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Philipp Pirro

Publications and source records attributed to Philipp Pirro.

At least 55 records · Page 3Linked to original sources

Nonlinear erasing of propagating spin-wave pulses in thin-film Ga:YIG

Nonlinear phenomena are key for magnon-based information processing, but the nonlinear interaction between two spin-wave signals requires their spatio-temporal overlap which can be challenging for directional processing devices. Our study focuses on a gallium-substituted yttrium iron garnet film, which exhibits an exchange-dominated dispersion relation and thus provides a particularly broad range of group velocities compared to pure YIG. Using time- and space-resolved Brillouin light scattering spectroscopy, we demonstrate the excitation of time-separated spin-wave pulses at different frequencies from the same source, where the delayed pulse catches up with the previously excited pulse and outruns it due to its higher group velocity. By varying the excitation power of the faster pulse, the outcome can be finely tuned from a linear superposition to a nonlinear interaction of both pulses, resulting in a full attenuation of the slower pulse. Therefore, our findings demonstrate the all-magnonic erasing process of a propagating magnonic signal, which enables the realization of complex temporal logic operations with potential application, e.g., in inhibitory neuromorphic functionalities.

cond-mat.mtrl-sci↗

Nanoscaled magnon transistor based on stimulated three-magnon splitting

Magnonics is a rapidly growing field, attracting much attention for its potential applications in data transport and processing. Many individual magnonic devices have been proposed and realized in laboratories. However, an integrated magnonic circuit with several separate magnonic elements has yet not been reported due to the lack of a magnonic amplifier to compensate for transport and processing losses. The magnon transistor reported in [Nat. Commun. 5, 4700, (2014)] could only achieve a gain of 1.8, which is insufficient in many practical cases. Here, we use the stimulated three-magnon splitting phenomenon to numerically propose a concept of magnon transistor in which the energy of the gate magnons at 14.6 GHz is directly pumped into the energy of the source magnons at 4.2 GHz, thus achieving the gain of 9. The structure is based on the 100 nm wide YIG nano-waveguides, a directional coupler is used to mix the source and gate magnons, and a dual-band magnonic crystal is used to filter out the gate and idler magnons at 10.4 GHz frequency. The magnon transistor preserves the phase of the signal and the design allows integration into a magnon circuit.

cond-mat.mes-hall↗

Coherent phonon-magnon interactions detected by micro-focused Brillouin light scattering spectroscopy

We investigated the interaction of surface acoustic waves and spin waves with spatial resolution by micro-focused Brillouin light scattering spectroscopy in a Co$_{40}$Fe$_{40}$B$_{20}$ ferromagnetic layer on a LiNbO$_{3}$-piezoelectric substrate. We experimentally demonstrate that the magnetoelastic excitation of magnons by phonons is coherent by studying the interfering BLS-signals of the phonons and magnons during their conversion process.We find a pronounced spatial dependence of the phonon annihilation and magnon excitation which we map as a function of the magnetic field. The coupling efficiency of the surface acoustic waves (SAWs) and the spin waves (SWs) is characterized by a magnetic field dependent decay of the SAWs amplitude.

physics.app-ph↗

Perspective on Nanoscaled Magnonic Networks

With the rapid development of artificial intelligence in recent years, mankind is facing an unprecedented demand for data processing. Today, almost all data processing is performed using electrons in conventional complementary metal-oxide-semiconductor (CMOS) circuits. Over the past few decades, scientists have been searching for faster and more efficient ways to process data. Now, magnons, the quanta of spin waves, show the potential for higher efficiency and lower energy consumption in solving some specific problems. While magnonics remains predominantly in the realm of academia, significant efforts are being made to explore the scientific and technological challenges of the field. Numerous proof-of-concept prototypes have already been successfully developed and tested in laboratories. In this article, we review the developed magnonic devices and discuss the current challenges in realizing magnonic circuits based on these building blocks. We look at the application of spin waves in neuromorphic networks, stochastic and reservoir computing and discuss the advantages over conventional electronics in these areas. We then introduce a new powerful tool, inverse design magnonics, which has the potential to revolutionize the field by enabling the precise design and optimization of magnonic devices in a short time. Finally, we provide a theoretical prediction of energy consumption and propose benchmarks for universal magnonic circuits.

