arXiv subjects

Philipp Treutlein

Publications and source records attributed to Philipp Treutlein.

At least 19 recordsLinked to original sources

arXiv2025

Multiparameter estimation with an array of entangled atomic sensors

In quantum metrology, entangled states of many-particle systems are investigated to enhance measurement precision of the most precise clocks and field sensors. While single-parameter quantum metrology is well established, many metrological tasks require joint multiparameter estimation, which poses new conceptual challenges that have so far only been explored theoretically. We experimentally demonstrate multiparameter quantum metrology with an array of entangled atomic ensembles. By splitting a spin-squeezed ensemble, we create an atomic sensor array featuring inter-sensor entanglement that can be flexibly configured to enhance measurement precision of multiple parameters jointly. Using an optimal estimation protocol, we achieve significant gains over the standard quantum limit in key multiparameter estimation tasks, thus grounding the concept of quantum enhancement of field sensor arrays and imaging devices.

quant-ph↗

arXiv2025

Squeezing light with optomechanical and spin-light quantum interfaces

We investigate squeezing of light through quantum-noise-limited interactions with two different material systems: an ultracold atomic spin ensemble and a micromechanical membrane. Both systems feature a light-matter quantum interface that we exploit, respectively, to generate polarization squeezing of light through Faraday interaction with the collective atomic spin precession, and ponderomotive quadrature squeezing of light through radiation pressure interaction with the membrane vibrations in an optical cavity. Both experiments are described in a common theoretical framework, highlighting the conceptual similarities between them. The observation of squeezing certifies light-matter coupling with large quantum cooperativity, a prerequisite for applications in quantum science and technology. In our experiments, we obtain a maximal cooperativity of $C_\mathrm{qu} =10$ for the spin and $C_\mathrm{qu} = 9$ for the membrane. In particular, our results pave the way for hybrid quantum systems where spin and mechanical degrees of freedom are coherently coupled via light, enabling new protocols for quantum state transfer and entanglement generation over macroscopic distances.

quant-ph↗

arXiv2024

Effective Faraday interaction between light and nuclear spins of Helium-3 in its ground state: a semiclassical study

We derive the semiclassical evolution equations for a system consisting of helium-3 atoms in the $2^3S$ metastable state interacting with a light field far-detuned from the $2^3S-2^3P$ transition, in the presence of metastability exchange collisions with ground state helium atoms and a static magnetic field. For two configurations, each corresponding to a particular choice of atom-light detuning in which the contribution of either the metastable level $F=1/2$ or $F=3/2$ is dominant, we derive a simple model of three coupled collective spins from which we can analytically extract an effective coupling constant between the collective nuclear spin and light. In these two configurations, we compare the predictions of our simplified model with the full model.

quant-ph↗

arXiv2024

Broad Instantaneous Bandwidth Microwave Spectrum Analyzer with a Microfabricated Atomic Vapor Cell

We report on broad instantaneous bandwidth microwave spectrum analysis with hot $^{87}\mathrm{Rb}$ atoms in a microfabricated vapor cell in a large magnetic field gradient. The sensor is a MEMS atomic vapor cell filled with isotopically pure $^{87}\mathrm{Rb}$ and $\mathrm{N}_2$ buffer gas to localize the motion of the atoms. The microwave signals of interest are coupled through a coplanar waveguide to the cell, inducing spin flip transitions between optically pumped ground states of the atoms. A static magnetic field with large gradient maps the $\textit{frequency spectrum}$ of the input microwave signals to a position-dependent $\textit{spin-flip pattern}$ on absorption images of the cell recorded with a laser beam onto a camera. In our proof-of-principle experiment, we demonstrate a microwave spectrum analyzer that has $\approx$ 1 GHz instantaneous bandwidth centered around 13 GHz, 3 MHz frequency resolution, 2 kHz refresh rate, and a -23 dBm single-tone microwave power detection limit in 1 s measurement time. A theoretical model is constructed to simulate the image signals by considering the processes of optical pumping, microwave interaction, diffusion of $^{87}\mathrm{Rb}$ atoms, and laser absorption. We expect to reach more than 25 GHz instantaneous bandwidth in an optimized setup, limited by the applied magnetic field gradient. Our demonstration offers a practical alternative to conventional microwave spectrum analyzers based on electronic heterodyne detection.

