fading memory

Magnonics offers nanometer-scale wave propagation and strong nonlinearities, making it attractive for neuromorphic applications such as artificial neurons. Yet, magnonic elements with interconnections solely within the magnonic system remain challenging, preventing the realization of interconnected magnonic neurons to date. Here, we experimentally demonstrate an all-magnonic neuron that reacts to magnon inputs with thresholded, amplified magnon firing and subsequent self-reset, enabling all-magnonic operation and cascading. Our approach is based on micro-antenna excitation on an ultra-low damping garnet with perpendicular magnetic anisotropy (PMA), where we exploit the positive magnon frequency shift to realize nonlinear activation. Using Brillouin light scattering spectroscopy, we uncover a transient neuron response with tunable fading memory: A 25% change in pump power results in a 3-order-of-magnitude tuning in memory time, which we harness, demonstrating temporal integration of up to 50 magnon pulses. Finally, we realize neuron triggering in a cascade of 3 neurons, highlighting its potential for connected magnonic circuits.

cond-mat.mtrl-sci

YSGAG: The Ideal Substrate for YIG in Quantum Magnonics

Quantum magnonics leverages the quantum properties of magnons to advance nanoscale quantum information technologies. Ferrimagnetic yttrium iron garnet (YIG), known for exceptionally long magnon lifetimes, is a cornerstone material typically grown as thin films on gadolinium gallium garnet (GGG) for lattice matching. However, paramagnetic GGG introduces detrimental damping at low temperatures due to substrate magnetization, undermining quantum applications. Here, we study magnetic damping in a 150$\,$nm-thick YIG film on a yttrium scandium gallium aluminum garnet (YSGAG) substrate, a newly developed diamagnetic alternative to GGG. Using ferromagnetic resonance spectroscopy down to 30$\,$mK, we compare YIG/YSGAG with a conventional YIG/GGG reference system. We demonstrate that the YIG/YSGAG system maintains low damping from 300$\,$K to 30$\,$mK, with $\alpha = 4.29\times10^{-5}$ at room temperature, comparable to the best YIG/GGG films and bulk YIG, with no low-temperature upturn. The diamagnetic substrate eliminates the dissipation mechanisms that dominate on magnetized GGG, preserving low magnetic damping across the full temperature range. Consequently, YSGAG serves as an ideal substrate for YIG films in quantum magnonics and is paving the way for the development of spin-wave-based quantum technologies.

cond-mat.mes-hall