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Pierre Chantelot

Publications and source records attributed to Pierre Chantelot.

10 recordsLinked to original sources

Guided elastic waves for soft elastomer characterization: an alternative to conventional rheometry

Elastic wave propagation is intrinsically sensitive to the mechanical properties of the medium through which it travels. In soft elastomers, this makes guided elastic waves natural probes of viscoelastic and acoustoelastic behavior over a broad frequency range. In this work, we introduce a wave-based mechanical characterization method in which a thin elastomer strip acts as a waveguide supporting multiple in-plane guided modes. By combining stroboscopic measurements of monochromatic wave fields with a theoretical framework that couples frequency-dependent viscoelasticity and elongation-dependent acoustoelasticity, we extract complex-valued dispersion relations for guided modes under controlled static elongation. A dedicated numerical implementation allows these experimental dispersion curves to be quantitatively matched to theory, enabling identification of the material's rheological and hyperelastic parameters. Applied to several commercial silicone elastomers, the method yields mechanical parameters that are consistent with conventional plate-plate rheometry, while extending the accessible frequency range beyond that of conventional techniques. By exploiting the richness of guided-wave dispersion and the sensitivity of waves to both frequency and pre-stress, this approach provides a unified, broadband, and experimentally simple route to the mechanical characterization of soft elastomers.

cond-mat.soft

Guided elastic waves informed material modelling of soft incompressible media

Identifying a universal material constitutive law, that describes the mechanical response of rubber-like solids for all deformation fields and achievable extensions, is an outstanding challenge. Here, we propose to exploit the propagation of elastic waves and demonstrate that monitoring incremental guided wave propagation in an elastomer plate undergoing uniaxial extension reveals model sensitivities that are inaccessible in the corresponding static test. We measure the dispersion relations of the three zero-order guided modes, propagating parallel and perpendicular to the direction of imposed elongation. We compare them with predictions from the acoustoelastic theory, that also take into account material rheology, using parameters extracted from fitting the uniaxial stress-strain curve across three successive elongation regimes, following the methodical procedure of Destrade $\textit{et al.}$ (Proc. R. Soc. A 2017). We evidence that our approach lifts the degeneracy between hyperelastic models with different functional forms of the so-called $C_2$ term, which remain undistinguishable from static uniaxial tension stress-strain measurements alone. However, like their static counterpart, our dynamics measurements cannot distinguish between different generalized neo-Hookean models.

cond-mat.soft

Wave propagation in a model artery

Fluid filled pipes are ubiquitous in both man-made constructions and living organisms. In the latter, biological pipes, such as arteries, have unique properties as their walls are made of soft, incompressible, highly deformable materials. In this article, we experimentally investigate wave propagation in a model artery: an elastomer strip coupled to a rigid water channel. We measure out-of-plane waves using synthetic Schlieren imaging, and evidence a single dispersive mode which resembles the pulse wave excited by the heartbeat. By imposing an hydrostatic pressure difference, we reveal the strong influence of pre-stress on the dispersion of this wave. Using a model based on the acoustoelastic theory accounting for the material rheology and for the large static deformation of the strip, we demonstrate that the imposed pressure affects wave propagation through an interplay between stretching, orthogonal to the propagation direction, and curvature-induced rigidity. We finally highlight the relevance of our results in the biological setting, by discussing the determination of the arterial wall's material properties from pulse wave velocity measurements in the presence of pre-stress.

cond-mat.soft

Drop impact on superheated surfaces: from capillary dominance to non-linear advection dominance

Ambient air cushions the impact of drops on solid substrates, an effect usually revealed by the entrainment of a bubble, trapped as the air squeezed under the drop drains and liquid-solid contact occurs. The presence of air becomes evident for impacts on very smooth surfaces, where the gas film can be sustained, allowing drops to bounce without wetting the substrate. In such a non-wetting situation, Mandre & Brenner (2012) numerically and theoretically evidenced that two physical mechanisms can act to prevent contact: surface tension and non-linear advection. However, the advection dominated regime has remained hidden in experiments as liquid-solid contact prevents to realize rebounds at sufficiently large impact velocities. By performing impacts on superheated surfaces, in the so-called dynamical Leidenfrost regime Tran et al. (2012), we enable drop rebound at higher impact velocities, allowing us to reveal this regime. Using high-speed total internal reflection, we measure the minimal gas film thickness under impacting drops, and provide evidence for the transition from the surface tension to the non-linear inertia dominated regime. We rationalise our measurements through scaling relationships derived by coupling the liquid and gas dynamics, in the presence of evaporation.

physics.flu-dyn

When does an impacting drop stop bouncing?