physics.atom-ph↗

arXiv2023

Electromagnetically Induced Transparency and Optical Pumping in the Hyperfine Paschen-Back Regime

We report spectroscopy experiments of rubidium vapor in a high magnetic field under conditions of electromagnetically induced transparency (EIT) and optical pumping. The 1.1 T static magnetic field decouples nuclear and electronic spins and shifts each magnetic state via the Zeeman effect, allowing us to resolve individual optical transitions of the D$_2$ line in a Doppler-broadened medium. By varying the control laser power driving one leg of a spectrally isolated $\Lambda$ system we tune the vapor from the EIT regime to conditions of Autler-Townes line splitting. The resulting spectra conform to simple three-level models demonstrating the effective simplification of the energetic structure. Further, we quantify the viability of state preparation via optical pumping on nuclear spin-forbidden transitions. We conclude that the ``cleanliness'' of this system greatly enhances the capabilities of quantum control in hot vapor, offering advantages in a broad variety of quantum applications plagued by spurious light-matter interaction processes, such as atomic quantum memories for light.

quant-ph↗

arXiv2023

Optical Memory in a Microfabricated Rubidium Vapor Cell

Scalability presents a central platform challenge for the components of current quantum network implementations that can be addressed by microfabrication techniques. We demonstrate a high-bandwidth optical memory using a warm alkali atom ensemble in a microfabricated vapor cell compatible with wafer-scale fabrication. By applying an external tesla-order magnetic field, we explore a novel ground-state quantum memory scheme in the hyperfine Paschen-Back regime, where individual optical transitions can be addressed in a Doppler-broadened medium. Working on the $^{87}$Rb D$_2$ line, where deterministic quantum dot single-photon sources are available, we demonstrate bandwidth-matching with hundreds of megahertz broad light pulses keeping such sources in mind. For a storage time of 80 ns we measure an end-to-end efficiency of $\eta_{e2e}^{\text{80ns}} = 3.12(17)\%$, corresponding to an internal efficiency of $\eta_{\text{int}}^{\text{0ns}} = 24(3)\%$, while achieving a signal-to-noise ratio of $\text{SNR} = 7.9(8)$ with coherent pulses at the single-photon level.

quant-ph↗

arXiv2022

Einstein-Podolsky-Rosen experiment with two Bose-Einstein condensates

In 1935, Einstein, Podolsky and Rosen (EPR) conceived a Gedankenexperiment which became a cornerstone of quantum technology and still challenges our understanding of reality and locality today. While the experiment has been realized with small quantum systems, a demonstration of the EPR paradox with spatially separated, massive many-particle systems has so far remained elusive. We observe the EPR paradox in an experiment with two spatially separated Bose-Einstein condensates containing about 700 Rubidium atoms each. EPR entanglement in conjunction with individual manipulation of the two condensates on the quantum level, as demonstrated here, constitutes an important resource for quantum metrology and information processing with many-particle systems. Our results show that the conflict between quantum mechanics and local realism does not disappear as the system size is increased to over a thousand massive particles.

