arXiv subjects

Pratim K. Saha

Publications and source records attributed to Pratim K. Saha.

3 recordsLinked to original sources

arXiv2026

Size-Limited Room Temperature Single-Photon Emission from Sidewall-Treated Fractional Dimension InGaN Quantum Dots: Determined by Density-of-States-Corrected Ultrafast Carrier Dynamics and Improved Signal-to-Noise Ratio

Room-temperature single-photon emission (SPE) resulting from a biexciton-exciton cascaded decay is demonstrated for the first time from chemically and photoelectrochemically etched site-controlled In0.14Ga0.86N quantum dots (QDs) embedded in vertical GaN nanowires. Diameter-dependent biexciton-exciton dynamics are analysed to determine the eligibility of QD as a single-photon emitter. The signal-to-noise ratio degrades with increasing QD diameter. Background noise photons pose a bottleneck to achieving SPE. This is also explained from a carrier dynamics perspective. Surface recombination contributes to inhomogeneous broadening at QD diameters larger than 35 nm. Below 35 nm, density-of-states-corrected Auger gradually becomes the principal biexciton-decay route with further reduction in QD diameter, thereby quenching the possibility of thermal broadening and setting a threshold for SPE. Below 9 nm, the Auger recombination rate becomes manyfold of other decay rates, causing multi-photon suppression via single Auger decay to form an exciton. Surface recombination probability of this exciton is minimized while biexciton state filling probability is maximized by reducing sidewall surface states through wet-treatment. These improve biexciton state preparation and enhance the single-photon purity of the exciton towards the exciton Bohr radius (3 nm) regime. Far away from this regime, higher-order autocorrelations to characterize quantum emission involving multi-photon events are discussed. This study establishes a generalized physical framework for predetermining SPE probability as a function of QD surface and geometry down to the exciton Bohr radius regime, with practical implementations. This work shows the pathway to design and develop next-generation semiconductor QDs for high-purity room-temperature SPE.

cond-mat.mes-hall↗

arXiv2026

Gigahertz-clocked Generation of Highly Indistinguishable Photons at C-band Wavelengths

High-performance single-photon sources at telecom C-band wavelentghs are key building blocks for applications in long-distance quantum communication. Here, we report the generation of highly indistinguishable, single photons at a clock-rate of 2.5 GHz. This is achieved by coherently driving the biexciton transition ($T_1^\mathrm{XX}=64(1)\,$ps) of a semiconductor quantum dot embedded in a microcavity with strong asymmetric Purcell enhancement. Employing pulsed two-photon resonant excitation, strong multiphoton suppression with $g^{(2)}(0) < 4\%$ and high two-photon-interference visibility of $V_\mathrm{raw}> 85\%$ is observed. The observed photon indistinguishability is close to the theoretical limit expected for the photonically engineered radiative cascade and matches values obtained at lower repetition rates. Our results show a substantial advancement towards interference-based quantum information protocols at unprecedented data rates in the telecom C-Band.

cond-mat.mes-hall↗

arXiv2026

Highly-Indistinguishable Single-Photons at 1550 nm from a Two-photon Resonantly Excited Purcell-enhanced Quantum Dot

In this work we present a cavity-enhanced InAs/$\mathrm{In_{0.53}Al_{0.23}Ga_{0.24}As}$ quantum dot (QD) single-photon source in the telecom C-band with a record-low biexciton emitter decay time of \SI{67.4(2)}{ps} under resonant two-photon excitation (TPE). We observe strong multiphoton suppression associated with $g^{(2)}_\mathrm{X}(0) = 0.006(1)$ and $g^{(2)}_\mathrm{XX}(0) = 0.007(1)$ for the exciton (X) and biexciton (XX) emission, respectively. Due to a asymmetric Purcell enhancement of the XX-X cascade, the two-photon interference (TPI) visibility of XX photons under $π$-pulse excitation of $V_{\rm{TPI}} = 90(3)\%$ reaches the theoretical limit and clearly exceeds the $\sim60\%$ expected for standard XX-X cascades without photonic engineering. Furthermore, adding a second timed laser pulse coinciding with XX emission energy, we demonstrate stimulated TPE in the telecom C-Band. The result is an improved TPI visibility of the X photons of $V_{\rm{TPI}}=0.69(3)$ compared to TPE with $V_{\rm{TPI}}=0.61(4)$, with both being reduced compared to the theoretical values due to present dephasing effects. The advances presented in this work hold important promises for the implementation of advanced schemes of quantum communication using deterministic quantum light sources.

cond-mat.mes-hall↗