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Piers Coleman

Publications and source records attributed to Piers Coleman.

At least 37 records · Page 2Linked to original sources

Quantum order by disorder in Frustrated Spin Nanotubes

We investigate quantum order by disorder in a frustrated spin nanotube formed by wrapping a $J_1$-$J_2$ Heisenberg model at 45$^\circ$ around a cylinder. Using Schwinger boson theory and Density Matrix Renormalization Group (DMRG), we have computed the ground-state phase diagram to reveal a $\mathbb{Z}_2$ phase in which collinear spin stripes form a right or left handed helix around the nanotube. We have derived an analytic estimate for the critical $η_c=J_1/2J_2$ of the $\mathbb{Z}_2$ helical phase transition, which is in agreement with the DMRG results. By evaluating the entanglement spectrum and nonlocal string order parameters we discuss the topology of the $\mathbb{Z}_2$-helical phase.

cond-mat.str-el↗

Analytic calculation of the vison gap in the Kitaev spin liquid

Although the ground-state energy of the Kitaev spin liquid can be calculated exactly, the associated vison gap energy has to date only been calculated numerically from finite size diagonalization. Here we show that the phase shift for scattering Majorana fermions off a single bond-flip can be calculated analytically, leading to a closed-form expression for the vison gap energy $Δ= 0.2633J$. Generalizations of our approach can be applied to Kitaev spin liquids on more complex lattices such as the three dimensional hyper-octagonal lattice.

cond-mat.str-el↗

Flat bands, strange metals, and the Kondo effect

Flat band materials such as the kagome metals or moiré superlattice systems are of intense current interest. Flat bands can result from the electron motion on numerous (special) lattices and usually exhibit topological properties. Their reduced bandwidth proportionally enhances the effect of Coulomb interaction, even when the absolute magnitude of the latter is relatively small. Seemingly unrelated to these cases is the large family of strongly correlated electron systems, which includes the heavy fermion compounds, cuprate and pnictide superconductors. In addition to itinerant electrons from large, strongly overlapping orbitals, they frequently contain electrons from more localized orbitals, which are subject to a large Coulomb interaction. The question then arises as to what commonality in the physical properties and microscopic physics, if any, exists between the two broad categories of materials? A rapidly increasing body of strikingly similar phenomena across the different platforms -- from electronic localization-delocalization transitions to strange metal behavior and unconventional superconductivity -- suggests that similar underlying principles could be at play. Indeed, it has recently been suggested that flat band physics can be understood in terms of Kondo physics. Inversely, the concept of electronic topology from lattice symmetry, which is fundamental in flat band systems, is enriching the field of strongly correlated electron systems where correlation-driven topological phases are increasingly being investigated. Here we elucidate this connection, survey the new opportunities for cross-fertilization in understanding across the platforms, and assess the prospect for new insights that may be gained into both the correlation physics and its intersection with electronic topology.

cond-mat.str-el↗

TBG as Topological Heavy Fermion: II. Analytical approximations of the model parameters

The recently-introduced Topological Heavy Fermion (THF) model [Phys. Rev. Lett. 129, 047601] of twisted bilayer graphene (TBG) aims to reconcile the quantum-dot-like electronic structure of the latter observed by scanning tunneling microscopy, with its electron delocalization seen in transport measurements. The THF model achieves this by coupling localized (heavy) fermions with anomalous conduction electrons. Originally, the parameters of the THF model were obtained numerically from the Bistritzer-Macdonald (BM) model of TBG [Phys. Rev. Lett. 129, 047601]. In this work, we derive analytical expressions for the THF model parameters as a function of the twist angle, the ratio between the tunneling amplitudes at the $AA$ and $AB$ regions ($w_0 / w_1$), and the screening length of the interaction potential. By numerically computing the THF model parameters across an extensive experimentally-relevant parameter space, we show that the resulting approximations are remarkably good, i.e. within the 30% relative error for almost the entire parameter space. At the single-particle level, the THF model accurately captures the energy spectrum of the BM model over a large phase space of angles and tunneling amplitude ratios. When interactions are included, we also show that the THF description of TBG is good around the magic angle for realistic values of the tunneling amplitude ratios ($0.6 \leq w_0/w_1 \leq 1.0$), for which the hybridization between the localized and conduction fermions $γ$ is smaller than the onsite repulsion of the heavy fermions $U_1$ (i.e. $|γ| < U_1$).

