arXiv subjects

Q. Wu

Publications and source records attributed to Q. Wu.

At least 55 records · Page 3Linked to original sources

arXiv2021

Unconventional charge density wave and photoinduced lattice symmetry change in Kagome Metal CsV$_3$Sb$_5$ probed by time-resolved spectroscopy

Recently, kagome lattice metal AV$_3$Sb$_5$ (A = K, Rb, Cs) family has received wide attention due to its presence of superconductivity, charge density wave (CDW) and peculiar properties from topological nontrivial electronic structure. With time-resolved pump-probe spectroscopy, we show that the excited quasiparticle relaxation dynamics can be explained by formation of energy gap below the phase transition being similar to a usual second-order CDW condensate, by contrast, the structure change is predominantly first order phase transition. Furthermore, no CDW amplitude mode is identified in the ordered phase. The results suggest that the CDW order is very different from the traditional CDW condensate. We also find that weak pump pulse can non-thermally melt the CDW order and drive the sample into its high temperature phase, revealing the fact that the difference in lattice potential between those phases is small.

cond-mat.supr-con↗

arXiv2021

Prediction of anomalous LA-TA splitting in electrides

Electrides are an emerging class of materials with excess electrons localized in interstices and acting as anionic interstitial quasi-atoms (ISQs). The spatial ion-electron separation means that electrides can be treated physically as ionic crystals, and this unusual behavior leads to extraordinary physical and chemical phenomena. Here, a completely different effect in electrides is predicted. By recognizing the long-range Coulomb interactions between matrix atoms and ISQs that are unique in electrides, a nonanalytic correction to the forces exerted on matrix atoms is proposed. This correction gives rise to an LA-TA splitting in the acoustic branch of lattice phonons near the zone center, similar to the well-known LO-TO splitting in the phonon spectra of ionic compounds. The factors that govern this splitting are investigated, with isotropic fcc-Li and anisotropic hP4-Na as the typical examples. It is found that not all electrides can induce a detectable splitting, and criteria are given for this type of splitting. The present prediction unveils the rich phenomena in electrides and could lead to unprecedented applications.

cond-mat.mtrl-sci↗

arXiv2021

Interplay of anionic quasi-atom and interstitial point defects in electrides: abnormal interstice occupation and colossal charge state of point defects in dense FCC-lithium

Electrides are an emerging class of materials with highly-localized electrons in the interstices of a crystal that behave as anions. The presence of these unusual interstitial quasi-atom (ISQ) electrons leads to interesting physical and chemical properties, and wide potential applications for this new class of materials. Crystal defects often have a crucial influence on the properties of materials. Introducing impurities has been proved to be an effective approach to improve the properties of a material and to expand its applications. However, the interactions between the anionic ISQs and the crystal defects in electrides are as yet unknown. Here, dense FCC-Li was employed as an archetype to explore the interplay between anionic ISQs and interstitial impurity atoms in this electride. This work reveals a strong coupling among the interstitial impurity atoms, the ISQs, and the matrix Li atoms near to the defects. This complex interplay and interaction mainly manifest as the unexpected tetrahedral interstitial occupation of impurity atoms and the enhancement of electron localization in the interstices. Moreover, the Be impurity occupying the octahedral interstice shows the highest negative charge state (Be8-) discovered thus far. These results demonstrate the rich chemistry and physics of this emerging material, and provide a new basis for enriching their variants for a wide range of applications.

cond-mat.mtrl-sci↗

arXiv2021

Multi-Objective Resource Allocation for IRS-Aided SWIPT

In this letter, we study the resource allocation for a multiuser intelligent reflecting surface (IRS)-aided simultaneous wireless information and power transfer (SWIPT) system. Specifically, a multi-antenna base station (BS) transmits energy and information signals simultaneously to multiple energy harvesting receivers (EHRs) and information decoding receivers (IDRs) assisted by an IRS. Under this setup, we introduce a multi-objective optimization (MOOP) framework to investigate the fundamental trade-off between the data sum-rate maximization and the total harvested energy maximization, by jointly optimizing the energy/information beamforming vectors at the BS and the phase shifts at the IRS. This MOOP problem is first converted to a single-objective optimization problem (SOOP) via the $ε$-constraint method and then solved by majorization minimization (MM) and inner approximation (IA) techniques. Simulation results unveil a non-trivial trade-off between the considered competing objectives, as well as the superior performance of the proposed scheme as compared to various baseline schemes.

