arXiv subjects

Philipp Stammer

Publications and source records attributed to Philipp Stammer.

At least 19 recordsLinked to original sources

arXiv2026

Geometric Control of Cat States in High Harmonic Generation

High-harmonic generation (HHG) provides a powerful platform for exploring the interaction between intense laser fields and matter on ultrafast timescales. Beyond its conventional description in terms of emitted radiation and electron dynamics, a fully quantum treatment of HHG reveals that the nonlinear light-matter interaction can modify the quantum state of the driving field itself, establishing correlations between the fundamental and harmonic modes. This perspective opens new possibilities for using HHG as a tool to engineer and control nonclassical states of light. In this work, we investigate the geometric properties of optical Schroedinger cat states generated in HHG via conditioning and post-selection. By analyzing the coherent-state displacements induced by different structured driving fields, we characterize the resulting phase-space evolution and the associated geometric phases of the generated quantum states. Particular emphasis is placed on how the polarization and spatial-mode structure of the driving light influence the geometry and evolution of displaced coherent states. Our results demonstrate that structured light offers a versatile means of controlling the geometric dynamics of HHG-generated cat states across the parameter space. Furthermore, we discuss the prospects for realizing genuinely topological optical cat states by exploiting more complex structured light configurations.

physics.optics↗

arXiv2026

Two-Electron Effects Extend High-Harmonic Generation into the keV Regime

Two-electron processes can generate high harmonics beyond the conventional single-active-electron cutoff. Motivated by recent experimental evidence of an extended secondary plateau in the helium high-harmonic spectrum [S. Wang et al, Optica, (2023); S. Wang et al, In Print in Nature Photon., (2026)], we present a two-electron generalisation of the strong-field approximation. We analyse the resulting expressions using the saddle-point method and determine the extended cutoff. We find good agreement with classical predictions of cutoff scalings of $4.7$ and $5.5$ times the ponderomotive energy, which significantly exceed the established single-electron scaling of 3.17. We calculate high-harmonic spectra generated via a two-electron process in helium atoms driven by an intense few-cycle infrared laser pulse. Our results demonstrate that the harmonic spectrum extends far beyond the water window, reaching photon energies up to $\approx 1.2\,\mathrm{keV}$ in the soft x-ray region. The large spectral bandwidth can support the generation of sub-attosecond soft x-ray pulses, which are of particular interest for probing ultrafast dynamics across matter, including applications in core-level spectroscopy and biological imaging.

physics.atom-ph↗

arXiv2026

Photon anti-bunching in high harmonic generation

Photon anti-bunching is the direct evidence for the existence of photons without having a classical counterpart. Unlike bunching of photons, which can have a semi-classical description, the effect of photon anti-bunching can only be understood with quantized electromagnetic fields. However, for the process of high harmonic generation (HHG), where many photons of the driving field are upconverted to a single photon of higher energy, there is yet no clear evidence for the presence of individual photon emission. The key result of this work is the prediction of photon anti-bunching in the process of HHG, marking it the first theoretical discovery of non-classicality in the temporal correlations of HHG photons. While other non-classical signatures in HHG, such as sub-Poissonian statistics or squeezing, have been discussed for an ensemble of photons, the anti-bunching signature reported here is a signature of a single photon. This is achieved by using the recently developed Heisenberg picture approach for quantum optical HHG, revealing clear anti-bunching signatures in the intensity correlation function across the entire harmonic spectrum.

quant-ph↗

arXiv2026

Fluctuation-induced symmetry breaking in high harmonic generation for bicircular quantum light

Symmetries are ubiquitous in physics and play a pivotal role in light-matter interactions, where they determine the selection rules governing allowed atomic transitions and define the associated conserved quantities. For the up-conversion process of high harmonic generation, the symmetries of the driving field determine the allowed frequencies and the polarization properties of the resulting harmonics. As a consequence, it is possible to establish classical selection rules when the process is driven by coherent radiation. In this work, we show that fluctuation-induced symmetry breaking in the driving field leads to the appearance of otherwise forbidden harmonics. This is achieved by considering bicircular quantum light, and demonstrate that the enhanced quantum fluctuations due to squeezing in the driving field break the classical selection rules. To this end, we develop a quantum optical description of the dynamical symmetries in the process of high harmonic generation, revealing corrections to the classical selection rules. Moreover, we show that the new harmonics show squeezing-like signatures in their photon statistics, allowing them to be clearly distinguished from classical thermal fluctuations.