cond-mat.str-el↗

Light-Driven Transitions in Quantum Paraelectrics

Motivated by recent experiments on pump-induced polar ordering in the quantum paraelectric SrTiO$_3$, we study a driven phonon system close to a second order phase transition. Analyzing its classical dynamics, we find that sufficiently strong driving leads to transitions into polar phases whose structures, determined by the light polarization, are not all accessible in equilibrium. In addition, for certain intensity profiles we demonstrate the possibility of two-step transitions as a function of fluence. For even stronger field intensities, the possibility of period-doubling and chaotic behavior is demonstrated. Finally we develop a generalized formalism that allows us to consider quantum corrections to the classical dynamics in a systematic fashion. We predict a shift in the critical pump fluence due to quantum fluctuations with a characteristic dependence on the fluence increase rate, which can be observed in experiments.

cond-mat.mes-hall↗

Triplet pairing, orbital selectivity and correlations in Iron-based superconductors

We use a slave-boson approach to study the band renormalization and pair susceptibility in the normal state of Iron-based superconductors in presence of strong Coulomb repulsion and Hund's interaction. Our results show orbital selectivity toward localization of $xy$ orbitals and its interplay with superconductivity. We also compare the recently proposed triplet resonating valence bond theory of superconductivity in Iron-based superconductors with the more conventional $s_\pm$ pairing and show that both favor a superconductivity when the $xy$ orbital is delocalized.

cond-mat.supr-con↗

Matrix Product Study of Spin Fractionalization in the 1D Kondo Insulator

The Kondo lattice is one of the classic examples of strongly correlated electronic systems. We conduct a controlled study of the Kondo lattice in one dimension, highlighting the role of excitations created by the composite fermion operator. Using time-dependent matrix-product-state methods we compute various correlation functions and contrast them with both large-N mean-field theory and the strong-coupling expansion. We show that the composite fermion operator creates long-lived, charge-e and spin-1/2 excitations, which cover the low-lying single-particle excitation spectrum of the system. Furthermore, spin excitations can be thought to be composed of such fractionalized quasi-particles with a residual interaction which tend to disappear at weak Kondo coupling.

cond-mat.str-el↗

Triplet pairing mechanisms from Hund's-Kondo models: applications to UTe$_{2}$ and CeRh$_{2}$As$_{2}$

Observing that several U and Ce based candidate triplet superconductors share a common structural motif, with pairs of magnetic atoms separated by an inversion center, we hypothesize a triplet pairing mechanism based on an interplay of Hund's and Kondo interactions that is unique to this structure. In the presence of Hund's interactions, valence fluctuations generate a triplet superexchange between electrons and local moments. The offset from the center of symmetry allows spin-triplet pairs formed by the resulting Kondo effect to delocalize onto the Fermi surface, precipitating superconductivity. We demonstrate this mechanism within a minimal two-channel Kondo lattice model and present support for this pairing mechanism from existing experiments.

cond-mat.supr-con↗

Interplay of charge and spin fluctuations in a Hund's coupled impurity

In Hund's metals, the local ferromagnetic interaction between orbitals leads to an emergence of complex electronic states with large and slowly fluctuating magnetic moments. Introducing the Hund's coupled mixed valence quantum impurity, we gain analytic insight into recent numerical renormalization group studies. We show that valence fluctuations drastically impede the development of a large fluctuating moment over a wide range of temperatures and energy, characterized by quenched orbital degrees of freedom and a singular logarithmic behavior of the spin susceptibility $χ_{\rm sp}''(ω) \propto [ω\ln(ω/T_K^{\rm eff})^2]^{-1}$, closely resembling power-law scaling $χ_{\rm sp}''(ω) \sim ω^{-γ}$. Such singular spin fluctuations are suspected to play an important role in future models of Hund's driven Cooper pairing.