physics.app-ph↗

Stimulated amplification of propagating spin waves

Spin-wave amplification techniques are key to the realization of magnon-based computing concepts. We introduce a novel mechanism to amplify spin waves in magnonic nanostructures. Using the technique of rapid cooling, we create a non-equilibrium state in excess of high-energy magnons and demonstrate the stimulated amplification of an externally seeded, propagating spin wave. Using an extended kinetic model, we qualitatively show that the amplification is mediated by an effective energy flux of high energy magnons into the low energy propagating mode, driven by a non-equilibrium magnon distribution.

cond-mat.mtrl-sci↗

Enhanced thermally-activated skyrmion diffusion with tunable effective gyrotropic force

Magnetic skyrmions, topologically-stabilized spin textures that emerge in magnetic systems, have garnered considerable interest due to a variety of electromagnetic responses that are governed by the topology. The topology that creates a microscopic gyrotropic force also causes detrimental effects, such as the skyrmion Hall effect, which is a well-studied phenomenon highlighting the influence of topology on the deterministic dynamics and drift motion. Furthermore, the gyrotropic force is anticipated to have a substantial impact on stochastic diffusive motion; however, the predicted repercussions have yet to be demonstrated, even qualitatively. Here we demonstrate enhanced thermally-activated diffusive motion of skyrmions in a specifically designed synthetic antiferromagnet. Suppressing the effective gyrotropic force by tuning the angular momentum compensation leads to a more than 10 times enhanced diffusion coefficient compared to that of ferromagnetic skyrmions. Consequently, our findings not only demonstrate the gyro-force dependence of the diffusion coefficient but also enable ultimately energy-efficient unconventional stochastic computing.

cond-mat.mtrl-sci↗

Coherent and incoherent magnons induced by strong ultrafast demagnetization in thin permalloy films

Understanding spin dynamics on femto- and picosecond timescales offers new opportunities for faster and more efficient spintronic devices. Here, we experimentally investigate the coherent spin dynamics after ultrashort laser excitation by time-resolved magneto optical Kerr effect (TR-MOKE) in thin Ni80Fe20 films. We provide a detailed study of the magnetic field and pump fluence dependence of the coherent precessional dynamics. We show that the coherent precession lifetime increases with the applied external magnetic field which cannot be understood by viscous Gilbert damping of the coherent magnons. Instead, it can be explained by nonlinear magnon interactions and by the change in the fraction of incoherent magnons. This interpretation is in agreement with the observed trends of the coherent magnon amplitude and lifetime as a function of the exciting laser fluence. Our results provide a new insight into the magnetization relaxation processes in ferromagnetic thin films, which is of great importance for further spintronic applications.

cond-mat.mes-hall↗

Investigation of Spin-Wave Dynamics in Gyroid Nanostructures

A new concept in magnonics studies the dynamics of spin waves (SWs) in three-dimensional nanosystems. It is a natural evolution from conventionally used planar systems to explore magnetization configurations and dynamics in 3D nanostructures with lengths near intrinsic magnetic scales. In this work, we perform broadband ferromagnetic resonance (BBFMR) measurements and micromagnetic simulations of nanoscale magnetic gyroids - a periodic chiral structure consisting entirely of chiral triple junctions. Our results show unique properties of the network, such as the localization of the SW modes, evoking their topological properties, and the substantial sensitivity to the direction of the static magnetic field. The presented results open a wide range of applications in the emerging field of 3D magnonic crystals and spintronics.

cond-mat.mes-hall↗

Symmetry and nonlinearity of spin wave resonance excited by focused surface acoustic waves

The use of a complex ferromagnetic system to manipulate GHz surface acoustic waves is a rich current topic under investigation, but the high-power nonlinear regime is under-explored. We introduce focused surface acoustic waves, which provide a way to access this regime with modest equipment. Symmetry of the magneto-acoustic interaction can be tuned by interdigitated transducer design which can introduce additional strain components. Here, we compare the impact of focused acoustic waves versus standard unidirectional acoustic waves in significantly enhancing the magnon-phonon coupling behavior. Analytical simulation results based on modified Landau-Lifshitz-Gilbert theory show good agreement with experimental findings. We also report nonlinear input power dependence of the transmission through the device. This experimental observation is supported by the micromagnetic simulation using mumax3 to model the nonlinear dependence. These results pave the way for extending the understanding and design of acoustic wave devices for exploration of acoustically driven spin wave resonance physics.

