arXiv subjects

Philippa M. Shepley

Publications and source records attributed to Philippa M. Shepley.

5 recordsLinked to original sources

arXiv2023

Temperature dependence of magnetic anisotropy and domain wall tuning in BaTiO3(111)/CoFeB multiferroics

Artificial multiferroics consist of two types of ferroic materials, typically a ferroelectric and ferromagnet, often coupled interfacially by magnetostriction induced by the lattice elongations in the ferroelectric. In BaTiO3 the magnitude of strain induced by these elongations is heavily temperature dependent, varying greatly between each of the polar crystal phases and exerting a huge influence over the properties of a coupled magnetic film. Here we demonstrate that temperature, and thus strain, is an effective means of controlling the magnetic anisotropy in BaTiO3(111)/CoFeB heterostructures. We investigate the three polar phases of BaTiO3: tetragonal (T) at room temperature, orthorhombic (O) below 280 K and rhombohedral (R) below 190 K, across a total range of 77 K to 420 K. We find two distinct responses; a step-like change in the anisotropy across the low-temperature phase transitions, and a sharp high-temperature reduction around the ferroelectric Curie temperature, measured from hard axis hysteresis loops. Using our measurements of this anisotropy strength we are then able to show by micromagnetic simulation the behaviour of all possible magnetic domain wall states and determine their scaling as a function of temperature. The most significant changes occur in the head-to-head domain wall states, with a maximum change of 210 nm predicted across the entire range effectively doubling the size of the domain wall as compared to room temperature. Notably, similar changes are seen for both high and low temperatures which suggest different routes for potential control of magnetic anisotropy and elastically pinned magnetic domain walls.

cond-mat.mtrl-sci↗

arXiv2022

Strain Coupled Domains in BaTiO3(111)-CoFeB Heterostructures

Domain pattern transfer from ferroelectric to ferromagnetic materials is a critical step for the electric field control of magnetism and has the potential to provide new schemes for low-power data storage and computing devices. Here we investigate domain coupling in BaTiO$_3$(111)/CoFeB heterostructures by direct imaging in a wide-field Kerr microscope. The magnetic easy axis is found to locally change direction as a result of the underlying ferroelectric domains and their polarisation. By plotting the remanent magnetisation as a function of angle in the plane of the CoFeB layer, we find that the magnetic easy axes in adjacent domains are angled at 60$^\circ$ or 120$^\circ$, corresponding to the angle of rotation of the polarisation from one ferroelectric domain to the next, and that the magnetic domain walls may be charged or uncharged depending on the magnetic field history. Micromagnetic simulations show that the properties of the domain walls vary depending on the magnetoelastic easy axis configuration and the charged or uncharged nature of the wall. The configuration where the easy axis alternates by 60$^\circ$ and a charged wall is initialised exhibits the largest change in domain wall width from 192 nm to 119 nm as a function of in-plane magnetic field. Domain wall width tuning provides an additional degree of freedom for devices that seek to manipulate magnetic domain walls using strain coupling to ferroelectrics.

cond-mat.mtrl-sci↗

arXiv2018

Magnetic properties, domain wall creep motion and the Dzyaloshinskii-Moriya interaction in Pt/Co/Ir thin films

We study the magnetic properties of perpendicularly magnetised Pt/Co/Ir thin films and investigate the domain wall creep method of determining the interfacial Dzyaloshinskii-Moriya (DM) interaction in ultra-thin films. Measurements of the Co layer thickness dependence of saturation magnetisation, perpendicular magnetic anisotropy, and symmetric and antisymmetric (i.e. DM) exchange energies in Pt/Co/Ir thin films have been made to determine the relationship between these properties. We discuss the measurement of the DM interaction by the expansion of a reverse domain in the domain wall creep regime. We show how the creep parameters behave as a function of in-plane bias field and discuss the effects of domain wall roughness on the measurement of the DM interaction by domain expansion. Whereas modifications to the creep law with DM field and in-plane bias fields have taken into account changes in the energy barrier scaling parameter $α$, we find that both $α$ and the velocity scaling parameter $v_{0}$ change as a function of in-plane bias field.

cond-mat.mes-hall↗

arXiv2018

Dielectric properties of relaxor-ferroelectric ceramic and single crystal Pb(In$_{1/2}$Nb$_{1/2}$)O$_{3}$-Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$-PbTiO$_{3}$ at cryogenic temperatures

We investigate the low temperature behaviour of Pb(In$_{1/2}$Nb$_{1/2}$)O$_{3}$-Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$-PbTiO$_{3}$ using dielectric permittivity measurements. We compare single crystal plates measured in the [001] and [111] directions with a polycrystalline ceramic of the same composition. Poled crystals behave very differently to unpoled crystals, whereas the dielectric spectrum of the ceramic changes very little on poling. A large, frequency dependent dielectric relaxation seen in the poled [001] crystal around 100 K is much less prominent in the [111] crystal, and doesn't occur in the ceramic. Preparation conditions and the microstructure of the material play a role in the low temperature dynamics of relaxor-ferroelectric crystals.

cond-mat.mtrl-sci↗

arXiv2016

Effect of interfacial intermixing on the Dzyaloshinskii-Moriya interaction in Pt/Co/Pt

We study the effect of sputter-deposition conditions, namely substrate temperature and chamber base pressure, upon the interface quality of epitaxial Pt/Co/Pt thin films with perpendicular magnetic anisotropy. Here we define interface quality to be the inverse of the sum in quadrature of roughness and intermixing. We find that samples with the top Co/Pt layers grown at 250 degrees C exhibit a local maximum in roughness-intermixing and that the interface quality is better for lower or higher deposition temperatures, up to 400 degrees C, above which the interface quality degrades. Imaging the expansion of magnetic domains in an in-plane field using wide-field Kerr microscopy, we determine the interfacial Dzyaloshinskii-Moriya interaction (DMI) in films in the deposition temperature range 100 degrees C to 300 degrees C. The net DMI is linked to the difference in top and bottom Co interface qualities; the net DMI increases as the difference between top and bottom Co interface quality increases. Furthermore, for sufficiently low base pressures, the net DMI increases linearly with the deposition temperature, indicating that fine-tuning of the DMI may be achieved via the deposition conditions.

cond-mat.mes-hall↗