arXiv subjects

Q. Y. Chen

Publications and source records attributed to Q. Y. Chen.

At least 19 recordsLinked to original sources

arXiv2026

Shell model description of the $N=82$ isotonic chain with a new effective interaction

In this work, we present a systematic study of low-lying states and electromagnetic properties of the semi-magic $N = 82$ isotonic chain with proton number $Z=51$-77, using the full configuration interaction shell model with a newly developed high-quality effective interaction. The calculations are performed in a large model space that includes all proton orbitals between $Z = 50$ and 82: $0g_{7/2}$, $1d_{5/2}$, $1d_{3/2}$, $2s_{1/2}$, and $0h_{11/2}$. The effective interaction is derived through the principal component analysis approach, starting from 160 two-body matrix elements and 5 single-particle energies and considering up to 30 degrees of freedom. Those are optimized by fitting to 204 available experimental energy levels. The resulting root-mean-square deviation is as low as 102 keV. The new interaction successfully reproduces the binding energies, low-lying spectra, electric quadrupole transition probabilities $B(E2)$, and magnetic dipole moments across both even-even and odd-mass isotones. The nuclear structure of low-lying states is analyzed in detail. Additionally, predictions are made for several more proton-rich nuclei beyond current experimental reach, including $^{155}\mathrm{Ta}$, $^{156}\mathrm{W}$, $^{157}\mathrm{Re}$, $^{158}\mathrm{Os}$, and $^{159}\mathrm{Ir}$.

nucl-th↗

arXiv2024

Practical identifiability and parameter estimation of compartmental epidemiological models

Practical parameter identifiability in ODE-based epidemiological models is a known issue, yet one that merits further study. It is essentially ubiquitous due to noise and errors in real data. In this study, to avoid uncertainty stemming from data of unknown quality, simulated data with added noise are used to investigate practical identifiability in two distinct epidemiological models. Particular emphasis is placed on the role of initial conditions, which are assumed unknown, except those that are directly measured. Instead of just focusing on one method of estimation, we use and compare results from various broadly used methods, including maximum likelihood and Markov Chain Monte Carlo (MCMC) estimation. Among other findings, our analysis revealed that the MCMC estimator is overall more robust than the point estimators considered. Its estimates and predictions are improved when the initial conditions of certain compartments are fixed so that the model becomes globally identifiable. For the point estimators, whether fixing or fitting the that are not directly measured improves parameter estimates is model-dependent. Specifically, in the standard SEIR model, fixing the initial condition for the susceptible population S(0) improved parameter estimates, while this was not true when fixing the initial condition of the asymptomatic population in a more involved model. Our study corroborates the change in quality of parameter estimates upon usage of pre-peak or post-peak time-series under consideration. Finally, our examples suggest that in the presence of significantly noisy data, the value of structural identifiability is moot.

stat.ME↗

arXiv2023

Vaccination compartmental epidemiological models for the delta and omicron SARS-CoV-2 variants

We explore the inclusion of vaccination in compartmental epidemiological models concerning the delta and omicron variants of the SARS-CoV-2 virus that caused the COVID-19 pandemic. We expand on our earlier compartmental-model work by incorporating vaccinated populations. We present two classes of models that differ depending on the immunological properties of the variant. The first one is for the delta variant, where we do not follow the dynamics of the vaccinated individuals since infections of vaccinated individuals were rare. The second one for the far more contagious omicron variant incorporates the evolution of the infections within the vaccinated cohort. We explore comparisons with available data involving two possible classes of counts, fatalities and hospitalizations. We present our results for two regions, Andalusia and Switzerland (including the Principality of Liechtenstein), where the necessary data are available. In the majority of the considered cases, the models are found to yield good agreement with the data and have a reasonable predictive capability beyond their training window, rendering them potentially useful tools for the interpretation of the COVID-19 and further pandemic waves, and for the design of intervention strategies during these waves.