cond-mat.mtrl-sci↗

Competing signatures of intersite and interlayer spin transfer in the ultrafast magnetization dynamics

Optically driven intersite and interlayer spin transfer are individually known as the fastest processes for manipulating the spin order of magnetic materials on the sub 100 fs time scale. However, their competing influence on the ultrafast magnetization dynamics remains unexplored. In our work, we show that optically induced intersite spin transfer (also known as OISTR) dominates the ultrafast magnetization dynamics of ferromagnetic alloys such as Permalloy (Ni80Fe20) only in the absence of interlayer spin transfer into a substrate. Once interlayer spin transfer is possible, the influence of OISTR is significantly reduced and interlayer spin transfer dominates the ultrafast magnetization dynamics. This provides a new approach to control the magnetization dynamics of alloys on extremely short time scales by fine-tuning the interlayer spin transfer.

cond-mat.mtrl-sci↗

Coherent magnetization dynamics in strongly quenched Ni thin films

The remagnetization process after ultrafast demagnetization can be described by relaxation mechanisms between the spin, electron, and lattice reservoirs. Thereby, collective spin excitations in form of spin waves and their angular momentum transfer play an important role on the longer timescales. In this work, we address the question whether the strength of demagnetization affects the coherency and the phase of the excited spin waves. We present a study of coherent magnetization dynamics in thin nickel films after ultrafast demagnetization using the all-optical, time-resolved magneto-optical Kerr-effect (tr-MOKE) technique. The largest coherent oscillation amplitude was observed for strongly quenched systems, showing the conservation of coherency for demagnetizations of up to 90%. Moreover, the phase of the excited spin-waves increases with pump power, indicating a delayed start of the precession during the remagnetization.

cond-mat.mtrl-sci↗

Coupling of ferromagnetic and antiferromagnetic spin dynamics in Mn$_{2}$Au/NiFe thin-film bilayers

We investigate magnetization dynamics of Mn$_{2}$Au/Py (Ni$_{80}$Fe$_{20}$) thin film bilayers using broadband ferromagnetic resonance (FMR) and Brillouin light scattering spectroscopy. Our bilayers exhibit two resonant modes with zero-field frequencies up to almost 40 GHz, far above the single-layer Py FMR. Our model calculations attribute these modes to the coupling of the Py FMR and the two antiferromagnetic resonance (AFMR) modes of Mn2Au. The coupling-strength is in the order of 1.6 T$\cdot$nm at room temperature for nm-thick Py. Our model reveals the dependence of the hybrid modes on the AFMR frequencies and interfacial coupling as well as the evanescent character of the spin waves that extend across the Mn$_{2}$Au/Py interface

cond-mat.mtrl-sci↗

Quantifying symmetric exchange in ultrathin ferromagnetic films with chirality

The symmetric (Heisenberg) exchange interaction is fundamental to magnetism and assumes critical importance in designing magnetic materials for novel emergent phenomena and device applications. However, quantifying exchange is extremely challenging for ultrathin ($\sim$ 1 nm) magnetic films, as techniques and approximations reliably used for bulk materials are largely inapplicable in the two-dimensional (2D) limit. Here we present and contrast the measurement of exchange stiffness, $A$, by several methods on a series of five Co/Pt-based ultrathin ($1-2$ nm) films. We compare results from (a) spin-wave spectroscopy by Brillouin light scattering (BLS), (b) three analytical models describing the temperature dependence of magnetization obtained by magnetometry, (c) microscopic domain periodicity measurements and simulations, and (d) ab initio density functional theory (DFT) calculations. While different methods present some qualitatively consistent trends across samples, we note, for any given sample, considerable differences (up to $5\times$) in the absolute values of $A$ across the techniques, consistent with discrepancies of $A$ reported in literature for nominally similar samples. We analyze possible sources of the discrepancies across various methods, notably including their relationship to the spin-wave dispersion, and the wave-vector ranges probed. We compare the strengths and limitations of the techniques, and outline directions for their future use in characterizing exchange interactions in ultrathin films.

cond-mat.mtrl-sci↗

Parametric Excitation and Instabilities of Spin Waves driven by Surface Acoustic Waves

