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Prasad P. Iyer

Publications and source records attributed to Prasad P. Iyer.

11 recordsLinked to original sources

Pulse-driven photonic transitions and nonreciprocity in space-time modulated metasurfaces

Time-varying photonic systems open new possibilities for controlling light, enabling photonic time crystals, time reflection and refraction, frequency conversion, synthetic gauge fields, optical nonreciprocity, among others. These effects emerge from the dynamic modulation of optical properties, which can mediate photonic transitions between eigenstates of different frequencies and/or wavevectors. To achieve such transitions, conventional approaches rely on periodic modulation schemes that demand ultrafast modulation rates and continuous energy input, posing significant practical challenges at optical frequencies. Here, we demonstrate that periodic-modulation-driven photonic transitions within the radiation continuum can be effectively mimicked using a single-period ultrafast pulse modulation, eliminating the need for sustained continuous modulation. By leveraging dispersion engineering in metasurfaces to tailor the density of states in the radiation continuum, we achieve controlled frequency transitions and theoretically demonstrate strong nonreciprocity for free-space waves as a key application. Our findings may guide future experimental research on time-varying photonics using materials such as transparent conductive oxides and semiconductors, expanding the possibilities for ultrafast and reconfigurable optical technologies. More broadly, our work may establish a practical and energy-efficient framework for dynamic photonic systems, with potential applications ranging from spatio-temporal wavefront manipulation to photonic computing and ultrafast signal processing.

physics.optics↗

Learning interpretable surface elasticity properties from bulk properties

Surface elasticity is central to understanding the mechanics and stability of surfaces and interfaces. It is characterized by quantities such as surface tension, residual surface stress, and surface stiffness, however their analytical expressions are typically difficult to derive from atomistic data, and depend strongly on modeling choices. This work presents a neural network-based equation learner which combines customized activation functions and connection-based pruning to discover parsimonious, closed-form equations for surface elasticity from atomistic simulations. Applying the method to seven face centered cubic (FCC) metals, our equation learner uncovers interpretable equations that describe both low-Miller index and high-Miller index surface properties, capturing long-tail property distributions accurately. The discovered expressions are decoupled into two components: a universal, geometry-driven orientation function, and material-specific baseline coefficients. We find that lower-order properties such as surface tension are fundamentally geometry dependent, while higher-order properties such as surface stress and elasticity show more complex geometry and material dependence. We also relate material dependent coefficients to bulk properties, forming a clear map from bulk material properties to surface elasticity. Overall, this approach demonstrates that interpretable neurosymbolic machine learning can bridge the gap between atomistic simulations and physical laws, enabling the discovery of generalizable structure-property relationships for materials science phenomena such as surface elasticity.

cond-mat.mtrl-sci↗

High-Q, size-independent, and reconfigurable optical antennas via zero-index material dispersion engineering

Enhancing light-matter interactions at the nanoscale is foundational to nanophotonics, with epsilon near zero (ENZ) materials demonstrating significant potential.High-quality (Q) factor resonances maximizing these interactions are typically realized in photonic crystals requiring sub-50 nm precision nanofabrication over large areas, limiting scalability and increasing complexity. Mie resonances offer an alternative but are constrained by low Q factors due to the scarcity of high refractive index materials, necessitating large refractive index changes for effective resonance switching and limiting dynamic reconfigurability. We overcome these limitations by embedding Mie resonators within ENZ media, thereby enhancing Q- factors, mitigating geometric dispersion and fabrication challenges, and maximizing optical reconfigurability. We introduce three resonator-ENZ configurations - voids in AlN, Ge in $SiO_2$, and intrinsic InSb in doped InSb - spanning from low-loss phononic to lossy plasmonic ENZ modes.Using novel epitaxial regrowth techniques, we achieve significant Q-factor improvements over non-embedded resonators. Notably, an air-based Mie resonator embedded in AlN supports resonant Q-factors exceeding 100, with negligible geometric dispersion across sizes from 800 nm to 2,800 nm. Additionally, we demonstrate dynamic reconfigurability of intrinsic InSb resonators by thermally tuning the ENZ wavelength over a 2$μ$m range in the mid-infrared (11-16 $μ$m) wavelength regime. These results showcase the potential of Mie resonators embedded in ENZ media for high-fidelity sensors, thermal emitters, and reconfigurable metasurfaces, bridging theoretical predictions with practical applications, advancing the development of dynamic, high-Q optical devices.

