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Q. Huang

Publications and source records attributed to Q. Huang.

At least 37 records · Page 2Linked to original sources

Survival of itinerant excitations and quantum spin state transitions in YbMgGaO$_4$ with chemical disorder

A recent focus of quantum spin liquid (QSL) studies is how disorder/randomness in a QSL candidate affects its true magnetic ground state. The ultimate question is whether the QSL survives disorder or the disorder leads to a "spin-liquid-like" state, such as the proposed random-singlet (RS) state. Since disorder is a standard feature of most QSL candidates, this question represents a major challenge for QSL candidates. YbMgGaO$_4$, a triangular lattice antiferromagnet with effective spin-1/2 Yb$^{3+}$ ions, is an ideal system to address this question, since it shows no long-range magnetic ordering with Mg/Ga site disorder. Despite the intensive study, it remains unresolved as to whether YbMgGaO$_4$ is a QSL or in the RS state. Here, through ultralow-temperature thermal conductivity and magnetic torque measurements, plus specific heat and DC magnetization data, we observed a residual $κ_0/T$ term and series of quantum spin state transitions in the zero temperature limit for YbMgGaO$_4$. These observations strongly suggest that a QSL state with itinerant excitations and quantum spin fluctuations survives disorder in YbMgGaO$_4$.

cond-mat.str-el↗

Evolution of magnetic-field-induced ordering in the layered structure quantum Heisenberg triangular-lattice antiferromagnet Ba$_3$CoSb$_2$O$_9$

Quantum fluctuations in the effective spin one-half layered structure triangular-lattice quantum Heisenberg antiferromagnet Ba$_3$CoSb$_2$O$_9$ lift the classical degeneracy of the antiferromagnetic ground state in magnetic field, producing a series of novel spin structures for magnetic fields applied within the crystallographic ab plane. Theoretically unresolved, however, are the effects of interlayer antferromagnetic coupling and transverse magnetic fields on the ground states of this system. To address these issues, we have used specific heat, neutron diffraction, thermal conductivity, and magnetic torque measurements to map out the phase diagram as a function of magnetic field intensity and orientation relative to the crystallographic ab plane. For H parallel to the ab plane, we have discovered an additional, previously unreported magnetic-field-induced phase transition at low temperature and an unexpected tetracritical point in the high field phase diagram, which - coupled with the apparent second-order nature of the phase transitions - eliminates several theoretically proposed spin structures for the high field phases. Our calorimetric measurements as a function of magnetic field orientation are in general agreement with theory for field-orientation angles close to plane parallel but diverge at angles near plane perpendicular; a predicted convergence of two phase boundaries at finite angle and a corresponding change in the order of the field induced phase transition is not observed experimentally. Our results emphasize the role of interlayer coupling in selecting and stabilizing field-induced phases, provide new guidance into the nature of the magnetic order in each phase, and reveal the need for new physics to account for the nature of magnetic ordering in this archetypal 2D spin one-half triangular lattice quantum Heisenberg antiferromagnet.

cond-mat.str-el↗

Differential cross sections for Λ(1520) using photoproduction at CLAS

The reaction $γp \rightarrow K^{+} Λ(1520)$ using photoproduction data from the CLAS $g12$ experiment at Jefferson Lab is studied. The decay of $Λ(1520)$ into two exclusive channels, $Σ^{+}π^{-}$ and $Σ^{-}π^{+}$, is studied from the detected $K^{+}$, $π^{+}$, and $π^{-}$ particles. A good agreement is established for the $Λ(1520)$ differential cross sections with the previous CLAS measurements. The differential cross sections as a function of CM angle are extended to higher photon energies. Newly added are the differential cross sections as a function of invariant 4-momentum transfer $t$, which is the natural variable to use for a theoretical model based on a Regge-exchange reaction mechanism. No new $N^*$ resonances decaying into the $K^+Λ(1520)$ final state are found.

hep-ex↗

Beam spin asymmetry in semi-inclusive electroproduction of a hadron pair

A first measurement of the longitudinal beam spin asymmetry ALU in the semi-inclusive electroproduction of pairs of charged pions is reported. ALU is a higher-twist observable and offers the cleanest access to the nucleon twist-3 parton distribution function e(x). Data have been collected in the Hall-B at Jefferson Lab by impinging a 5.498 GeV electron beam on a liquid-hydrogen target, and reconstructing the scattered electron and the pion pair with the CLAS detector. One-dimensional projections of the sin(phiR) moments of ALU are extracted for the kinematic variables of interest in the valence quark region. The understanding of di-hadron production is essential for the interpretation of observables in single hadron production in semi-inclusive DIS, and pioneering measurements of single spin asymmetries in di-hadron production open a new avenue in studies of QCD dynamics.

