arXiv subjects

Pietro Musumeci

Publications and source records attributed to Pietro Musumeci.

At least 19 recordsLinked to original sources

arXiv2026

High temporal resolution THz streaking of high brightness relativistic electron beams

We report a systematic experimental study of terahertz (THz) streaking structures for ultrafast characterization of relativistic, high-brightness electron beams. Horn-coupled waveguide geometries are investigated, enabling a comparative characterization of streaking strength, dispersion, transmission, and temporal fidelity. Analytical models and electromagnetic simulations are used to describe the dependence of streaking power on the waveguide dimensions and the drive frequency. Experimentally, the structures are characterized using compressed electron beam from an RF photoinjector over a range of THz field strengths, beam energies, and bunch durations. These results establish general design principles and performance limits for THz streaking structures applicable to ultrafast electron beam diagnostics.

physics.acc-ph↗

arXiv2025

Experimental verification of space-charge saturation scaling laws in high-gradient photocathode RF guns

We investigate the limits of photoemission yield in a high-gradient S-band radiofrequency photoinjector in the space-charge-dominated regime. Using an RF phase-scan technique, where the emitted charge is measured as a function of the RF-field phase in the gun, we directly monitor photoemission over a range of launch fields and laser parameters, enabling quantitative characterization of space-charge saturation. Measurements, supported by simulations and analytic modeling, confirm the characteristic charge-field scaling laws for pancake beams and provide the first experimental verification of cigar-regime scaling in an RF photogun. These results establish a predictive framework for identifying the onset of space-charge saturation and guide the optimization of photoinjectors for ultrafast electron diffraction, microscopy, and high-brightness light sources operating at ultra-high gradients.

physics.acc-ph↗

arXiv2025

Dynamic control of laser driven electron acceleration in a photonic structure using programmable optical pulses

Progress in optical techniques has made precision control of the phase profile in optical pulses common and accessible in scientific laboratories. Carefully shaping the field profile of a laser pulse can be used to master the dynamics of electrons traveling in photonic accelerating structures such as the ones obtained by precisely aligning two dielectric gratings. Here we show that by applying a liquid-crystal-mask to program the phase and amplitude of an infrared laser pulse in combination with a pulse front tilt scheme, it is possible to implement dynamic control on a laser accelerator. This results in a nearly limitless live tuning capability of the accelerator beam dynamics, allowing the demonstration software-based correction of structure and optical front imperfections, implementation of transverse focusing schemes, control of the energy and charge of the output beam, and ultimately optimization of the interaction length, leading to measured energy gains of up to 0.55 MeV.

physics.acc-ph↗

arXiv2025

Sub-5-fs compression and synchronization of relativistic electron bunches enabled by a high-gradient $\alpha$-magnet and low-jitter photoinjector

Generating high-brightness relativistic electron bunches with few-femtosecond duration, while simultaneously achieving few-fs synchronization with ultrafast lasers, remains an outstanding challenge at the frontier of accelerator physics and ultrafast science. In this Letter, we present the beam physics and experimental demonstration of a new method that, for the first time, enables simultaneous control of bunch duration and synchronization with few-fs precision. Timing stabilization is achieved using a tailored high-gradient $\alpha$-magnet that optimizes the correlation between time of flight and momentum, together with a photocathode RF gun designed to suppress the effect of RF-to-laser timing jitter. Compression is realized by manipulating the time-momentum correlation in phase space, primarily through space-charge effects. Sub-5-fs rms bunch duration and synchronization are demonstrated. This method establishes a new regime in electron bunch control, unlocking new capabilities for ultrafast beam physics and applications.

physics.acc-ph↗

arXiv2025

Topological phase transition to a hidden charge density wave liquid

Charge density waves (CDWs), electronic crystals that form within a host solid, have long been speculated to melt into a spatially textured electronic liquid. Though they have not been previously detected, liquid CDWs may nonetheless be fundamental to the phase diagrams of many correlated electron systems, including high temperature superconductors and quantum Hall states. In one of the most promising candidate materials capable of hosting a liquid CDW, 1T-TaS2, a structural phase transition impedes its observation. Here, by irradiating the material with a femtosecond light pulse, we circumvent the structural phase transition to reveal how topological defect dynamics govern the otherwise invisible CDW correlations. Upon photoexcitation, the CDW diffraction peaks broaden azimuthally, initially revealing a hexatic state. At higher temperatures, photoexcitation completely destroys translational and orientational order and only a ring of diffuse scattering is observed, a key signature of a liquid CDW. Our work provides compelling evidence for a defect-unbinding transition to a CDW liquid and presents a protocol for uncovering states that are hidden by other transitions in thermal equilibrium.