physics.optics↗

AutoSciLab: A Self-Driving Laboratory For Interpretable Scientific Discovery

Advances in robotic control and sensing have propelled the rise of automated scientific laboratories capable of high-throughput experiments. However, automated scientific laboratories are currently limited by human intuition in their ability to efficiently design and interpret experiments in high-dimensional spaces, throttling scientific discovery. We present AutoSciLab, a machine learning framework for driving autonomous scientific experiments, forming a surrogate researcher purposed for scientific discovery in high-dimensional spaces. AutoSciLab autonomously follows the scientific method in four steps: (i) generating high-dimensional experiments (x \in R^D) using a variational autoencoder (ii) selecting optimal experiments by forming hypotheses using active learning (iii) distilling the experimental results to discover relevant low-dimensional latent variables (z \in R^d, with d << D) with a 'directional autoencoder' and (iv) learning a human interpretable equation connecting the discovered latent variables with a quantity of interest (y = f(z)), using a neural network equation learner. We validate the generalizability of AutoSciLab by rediscovering a) the principles of projectile motion and b) the phase transitions within the spin-states of the Ising model (NP-hard problem). Applying our framework to an open-ended nanophotonics challenge, AutoSciLab uncovers a fundamentally novel method for directing incoherent light emission that surpasses the current state-of-the-art (Iyer et al. 2023b, 2020).

cs.LG↗

Self-driving lab discovers principles for steering spontaneous emission

We developed an autonomous experimentation platform to accelerate interpretable scientific discovery in ultrafast nanophotonics, targeting a novel method to steer spontaneous emission from reconfigurable semiconductor metasurfaces. Controlling spontaneous emission is crucial for clean-energy solutions in illumination, thermal radiation engineering, and remote sensing. Despite the potential of reconfigurable semiconductor metasurfaces with embedded sources for spatiotemporal control, achieving arbitrary far-field control remains challenging. Here, we present a self-driving lab (SDL) platform that addresses this challenge by discovering the governing equations for predicting the far-field emission profile from light-emitting metasurfaces. We discover that both the spatial gradient (grating-like) and the curvature (lens-like) of the local refractive index are key factors in steering spontaneous emission. The SDL employs a machine-learning framework comprising: (1) a variational autoencoder for generating complex spatial refractive index profiles, (2) an active learning agent for guiding experiments with real-time closed-loop feedback, and (3) a neural network-based equation learner to uncover structure-property relationships. The SDL demonstrated a four-fold enhancement in peak emission directivity (up to 77%) over a 72° field of view within ~300 experiments. Our findings reveal that combinations of positive gratings and lenses are as effective as negative lenses and gratings for all emission angles, offering a novel strategy for controlling spontaneous emission beyond conventional Fourier optics.

physics.optics↗

Terahertz pulse generation with binary phase control in non-linear InAs metasurface

The effect of terahertz (THz) pulse generation has revolutionized broadband coherent spectroscopy and imaging at THz frequencies. However, THz pulses typically lack spatial structure, whereas structured beams are becoming essential for advanced spectroscopy applications. Non-linear optical metasurfaces with nanoscale THz emitters can provide a solution by defining the beam structure at the generation stage. We develop a non-linear InAs metasurface consisting of nanoscale optical resonators for simultaneous generation and structuring of THz beams. We find that THz pulse generation in the resonators is governed by optical rectification. It is more efficient than in ZnTe crystals, and it allows us to control the pulse polarity and amplitude, offering a platform for realizing binary-phase THz metasurfaces. To illustrate this capability, we demonstrate an InAs metalens, which simultaneously generates and focuses THz pulses. The control of spatiotemporal structure using nanoscale emitters opens doors for THz beam engineering and advanced spectroscopy and imaging applications.

physics.optics↗

Sub picosecond steering of ultrafast incoherent emission from semiconductor metasurfaces

The ability to dynamically steer fs pulses from a monolithically integrated source is a critical milestone for the fields of nanophotonics and ultrafast optics. The nascent field of reconfigurable metasurfaces -- made of optically resonant meta-atoms -- has shown great promise in manipulating light-matter interactions through subwavelength control of the phase, amplitude, and polarization of light. These active metasurfaces arbitrarily transform an incident wavefront using a reconfigurable spatial phase profile and thus have been limited to manipulating coherent external sources. Light emitting metasurfaces obtained through integration of incoherent emitters with meta-atoms, have been used to statically increase the quantum efficiency of the emission through Purcell factor enhancement and control the far-field emission properties of the light to collimate and focus spontaneous emission. Active manipulation of such incoherent light sources, however, remains a challenge as current phase-sensitive approaches used for coherent sources cannot be directly applied. Spatiotemporal control at ultrafast timescales of incoherent light emission could lead to a transformative technological leap allowing low-power light emitting diodes (LEDs) to replace high-power coherent laser sources, enabling holographic LED displays and other key optical transceiver applications including remote-sensing, perception, and high-speed optical communication systems. In this work, we theoretically predict and experimentally demonstrate for the first time, sub-picosecond steering over a 70° range of ultrafast incoherent emission from a light emitting metasurface.