quant-ph↗

arXiv2026

Generation of circular polarized high-order harmonics from single color quantum light

The atomic response to an ultra-intense driving field produces a characteristic high-harmonic spectrum featuring a rapid drop in intensity for the lower harmonics, followed by a plateau and a sharp cutoff. This response vanishes for circularly polarized classical drivers -- a limitation that can be overcome by introducing quantum features into the driving field. In this work, we show that squeezed highly elliptically polarized drivers not only enable the high-harmonic generation (HHG) process in classically forbidden regimes of large ellipticity, but also yield highly elliptical harmonic radiation with pronounced super-Poissonian photon statistics. Moreover, we show that the HHG spectral features encode information about the quantum nature of the driving field, revealing the presence of its squeezed field fluctuations. By analyzing the HHG spectral intensity dependence as a function of the driver's ellipticity and squeezing orientation, we identify a means to probe the driving field's quantum properties that intrinsically lie in the high-photon number regime.

quant-ph↗

arXiv2025

Attosecond quantum optical interferometry

In this work, we explore the scheme of attosecond quantum interferometry (AQI), the quantum optical version of classical attosecond interferometry, which allows to measure quantum optical properties on the attosecond time-scale. We develop how the scheme of AQI can be used for engineering the phase-space and photon statistics properties of the emitted harmonics, using the relative phase of a two-color driving field as a control, and further enables to manipulate the field correlations as well as their entanglement characteristics. In addition, this scheme allows us to learn properties of the phase-space distribution of the harmonic quantum state, by means of measuring an attosecond quantum tomography trace. This serves as a new type of protocol for in situ attosecond measurements of quantum optical observables. With this, we achieve to further connect all-optical attosecond measurement schemes with quantum optics, allowing for a rich manifold of observations.

quant-ph↗

arXiv2025

Quantum Optics and Quantum Electrodynamics of Strong Field Processes

In its beginnings, the physics of intense laser-matter interactions was the physics of multiphoton processes. The theory was reduced then to high-order perturbation theory, while treating matter and light in a quantum manner. With the advent of chirped pulse amplification developed by D. Strickland and G. Mourou, which enabled generation of ultra-intense, ultra-short, coherent laser pulses, the need for a quantum electrodynamics description of electromagnetic (EM) fields practically ceased to exist and lost relevance. Contemporary attoscience (AS), and more generally ultrafast laser physics, awarded the Nobel Prize in 2023 to P. Agostini, F. Krausz, and A. L'Huillier, commonly uses the classical description of EM fields while keeping a fully quantum description of matter. The progress and successes of AS in the last 40 years have been spectacular, with an enormous amount of fascinating investigations in basic research and technology. Yet a central question remains: can ultrafast laser physics continue to advance without reintroducing quantum electrodynamics and quantum optics into its description of light-matter interactions? This article discusses future perspectives at the intersection of strong-field physics and quantum optics.

quant-ph↗

arXiv2025

High harmonic generation from a Bose-Einstein condensate

Lasers provide intense coherent radiation, essential to cool and trap atoms into a Bose-Einstein condensate or can alternatively drive the non-linear dynamics of high-order harmonic generation. Yet, these two fundamental processes remained of independent consideration. Here, we connect matter waves at ultracold temperatures with radiation bursts on the ultrafast attosecond timescale. We do this by exploring high harmonic generation from a Bose-Einstein condensate. We show that the quantum state of the generated harmonics of a driven Bose gas is a classical mixture, while below the critical temperature of Bose-Einstein condensation the emitted harmonic radiation is in a pure quantum state. These states furthermore exhibit squeezing and entanglement across all field modes.

quant-ph↗

arXiv2025

Propagation of intense squeezed vacuum light in non-linear media

Recent developments in quantum light engineering have enabled the use of infrared bright squeezed vacuum (BSV) femtosecond pulses in highly nonlinear optics, particularly strong field physics and high-harmonic generation. However, theoretical studies were focused on the microscopic interaction with a single atom, neglecting the crucial macroscopic aspect of light propagation through the media. This raises a key question: How does BSV propagates in strongly light-driven nonlinear media and how this affects the generation of non-linear optical signals? We address this question by introducing a fully quantized framework that accounts for the propagation in gas media. We find that atomic ionization caused by strong BSV fluctuations and the associated infrared photon losses introduce decoherence effects that can substantially limit the propagation length in the medium, reduce the harmonic yield, and decrease the number of emitted harmonics at high intensities. However, these effects are not detrimental. We identify conditions under which propagation-induced decoherence is minimized while the generated harmonics remain clearly detectable--an issue of particular importance for future studies exploring the connection between strong-field physics and quantum optics. Our results lay the foundation for future studies of BSV in strong-field physics, nonlinear optics, and ultrafast science, and establish a basis for exploring its propagation through all states of matter in a fully quantized framework.

