arXiv subjects

Puneet A. Murthy

Publications and source records attributed to Puneet A. Murthy.

11 recordsLinked to original sources

arXiv2026

Photon correlation microscopy of quantum matter

Light and matter share fundamental statistical properties, yet the experimental probes of quantum optics and many-body physics have largely evolved along separate trajectories. While many-body physics explores emergent collective phenomena, quantum optics has refined the measurement of correlations between individual photons. Here, we introduce photon correlation microscopy (PCM) - which bridges the two domains by leveraging correlations of emitted light to probe the correlations in quantum matter at mesoscopic scales. We demonstrate this approach using a one-dimensional (1D) ensemble of dipolar excitons confined at a lateral monolayer MoSe$_2$-WSe$_2$ heterojunction. We use gate-defined potentials to confine the 1D excitons to a mesoscopic lengthscale to enhance the visibility of matter correlations in the emitted photon field. Power-dependent spectroscopy reveals a transition from a compressible to an incompressible phase, signaled by the simultaneous saturation of the emission intensity and energy blueshift, which is supported by numerical simulations. Through this crossover, photon correlation measurements show a striking evolution from bunching at low densities to antibunching at high densities. This constitutes a many-body blockade of photon emission emerging directly from a number-stabilized state, driven by collective dipolar repulsion. Our results establish PCM as a powerful probe of many-body physics through the lens of quantum optics, extensible to a broad class of correlated electronic phases, while pointing toward a route to generating non-classical light through many-body correlations.

cond-mat.mes-hall↗

arXiv2026

Dipolar excitonic quantum wires at atomically sharp lateral interfaces

One-dimensional (1D) quantum systems are a cornerstone of many-body physics. However, their realization in solids has traditionally relied on top-down methods, which are limited by structural disorder and coarse confinement. Here, we demonstrate a fundamentally distinct route: the emergence of 1D quantum matter at the atomically sharp interface between monolayer semiconductors. Using lateral $MoSe_2-WSe_2$ heterostructures, we identify interfacial excitonic quasiparticles that are bound to the crystal junction. Photoluminescence spectroscopy resolves these excitons into a ladder of discrete states, establishing nanoscopic 1D confinement at length scales of 3 nm. These excitons possess exceptional large permanent in-plane electric dipole moments exceeding e x 2 nm, and exhibit micron-scale, highly anisotropic diffusion confined to the interface. Crucially, the lateral geometry enables dynamic, in-situ reconfiguration of the exciton's internal structure. By introducing electrostatic doping, we demonstrate a collapse of the dipole moment and a 20-fold reduction in radiative lifetime. This structural tunability establishes lateral interfaces as a uniquely powerful platform for the 'bottom-up' engineering of 1D quantum matter. By enabling the dynamic tuning of wavefunctions within a single atomic monolayer, this work opens a scalable route toward 1D excitonic circuits and strongly correlated 1D bosonic phases.

cond-mat.mes-hall↗

arXiv2025

Resonantly enhanced superconductivity mediated by spinor condensates

Achieving strong interactions in fermionic many-body systems is a major theme of research in condensed matter physics. It is well-known that interactions between fermions can be mediated through a bosonic medium, such as a phonon bath or Bose-Einstein condensate (BEC). Here we show that such induced attraction can be resonantly enhanced when the bosonic medium is a two-component spinor BEC. The strongest interaction is achieved by tuning the boson-boson scattering to the quantum critical spinodal point of the BEC where the sound velocity vanishes. The fermion pairing gap and the superconducting critical temperature can thus be dramatically enhanced. We propose two experimental realizations of this scenario, with exciton-polariton systems in two-dimensional semiconductors and ultracold atomic Bose-Fermi mixtures.