quant-ph↗

arXiv2022

Optical coherent feedback control of a mechanical oscillator

Feedback is a powerful and ubiquitous technique both in classical and quantum system control. Its standard implementation relies on measuring the state of a system, processing the classical signal, and feeding it back to the system. In quantum physics, however, measurements not only read out the state of the system but also modify it irreversibly. Coherent feedback is a different kind of feedback that coherently processes and feeds back quantum signals without actually measuring the system. Here, we report on the experimental realization and the theoretical analysis of an optical coherent feedback platform to control the motional state of a nanomechanical membrane in an optical cavity. The coherent feedback loop consists of a light field interacting twice with the same mechanical mode through different cavity modes, without {performing any} measurement. Tuning the optical phase and delay of the feedback loop allows us to control the motional state of the mechanical oscillator, its resonance frequency and also its damping rate, which we use to cool the membrane close to the quantum ground state. Our theoretical analysis provides the optimal cooling conditions, showing that this new technique enables ground-state cooling. Experimentally, we show that we can cool the membrane to a state with $\bar{n}_m = 4.89 \pm 0.14 $ phonons (${480}\,{\mu \mathrm{K}}$) in a ${20}\,\mathrm{K}$ environment. This lies below the theoretical limit of cavity dynamical backaction cooling in the unresolved sideband regime and is achieved with only 1$\%$ of the optical power required for cavity cooling. Our feedback scheme is very versatile, offering new opportunities for quantum control in a variety of optomechanical systems.

quant-ph↗

arXiv2022

Single-Photon Storage in a Ground-State Vapor Cell Quantum Memory

Interfaced single-photon sources and quantum memories for photons together form a foundational component of quantum technology. Achieving compatibility between heterogeneous, state-of-the-art devices is a long-standing challenge. We built and successfully interfaced a heralded single-photon source based on cavity-enhanced spontaneous parametric down-conversion in ppKTP and a matched memory based on electromagnetically induced transparency in warm $^{87}$Rb vapor. The bandwidth of the photons emitted by the source is 370 MHz, placing its speed in the technologically relevant regime while remaining well within the acceptance bandwidth of the memory. Simultaneously, the experimental complexity is kept low, with all components operating at or above room temperature. Read-out noise of the memory is considerably reduced by exploiting polarization selection rules in the hyperfine structure of spin-polarized atoms. For the first time, we demonstrate single-photon storage and retrieval in a ground-state vapor cell memory, with $g_{c,\text{ret}}^{(2)}=0.177(23)$ demonstrating the single-photon character of the retrieved light. Our platform of single-photon source and atomic memory is attractive for future experiments on room-temperature quantum networks operating at high bandwidth.

quant-ph↗

arXiv2021

Coherent feedback cooling of a nanomechanical membrane with atomic spins

Coherent feedback stabilises a system towards a target state without the need of a measurement, thus avoiding the quantum backaction inherent to measurements. Here, we employ optical coherent feedback to remotely cool a nanomechanical membrane using atomic spins as a controller. Direct manipulation of the atoms allows us to tune from strong-coupling to an overdamped regime. Making use of the full coherent control offered by our system, we perform spin-membrane state swaps combined with stroboscopic spin pumping to cool the membrane in a room-temperature environment to ${T}={216}\,\mathrm{mK}$ ($\bar{n}_{m} = 2.3\times 10^3$ phonons) in ${200}\,\mathrm{{\mu}s}$. We furthermore observe and study the effects of delayed feedback on the cooling performance. Starting from a cryogenically pre-cooled membrane, this method would enable cooling of the mechanical oscillator close to its quantum mechanical ground state and the preparation of nonclassical states.

quant-ph↗

arXiv2020

Nuclear spin squeezing by continuous quantum non-demolition measurement: a theoretical study