The parametric excitation of spin waves by coherent surface acoustic waves is demonstrated experimentally in metallic magnetic thin film structures. The involved magnon modes are analyzed with micro-focused Brillouin light scattering spectroscopy and complementary micromagnetic simulations combined with analytical modelling are used to determine the origin of the spin-wave instabilities. Depending on the experimental conditions, we observe spin-wave instabilities originating from different phonon-magnon and magnon-magnon scattering processes. Our results demonstrate that an efficient excitation of high amplitude, strongly nonlinear magnons in metallic ferromagnets is possible by surface acoustic waves, which opens novel ways to create micro-scaled nonlinear magnonic systems for logic and data processing that can profit from the high excitation efficiency of phonons using piezoelectricity.

cond-mat.other↗

Deeply nonlinear excitation of self-normalised exchange spin waves

Spin waves are ideal candidates for wave-based computing, but the construction of magnetic circuits is blocked by a lack of an efficient mechanism to excite long-running exchange spin waves with normalised amplitudes. Here, we solve the challenge by exploiting the deeply nonlinear phenomena of forward-volume spin waves in 200 nm wide nanoscale waveguides and validate our concept with microfocused Brillouin light scattering spectroscopy. An unprecedented nonlinear frequency shift of >2 GHz is achieved, corresponding to a magnetisation precession angle of 55° and enabling the excitation of exchange spin waves with a wavelength of down to ten nanometres with an efficiency of >80%. The amplitude of the excited spin waves is constant and independent of the input microwave power due to the self-locking nonlinear shift, enabling robust adjustment of the spin wave amplitudes in future on-chip magnonic integrated circuits.

physics.app-ph↗

Parametric generation of spin waves in nano-scaled magnonic conduits

The research feld of magnonics proposes a low-energy wave-logic computation technology based on spin waves to complement the established CMOS technology and provide a basis for emerging unconventional computation architectures. However, magnetic damping is a limiting factor for all-magnonic logic circuits and multi-device networks, ultimately rendering mechanisms to effciently manipulate and amplify spin waves a necessity. In this regard, parallel pumping is a versatile tool since it allows to selectively generate and amplify spin waves. While extensively studied in microscopic systems, nano-scaled systems are lacking investigation to assess the feasibility and potential future use of parallel pumping in magnonics. Here, we investigate a longitudinally magnetized 100 nm-wide magnonic nano-conduit using space and time-resolved micro-focused Brillouin-light-scattering spectroscopy. Employing parallel pumping to generate spin waves, we observe that the non-resonant excitation of dipolar spin waves is favored over the resonant excitation of short wavelength exchange spin waves. In addition, we utilize this technique to access the effective spin-wave relaxation time of an individual nano-conduit, observing a large relaxation time up to (115.0 +- 7.6) ns. Despite the significant decrease of the pumping effciency in the investigated nano-conduit, a reasonably small threshold is found rendering parallel pumping feasible on the nano-scale.

cond-mat.mes-hall↗

Fully Resonant Magneto-elastic Spin-wave Excitation by Surface Acoustic Waves under Conservation of Energy and Linear Momentum

We report on the resonant excitation of spin waves in micro-structured magnetic thin films by surface acoustic waves (SAWs). The spin waves as well as the acoustic waves are studied by micro-focused Brillouin light scattering spectroscopy. Besides the excitation of the ferromagnetic resonance, a process which does not fulfill momentum conservation, also the excitation of finite-wavelength spin waves can be observed at low magnetic fields. Using micromagnetic simulations, we verify that during this excitation both energy and linear momentum are conserved and fully transferred from the SAW to the spin wave.

cond-mat.other↗

Higgs and Goldstone spin-wave modes in striped magnetic texture

Spontaneous symmetry breaking is ubiquitous in physics. Its spectroscopic signature consists in the softening of a specific mode upon approaching the transition from the high symmetry side and its subsequent splitting into a zero-frequency "Goldstone" mode and a non-zero-frequency "Higgs" mode. Although they determine the whole system dynamics, these features are difficult to address in practice because of their vanishing coupling to most experimental probes and/or their strong interaction with other fluctuations. In this work, we consider a periodic magnetic modulation occurring in a ferromagnetic film with perpendicular-to-plane magnetic anisotropy and directly observe its Goldstone and Higgs spin-wave modes at room temperature using microwave and optical techniques. This simple system constitutes a particularly convenient platform for further exploring the dynamics of symmetry breaking.

cond-mat.mes-hall↗