cs.IT↗

arXiv2021

A parsec-scale faint jet in the nearby changing-look Seyfert galaxy Mrk 590

Broad Balmer emission lines in active galactic nuclei (AGN) may display dramatic changes in amplitude, even disappearance and re-appearance in some sources. As a nearby galaxy at a redshift of z = 0.0264, Mrk 590 suffered such a cycle of Seyfert type changes between 2006 and 2017. Over the last fifty years, Mrk 590 also underwent a powerful continuum outburst and a slow fading from X-rays to radio wavelengths with a peak bolometric luminosity reaching about ten per cent of the Eddington luminosity. To track its past accretion and ejection activity, we performed very long baseline interferometry (VLBI) observations with the European VLBI Network (EVN) at 1.6 GHz in 2015. The EVN observations reveal a faint (~1.7 mJy) radio jet extending up to ~2.8 mas (projected scale ~1.4 pc) toward north, and probably resulting from the very intensive AGN activity. To date, such a parsec-scale jet is rarely seen in the known changing-look AGN. The finding of the faint jet provides further strong support for variable accretion as the origin of the type changes in Mrk 590.

astro-ph.HE↗

arXiv2020

Neutron-rich calcium isotopes within realistic Gamow shell model calculations with continuum coupling

Based on the realistic nuclear force of the high-precision CD-Bonn potential, we have performed comprehensive calculations for neutron-rich calcium isotopes using the Gamow shell model (GSM) which includes resonance and continuum. The realistic GSM calculations produce well binding energies, one- and two-neutron separation energies, predicting that $^{57}$Ca is the heaviest bound odd isotope and $^{70}$Ca is the dripline nucleus. Resonant states are predicted, which provides useful information for future experiments on particle emissions in neutron-rich calcium isotopes. Shell evolutions in the calcium chain around neutron numbers \textit{N} = 32, 34 and 40 are understood by calculating effective single-particle energies, the excitation energies of the first $2^+$ states and two-neutron separation energies. The calculations support shell closures at $^{52}$Ca (\textit{N} = 32) and $^{54}$Ca (\textit{N} = 34) but show a weakening of shell closure at $^{60}$Ca (\textit{N} = 40). The possible shell closure at $^{70}$Ca (\textit{N} = 50) is predicted.

nucl-th↗

arXiv2020

Understanding FRB 200428 in the synchrotron maser shock model: consistency and possible challenge

Recently, the discovery of Galactic FRB 200428 associated with a X-ray burst (XRB) of SGR 1935+2154 has built a bridge between FRBs and magnetar activities. In this paper, we assume that the XRB occurs in the magnetar magnetosphere. We show that the observational properties of FRB 200428 and the associated XRB are consistent with the predictions of synchrotron maser emission at ultrarelativistic magnetized shocks, including radiation efficiency, similar energy occurrence frequency distributions, and simultaneous arrive times. It requires that the upstream medium is a mildly relativistic baryonic shell ejected by a previous flare. The energy injection by flares responsible for the radio bursts will produce a magnetar wind nebula, which has been used to explain the persistent radio source associated FRB 121102. We find that the radio continuum around SGR 1935+2154 can be well understood in the magnetar wind nebula model, by assuming the same energy injection rate $\dot{E} \propto t^{-1.37}$ as FRB 121102. The required baryonic mass is also estimated form the observations of FRB 121102 by GBT and FAST. By assuming the same radiation efficiency $η\sim 10^{-5}$, the total baryonic mass ejected from the central magnetar is about 0.005 solar mass. This value is much larger than the typical mass of a magnetar outer crust, but is comparable to the total mass of a magnetar crust.