We propose to take advantage of the weak coupling of ground-state helium-3 nuclear spin to its environment to produce long-lived macroscopic quantum states, nuclear spin squeezed states, in a gas cell at room temperature. To perform a quantum non-demolition measurement of a transverse component of the polarized collective nuclear spin, we maintain a population in helium-3 metastable state with a discharge. The collective spin associated to $F=1/2$ metastable level hybridizes with the ground state one by metastability exchange collisions. To access nuclear spin fluctuations, one continuously measures the light leaking out of an optical cavity, where it has interacted dispersively with the metastable state collective spin. In a three coupled collective spin model (nuclear, metastable and Stokes), we calculate moments of the nuclear spin squeezed component $I_z$ conditioned on the time averaged optical signal. In the photon counting scheme, the squeezed observable is $I_z^2$ rather than $I_z$. In the homodyne detection scheme, we solve the stochastic equation for the system state conditioned on the measurement; the conditional expectation value of $I_z$ depends linearly on the signal and the conditional variance of $I_z$ does not depend on it. The conditional variance decreases as $(\Gamma_{\rm sq}t)^{-1}$, where the squeezing rate $\Gamma_{\rm sq}$ depends linearly on the light intensity in the cavity at weak atom-field coupling and saturates at strong coupling to the ground state metastability exchange effective rate, proportional to the metastable atom density. Including de-excitation of metastable atoms at the walls, which induces nuclear spin decoherence with an effective rate $\gamma_\alpha$, we find a limit $\propto(\gamma_\alpha/\Gamma_{\rm sq})^{1/2}$ on the conditional variance reached in a time $\propto(\gamma_\alpha\Gamma_{\rm sq})^{-1/2}$.

physics.atom-ph↗

arXiv2020

Nuclear spin squeezing in Helium-3 by continuous quantum nondemolition measurement

We propose a technique to control the macroscopic collective nuclear spin of a Helium-3 vapor in the quantum regime using light. The scheme relies on metastability exchange collisions to mediate interactions between optically accessible metastable states and the ground-state nuclear spin, giving rise to an effective nuclear spin-light quantum nondemolition interaction of the Faraday form. Our technique enables measurement-based quantum control of nuclear spins, such as the preparation of spin-squeezed states. This, combined with the day-long coherence time of nuclear spin states in Helium-3, opens the possibility for a number of applications in quantum technology.

quant-ph↗

arXiv2020

Large-Range Frequency Tuning of a Narrow-Linewidth Quantum Emitter

A hybrid system of a semiconductor quantum dot single photon source and a rubidium quantum memory represents a promising architecture for future photonic quantum repeaters. One of the key challenges lies in matching the emission frequency of quantum dots with the transition frequency of rubidium atoms while preserving the relevant emission properties. Here, we demonstrate the bidirectional frequency-tuning of the emission from a narrow-linewidth (close-to-transform-limited) quantum dot. The frequency tuning is based on a piezoelectric strain-amplification device, which can apply significant stress to thick bulk samples. The induced strain shifts the emission frequency of the quantum dot over a total range of $1.15\ \text{THz}$, about three orders of magnitude larger than its linewidth. Throughout the whole tuning process, both the spectral properties of the quantum dot and its single-photon emission characteristics are preserved. Our results show that external stress can be used as a promising tool for reversible frequency tuning of high-quality quantum dots and pave the wave towards the realisation of a quantum dot -- rubidium atoms interface for quantum networking.

cond-mat.mes-hall↗

arXiv2020

Light-mediated strong coupling between a mechanical oscillator and atomic spins one meter apart

Engineering strong interactions between quantum systems is essential for many phenomena of quantum physics and technology. Typically, strong coupling relies on short-range forces or on placing the systems in high-quality electromagnetic resonators, restricting the range of the coupling to small distances. We use a free-space laser beam to strongly couple a collective atomic spin and a micromechanical membrane over a distance of one meter in a room-temperature environment. The coupling is highly tunable and allows the observation of normal-mode splitting, coherent energy exchange oscillations, two-mode thermal noise squeezing and dissipative coupling. Our approach to engineer coherent long-distance interactions with light makes it possible to couple very different systems in a modular way, opening up a range of opportunities for quantum control and coherent feedback networks.