cond-mat.quant-gas↗

arXiv2024

Fermionization and collective excitations of 1D polariton lattices

We theoretically demonstrate that the hallmarks of correlation and fermionization in a one-dimensional exciton-polaritons gas can be observed with state-of-the-art technology. Our system consists of a chain of excitonic quantum dots coupled to a photonic waveguide, with a low filling of polaritons. We analytically identify the Tonks-Girardeau, Tavis-Cummings and mean-field limits and relate them to different regimes of the excitonic anharmonicity and photonic bandwidth. Using matrix-product states, we numerically calculate the ground-state energies, correlation functions and dynamic structure factor of the system. In particular, the latter has a finite weight in the Lieb-Liniger hole branch, and the density-density correlator displays Friedel-like oscillations for realistic parameters, which reveal the onset of fermionization close to the Tonks-Girardeau regime. Our work encourages future experiments aimed at observing, for the first time and in spite of the moderate excitonic anharmonicity, strongly correlated exciton-polariton physics.

quant-ph↗

arXiv2023

Quantum control of exciton wavefunctions in 2D semiconductors

Excitons -- bound electron-hole pairs -- play a central role in light-matter interaction phenomena, and are crucial for wide-ranging applications from light harvesting and generation to quantum information processing. A long-standing challenge in solid-state optics has been to achieve precise and scalable control over the quantum mechanical state of excitons in semiconductor heterostructures. Here, we demonstrate a technique for creating tailored and tunable potential landscapes for optically active excitons in 2D semiconductors that enables in-situ wavefunction shaping at the nanoscopic lengthscale. Using nanostructured gate electrodes, we create localized electrostatic traps for excitons in diverse geometries such as quantum dots and rings, and arrays thereof. We show independent spectral tuning of multiple spatially separated quantum dots, which allows us to bring them to degeneracy despite material disorder. Owing to the strong light-matter coupling of excitons in 2D semiconductors, we observe unambiguous signatures of confined exciton wavefunctions in optical reflection and photoluminescence measurements. Our work introduces a new approach to engineering exciton dynamics and interactions at the nanometer scale, with implications for novel optoelectronic devices, topological photonics, and many-body quantum nonlinear optics.

cond-mat.mes-hall↗

arXiv2022

Tunable quantum confinement of neutral excitons using electric fields and exciton-charge interactions

Quantum confinement is the discretization of energy when motion of particles is restricted to length scales smaller than their de Broglie wavelength. The experimental realization of this effect has had wide ranging impact in diverse fields of physics and facilitated the development of new technologies. In semiconductor physics, quantum confinement of optically excited quasiparticles, such as excitons or trions, is typically achieved by modulation of material properties - an approach crucially limited by the lack of insitu tunability and scalability of confining potentials. Achieving fully tunable quantum confinement of optical excitations has therefore been an outstanding goal in quantum photonics. Here, we demonstrate electrically controlled quantum confinement of neutral excitons in a gate-defined monolayer p-i-n diode. A combination of dc Stark shift induced by large in-plane fields and a previously unknown confining mechanism based on repulsive interaction between excitons and free charges ensures tight exciton confinement in the narrow neutral region. Quantization of exciton motion manifests in multiple discrete, spectrally narrow, voltage-dependent optical resonances that emerge below the free exciton resonance. Our measurements reveal several unique physical features of these quantum confined excitons, including an in-plane dipolar character, one-dimensional center-of-mass confinement, and strikingly enhanced exciton size in the presence of magnetic fields. Our method provides an experimental route towards creating scalable arrays of identical single photon sources, which will constitute building blocks of strongly correlated photonic systems.