cond-mat.str-el↗

arXiv2024

Single-Shot Ionization-Based Transverse Profile Monitor for Pulsed Electron Beams

We present an experimental demonstration of a single-shot, non-destructive electron beam diagnostic based on the ionization of a low-density pulsed gas jet. In our study, 7~MeV electron bunches from a radio frequency (RF) photoinjector, carrying up to 100 pC of charge, traversed a localized distribution of nitrogen gas (N$_2$). The interaction of the electron bunches with the N$_2$ gas generated a correlated signature in the ionized particle distribution, which was spatially magnified using a series of electrostatic lenses and recorded with a micro-channel-plate detector. Various modalities, including point-to-point imaging and velocity mapping, are investigated. A temporal trace of the detector current enabled the identification of single- and double-ionization events. The characteristics of the ionization distribution, dependence on gas density, total bunch charge, and other parameters, are described. Approaches to scaling to higher electron bunch density and energy are suggested. Additionally, the instrument proves useful for comprehensive studies of the ionization process itself.

physics.ins-det↗

arXiv2024

Vector-based feedback of continuous wave radiofrequency compression cavity for ultrafast electron diffraction

The temporal resolution of ultrafast electron diffraction (UED) at weakly relativistic beam energies ($\lesssim$ 100 keV) suffers from space-charge induced electron pulse broadening. We describe the implementation of a radio frequency (RF) cavity operating in the continuous wave regime to compress high repetition rate electron bunches from a 40.4 kV DC photoinjector for ultrafast electron diffraction applications. Active stabilization of the RF amplitude and phase through a feedback loop based on the demodulated in-phase and quadrature components of the RF signal is demonstrated. This scheme yields 144$\pm$19 fs RMS temporal resolution in pump-probe studies.

physics.acc-ph↗

arXiv2023

Extended Interaction Length Laser-Driven Acceleration in a Tunable Dielectric Structure

The development of long, tunable structures is critical to increasing energy gain in laser-driven dielectric accelerators (DLAs). Here we combine pulse-front-tilt illumination with slab-geometry structures assembled by precisely aligning off-the-shelf 4~mm long transmission gratings to achieve up to 200 keV energy modulation for 6 MeV injected electrons. The effective interaction length is longer than 1~mm, limited by dephasing of the accelerated particles in the structure. The piezo-based independent mounting system for the gratings allows tuning of the gap and field distribution inside the structure.

physics.acc-ph↗

arXiv2023

Virtual-Diagnostic-Based Time Stamping for Ultrafast Electron Diffraction

In this work, non-destructive virtual diagnostics are applied to retrieve the electron beam time of arrival and energy in a relativistic ultrafast electron diffraction (UED) beamline using independently-measured machine parameters. This technique has the potential to improve temporal resolution of pump and probe UED scans. Fluctuations in time of arrival have multiple components, including a shot-to-shot jitter and a long-term drift which can be separately addressed by closed loop feedback systems. A linear-regression-based model is used to fit the beam energy and time of arrival and is shown to be able to predict accurately behavior for both on long and short time scales. More advanced time-series analysis based on machine learning techniques can be applied to improve this prediction further.

physics.acc-ph↗

arXiv2022

C$^3$ Demonstration Research and Development Plan

C$^3$ is an opportunity to realize an e$^+$e$^-$ collider for the study of the Higgs boson at $\sqrt{s} = 250$ GeV, with a well defined upgrade path to 550 GeV while staying on the same short facility footprint. C$^3$ is based on a fundamentally new approach to normal conducting linear accelerators that achieves both high gradient and high efficiency at relatively low cost. Given the advanced state of linear collider designs, the key system that requires technical maturation for C$^3$ is the main linac. This white paper presents the staged approach towards a facility to demonstrate C$^3$ technology with both Direct (source and main linac) and Parallel (beam delivery, damping ring, ancillary component) R&D. The white paper also includes discussion on the approach for technology industrialization, related HEP R&D activities that are enabled by C$^3$ R&D, infrastructure requirements and siting options.