quant-ph↗

arXiv2025

Weak measurement in strong laser field physics

The advantage of attosecond measurements is the possibility of time-resolving ultrafast quantum phenomena of electron dynamics. Many such measurements are of interferometric nature, and therefore give access to the phase. Likewise, weak measurements are intrinsically interferometric and specifically take advantage of interfering probability amplitudes, therefore encoding the phase information of the process. In this work, we show that attosecond interferometry experiments can be seen as a weak measurement, which unveils how this notion is connected to strong field physics and attosecond science. In particular, we show how the electron trajectory picks up a new phase, which occurs due to the weak measurement of the process. This phase can show significant contributions in the presence of spectral features of the measured system. Furthermore, extending this approach to include non-classical driving fields shows that the generated harmonics exhibit non-trivial features in their quantum state and photon statistics. This opens the path towards investigations of attosecond quantum interferometry experiments.

quant-ph↗

arXiv2025

Quantum stochastic analysis of non-linear driven light emission

This work extends quantum optical models of high harmonic generation by considering a quantum stochastic analysis of the field modes coupled to an environment. In particular, we study the open system dynamics by solving the quantum Langevin equation for a non-linear driven cavity coupled to the environment. For an unstructured environment without memory, we show that the emission characteristics of the intense driven cavity is isomorphic to the process of high harmonic generation and a non-linear antenna. This is achieved by using the quantum regression theorem for the Markovian dynamics, and further allows to obtain the upper bound of the radiated power due to the emitter fluctuations. This opens the path to connect current quantum optical approaches of HHG with open system descriptions and towards driven-dissipative systems in the non-linear regime.

quant-ph↗

arXiv2025

Quantum Kramers-Henneberger Transformation

The classical Kramers-Henneberger transformation connects, via a series of unitary transformations, the dynamics of a quantum particle of mass $m$ located in a trap at position $\alpha(t)$, with the dynamics of a charge $e$ moving in an electric field $eE(t)=-m\ddot{\alpha}(t)$ within the dipole approximation. In this paper, we extend the classical Kramers-Henneberger transformation to the quantum electrodynamic and quantum optical realm, by explicitly treating the trap location quantum mechanically, thus taking into account the quantum fluctuations of the time-dependent displacement force. Compared to the classical case, we show that quantum electrodynamic corrections appear, and we propose an optomechanical realization for the quantized position of the trap to show that such corrections can manifest in state-of-the-art experiments. These results open the path to novel quantum simulation of quantum electrodynamics and quantum optics of attoscience and ultrafast physics by using ultracold trapped atoms and ions.

quant-ph↗

arXiv2025

Theory of quantum optics and optical coherence in high harmonic generation

Optical coherence encodes information about the correlations of the electromagnetic field. In combination with quantum optical approaches, it allows for the study of the correlations between photons. Since the pioneering papers of Glauber, studies of optical coherence have facilitated many fundamental insights into non-classical signatures of light emission processes, with wide applicability in modern quantum technologies. However, when it comes to the photon up-conversion process of high-order harmonic generation the description has focused on semi-classical methods for decades. In this work, we overcome this limitation and establish a quantum optical theory of field correlations for the process of high harmonic generation (HHG). In effect, we introduce the notion of optical coherence at the intersection of quantum optics and strong laser-driven processes, and obtain the harmonic field correlation functions. In particular, we focus on the first and second order field correlation, which allow to understand the origin of the classical properties of the HHG spectrum, and its departure into the quantum regime. Further, we develop the theory for two-time intensity correlation functions of the harmonic field, and demonstrate the onset of anti-bunching signatures in HHG. We study the correlation functions in the regime of a single, few and many emitters in atomic HHG, showing the transition from quantum to classical signatures in the correlations. Since the theory is generic, it can be extended to multi-time correlation functions of any order, and allows to consider the interaction of light with arbitrary material systems.

quant-ph↗

arXiv2024

Information-theoretic perspective on energy conservation in high harmonic generation

