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Pieter J. van Essen

Publications and source records attributed to Pieter J. van Essen.

6 recordsLinked to original sources

Transient High-Harmonic Generation from Solids: From Spectroscopy and Control to Programmable Emission

High-harmonic generation (HHG) from solids has emerged as a powerful probe of electronic structure and ultrafast dynamics in condensed matter systems. In this chapter, we review recent advances in solid-state HHG spectroscopy and control, with a focus on semiconductors and correlated materials. We discuss the theoretical foundations of HHG and summarize experimental approaches for extracting information from harmonic emission. HHG has been shown to be sensitive to a wide range of microscopic properties, including band structure, transition dipole moments, Berry phases, crystal symmetry, carrier populations, dephasing processes, and lattice dynamics. This sensitivity enables access to electronic and structural dynamics on femtosecond and attosecond timescales and has established HHG as a versatile spectroscopic tool. At the same time, the strong dependence of HHG on many coupled material and excitation parameters makes the emitted harmonics intrinsically difficult to associate with a single microscopic quantity. Rather than representing a limitation alone, this sensitivity also provides numerous pathways for control. We review how photoexcitation, multicolor driving fields, waveform engineering, and transient modification of material properties can be used to enhance, suppress, and shape harmonic emission. These developments position solid-state HHG not only as a spectroscopic technique, but also as a platform for programmable nonlinear optics with applications ranging from compact extreme-ultraviolet sources to super-resolution microscopy and ultrafast photonic devices.

physics.optics↗

Programmable high-harmonic emission in solids through photon pathways

Ultrafast all-optical control of light emission is a central goal of extreme nonlinear optics, with implications for compact short-wavelength sources, petahertz optoelectronics, and label-free superresolution microscopy. High-harmonic generation in solids is a particularly attractive platform for this goal because it is highly sensitive to both the driving field and the material response, yet a generally applicable framework for controlling harmonic emission has remained elusive. Here, we demonstrate programmable control of high-harmonic emission in solids and show that it can be quantitatively described within a photon-pathway framework. We find that harmonic emission can be suppressed or enhanced by tuning two experimentally accessible quantities: the effective nonlinear order and the intrinsic emission phase. Across a wide range of semiconductors and dielectrics, this approach unifies parametric and non-parametric modulation, explains distinct delay-dependent spectral responses, and reproduces strong suppression, enhancement, and higher-order pathway revivals. Semiconductor Bloch equation simulations support the model and provide a complementary time-domain picture in which the control field reshapes the interference of sub-cycle emission events. These results establish high-harmonic generation in solids as a programmable emission process and provide a general route towards ultrafast optical switching, compact coherent short-wavelength sources, and label-free attosecond super-resolution microscopy.

physics.optics↗

Attosecond high-harmonic interferometry probes orbital- and band-dependent dipole phase in magnesium oxide

Control over the spatial coherence, wavefront, and focusability of emitted light relies on understanding the intrinsic phase of the emission process, and vice versa, measuring phase can reveal insights about microscopic generation mechanisms. A thorough understanding of the origin of the dipole phase in solid-state high-harmonic generation is currently missing. Here, by employing attosecond interferometry with phase-locked XUV pulses, we directly assess the intensity- and frequency-dependent dipole phases in magnesium oxide (MgO) in solid-state HHG. We also quantify a nonlinear phase shift of the fundamental and disentangle its contribution from the dipole phase. Theoretical models (analytical, two-band, and full-band numerical simulations) support our results. The analytical approach aids future solid-state HHG experiments and simulations, while the full numerical model details orbital- and band-resolved current contributions to the dipole phase. Our research delivers the first combined quantitative measurement and rigorous theoretical description of the harmonic emission phase in solids.

physics.optics↗

Extreme Ultraviolet High-Harmonic Interferometry of Excitation-Induced Bandgap Dynamics in Solids

Interferometry is a fundamental technique in physics, enabling precise measurements through the interference of waves. High-harmonic generation (HHG) in solids has emerged as a powerful method for probing ultrafast electronic dynamics within crystalline structures. In this study, we employed extreme ultraviolet (XUV) high-harmonic interferometry with phase-locked XUV pulse pairs to investigate excitation-induced bandgap dynamics in solids. Our experiments on amorphous SiO2 and crystalline MgO, complemented by analytical modeling and semiconductor Bloch equation simulations, reveal a correlation between transient bandgap modifications and variations in the phase of harmonic emission. These findings suggest a potential pathway for sub-cycle, all-optical control of band structure modifications, advancing prospects for petahertz-scale electronic applications and attosecond diagnostics of carrier dynamics.

physics.optics↗

Spatial polarization gating of high-harmonic generation in solids

High-harmonic generation from solids can be utilized as probe of ultrafast dynamics, but thus far only over extended sample areas, since its spatial resolution is diffraction-limited. Here we propose spatial polarization gating, that is using a spatially varying ellipticity of a driving laser pulse to reduce the spatial profile of high-harmonic emission below the diffraction limit and hence increase spatial resolution. We show experimentally and by numerical simulations that our method is generally applicable as suppressing high harmonics in elliptical fields is a common response in all solids. We also briefly explore the possibility of applying this technique to widefield imaging, specifically to nonlinear structured illumination microscopy. Our findings indicate that spatial polarization gating can enable all-optical femto-to-attosecond label-free imaging beyond the Abbe limit.

physics.optics↗

Towards complete all-optical emission control of high-harmonic generation from solids

Optical modulation of high-harmonics generation in solids enables the detection of material properties such as the band structure and promising new applications such as super-resolution imaging in semiconductors. Various recent studies have shown optical modulation of high-harmonics generation in solids, in particular, suppression of high-harmonics generation has been observed by synchronized or delayed multi-pulse sequences. Here we provide an overview of the underlying mechanisms attributed to this suppression and provide a perspective on the challenges and opportunities regarding these mechanisms. All-optical control of high-harmonic generation allows for femtosecond, and in the future possibly subfemtosecond, switching, which has numerous possible applications: These range from super-resolution microscopy, to nanoscale controlled chemistry, and highly tunable nonlinear light sources.

physics.optics↗