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Purbasha Ray

Publications and source records attributed to Purbasha Ray.

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Photon correlation microscopy of quantum matter

Light and matter share fundamental statistical properties, yet the experimental probes of quantum optics and many-body physics have largely evolved along separate trajectories. While many-body physics explores emergent collective phenomena, quantum optics has refined the measurement of correlations between individual photons. Here, we introduce photon correlation microscopy (PCM) - which bridges the two domains by leveraging correlations of emitted light to probe the correlations in quantum matter at mesoscopic scales. We demonstrate this approach using a one-dimensional (1D) ensemble of dipolar excitons confined at a lateral monolayer MoSe$_2$-WSe$_2$ heterojunction. We use gate-defined potentials to confine the 1D excitons to a mesoscopic lengthscale to enhance the visibility of matter correlations in the emitted photon field. Power-dependent spectroscopy reveals a transition from a compressible to an incompressible phase, signaled by the simultaneous saturation of the emission intensity and energy blueshift, which is supported by numerical simulations. Through this crossover, photon correlation measurements show a striking evolution from bunching at low densities to antibunching at high densities. This constitutes a many-body blockade of photon emission emerging directly from a number-stabilized state, driven by collective dipolar repulsion. Our results establish PCM as a powerful probe of many-body physics through the lens of quantum optics, extensible to a broad class of correlated electronic phases, while pointing toward a route to generating non-classical light through many-body correlations.

cond-mat.mes-hall

Multi Moire Networks in Engineered Lateral Hetero-Bilayers: Programmable Phononic Reconfiguration and Second Harmonic Generation

Moire engineering in two-dimensional transition metal dichalcogenides enables access to correlated quantum phenomena. Realizing such effects demands simultaneous control over twist angle and material composition to modulate phonons, excitons, and their interactions. However, most studies rely on exfoliated flakes, limiting scalability and systematic exploration. Here, we demonstrate a scalable multi-moire network by vertically stacking CVD-grown monolayer lateral heterostructures. Signatures of moire non-rigidity, including phonon frequency softening, linewidth broadening, and strain localization, are attributed to two lattice relaxation modes; rotational reconstruction and volumetric dilation. Micro-angle-resolved photoemission spectroscopy reveals that interfacial orbital interactions modulate interlayer coupling. At aligned angles, molybdenum diselenides exhibit reduced valley polarization and Davydov splitting, indicating strain-induced symmetry breaking and chiral phonon effects. Notably, SHG modulation was obderved with variation in twist angle due to lower coherence and band-offset-driven phase delay. First-principles calculations support these findings. This work provides a route to programmable, scalable multi-moire platforms for opto-straintronics, quantum sensing, and on-chip photonics.

cond-mat.mes-hall