physics.acc-ph↗

arXiv2022

Ultrafast Electron Diffraction: Visualizing Dynamic States of Matter

Since the discovery of electron-wave duality, electron scattering instrumentation has developed into a powerful array of techniques for revealing the atomic structure of matter. Beyond detecting local lattice variations in equilibrium structures, recent research efforts have been directed towards the long sought-after dream of visualizing the dynamic evolution of matter in real-time. The atomic behavior at ultrafast timescales carries critical information on phase transition and chemical reaction dynamics, the coupling of electronic and nuclear degrees of freedom in materials and molecules, the correlation between structure, function and previously hidden metastable or nonequilibrium states of matter. Ultrafast electron pulses play an essential role in this scientific endeavor, and their generation has been facilitated by rapid technical advances in both ultrafast laser and particle accelerator technologies. This review presents a summary of the remarkable developments in this field over the last few decades. The physics and technology of ultrafast electron beams is presented with an emphasis on the figures of merit most relevant for ultrafast electron diffraction (UED) experiments. We discuss recent developments in the generation, manipulation and characterization of ultrashort electron beams aimed at improving the combined spatio-temporal resolution of these measurements. The fundamentals of electron scattering from atomic matter and the theoretical frameworks for retrieving dynamic structural information from solid-state and gas-phase samples are described, together with essential experimental techniques and several landmark works. Ultrafast electron probes with ever improving capabilities, combined with other complementary photon-based or spectroscopic approaches, hold tremendous potential for revolutionizing our ability to observe and understand energy and matter at atomic scales.

physics.ins-det↗

arXiv2022

Electro-optic sampling based characterization of broad-band high efficiency THz-FEL

Extremely high beam-to-radiation energy conversion efficiencies can be obtained in a THz FEL using a strongly tapered helical undulator at the zero-slippage resonant condition, where a circular waveguide is used to match the radiation group velocity to the electron beam longitudinal velocity. In this paper we report on the first electro-optic sampling (EOS) based measurements of the broadband THz FEL radiation pulses emitted in this regime. The THz field waveforms are reconstructed in the spatial and temporal domains using multi-shot and single-shot EOS schemes respectively. The measurements are performed varying the input electron beam energy in the undulator providing insights on the complex dynamics in a waveguide FEL.

physics.acc-ph↗

arXiv2022

Feedback and control systems for future linear colliders: White Paper for Snowmass 2021 Topical Group AF07-RF

Particle accelerators for high energy physics will generate TeV-scale particle beams in large, multi-Km size machines colliding high brightness beams at the interaction point [1-4]. The high luminosity in such machines is achieved by producing very small asymmetric beam size at the interaction point, with short durations to minimize beam-beam effects. Tuning energy, timing and position of the beam for optimal performance will require high-precision controls of amplitude and phase of high-frequency electromagnetic fields and real-time processing of complex algorithms. The stability of the colliding beams has a large impact on the collider's effective luminosity. Therefore, the technology readiness level of diagnostic and control systems will be a major consideration in the collider design. The technical requirements of such systems depend on the specifics of beam parameters, such as transverse and longitudinal dimensions, charge/pulse and beam pulse format, which are driven by the accelerating technology of choice. While feedback systems with single bunch position monitor resolution below 50 nm and latency <300 ns have been demonstrated in beam test facilities, many advanced collider concepts make use of higher repetition rates, brighter beams and higher accelerating frequencies, and will require better performance, up to 1-2 order of magnitude, demanding aggressive R&D to be able to deliver and maintain the targeted luminosity.

physics.acc-ph↗

arXiv2021

Ultrafast optical melting of trimer superstructure in layered 1T'-TaTe2

Quasi-two-dimensional transition-metal dichalcogenides are a key platform for exploring emergent nanoscale phenomena arising from complex interactions. Access to the underlying degrees-of-freedom on their natural time scales motivates the use of advanced ultrafast probes sensitive to self-organised atomic-scale patterns. Here, we report the first ultrafast investigation of TaTe2, which exhibits unique charge and lattice trimer order characterised by a transition upon cooling from stripe-like chains into a $(3 \times 3)$ superstructure of trimer clusters. Utilising MeV-scale ultrafast electron diffraction, we capture the photo-induced TaTe2 structural dynamics -- exposing a rapid $\approx\!1.4$ ps melting of its low-temperature ordered state followed by recovery via thermalisation into a hot cluster superstructure. Density-functional calculations indicate that the initial quench is triggered by intra-trimer Ta charge transfer which destabilises the clusters, unlike melting of charge density waves in other TaX2 compounds. Our work paves the way for further exploration and ultimately rapid optical and electronic manipulation of trimer superstructures.