q-bio.PE↗

arXiv2022

Backcasting COVID-19: A Physics-Informed Estimate for Early Case Incidence

It is widely accepted that the number of reported cases during the first stages of the COVID-19 pandemic severely underestimates the number of actual cases. We leverage delay embedding theorems of Whitney and Takens and use Gaussian Process regression to estimate the number of cases during the first 2020 wave based on the second wave of the epidemic in several European countries, South Korea, and Brazil. We assume that the second wave was more accurately monitored and hence that it can be trusted. We then construct a manifold diffeomorphic to that of the implied original dynamical system, using fatalities or hospitalizations only. Finally, we restrict the diffeomorphism to the reported cases coordinate of the dynamical system. Our main finding is that in the European countries studied, the actual cases are under-reported by as much as 50\%. On the other hand, in South Korea -- which had an exemplary and proactive mitigation approach -- a far smaller discrepancy between the actual and reported cases is predicted, with an approximately 17\% predicted under-estimation. We believe that our backcasting framework is applicable to other epidemic outbreaks where (due to limited or poor quality data) there is uncertainty around the actual cases.

q-bio.QM↗

arXiv2021

Cross-over behavior of the localized to itinerant transition of 5f electrons in the antiferromagnetic Kondo lattice USb2

In Uranium-based heavy fermion system, the 5f electrons display an intermediate character between partial localization and partial itinerancy, which makes the Kondo problem more complicated. Here we use scanning tunneling microscopy/spectroscopy to investigate the (001) surface of the Kondo lattice antiferromagnet USb2. Temperature-dependent dI/dV spectra from 4.7 K up to 140 K reveal several peak structures around the Fermi level. Two pronounced peaks are originated from the hybridization between the conduction and 5f electrons. We did not observe the mysteriously abrupt change of the electronic state at 45 K, which is previously reported by another STM group and attributed to a novel first-order like transition. Instead, we only observe continuous evolution of the dI/dV spectra with temperature. Furthermore, in some scanning regions, we find significant Sb atoms missing from the top layer, which gives us the opportunity to investigate the electronic structure of the U-terminated surface. For the U-terminated surface, an additional sharp peak emerges, which is closely related to the magnetic order.

cond-mat.str-el↗

arXiv2021

Kondo effect and subatomic structures of single U atoms on graphene/6H-SiC(0001)

The Kondo effect typically arises from the spin-flip scattering between the localized magnetic moment of the impurity and the delocalized electrons in the metallic host, which leads to a variety of intriguing phenomena. Here, by using scanning tunnelling microscopy/spectroscopy (STM/STS), we present the Kondo effect and subatomic features of single U adatom on graphene/6H-SiC(0001). A dip spectral feature can be observed around the Fermi energy, which is termed as the "fingerprint" of the Kondo resonance in STS; in addition, two subatomic features with different symmetries: a three-lobe structure and a donghnut-like structure can be observed from the dI/dV maps. The Kondo resonance is only detectable within 5~Å~of the lateral distance from the U atom center, which is much smaller than the distances observed in Co atoms on different surfaces, indicating the more localized 5$f$ states than 3$d$ orbitals. By comparing with density functional theory calculations, we find that the two subatomic features displaying different symmetries originate from the selective hybridization between U 6$d$, 5$f$ orbitals and the $p_z$ orbitals from two inequivalent C atoms of the multilayer graphene.

cond-mat.str-el↗

arXiv2019

Orbital-selective Kondo entanglement and antiferromagnetic order in USb$_2$

In heavy-fermion compounds, the dual character of $f$ electrons underlies their rich and often exotic properties like fragile heavy quasipartilces, variety of magnetic orders and unconventional superconductivity. 5$f$-electron actinide materials provide a rich setting to elucidate the larger and outstanding issue of the competition between magnetic order and Kondo entanglement and, more generally, the interplay among different channels of interactions in correlated electron systems. Here, by using angle-resolved photoemission spectroscopy, we present detailed electronic structure of USb$_2$ and observed two different kinds of nearly flat bands in the antiferromagnetic state of USb$_2$. Polarization-dependent measurements show that these electronic states are derived from 5$f$ orbitals with different characters; in addition, further temperature-dependent measurements reveal that one of them is driven by the Kondo correlations between the 5$f$ electrons and conduction electrons, while the other reflects the dominant role of the magnetic order. Our results on the low-energy electronic excitations of USb$_2$ implicate orbital selectivity as an important new ingredient for the competition between Kondo correlations and magnetic order and, by extension, in the rich landscape of quantum phases for strongly correlated $f$ electron systems.