hep-ex↗

Orbital competition of Mn3+ and V3+ ions in Mn1+xV2-xO4

The structure and magnetic properties of Mn1+xV2-xO4 (0 a) phase transition was observed. For x > 0.3, the system maintained the tetragonal lattice. The collinear and noncollinear magnetic transition was also observed for all compositions. To reveal the dynamics of the ground state, first principle simulation was applied to not only analyze the orbital effects of Mn2+, Mn3+, and V3+ ions, but also the related exchange energies.

cond-mat.str-el↗

Possible itinerant excitations and quantum spin state transitions in the effective spin-1/2 triangular-lattice antiferromagnet Na$_2$BaCo(PO$_4$)$_2$

The most fascinating feature of certain two-dimensional (2D) gapless quantum spin liquid (QSL) is that their spinon excitations behave like the fermionic carriers of a paramagnetic metal. The spinon Fermi surface is then expected to produce a linear increase of the thermal conductivity with temperature that should manifest via a residual value ($κ_0/T$) in the zero-temperature limit. However, this linear in T behavior has been reported for very few QSL candidates. Here, we studied the ultralow-temperature thermal conductivity of an effective spin-1/2 triangular QSL candidate Na$_2$BaCo(PO$_4$)$_2$, which has an antiferromagnetic order at very low temperature ($T_N \sim$ 148 mK), and observed a finite $κ_0/T$ extrapolated from the data above $T_N$. Moreover, while approaching zero temperature, it exhibits series of quantum spin state transitions with applied field along the $c$ axis. These observations indicate that Na$_2$BaCo(PO$_4$)$_2$ possibly behaves as a gapless QSL with itinerant spin excitations above $T_N$ and its strong quantum spin fluctuations persist below $T_N$.

cond-mat.str-el↗

Unraveling the Topological Phase of ZrTe$_5$ via Magneto-infrared Spectroscopy

For materials near the phase boundary between weak and strong topological insulators (TIs), their band topology depends on the band alignment, with the inverted (normal) band corresponding to the strong (weak) TI phase. Here, taking the anisotropic transition-metal pentatelluride ZrTe$_5$ as an example, we show that the band inversion manifests itself as a second extremum (band gap) in the layer stacking direction, which can be probed experimentally via magneto-infrared spectroscopy. Specifically, we find that the band anisotropy of ZrTe$_5$ features a slow dispersion in the layer stacking direction, along with an additional set of optical transitions from a band gap away from the Brillouin zone center. Our work identifies ZrTe5 as a strong TI at liquid helium temperature and provides a new perspective in determining band inversion in layered topological materials.

cond-mat.mes-hall↗

Comprehensive Control of Metamagnetic Transition of Antiferromagnetic Mott Insulator Sr2IrO4 by in-situ Anisotropic Strain

Metamagnetism in antiferromagnets exhibits distinct critical behaviors and dynamics when invoking spin reversal and rotation. Here we show a 0.05% anisotropic strain suffices to in-situ modulate the metamagnetic critical field of the Mott insulator Sr2IrO4 by over 50%, enabling electrical switching of the transition. Resonant x-ray scattering and model simulation reveal that the transition is completely tuned from the spin-flop to spin-flip type as the strain introduces C4-symmetry-breaking magnetic anisotropy. Simultaneous transport study indicates the metamagnetic responses are reflected in the large elasto- and magnetoconductance, highlighting the active charge degree of freedom in the spin-orbit-coupled Mott state and its potential for spin-electronics.

cond-mat.str-el↗

Magnetoelectric effect arising from a field-induced pseudo Jahn-Teller distortion in a rare earth magnet

Magnetoelectric materials are attractive for several applications, including actuators, switches, and magnetic field sensors. Typical mechanisms for achieving a strong magnetoelectric coupling are rooted in transition metal magnetism. In sharp contrast, here we identify CsEr(MoO4)2 as a magnetoelectric material without magnetic transition metal ions, thus ensuring that the Er ions play a key role in achieving this interesting property. Our detailed study includes measurements of the structural, magnetic, and electric properties of this material. Bulk characterization and neutron powder diffraction show no evidence for structural phase transitions down to 0.3 K and therefore CsEr(MoO4)2 maintains the room temperature P2/c space group over a wide temperature range without external magnetic field. These same measurements also identify collinear antiferromagnetic ordering of the Er3+ moments below TN = 0.87 K. Complementary dielectric constant and pyroelectric current measurements reveal that a ferroelectric phase (P ~ 0.5 nC/cm2) emerges when applying a modest external magnetic field, which indicates that this material has a strong magnetoelectric coupling. We argue that the magnetoelectric coupling in this system arises from a pseudo Jahn-Teller distortion induced by the magnetic field.

cond-mat.mtrl-sci↗

Absence of long-range order in an $XY$ pyrochlore antiferromagnet Er$_2$AlSbO$_7$