Non-wetting substrates allow impacting liquid drops to spread, recoil, and takeoff, provided they are not too heavy (Biance et al. 2006) or too viscous (Jha et al. 2020). In this article, using direct numerical simulations with the volume of fluid method, we investigate how viscous stresses and gravity conspire against capillarity to inhibit drop rebound. Close to the bouncing to non-bouncing transition, we evidence that the initial spreading stage can be decoupled from the later retraction and takeoff, allowing to understand the rebound as a process converting the surface energy of the spread liquid into kinetic energy. Drawing an analogy with coalescence induced jumping, we propose a criterion for the transition from the bouncing to the non-bouncing regime, namely by the condition $Oh_c + Bo_c \sim 1$, where $Oh_c$ and $Bo_c$ are the Ohnesorge number and Bond number at the transition, respectively. This criterion is in excellent agreement with the numerical results. We also elucidate the mechanisms of bouncing inhibition in the heavy and viscous drops limiting regimes by calculating the energy budgets and relating them to the drop's shape and internal flow.

physics.flu-dyn

Drop impact on viscous liquid films

When a liquid drop falls on a solid substrate, the air layer in between them delays the occurrence of liquid--solid contact. For impacts on smooth substrates, the air film can even prevent wetting, allowing the drop to bounce off with dynamics identical to that observed for impacts on superamphiphobic materials. In this article, we investigate similar bouncing phenomena, occurring on viscous liquid films, that mimic atomically smooth substrates, with the goal to probe their effective repellency. We elucidate the mechanisms associated to the bouncing to non-bouncing (floating) transition using experiments, simulations, and a minimal model that predicts the main characteristics of drop impact, the contact time, and the coefficient of restitution. In the case of highly viscous or very thin films, the impact dynamics is not affected by the presence of the viscous film. Within this substrate--independent limit, bouncing is suppressed once the drop viscosity exceeds a critical value as on superamphiphobic substrates. For thicker or less viscous films, both the drop and film properties influence the rebound dynamics and conspire to inhibit bouncing above a critical film thickness. This substrate--dependent regime also admits a limit, for low viscosity drops, in which the film properties alone determine the limits of repellency.

physics.flu-dyn

Non-wetting drop dynamics

The impact of droplets on solids or weakly-deformable surfaces can lead to non-wetting outcomes, depending on the control parameters. Here, we perform experiments and develop a simple model to understand the impact dynamics by varying three important drop parameters: the Ohnesorge number $\mathcal{O}h$, the Bond number $\mathcal{B}o$ and the Weber number $\mathcal{W}e$. The model suggests that the droplet dynamics is captured by only two non-dimensional groups, namely $\ \mathcal{O}h$ and $ξ= \mathcal{B}o/\sqrt{\mathcal{W}e}$. For $ξ\ll 1$, the droplet dynamics is fully dominated by $\mathcal{O}h$, but for $ξ\gg 1$, the dynamics depends both on $\mathcal{O}h$ and $ξ$. While the model results show some discrepancies for small $\mathcal{O}h$, they are in very good agreement with the experiments for moderately large $\mathcal{O}h$. The work thereby offers an elaborate description of the droplet impact dynamics in a non-wetting scenario.

physics.flu-dyn

The Leidenfrost effect as a directed percolation phase transition

Volatile drops deposited on a hot solid can levitate on a cushion of their own vapor, without contacting the surface. We propose to understand the onset of this so-called Leidenfrost effect through an analogy to non-equilibrium systems exhibiting a directed percolation phase transition. When performing impacts on superheated solids, we observe a regime of spatiotemporal intermittency in which localized wet patches coexist with dry regions on the substrate. We report a critical surface temperature, which marks the upper bound of a large range of temperatures in which levitation and contact coexist. In this range, with decreasing temperature, the equilibrium wet fraction increases continuously from zero to one. Also, the statistical properties of the spatio-temporally intermittent regime are in agreement with that of the directed percolation universality class. This analogy allows us to redefine the Leidenfrost temperature and shed light on the physical mechanisms governing the transition to the Leidenfrost state.

physics.flu-dyn

Drop impact on superheated surfaces: short-time dynamics and transition to contact

When a volatile drop impacts on a superheated solid, air drainage and vapor generation conspire to create an intermediate gas layer that delays or even prevents contact between the liquid and the solid. In this article, we use high-speed synchronized reflection interference and total internal reflection imaging to measure the short-time dynamics of the intermediate gas film and to probe the transition between levitation and contact. We observe that the substrate temperature strongly affects the vertical position of the liquid-gas interface and that the dynamic Leidenfrost transition is influenced by both air and vapor drainage (\emph{i.e}, gas drainage), and evaporation, the later giving rise to hitherto unreported vertical oscillations of the gas film that can trigger liquid-solid contact. We first derive scaling relations for the height of the gas film trapped under the drop's centerline, called the dimple height, and the minimum film thickness at short times. The former is set by a competition between gas drainage and liquid inertia, similarly as for isothermal impacts, while the later strongly depends on the vapor production. The gas pressure, at the location where the minimum thickness is reached, is determined by liquid inertia and vapor production and ultimately balanced by the increasing interfacial curvature, determining the minimum thickness. We show that, in the low impact velocity limit, the transient stability of the draining gas film remarkably makes dynamic levitation less demanding than static levitation. We characterise the vertical gas film oscillations by measuring their frequency and monitoring their occurrence in the parameter space spanned by surface temperature and impact velocity. Finally, we model the occurrence of these oscillations and account for their frequency through an hydrodynamic mechanism.

physics.flu-dyn

Drop Trampoline

Rigid superhydrophobic materials have the ability to repel millimetric water drops, in typically 10 ms. Yet, most natural water-repellent materials can be deformed by impacting drops. To test the effect of deformability, we perform impacts of non-wetting drops onto thin ($\sim$ 10 \micro m), circular PDMS membranes. The bouncing mechanism is markedly modified compared to that on a rigid material: the liquid leaves the substrate as it is kicked upwards by the membrane. We show that the rebound is controlled by an interplay between the dynamics of the drop and that of the soft substrate, so that we can continuously vary the contact time by playing on the membrane's characteristics and reduce it up to 70\%.

cond-mat.soft