astro-ph.HE↗

arXiv2020

A New Method to Measure Hubble Parameter $H(z)$ using Fast Radio Bursts

The Hubble parameter $H(z)$ is directly related to the expansion of our Universe. It can be used to study dark energy and constrain cosmology models. In this paper, we propose that $H(z)$ can be measured using fast radio bursts (FRBs) with redshift measurements. We use dispersion measures contributed by the intergalactic medium, which is related to $H(z)$, to measure Hubble parameter. We find that 500 mocked FRBs with dispersion measures and redshift information can accurately measure Hubble parameters using Monte Carlo simulation. The maximum deviation of $H(z)$ from standard $Λ$CDM model is about 6\% at redshift $z= 2.4$. We also test our method using Monte Carlo simulation. Kolmogorov-Smirnov (K-S) test is used to check the simulation. The $p$-value of K-S test is 0.23, which confirms internal consistency of the simulation. In future, more localizations of FRBs make it as an attractive cosmological probe.

astro-ph.CO↗

arXiv2020

Orbital localization error of density functional theory in shear properties of vanadium and niobium

It is believed that the density functional theory (DFT) describes most elements with s, p and d orbitals very well, except some materials that having strongly localized and correlated valence electrons. In this work, we find that the widely employed exchange-correlation (xc) functionals, including LDA, GGA and meta-GGA, underestimate the shear modulus and phase stability of V and Nb greatly. The advanced hybrid functional that is usually better for correlated system, on the other hand, completely fails in these two simple metals. This striking failure is revealed due to the orbital localization error in GGA, which is further deteriorated by hybrid functionals. This observation is corroborated by a similar failure of DFT+U and van der Waals functionals when applied to V and Nb. To remedy this problem, an semi-empirical approach of DFT+J is proposed which can delocalize electrons by facilitating the on-site exchange. Furthermore, it is observed that including density derivatives slightly improves the performance of the semi-local functionals, with meta-GGA outperforms GGA, and the latter is better than LDA. This discovery indicates the possibility and necessity to include higher-order density derivatives beyond the Laplacian level for the purpose to remove the orbital localization error (mainly from d orbitals) and delocalization error (mainly from s and p orbitals) completely in V and Nb, so that to achieve a better description of their electronic structures. The same strategy can be applied to other d electron system and f electron system.

cond-mat.mtrl-sci↗

arXiv2020

Thermodynamic anomalies and three distinct liquid-liquid transitions in warm dense liquid hydrogen

The properties of hydrogen at high pressure have wide implications in astrophysics and high-pressure physics. Its phase change in the liquid is variously described as a metallization, H2-dissociation, density discontinuity or plasma phase transition. It has been tacitly assumed that these phenomena coincide at a first-order liquid-liquid transition (LLT). In this work, the relevant pressure-temperature conditions are thoroughly explored with first-principles molecular dynamics. We show there is a large dependency on exchange-correlation functional and significant finite size effects. We use hysteresis in a number of measurable quantities to demonstrate a first-order transition up to a critical point, above which molecular and atomic liquids are indistinguishable. At higher temperature beyond the critical point, H2-dissociation becomes a smooth cross-over in the supercritical region that can be modelled by a pseudo-transition, where the H2-2H transformation is localized and does not cause a density discontinuity at metallization. Thermodynamic anomalies and counter-intuitive transport behavior of protons are also discovered even far beyond the critical point, making this dissociative transition highly relevant to the interior dynamics of Jovian planets. Below the critical point, simulation also reveals a dynamic H2-2H chemical equilibrium with rapid interconversion, showing that H2 and H are miscible. The predicted critical temperature lies well below the ionization temperature. Our calculations unequivocally demonstrate that there are three distinct regimes in the liquid-liquid transition of warm dense hydrogen.

cond-mat.mtrl-sci↗

arXiv2020

Nuclear multipole responses from chiral effective field theory interaction

We probe nuclear multipole resonances in the framework of the random-phase approximation by using the interaction obtained from the chiral effective field theory. The three-nucleon force is included in a form of the in-medium two-nucleon interaction which was derived from the chiral three-nucleon force. The isoscalar monopole, isoscalar dipole, isovector dipole and isoscalar quadrupole resonances of the closed-shell $^{56,68,78}$Ni have been investigated. The calculations reasonably reproduce the experimental multipole resonances of $^{56,68}$Ni, and well describe the pygmy dipole resonance and dipole polarizability measured in $^{68}$Ni. The multipole resonances of $^{78}$Ni, including pygmy dipole resonance and dipole polarizability, are predicted. The detailed effects of the tensor force and three-body force are analyzed by dissecting the chiral interaction. We find that in general the tensor force effect on electric giant resonances is not as significant as the effect from the three-body force, although the tensor force provides more than half of the binding energy. The effect from three-body force is strong in light nuclei. Particularly, three-body force is crucial for the formation of the pygmy resonance in calculations.