cond-mat.mes-hall↗

arXiv2021

Freeform nanostructuring of hexagonal boron nitride

Hexagonal boron nitride (hBN)-long-known as a thermally stable ceramic-is now available as atomically smooth, single-crystalline flakes, revolutionizing its use in optoelectronics. For nanophotonics, these flakes offer strong nonlinearities, hyperbolic dispersion, and single-photon emission, providing unique properties for optical and quantum-optical applications. For nanoelectronics, their pristine surfaces, chemical stability, and wide bandgap have made them the key substrate, encapsulant, and gate dielectric for two-dimensional electronic devices. However, while exploring these advantages, researchers have been restricted to flat flakes or those patterned with basic slits and holes, severely limiting advanced architectures. If freely varying flake profiles were possible, the hBN structure would present a powerful design parameter to further manipulate the flow of photons, electrons, and excitons in next-generation devices. Here, we demonstrate freeform nanostructuring of hBN by combining thermal scanning-probe lithography and reactive-ion etching to shape flakes with surprising fidelity. We leverage sub-nanometer height control and high spatial resolution to produce previously unattainable flake structures for a broad range of optoelectronic applications. For photonics, we fabricate microelements and show the straightforward transfer and integration of such elements by placing a spherical hBN microlens between two planar mirrors to obtain a stable, high-quality optical microcavity. We then decrease the patterning length scale to introduce Fourier surfaces for electrons, creating sophisticated, high-resolution landscapes in hBN, offering new possibilities for strain and band-structure engineering. These capabilities can advance the discovery and exploitation of emerging phenomena in hyperbolic metamaterials, polaritonics, twistronics, quantum materials, and 2D optoelectronic devices.

physics.optics↗

arXiv2019

Direct imaging of the order parameter of an atomic superfluid using matterwave optics

We propose a method to directly measure the complex phase distribution, superfluid density and velocity field in an ultracold atomic superfluid. The method consists of mapping the momentum distribution of the gas to real space using matterwave focusing, and manipulating the amplitude and phase by means of tailor made optical potentials. This makes it possible to find analogues of well-known techniques in optical microscopy such as Zernike phase contrast imaging, dark field imaging and schlieren imaging. Applying these ideas directly at the level of the macroscopic wavefunction of the superfluid will allow visualization of interesting effects such as phase fluctuations and topological defects, and enable measurements of transport properties such as vorticity.

cond-mat.quant-gas↗

arXiv2018

Anomalous breaking of scale invariance in a two-dimensional Fermi gas

The frequency of the breathing mode of a classical two dimensional Fermi gas in a harmonic confinement is fixed by the scale invariance of the Hamiltonian. Scale invariance is broken on the quantum mechanical level by introducing the two dimensional scattering length as a regulator. This is an example of a quantum anomaly in the field of ultracold atoms and leads to a shift of the frequency of the collective breathing mode of the cloud. In this work, we study this anomalous frequency shift for a two component Fermi gas in the strongly interacting regime. We measure significant shifts away from the scale invariant result that depend strongly on both interactions and temperature. We find qualitative agreement with theoretical calculations at zero temperature.

cond-mat.quant-gas↗

arXiv2018

Quantum scale anomaly and spatial coherence in a 2D Fermi superfluid

Quantum anomalies are violations of classical scaling symmetries caused by quantum fluctuations. Although they appear prominently in quantum field theory to regularize divergent physical quantities, their influence on experimental observables is difficult to discern. Here, we discovered a striking manifestation of a quantum anomaly in the momentum-space dynamics of a 2D Fermi superfluid of ultracold atoms. We measured the position and pair momentum distribution of the superfluid during a breathing mode cycle for different interaction strengths across the BEC-BCS crossover. Whereas the system exhibits self-similar evolution in the weakly interacting BEC and BCS limits, we found a violation in the strongly interacting regime. The signature of scale-invariance breaking is enhanced in the first-order coherence function. In particular, the power-law exponents that characterize long-range phase correlations in the system are modified due to this effect, indicating that the quantum anomaly has a significant influence on the critical properties of 2D superfluids.

cond-mat.quant-gas↗

arXiv2017

High temperature pairing in a strongly interacting two-dimensional Fermi gas

We observe many-body pairing in a two-dimensional gas of ultracold fermionic atoms at temperatures far above the critical temperature for superfluidity. For this, we use spatially resolved radio-frequency spectroscopy to measure pairing energies spanning a wide range of temperatures and interaction strengths. In the strongly interacting regime where the scattering length between fermions is on the same order as the inter-particle spacing, the pairing energy in the normal phase significantly exceeds the intrinsic two-body binding energy of the system and shows a clear dependence on local density. This implies that pairing in this regime is driven by many-body correlations, rather than two-body physics. We find this effect to persist at temperatures close to the Fermi temperature which demonstrates that pairing correlations in strongly interacting two-dimensional fermionic systems are remarkably robust against thermal fluctuations.

cond-mat.quant-gas↗