quant-ph↗

arXiv2020

Fundamental limit of phase coherence in two-component Bose-Einstein condensates

We experimentally and theoretically study phase coherence in two-component Bose-Einstein condensates of $^{87}{\rm Rb}$ atoms on an atom chip. Using Ramsey interferometry we measure the temporal decay of coherence between the $|F=1,m_{F}=-1\rangle$ and $|F=2,m_{F}=+1\rangle$ hyperfine ground states. We observe that the coherence is limited by random collisional phase shifts due to the stochastic nature of atom loss. The mechanism is confirmed quantitatively by a quantum trajectory method based on a master equation which takes into account collisional interactions, atom number fluctuations, and losses in the system. This decoherence process can be slowed down by reducing the density of the condensate. Our findings are relevant for experiments on quantum metrology and many-particle entanglement with Bose-Einstein condensates and the development of chip-based atomic clocks.

physics.atom-ph↗

arXiv2019

Entanglement between identical particles is a useful and consistent resource

The existence of fundamentally identical particles represents a foundational distinction between classical and quantum mechanics. Due to their exchange symmetry, identical particles can appear to be entangled -- another uniquely quantum phenomenon with far-reaching practical implications. However, a long-standing debate has questioned whether identical particle entanglement is physical or merely a mathematical artefact. In this work, we provide such particle entanglement with a consistent theoretical description as a quantum resource in processes frequently encountered in optical and cold atomic systems. This leads to a plethora of applications of immediate practical impact. On one hand, we show that the metrological advantage for estimating phase shifts in systems of identical bosons amounts to a measure of their particle entanglement, with a clearcut operational meaning. On the other hand, we demonstrate in general terms that particle entanglement is the property resulting in directly usable mode entanglement when distributed to separated parties, with particle conservation laws in play. Application of our tools to an experimental implementation with Bose-Einstein condensates leads to the first quantitative estimation of identical particle entanglement. Further connections are revealed between particle entanglement and other resources such as optical nonclassicality and quantum coherence. Overall, this work marks a resolutive step in the ongoing debate by delivering a unifying conceptual and practical understanding of entanglement between identical particles.

quant-ph↗

arXiv2019

An efficient, tunable, and robust source of narrow-band photon pairs at the $^{87}$Rb D1 line

We present an efficient and robust source of photons at the $^{87}$Rb D1-line (795 nm) with a narrow bandwidth of $\delta=226(1)$ MHz. The source is based on non-degenerate, cavity-enhanced spontaneous parametric down-conversion in a monolithic optical parametric oscillator far below threshold. The setup allows for efficient coupling to single mode fibers. A heralding efficiency of $\eta_{\mathrm{heralded}}=45(5)$ % is achieved, and the uncorrected number of detected photon pairs is $3.8 \times 10^{3}/(\textrm{s mW})$. For pair generation rates up to $5\times 10^{5}/$s, the source emits heralded single photons with a normalized, heralded, second-order correlation function $g^{(2)}_{c}<0.01$. The source is intrinsically stable due to the monolithic configuration. Frequency drifts are on the order of $\delta/20$ per hour without active feedback on the emission frequency. We achieved fine-tuning of the source frequency within a range of $ > 2$ GHz by applying mechanical strain.

quant-ph↗

arXiv2019

Remote Hamiltonian Interactions Mediated by Light

We address a fundamental question of quantum optics: Can a beam of light mediate coherent Hamiltonian interactions between two distant quantum systems? This is an intriguing question whose answer is not a priori clear, since the light carries away information about the systems and might be subject to losses, giving rise to intrinsic decoherence channels associated with the coupling. Our answer is affirmative and we derive a particularly simple sufficient condition for the interactions to be Hamiltonian: The light field needs to interact twice with the systems and the second interaction has to be the time reversal of the first. We demonstrate that, even in the presence of significant optical loss, coherent interactions can be realized and generate substantial amounts of entanglement between the systems. Our method is directly applicable for building hybrid quantum systems, with relevant applications in the fields of optomechanics and atomic ensembles.

quant-ph↗