nucl-th↗

arXiv2020

An {\it ab-initio} Gamow shell model approach with a core

Gamow shell model (GSM) is usually performed within the Woods-Saxon (WS) basis in which the WS parameters need to be determined by fitting experimental single-particle energies including their resonance widths. In the multi-shell case, such a fit is difficult due to the lack of experimental data of cross-shell single-particle energies and widths. In this paper, we develop an {\it ab-initio} GSM by introducing the Gamow Hartree-Fock (GHF) basis that is obtained using the same interaction as the one used in the construction of the shell-model Hamiltonian. GSM makes use of the complex-momentum Berggren representation, then including resonance and continuum components. Hence, GSM gives a good description of weakly bound and unbound nuclei. Starting from chiral effective field theory and employing many-body perturbation theory (MBPT) (called nondegenerate $\hat Q$-box folded-diagram renormalization) in the GHF basis, a multi-shell Hamiltonian ({\it sd-pf} shells in this work) can be constructed. The single-particle energies and their resonance widths can also been obtained using MBPT. We investigated $^{23-28}$O and $^{23-31}$F isotopes, for which multi-shell calculations are necessary. Calculations show that continuum effects and the inclusion of the {\it pf} shell are important elements to understand the structure of nuclei close to and beyond driplines.

nucl-th↗

arXiv2019

Ultrafast Quasiparticle Dynamics and Electron-Phonon Coupling in (Li0.84Fe0.16)OHFe0.98Se

Distinctive superconducting behaviors between bulk and monolayer FeSe make it challenging to obtain a unified picture of all FeSe-based superconductors. We investigate the ultrafast quasiparticle (QP) dynamics of an intercalated superconductor (Li1-xFex)OHFe1-ySe, which is a bulk crystal but shares a similar electronic structure with single-layer FeSe on SrTiO3. We obtain the electron-phonon coupling (EPC) constant λA1g (0.22 +/- 0.04), which well bridges that of bulk FeSe crystal and single-layer FeSe on SrTiO3. Moreover, we find that such a positive correlation between λA1g and superconducting Tc holds among all known FeSe-based superconductors, even in line with reported FeAs-based superconductors. Our observation indicates possible universal role of EPC in the superconductivity of all known categories of iron-based superconductors, which is a critical step towards achieving a unified superconducting mechanism for all iron-based superconductors.

cond-mat.supr-con↗

arXiv2019

Ab initio Gamow in-medium similarity renormalization group with resonance and continuum

We have developed a novel ab initio Gamow in-medium similarity renormalization group (Gamow IMSRG) in the complex-energy Berggren framework. The advanced Gamow IMSRG is capable of describing the resonance and nonresonant continuum properties of weakly bound and unbound nuclear many-body systems. As test grounds, carbon and oxygen isotopes have been calculated with chiral two- and three-nucleon forces from the effective field theory. Resonant states observed in the neutron-dripline 24O are well reproduced. The halo structure of the known heaviest Borromean nucleus 22C is clearly seen by calculating the density distribution in which the continuum s channel plays a crucial role. Furthermore, we predict low-lying resonant excited states in 22C. The Gamow IMSRG provides tractable ab initio calculations of weakly bound and unbound open quantum systems.