Rare-earth pyrochlores are known to exhibit exotic magnetic phenomena. We report a study of crystal growth and characterizations of a new rare-earth compound Er$_2$AlSbO$_7$, in which Al$^{3+}$ and Sb$^{5+}$ ions share the same positions with a random distribution. The magnetism are studied by magnetic susceptibility, specific heat and thermal conductivity measurements at low temperatures down to several tens of milli-kelvin. Different from the other reported Er-based pyrochlores exhibiting distinct magnetically ordered states, a spin-freezing transition is detected in Er$_2$AlSbO$_7$ below 0.37 K, which is primarily ascribed to the inherent structural disorder. A cluster spin-glass state is proposed in view of the frequency dependence of the peak position in the ac susceptibility. In addition, the temperature and field dependence of thermal conductivity indicates rather strong spin fluctuations which is probably due to the phase competition.

cond-mat.mtrl-sci↗

Design, operation and performance of the PAON4 prototype transit interferometer

PAON4 is an L-band (1250-1500 MHz) small interferometer operating in transit mode deployed at the Nançay observatory in France, designed as a prototype instrument for Intensity Mapping. It features four 5~meter diameter dishes in a compact triangular configuration, with a total geometric collecting area of $\sim75 \mathrm{m^2}$, and equipped with dual polarization receivers. A total of 36 visibilities are computed from the 8 independent RF signals by the software correlator over the full 250~MHz RF band. The array operates in transit mode, with the dishes pointed toward a fixed declination, while the sky drifts across the instrument. Sky maps for each frequency channel are then reconstructed by combining the time-dependent visibilities from the different baselines observed at different declinations. This paper presents an overview of the PAON4 instrument design and goals, as a prototype for dish arrays to map the Large Scale Structure in radio, using intensity mapping of the atomic hydrogen $21~\mathrm{cm}$ line. We operated PAON4 over several years and use data from observations in different periods to assess the array performance. We present preliminary analysis of a large fraction of this data and discuss crucial issues for this type of instrument, such as the calibration strategy, instrument response stability, and noise behaviour.

astro-ph.IM↗

Ba8MnNb6O24: a model two-dimensional spin-5/2 triangular lattice antiferromagnet

We successfully synthesized and characterized the triangular lattice anitferromagnet Ba$_8$MnNb$_6$O$_{24}$, which comprises equilateral spin-5/2 Mn$^{2+}$ triangular layers separated by six non-magnetic Nb$^{5+}$ layers. The detailed susceptibility, specific heat, elastic and inelastic neutron scattering measurements, and spin wave theory simulation on this system reveal that it has a 120 degree ordering ground state below T$_N$ = 1.45 K with in-plane nearest-neighbor exchange interaction ~0.11 meV. While the large separation 18.9 A between magnetic layers makes the inter-layer exchange interaction virtually zero, our results suggest that a weak easy-plane anisotropy is the driving force for the k$_m$ = (1/3 1/3 0) magnetic ordering. The magnetic properties of Ba$_8$MnNb$_6$O$_{24}$, along with its classical excitation spectra, contrast with the related triple perovskite Ba$_3$MnNb$_2$O$_9$, which shows easy-axis anisotropy, and the iso-structural compound Ba$_8$CoNb$_6$O$_{24}$, in which the effective spin-1/2 Co$^{2+}$ spins do not order down to 60 mK and in which the spin dynamics shows sign of strong quantum effects.

cond-mat.mtrl-sci↗

Tin+1Cn MXene with fully saturated and thermally stable Cl terminations

MXenes are a rapidly growing family of 2D materials that exhibit a highly versatile structure and composition, allowing for significant tuning of the material properties. These properties are, however, ultimately limited by the surface terminations, which are typically a mixture of species, including F and O that are inherent to the MXene processing. Other and robust terminations are lacking. Here, we apply high-resolution scanning transmission electron microscopy (STEM), corresponding image simulations and first-principles calculations to investigate the surface terminations on MXenes synthesized from MAX phases through Lewis acidic melts. The results show that atomic Cl terminates the synthesized MXenes, with mere residual presence of other termination species. Furthermore, in situ STEM-electron energy loss spectroscopy (EELS) heating experiments show that the Cl terminations are stable up to 750 °C. Thus, we present an attractive new termination that widely expands the MXenes functionalization space and enable new applications.