cond-mat.mtrl-sci↗

arXiv2021

Resonant phase matching by oblique illumination of a dielectric laser accelerator

In dielectric laser-driven accelerators (DLA), careful tuning of drive-laser wavelength and structure periodicity is typically required in order to hit the resonant condition and match the phase velocity of the accelerating wave to the electron beam velocity. By aggressively detuning (up to 30 mrad) the angle of incidence of the drive laser on a double grating DLA structure, we show that it is possible to recover resonant phase matching and maximize the energy modulation of an externally injected 6 MeV beam in a 800 nm period structure driven using a 780 nm laser. These results show that it is possible to power DLA structures away from their design working point, and excite accelerating fields in the gap with phase profiles that change by a relatively large amount period-to-period. This flexibility is a key feature of DLAs and a critical element in the realization of phase-modulation based ponderomotive focusing to demonstrate MeV energy gain and large capture in a single DLA stage.

physics.acc-ph↗

arXiv2021

Terawatt attosecond X-ray source driven by a plasma accelerator

Plasma accelerators can generate ultra high brightness electron beams which open the door to light sources with smaller physical footprint and properties un-achievable with conventional accelerator technology. In this paper we show that electron beams from Plasma WakeField Accelerators (PWFAs) can generate few-cycle coherent tunable soft X-ray pulses with TW peak power and a duration of tens of attoseconds, an order of magnitude more powerful, shorter and with better stability than state-of-the-art X-ray Free Electron Lasers (XFELs). Such a light source would significantly enhance the ability to experimentally investigate electron dynamics on ultrafast timescales, having broad-ranging impact across multiple scientific fields. Rather than starting from noise as in typical XFELs, the X-rays emission in this approach is driven by coherent radiation from a pre-bunched, near Mega Ampere (MA) current electron beam of attosecond duration. This relaxes the restrictive tolerances which have hindered progress towards utilizing plasma accelerators as coherent X-ray drivers thus far, presenting a new paradigm for advanced-accelerator light source applications.

physics.acc-ph↗

arXiv2021

SHarD: A beam dynamics simulationcode for dielectric laser acceleratorsbased on spatial harmonic field expansion

In order to demonstrate acceleration of electrons to relativistic scales by an on chipdielectric laser accelerator (DLA), a ponderomotive focusing scheme capable of capturingand transporting electrons through nanometer-scale apertures over extended interactionlengths has been proposed. We present a Matlab-based numerical code (SHarD) utilizinga spatial harmonic expansion of the fields within the dielectric structure to simulate theevolution of the beam phase space distribution in this scheme. The code can be usedto optimize key-parameters for the accelerator performance such as the final energy,transverse spot size evolution and total number of electrons accelerated through currentlyfabricated structures. Eventually, the simulation model will be applied to inform thephase mask profile to be added to a pulse front tilt drive laser pulse using a liquid crystalmask in the experimental setup being assembled at UCLA Pegasus Laboratory.

physics.acc-ph↗

arXiv2021

Analytical Scaling Laws for Radiofrequency Based Pulse Compression in Ultrafast Electron Diffraction Beamlines

In this paper, we use an envelope equation-based approach to obtain analytical scaling laws for the shortest pulse length achievable using radiofrequency (RF) based bunch compression. The derived formulas elucidate the dependencies on the electron beam energy and beam charge and reveal how to obtain bunches containing 1 million electrons with single-digit fs pulse lengths; relativistic energies are strongly desirable. The effect of the non-linearities associated with the RF curvature and the beam propagation in a drift is shown to strongly limit the attainability of extreme compression ratios. Using an additional higher frequency RF cavity is proposed as a method to linearize the bunch compression and enable the generation of ultrashort beams in the sub-femtosecond regime.

physics.acc-ph↗