cond-mat.str-el↗

Soluble limit and criticality of fermions in Z2 gauge theories

Quantum information theory and strongly correlated electron systems share a common theme of macroscopic quantum entanglement. In both topological error correction codes and theories of quantum materials (spin liquid, heavy fermion and high-$T_c$ systems) entanglement is implemented by means of an emergent gauge symmetry. Inspired by these connections, we introduce a simple model for fermions moving in the deconfined phase of a $\mathbb Z_2$ gauge theory, by coupling Kitaev's toric code to mobile fermions. This permits us to exactly solve the ground state of this system and map out its phase diagram. Reversing the sign of the plaquette term in the toric code, permits us to tune the groundstate between an orthogonal metal and an orthogonal semimetal, in which gapless quasiparticles survive despite a gap in the spectrum of original fermions. The small-to-large Fermi surface transition between these two states occurs in a stepwise fashion with multiple intermediate phases. By using a novel diagrammatic technique we are able to explore physics beyond the integrable point, to examine various instabilities of the deconfined phase and to derive the critical theory at the transition between deconfined and confined phases. We outline how the fermionic toric code can be implemented as a quantum circuit thus providing an important link between quantum materials and quantum information theory.

cond-mat.str-el↗

A solvable 3D Kondo lattice exhibiting odd-frequency pairing and order fractionalization

The Kondo lattice model plays a key role in our understanding of quantum materials, but a lack of small parameters has posed a long-standing problem. We present a 3 dimensional S= 1/2 Kondo lattice model describing a spin liquid within an electron sea. Strong correlations in the spin liquid are treated exactly, enabling a controlled analytical approach. Like a Peierls or BCS phase, a logarithmically divergent susceptibility leads to an instability into a new phase at arbitrarily small Kondo coupling. Our solution captures a plethora of emergent phenomena, including odd-frequency pairing, pair density wave formation and order fractionalization. The ground-state state is a pair density wave with a fractionalized charge e, S = 1/2 order parameter, formed between electrons and Majorana fermions.

cond-mat.str-el↗

Order Fractionalization in a Kitaev-Kondo model

We describe a mechanism for order fractionalization in a two-dimensional Kondo lattice model, in which electrons interact with a gapless spin liquid of Majorana fermions described by the Yao-Lee (YL) model. When the Kondo coupling to the conduction electrons exceeds a critical value, the model develops a superconducting instability into a state where the spinor order parameter carries charge $e$ and spin $S=1/2$. The broken symmetry state develops a gapless Majorana Dirac cone in the bulk. By including an appropriate gauge string, we can show that the charge $e$, spinorial order develops off-diagonal long range order that allows electrons to coherently tunnel arbitrarily long distances through the spin liquid.

cond-mat.str-el↗

Quasi-uniaxial pressure induced superconductivity in stoichiometric compound UTe$_2$

The recent discovery of superconductivity in heavy Fermion compound UTe2, a candidate topological and triplet-paired superconductor, has aroused widespread interest. However, to date, there is no consensus on whether the stoichiometric sample of UTe2 is superconducting or not due to lack of reliable evidence to distinguish the difference between the nominal and real compositions of samples. Here, we are the first to clarify that the stoichiometric UT2 is non-superconducting at ambient pressure and under hydrostatic pressure up to 6 GPa, however we find that it can be compressed into superconductivity by application of quasi-uniaxial pressure. Measurements of resistivity, magnetoresistance and susceptibility reveal that the quasi-uniaxial pressure results in a suppression of the Kondo coherent state seen at ambient pressure, and then leads to a superconductivity initially emerged on the ab-plane at 1.5 GPa. At 4.8 GPa, the superconductivity is developed in three crystallographic directions. The superconducting state coexists with an exotic magnetic ordered state that develops just below the onset temperature of the superconducting transition. The discovery of the quasi-uniaxial-pressure-induced superconductivity with exotic magnetic state in the stoichiometric UTe2 not only provide new understandings on this compound, but also highlight the vital role of Te deficiency in developing the superconductivity at ambient pressures.

cond-mat.supr-con↗

Observation of a Critical Charge Mode in a Strange Metal

Quantum electronic matter has long been understood in terms of two limiting behaviors of electrons: one of delocalized metallic states, and the other of localized magnetic states. Understanding the strange metallic behavior which develops at the brink of localization demands new probes of the underlying electronic charge dynamics. Using a state-of-the-art technique, synchrotron-radiation-based Mossbauer spectroscopy, we have studied the longitudinal charge fluctuations of the strange metal phase of beta-YbAlB4 as a function of temperature and pressure. We find that the usual single absorption peak in the Fermi-liquid regime splits into two peaks upon entering the critical regime. This spectrum is naturally interpreted as a single nuclear transition, modulated by nearby electronic valence fluctuations whose long time-scales are further enhanced, due to the formation of charged polarons. Our results represent a direct observation of critical charge fluctuations as a new signature of strange metals.