The use of energy conservation arguments is ubiquitous in understanding the process of high harmonic generation, yet a complete quantum optical description of exact photon number exchange remained elusive. Here, we solve this gap in description by introducing the energy conserving subspace in high harmonic generation in which many photons of the driving field are absorbed to generate a single photon of higher energy. The presented solution to energy conservation in quantum optical high harmonic generation naturally results in highly entangled states of light with non-classical properties in their marginals and photon statistics. This new technique can be seen as an information-theoretic approach to the problem of photon exchange between field modes, providing a new kind of selection rule imposed on the quantum optical state by the structure of the Hilbert space. In addition to providing the quantum state satisfying exact energy conservation, it allows to explain recent experimental results for quantum state engineering of optical cat states.

quant-ph↗

arXiv2024

Quantum phenomena in attosecond science

Attosecond science has opened up new frontiers in our understanding of processes happening on the intrinsic timescale of electrons. The ability to manipulate and observe phenomena at the attosecond level has yielded groundbreaking insights into processes such as electron dynamics and the behavior of matter under extreme conditions. This interdisciplinary field bridges various research areas such as quantum optics, quantum chemistry and quantum information science facilitating a cohesive understanding. However, despite many emerging successful applications, the discussion about intrinsic quantum effects has mainly been ignored. In this Perspective, we explore the latest advancements in quantum phenomena within attosecond science, encompassing both experimental and theoretical progress. Specifically, in the context of high-harmonic generation and above-threshold ionization, we focus on discerning genuinely quantum observations and distinguishing them from classical phenomena. Additionally, we illuminate the often overlooked yet significant role of entanglement in attosecond processes, elucidating its influence on experimental outcomes.

quant-ph↗

arXiv2024

Analog simulation of high harmonic generation in atoms

The demanding experimental access to the ultrafast dynamics of materials challenges our understanding of their electronic response to applied strong laser fields. For this purpose, trapped ultracold atoms with highly controllable potentials have become an enabling tool to describe phenomena in a scenario where some effects are more easily accessible and twelve orders of magnitude slower. In this work, we introduce a mapping between the parameters of attoscience platform and atomic cloud simulators, and propose an experimental protocol to access the emission spectrum of high harmonic generation, a regime that has so far been elusive to cold atom simulation. As we illustrate, the benchmark offered by these simulators can provide new insights on the conversion efficiency of extended and short nuclear potentials, as well as the response to applied elliptical polarized fields or ultrashort few-cycle pulses.

physics.atom-ph↗

arXiv2024

Nonclassical states of light after high-harmonic generation in semiconductors: a Bloch-based perspective

High-harmonic generation has emerged as a pivotal process in strong-field physics, yielding extreme ultraviolet radiation and attosecond pulses with a wide range of applications. Furthermore, its emergent connection with the field of quantum optics has revealed its potential for generating non-classical states of light. Here, we investigate the process of high-harmonic generation in semiconductors under a quantum optical perspective while using a Bloch-based solid-state description. Through the implementation of quantum operations based on the measurement of high-order harmonics, we demonstrate the generation of non-classical light states similar to those found when driving atomic systems. These states are characterized using diverse quantum optical observables and quantum information measures, showing the influence of electron dynamics on their properties. Additionally, we analyze the dependence of their features on solid characteristics such as the dephasing time and crystal orientation, while also assessing their sensitivity to changes in driving field strength. This study provides insights into HHG in semiconductors and its potential for generating non-classical light sources.

quant-ph↗

arXiv2023

Metrological robustness of high photon number optical cat states

In the domain of quantum metrology, cat states have demonstrated their utility despite their inherent fragility with respect to losses. Here, we introduce noise robust optical cat states which exhibit a metrological robustness for phase estimation in the regime of high photon numbers. These cat states are obtained from the intense laser driven process of high harmonic generation (HHG), and show a resilience against photon losses. Focusing on a realistic scenario including experimental imperfections we opt for the case in which we can maximize the lower bound of the quantum Fisher information (QFI) instead of analyzing the best case scenario. We show that the decrease of the QFI in the lossy case is suppressed for the HHG-cat state compared to the even and odd counterparts. In the regime of small losses of just a single photon, the HHG-cat state remains almost pure while the even/odd cat state counterparts rapidly decohere to the maximally mixed state. More importantly, this translates to a significantly enhanced robustness for the HHG-cat against photon loss, demonstrating that high photon number optical cat states can indeed be used for metrological applications even in the presence of losses.

quant-ph↗