nucl-th↗

arXiv2019

Observation of Weyl nodes in robust type-II Weyl semimetal WP2

Distinct to type-I Weyl semimetals (WSMs) that host quasiparticles described by the Weyl equation, the energy dispersion of quasiparticles in type-II WSMs violates Lorentz invariance and the Weyl cones in the momentum space are tilted. Since it was proposed that type-II Weyl fermions could emerge from (W,Mo)Te2 and (W,Mo)P2 families of materials, a large numbers of experiments have been dedicated to unveil the possible manifestation of type-II WSM, e.g. the surface-state Fermi arcs. However, the interpretations of the experimental results are very controversial. Here, using angle-resolved photoemission spectroscopy supported by the first-principles calculations, we probe the tilted Weyl cone bands in the bulk electronic structure of WP2 directly, which are at the origin of Fermi arcs at the surfaces and transport properties related to the chiral anomaly in type-II WSMs. Our results ascertain that due to the spin-orbit coupling the Weyl nodes originate from the splitting of 4-fold degenerate band-crossing points with Chern numbers C = $\pm$2 induced by the crystal symmetries of WP2, which is unique among all the discovered WSMs. Our finding also provides a guiding line to observe the chiral anomaly which could manifest in novel transport properties.

cond-mat.mes-hall↗

arXiv2019

Higher order mode damper for low energy RHIC electron cooler SRF booster cavity

To improve RHIC luminosity for heavy ion beam energies below 10 GeV/nucleon, the Low Energy RHIC electron Cooler (LEReC) is currently under commissioning at BNL. The Linac of LEReC is designed to deliver a 1.6 MeV to 2.6 MeV electron beam, with rms dp/p less than 5e-4. A 704 MHz superconducting radio frequency (SRF) booster cavity in this Linac provides up to 2.2 MeV accelerating voltage. With such a low energy and very demanding energy spread requirement, control of Higher Order Modes (HOMs) in the cavities becomes critical and needs to be carefully evaluated to ensure minimum impact on the beam. In this paper, we report the multiphysics design of the HOM damper for this cavity to meet the energy spread requirement, as well as experimental results of the cavity with and without the HOM damper.

physics.acc-ph↗

arXiv2019

Strong Pseudospin-Lattice Coupling in Sr3Ir2O7: Coherent Phonon Anomaly and Negative Thermal Expansion

The similarities to cuprates make iridates an interesting potential platform for investigating superconductivity. Equally attractive are their puzzling complex intrinsic interactions. Here, we report an ultrafast optical spectroscopy investigation of a coherent phonon mode in Sr3Ir2O7, a bilayer Ruddlesden-Popper perovskite iridate. An anomaly in the A1g optical phonon (ν = 4.4 THz) is unambiguously observed below the Néel temperature (TN), which we attribute to pseudospin-lattice coupling (PLC). Significantly, we find that PLC is the dominant interaction at low temperature, and we directly measure the PLC coefficient to be λ = 150 +/- 20 cm-1, which is two orders of magnitude higher than that in manganites (< 2.4 cm-1) and comparable to that in CuO (50 cm-1, the strongest PLC or spin-lattice coupling (SLC) previously known). Moreover, we find that the strong PLC induces an anisotropic negative thermal expansion. Our findings highlight the key role of PLC in iridates and uncovers another intriguing similarity to cuprates.

cond-mat.str-el↗

arXiv2018

Resonances of unbound quantum many-body systems of nuclei

Resonance is a general phenomenon which can happen in classic or quantum systems. An unbound many-body quantum system can undergo a self-resonant process. It has long been a challenge how to describe unbound many-body quantum systems in resonances. In this paper, we develop a novel first-principles method that is capable of describing resonant quantum systems. We exploit, for the first time, the advanced in-medium similarity renormalization group (IMSRG) in the complex-energy Gamow-Berggren representation with resonance and non-resonant continuum. The ab initio Gamow IMSRG has broad applications, such as, to the electromagnetic-interaction systems of atoms, molecules or quantum dots, and strong-interaction atomic nuclei. In the present work, we apply the method to loosely bound or unbound nuclear systems. Carbon and oxygen isotopes have been investigated with an optimized chiral effective field theory potential. The resonant states observed in neutron-rich 22O and 24O are well reproduced. The loose halo structure of the Borromean nucleus 22C is clearly seen by the density calculation, in which the continuum s-waves play a crucial role. Further, we predict low-lying resonant excited states in 22C. This method provides rigorous and tractable theoretical calculations for weakly-bound or unbound open quantum systems.

nucl-th↗