cond-mat.str-el↗

arXiv2019

Electronic structure and 4f-electron character in Ce2PdIn8 studied by angle-resolved photoemission spectroscopy

The localized-to-itinerant transition of f electrons lies at the heart of heavy-fermion physics, but has only been directly observed in single-layer Ce-based materials. Here, we report a comprehensive study on the electronic structure and nature of the Ce 4f electrons in the heavy-fermion superconductor Ce2PdIn8, a typical n=2 CenMmIn3n+2m compound, using high-resolution and 4d-4f resonance photoemission spectroscopies. The electronic structure of this material has been studied over a wide temperature range, and hybridization between f and conduction electrons can be clearly observed to form a Kondo resonance near the Fermi level at low temperatures. The characteristic temperature of the localized-to-itinerant transition is around 120K, which is much higher than its coherence temperature Tcoh~30K.

cond-mat.str-el↗

arXiv2018

ARPES/STM study of the surface terminations and 5$f$-electron character in URu$_2$Si$_2$

Hidden order in URu$_2$Si$_2$ has remained a mystery now entering its 4th decade. The importance of resolving the nature of the hidden order has stimulated extensive research. Here we present a detailed characterization of different surface terminations in URu$_2$Si$_2$ by angle-resolved photoemission spectroscopy, in conjunction with scanning tunneling spectroscopy and DMFT calculations that may unveil a new piece of this puzzle. The U-terminated surface is characterized by an electron-like band around the $\bar{X}$ point, while a hole-like band for the Si-terminated surface. We also investigate temperature evolution of the electronic structure around the $\bar{X}$ point from 11 K up to 70 K, and did not observe any abrupt change of the electronic structure around the coherence temperature (55 K). The $f$ spectral weight gradually weakens upon increasing temperature, still some $f$ spectral weight can be found above this temperature. Our results suggest that surface terminations in URu$_2$Si$_2$ are an important issue to be taken into account in future work.

cond-mat.str-el↗

arXiv2018

Charge Transfer Effects in Naturally Occurring van der Waals Heterostructures (PbSe)1.16(TiSe2)m (m=1, 2)

Van der Waals heterostructures (VDWHs) exhibit rich properties and thus has potential for applications, and charge transfer between different layers in a heterostructure often dominates its properties and device performance. It is thus critical to reveal and understand the charge transfer effects in VDWHs, for which electronic structure measurements have proven to be effective. Using angle-resolved photoemission spectroscopy, we studied the electronic structures of (PbSe)1.16(TiSe2)m(m=1, 2), which are naturally occurring VDWHs, and discovered several striking charge transfer effects. When the thickness of the TiSe2 layers is halved from m=2 to m=1, the amount of charge transferred increases unexpectedly by more than 250%. This is accompanied by a dramatic drop in the electron-phonon interaction strength far beyond the prediction by first-principles calculations and, consequently, superconductivity only exists in the m=2 compound with strong electron-phonon interaction, albeit with lower carrier density. Furthermore, we found that the amount of charge transferred in both compounds is nearly halved when warmed from below 10 K to room temperature, due to the different thermal expansion coefficients of the constituent layers of these misfit compounds. These unprecedentedly large charge transfer effects might widely exist in VDWHs composed of metal-semiconductor contacts; thus, our results provide important insights for further understanding and applications of VDWHs.

cond-mat.str-el↗

arXiv2018

Unveiling the superconducting mechanism of Ba$_{0.51}$K$_{0.49}$BiO$_3$

Bismuthates were the first family of oxide high-temperature superconductors, exhibiting superconducting transition temperatures (Tc) up to 32K, but the superconducting mechanism remains under debate despite more than 30 years of extensive research. Our angle-resolved photoemission spectroscopy studies on Ba$_{0.51}$K$_{0.49}$BiO$_3$ reveal an unexpectedly 34% larger bandwidth than in conventional density functional theory calculations. This can be reproduced by calculations that fully account for long-range Coulomb interactions --- the first direct demonstration of bandwidth expansion due to the Fock exchange term, a long-accepted and yet uncorroborated fundamental effect in many body physics. Furthermore, we observe an isotropic superconducting gap with 2Δ$_0$/k$_B$ T$_c$ = 3.51 $\pm$ 0.05, and strong electron-phonon interactions with a coupling constant λ$\sim$ 1.3 $\pm$ 0.2. These findings solve a long-standing mystery --- Ba$_{0.51}$K$_{0.49}$BiO$_3$ is an extraordinary Bardeen-Cooper-Schrieffer (BCS) superconductor, where long-range Coulomb interactions expand the bandwidth, enhance electron-phonon coupling, and generate the high Tc. Such effects will also be critical for finding new superconductors.