cond-mat.mtrl-sci↗

Low-carrier density and fragile magnetism in a Kondo lattice system

Kondo-based semimetals and semiconductors are of extensive current interest as a viable platform for strongly correlated states. It is thus important to understand the routes towards such dilute-carrier correlated states. One established pathway is through Kondo effect in metallic non-magnetic analogues. Here we advance a new mechanism, through which Kondo-based semimetals develop out of conduction electrons with a low carrier-density in the presence of an even number of rare-earth sites. We demonstrate this effect by studying the Kondo material Yb3Ir4Ge13 along with its closed-f-shell counterpart, Lu3Ir4Ge13. Through magnetotransport, optical conductivity and thermodynamic measurements, we establish that the correlated semimetallic state of Yb3Ir4Ge13 below its Kondo temperature originates from the Kondo effect of a low carrier conduction-electron background. In addition, it displays fragile magnetism at very low temperatures, which, in turn, can be tuned to a non Fermi liquid regime through Lu-for-Yb substitution. These findings are connected with recent theoretical studies in simplified models. Our results open an entirely new venue to explore the strong correlation physics in a semimetallic environment.

cond-mat.str-el↗

Magnetic Properties of the low dimensional BaM$_2$Si$_2$O$_7$(M= Cu, Co, Mn) system

We performed susceptibility, magnetization, specific heat, and single crystal neutron diffraction measurements on single crystalline BaMn$_2$Si$_2$O$_7$. Based on the results, we revisited its spin structure with a more accurate solution and constructed a magnetic phase diagram with applied field along the $b$-axis, which contains a spin flop transition around 6 T. We also used susceptibility, magnetization, and specific heat results confirmed the ferrimagnetic-like magnetism in polycrystalline BaCo$_2$Si$_2$O$_7$. Furthermore, we performed LSDA + U calculations for the BaM$_2$Si$_2$O$_7$ (M = Cu, Co, and Mn) system. Our discussions based on the comparison among the obtained magnetic exchange interactions suggest the different structures and electronic configurations are the reasons for the different magnetic properties among the system members.

cond-mat.str-el↗

Impact of Building-Level Motor Protection on Power System Transient Behaviors

Protection strategies for transmission and distribution systems have been extensively investigated to facilitate better coordination of physical protection devices. A diverse range of functional motors with dedicated protection schemes are being used more and more in commercial, residential, and industrial buildings. This paper focuses on simulating several of the most popular protection schemes using the ElectroMagnetic Transient Program (EMTP) model for three-phase and single-phase induction motors in existing commercial buildings connected to typical distribution feeders. To investigate the behaviors of single-phase motors stalling, the actions of motor protection and reconnections, and the impacts of device-level protection on system-level dynamics, we imposed voltage depressions at the head of a feeder fully loaded with functional induction motors. Several distribution feeders are represented in a standard IEEE 39-bus transmission system to simulate fault-induced delayed voltage recovery (FIDVR) and explore mitigation strategies by optimally configuring the building-level motor protection settings.

eess.SP↗

Anomalous metamagnetism in the low carrier density Kondo lattice YbRh3Si7

We report complex metamagnetic transitions in single crystals of the new low carrier Kondo antiferromagnet YbRh3Si7. Electrical transport, magnetization, and specific heat measurements reveal antiferromagnetic order at T_N = 7.5 K. Neutron diffraction measurements show that the magnetic ground state of YbRh3Si7 is a collinear antiferromagnet where the moments are aligned in the ab plane. With such an ordered state, no metamagnetic transitions are expected when a magnetic field is applied along the c axis. It is therefore surprising that high field magnetization, torque, and resistivity measurements with H||c reveal two metamagnetic transitions at mu_0H_1 = 6.7 T and mu_0H_2 = 21 T. When the field is tilted away from the c axis, towards the ab plane, both metamagnetic transitions are shifted to higher fields. The first metamagnetic transition leads to an abrupt increase in the electrical resistivity, while the second transition is accompanied by a dramatic reduction in the electrical resistivity. Thus, the magnetic and electronic degrees of freedom in YbRh3Si7 are strongly coupled. We discuss the origin of the anomalous metamagnetism and conclude that it is related to competition between crystal electric field anisotropy and anisotropic exchange interactions.

cond-mat.str-el↗

Probing Anomalous Inelastic Scattering in Spin-ice Ho$_2$Ti$_2$O$_7$ through Resonant Raman Spectroscopy

We report on a study of the inelastic scattering properties of (001) and (111) Ho$_2$Ti$_2$O$_7$ single crystals at room temperature. Structural and compositional analysis along with absorption measurement confirms single crystalline phase of all samples. Room temperature polarized Raman measurements were performed on crystals in non-resonant and two different resonant conditions by using six different laser excitation lines. Lorentzian model fitting analysis is performed on all measured spectra in order to identify the difference in the Raman scattering cross-section in resonant and non-resonant conditions. Variations in the fitting parameters on account of different polarization configurations and crystallographic orientations has helped identifying their symmetry if present. Several possible scattering pathways are discussed in order to qualitatively explain the anomalous scattering results in Ho$_2$Ti$_2$O$_7$

cond-mat.str-el↗