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Preston Went

Publications and source records attributed to Preston Went.

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Apparatus Design for Measuring of the Strain Dependence of the Seebeck Coefficient of Single Crystals

We present the design and construction of an apparatus that measures the Seebeck coefficient of single crystals under in-situ tunable strain at cryogenic temperatures. A home-built three piezostack apparatus applies uni-axial stress to a single crystalline sample and modulates anisotropic strain up to 0.7%. An alternating heater system and cernox sensor thermometry measures the Seebeck coefficient along the uniaxial stress direction. To demonstrate the efficacy of this apparatus, we applied uniaxial stress to detwin single crystals of BaFe2As2 in the orthorhombic phase. The obtained Seebeck coefficient anisotropy is in good agreement with previous measurements using a mechanical clamp.

cond-mat.str-el

Bismuth-doping Alters Structural Phase Transitions in Methylammonium Lead Tribromide Single Crystals

We study the effects of bismuth doping on the crystal structure and phase transitions in single crystals of the perovskite semiconductor methylammonium lead tribromide, MAPbBr3. By measuring temperature-dependent specific heat capacity (Cp) we find that, as Bi doping increases, the phase transition assigned to the cubic to tetragonal phase boundary decreases in temperature. Furthermore, after doping we observe one phase transition between 135 and 155 K, in contrast to two transitions observed in the undoped single crystal. These results appear strikingly similar to previously reported effects of mechanical pressure on perovskite crystal structure. Using X-ray diffraction, we show that the lattice constant decreases as Bi is incorporated into the crystal, as predicted by density functional theory (DFT). We propose that bismuth substitutional doping on the lead site is dominant, resulting in BiPb+ centers which induce compressive chemical strain that alters the crystalline phase transitions.

cond-mat.mtrl-sci

Drastic suppression of superconducting $T_{c}$ by anisotropic strain near a nematic quantum critical point

High temperature superconductivity emerges in the vicinity of competing strongly correlated phases. In the iron-based superconductor $Ba(Fe_{1-x}Co_{x})_{2}As_{2}$, the superconducting state shares the composition-temperature phase diagram with an electronic nematic phase and an antiferromagnetic phase that break the crystalline rotational symmetry. Symmetry considerations suggest that anisotropic strain can enhance these competing phases and thus suppress the superconductivity. Here we study the effect of anisotropic strain on the superconducting transition in single crystals of $Ba(Fe_{1-x}Co_{x})_{2}As_{2}$ through electrical transport, magnetic susceptibility, and x-ray diffraction measurements. We find that in the underdoped and near-optimally doped regions of the phase diagram, the superconducting critical temperature is rapidly suppressed by both compressive and tensile stress, and in the underdoped case this suppression is enough to induce a strain-tuned superconductor to metal quantum phase transition.

cond-mat.supr-con

Evidence for a strain tuned topological phase transition in ZrTe5

A phase transition between topologically distinct insulating phases involves closing and reopening of the bandgap. Close to this topological phase transition, the bulk energy spectrum is characterized by a massive Dirac dispersion, where the mass plays the role of bandgap. Here we report the observation of a non-monotonic strain dependence of resistivity and negative longitudinal magnetoresistance in ZrTe5, which is known to host massive Dirac Fermions in the bulk. This non-monotonic strain dependence is consistent with the closing and reopening of the bandgap at the Brillouin-zone center, indicative of a topological phase transition. This observation suggests that the topological state of ZrTe5 is highly sensitive to uniaxial stress. Our study presents a promising platform for continuous in-situ control of nontrivial topological properties of materials.

cond-mat.str-el