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Pragati Sharma

Publications and source records attributed to Pragati Sharma.

4 recordsLinked to original sources

Interplay of spin-lattice and electronic coupling far above Neel ordering in 2D antiferromagnetic CrPS4 and its interface manifestation

A short-range spin correlation driven, strongly intercoupled spin-phonon-electronic state far above TN (~38K) is identified in the low dimensional van der Waals antiferromagnet CrPS4. Temperature-dependent Raman spectroscopy reveals spin-phonon coupling persisting up to T*~120K, concomitant with local lattice distortion. The setting of vibronic progression in photoluminescence spectra suggests the strengthening of electron-phonon coupling around T*. Furthermore, both the electrical transport and optoelectronic response also change significantly at T*. The results indicate that spin-phonon coupling above TN in CrPS4 originates from local lattice distortion induced by short range magnetic correlations which in turn enhances the electron-phonon interaction. Furthermore, using a CrPS4/In2Se3 heterostructure, we demonstrate that the anomaly associated with the coupled degrees of freedom in CrPS4 also influences the adjacent In2Se3 layer. The lattice dynamics of In2Se3 is significantly modified across the magnetic anomaly of CrPS4, and the coupled dynamics is observed at T*. These interfacial manifestation opens up new possibilities for achieving correlated multifunctionalities in artificially designed heterostructure.

cond-mat.mtrl-sci

Wavelength-dependent anisotropic light-matter interaction in 2D ferroelectric In2Se3

The anisotropic light-matter interactions in 2D materials have garnered significant attention for their potential to develop futuristic polarization-based optoelectronic devices, such as photodetectors and photo-actuators. In this study, we investigate the polarization-dependent interactions in ferroelectric 3R alpha-In2Se3 using Angle-Resolved Polarized Raman Spectroscopy (ARPRS) with different excitation lasers. Our experimental findings supported by complementary Density Functional Theory calculations demonstrate that the light-matter interactions depend not only on the crystallographic orientation but also on the excitation energy. Scanning transmission electron microscopy (STEM) confirms the highly anisotropic 3R crystal structure of alpha-In2Se3. This anisotropy in crystal structure facilitates significant optical anisotropy, driven by a complex interplay of electron-photon and electron-phonon interactions, which is reflected in the complex nature of the Raman tensor elements. These anisotropy interactions extend to the materials electrical response under light illumination. Remarkably, the anisotropic photo-response can be tuned by both polarization and wavelength of the incident light, making In2Se3 a promising material for advanced polarization-sensitive photodetection applications.

cond-mat.mtrl-sci

Room temperature Mott transistor based on resistive switching in disordered V2O3 films grown on Si

Electric field-induced giant resistive switching triggered by insulator-to-metal transition (IMT) is one of the promising approaches for developing a new class of electronics often referred to as Mottronics. Achieving this resistive switching by minimal external field at room temperature is of paramount research and technological interest. Mott-IMT is often associated with structural modification, which is very important for optoelectronic and actuator applications. Here, we report a giant resistive switching of about 900 % at room temperature in disordered polycrystalline V2O3-Si thin film stabilized at the IMT phase boundary and associated structural transformation under a small electric field. The increase of electron population in the a1g band under the field is responsible for the Mott gap collapse that drives the structural transition. Furthermore, we also fabricated a room temperature Mott-FET with a channel ON/OFF resistive ratio of about 15. This study provides a fundamental mechanism of the Mott-IMT in V2O3 as well as its device applications.

cond-mat.mtrl-sci

Survey on Wireless Information Energy Transfer (WIET) and Related Applications in 6G Internet of NanoThings (IoNT)

This article contains an overview of WIET and the related applications in 6G IoNT. Specifically, to explore the following, we: (i) introduce the 6G network along with the implementation challenges, possible techniques, THz communication and related research challenges, (ii) focus on the WIET architecture, and different energy carrying code words for efficient charging through WIET, (iii) discuss IoNT with techniques proposed for communication of nano-devices, and (iv) conduct a detailed literature review to explore the implicational aspects of the WIET in the 6G nano-network. In addition, we also investigate the expected applications of WIET in the 6G IoNT based devices and discuss the WIET implementation challenges in 6G IoNT for the optimal use of the technology. Lastly, we overview the expected design challenges which may occur during the implementation process, and identify the key research challenges which require timely solutions and which are significant to spur further research in this challenging area. Overall, through this survey, we discuss the possibility to maximize the applications of WIET in 6G IoNT.

cs.NI