cond-mat.str-el↗

Triplet resonating valence bond theory and transition metal chalcogenides

We develop a quantum spin liquid theory for quantum magnets with easy-plane ferromagnetic exchange. These strongly entangled quantum states are obtained by dimer coverings of 2D lattices with triplet $S = 1, m_z = 0$ bonds, forming a triplet resonating valence bond (tRVB) state. We discuss the conditions and the procedure to transfer well-known results from conventional singlet resonating valence bond theory to tRVB. Additionally, we present mean field theories of Abrikosov fermions on 2D triangular and square lattices, which can be controlled in an appropriate large $N$ limit. We also incorporate the effect of charge doping which stabilizes $p+ip$-wave superconductivity. Beyond the pure theoretical interest, our study may help to resolve contradictory statements on certain transition metal chalcogenides, including 1T-TaS$_2$, as a potential tRVB spin-liquid.

cond-mat.str-el↗

Frustrated Kondo impurity triangle: A simple model of deconfinement

The concepts of deconfinement and topological order are of great current interest for quantum information science and for our understanding of quantum materials. Here, we introduce a simple model of three antiferromagnetically coupled Kondo impurities, a Kondo triangle, which can be used to further extend the application of these concepts to electronic systems. We show that, by tuning the magnetic frustration, the Kondo triangle undergoes a quantum phase transition between two phases of unbroken symmetry, signaling a phase transition beyond the Landau paradigm. We demonstrate that the frustrated spin liquid phase is described by a three-channel Kondo (3CK) fixed point and thus displays an irrational ground state degeneracy. Using an Abrikosov pseudofermion representation, this quantum state is categorized by an emergent U(1) gauge field and its projective symmetry group. The gauge theory is deconfining in the sense that a miniature Wilson loop orders and topological defects (instantons in the gauge field) are expelled. This phase persists in the presence of moderate Kondo screening until proliferation of topological defects leads to a quantum phase transition to an unfrustrated Fermi liquid phase. Based on this evidence, we propose that the 3CK phase displays topological order in a similar sense as gapless spin liquids.

cond-mat.str-el↗

Superconductivity from energy fluctuations in dilute quantum critical polar metals

Superconductivity in low carrier density metals challenges the conventional electron-phonon theory due to the absence of retardation required to overcome Coulomb repulsion. In quantum critical polar metals, the Coulomb repulsion is heavily screened, while the critical transverse optic phonons decouple from the electron charge. In the resulting vacuum, the residual interactions between quasiparticles are carried by energy fluctuations of the polar medium, resembling the gravitational interactions of a dark matter universe. Here we demonstrate that pairing inevitably emerges from "gravitational'' interactions with the energy fluctuations, leading to a dome-like dependence of the superconducting $T_c$ on carrier density. Our estimates show that this mechanism may explain the critical temperatures observed in doped SrTiO$_3$. We provide predictions for the enhancement of superconductivity near polar quantum criticality in two and three dimensional materials that can be used to test our theory.

cond-mat.supr-con↗

Emergent Potts Order in a Coupled Hexatic-Nematic XY model

Addressing the nature of an unexpected smectic-A' phase in liquid crystal 54COOBC films, we perform large scale Monte Carlo simulations of a coupled hexatic-nematic XY model. The resulting finite-temperature phase diagram reveals a small region with composite Potts $\mathbb{Z}_3$ order above the vortex binding transition; this phase is characterized by relative hexatic-nematic ordering though both variables are disordered. The system develops algebraic hexatic and nematic order only at a lower temperature. This multi-step melting scenario agrees well with the experimental observations of a sharp specific heat anomaly that emerges above the onset of hexatic positional order. We therefore propose that the smectic-A' phase is characterized by composite Potts order and bound-states of fractional vortices.

cond-mat.stat-mech↗