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Piotr Habdas

Publications and source records attributed to Piotr Habdas.

5 recordsLinked to original sources

Local elastic perturbation of colloidal suspensions near the colloidal glass transition

Isolated microscopic magnetic particles are used to induce local perturbations in dense colloidal suspensions by rotating an external magnet. Confocal microscopy enables tracking of both the magnetic probe particle and adjacent colloidal particles. A probe particle moves with a circular trajectory. Knowing the external force and measuring the amplitude and phase of the probe motion allows us to infer the storage and loss moduli of colloidal suspensions at various volume fractions. These measurements are in qualitative agreement with previous results from conventional rheology. To further analyze the system's response, the oscillatory amplitude of colloidal particles is evaluated as a function of distance from the probe, revealing a 1/r decay in amplitude, consistent with a homogeneous viscoelastic material. These observations confirm that continuum descriptions of the colloidal samples are effective down to length scales comparable to the particle diameter.

cond-mat.soft

Stirring supercooled colloidal liquids at the particle scale

We study the decay of tangential velocity profiles with distance from a local disturbance in hard-sphere colloidal suspensions as the colloidal glass transition is approached. The disturbance, generated by a dimer of superparamagnetic particles rotated by an external magnetic field, enables a precise characterization of the system's response through confocal microscopy and tracking of individual particle dynamics. The tangential velocity profiles exhibit nearly exponential decay with distance. As particle density increases toward the colloidal glass transition, the characteristic length scale derived from exponential fits grows. We also observe that the colloidal particles slip against the rotating dimer, with less slip in samples which are closer to the glass transition.

cond-mat.soft

Local elastic response measured near the colloidal glass transition

We examine the response of a dense colloidal suspension to a local force applied by a small magnetic bead. For small forces, we find a linear relationship between the force and the displacement, suggesting the medium is elastic, even though our colloidal samples macroscopically behave as fluids. We interpret this as a measure of the strength of colloidal caging, reflecting the proximity of the samples' volume fractions to the colloidal glass transition. The strain field of the colloidal particles surrounding the magnetic probe appears similar to that of an isotropic homogeneous elastic medium. When the applied force is removed, the strain relaxes as a stretched exponential in time. We introduce a model that suggests this behavior is due to the diffusive relaxation of strain in the colloidal sample.

cond-mat.soft

Particle dynamics in colloidal suspensions above and below the glass-liquid re-entrance transition

We study colloidal particle dynamics of a model glass system using confocal and fluorescence microscopy as the sample evolves from a hard-sphere glass to a liquid with attractive interparticle interactions. The transition from hard-sphere glass to attractive liquid is induced by short-range depletion forces. The development of liquid-like structure is indicated by particle dynamics. We identify particles which exhibit substantial motional events and characterize the transition using the properties of these motional events. As samples enter the attractive liquid region, particle speed during these motional events increases by about one order of magnitude, and the particles move more cooperatively. Interestingly, colloidal particles in the attractive liquid phase do not exhibit significantly larger displacements than particles in the hard-sphere glass.

cond-mat.soft

Video Microscopy of Colloidal Suspensions and Colloidal Crystals

Colloidal suspensions are simple model systems for the study of phase transitions. Video microscopy is capable of directly imaging the structure and dynamics of colloidal suspensions in different phases. Recent results related to crystallization, glasses, and 2D systems complement and extend previous theoretical and experimental studies. Moreover, new techniques allow the details of interactions between individual colloidal particles to be carefully measured. Understanding these details will be crucial for designing novel colloidal phases and new materials, and for manipulating colloidal suspensions for industrial uses.

cond-mat.soft