physics.optics↗

Cascaded optical nonlinearities in dielectric metasurfaces

Since the discovery of the laser, optical parametric nonlinearities have been at the core of efficient light conversion sources. Typically, thick transparent crystals or quasi-phase matched waveguides, are utilized in conjunction with phase-matching techniques to select a single parametric process. In recent years, due to the rapid developments in artificially structured materials, optical frequency mixing has been achieved at the nanoscale in subwavelength resonators arrayed as metasurfaces. Phase matching becomes relaxed for these wavelength-scale structures, and all allowed nonlinear processes can, in principle, occur on an equal footing. This could promote harmonic generation via a cascaded (consisting of several frequency mixing steps) process. However, so far, all reported work on dielectric metasurfaces have assumed frequency mixing from a direct (single step) nonlinear process. In this work, we prove the existence of cascaded second-order optical nonlinearities by analyzing the second and third wave mixing from a highly nonlinear metasurface in conjunction with polarization selection rules and crystal symmetries. We find that the third wave mixing signal from a cascaded process can be of comparable strength to that from conventional third harmonic generation, and that surface nonlinearities are the dominant mechanism that contributes to cascaded second order nonlinearities

physics.optics↗

Widely Tunable Optical and Thermal Properties of Dirac Semimetal Cd$_3$As$_2$

In this paper we report a detailed analysis of the temperature-dependent optical properties of epitaxially grown cadmium arsenide (Cd$_3$As$_2$), a newly discovered three-dimensional Dirac semimetal. Dynamic Fermi level tuning -- instigated from Pauli-blocking in the linear Dirac cone -- and varying Drude response, generate large variations in the mid and far-infrared optical properties. We demonstrate thermo-optic shifts larger than those of traditional III-V semiconductors, which we attribute to the obtained large thermal expansion coefficient as revealed by first-principles calculations. Electron scattering rate, plasma frequency edge, Fermi level shift, optical conductivity, and electron effective mass analysis of Cd$_3$As$_2$ thin-films are quantified and discussed in detail. Our ab initio density functional study and experimental analysis of epitaxially grown Cd$_3$As$_2$ promise applications for nanophotonic and nanoelectronic devices, such as reconfigurable metamaterials and metasurfaces, nanoscale thermal emitters, and on-chip directional antennas.

physics.app-ph↗

Unidirectional Luminescence from Quantum Well Metasurfaces

III-Nitride light emitting diodes (LEDs) are the backbone of ubiquitous lighting and display applications. Imparting directional emission is an essential requirement for many LED implementations. Although optical packaging, nano-patterning and surface roughening techniques can enhance LED extraction, directing the emitted light requires bulky optical components. Optical metasurfaces provide precise control over transmitted and reflected waveforms, suggesting a new route for directing light emission. However, it is difficult to adapt metasurface concepts for incoherent light emission, due to the lack of a phase-locking incident wave. In this Letter, we demonstrate metasurface-based design of InGaN/GaN quantum-well structures that generate narrow, unidirectional transmission and emission lobes at arbitrary engineered angles. We show that the directions and polarization of emission differ significantly from transmission, in agreement with an analytical Local Density of Optical States (LDOS) model. The results presented in this Letter open a new paradigm for exploiting metasurface functionality in light emitting devices.

physics.optics↗

Beam engineering for selective and enhanced coupling to multipolar resonances

Multipolar electromagnetic phenomena in sub-wavelength resonators are at the heart of metamaterial science and technology. In this letter, we demonstrate selective and enhanced coupling to specific multipole resonances via beam engineering. We first derive an analytical method for determining the scattering and absorption of spherical nanoparticles (NPs) that depends only on the local electromagnetic field quantities within an inhomogeneous beam. Using this analytical technique, we demonstrate the ability to drastically manipulate the scattering properties of a spherical NP by varying illumination properties and demonstrate the excitation of a longitudinal quadrupole mode that cannot be accessed with conventional illumination. This work enhances the understanding of fundamental light-matter interactions in metamaterials, and lays the foundation for researchers to identify, quantify, and manipulate multipolar light-matter interactions through optical beam engineering.

physics.optics↗