cond-mat.supr-con↗

arXiv2018

Tracing crystal-field splittings in the rare earth-based intermetallic CeIrIn$_5$

Crystal electric field states in rare earth intermetallics show an intricate entanglement with the many-body physics that occurs in these systems and that is known to lead to a plethora of electronic phases. Here, we attempt to trace different contributions to the crystal electric field (CEF) splittings in CeIrIn$_5$, a heavy-fermion compound and member of the Ce$M$In$_5$ ($M$= Co, Rh, Ir) family. To this end, we utilize high-resolution resonant angle-resolved photoemission spectroscopy (ARPES) and present a spectroscopic study of the electronic structure of this unconventional superconductor over a wide temperature range. As a result, we show how ARPES can be used in combination with thermodynamic measurements or neutron scattering to disentangle different contributions to the CEF splitting in rare earth intermetallics. We also find that the hybridization is stronger in CeIrIn$_5$ than CeCoIn$_5$ and the effects of the hybridization on the Fermi volume increase is much smaller than predicted. By providing the first experimental evidence for $4f_{7/2}^{1}$ splittings which, in CeIrIn$_5$, split the octet into four doublets, we clearly demonstrate the many-body origin of the so-called $4f_{7/2}^{1}$ state.

cond-mat.str-el↗

arXiv2018

Band dependent inter-layer $f$-electron hybridization in CeRhIn$_5$

A key issue in heavy fermion research is how subtle changes in the hybridization between the 4$f$ (5$f$) and conduction electrons can result in fundamentally different ground states. CeRhIn$_5$ stands out as a particularly notable example: replacing Rh by either Co or Ir, located above or below Rh in the periodic table, antiferromagnetism gives way to superconductivity. In this photoemission study of CeRhIn$_5$, we demonstrate that the use of resonant ARPES with polarized light allows to extract detailed information on the 4$f$ crystal field states and details on the 4$f$ and conduction electron hybridization which together determine the ground state. We directly observe weakly dispersive Kondo resonances of $f$-electrons and identify two of the three Ce $4f_{5/2}^{1}$ crystal-electric-field levels and band-dependent hybridization, which signals that the hybridization occurs primarily between the Ce $4f$ states in the CeIn$_3$ layer and two more three-dimensional bands composed of the Rh $4d$ and In $5p$ orbitals in the RhIn$_2$ layer. Our results allow to connect the properties observed at elevated temperatures with the unusual low-temperature properties of this enigmatic heavy fermion compound.

cond-mat.str-el↗

arXiv2018

Seasonal Variation of the Underground Cosmic Muon Flux Observed at Daya Bay

The Daya Bay Experiment consists of eight identically designed detectors located in three underground experimental halls named as EH1, EH2, EH3, with 250, 265 and 860 meters of water equivalent vertical overburden, respectively. Cosmic muon events have been recorded over a two-year period. The underground muon rate is observed to be positively correlated with the effective atmospheric temperature and to follow a seasonal modulation pattern. The correlation coefficient $α$, describing how a variation in the muon rate relates to a variation in the effective atmospheric temperature, is found to be $α_{\text{EH1}} = 0.362\pm0.031$, $α_{\text{EH2}} = 0.433\pm0.038$ and $α_{\text{EH3}} = 0.641\pm0.057$ for each experimental hall.

physics.ins-det↗

arXiv2018

Direct observation of heavy quasiparticles in the Kondo lattice CeIn3

The electronic structure of the Kondo lattice CeIn3 has been studied by on-resonant angle-resolved photoemission spectroscopy and scanning tunneling microscopy/spectroscopy. A weakly dispersive quasiparticle band has been observed directly with an energy dispersion of 4 meV by photoemission, implying the existence of weak hybridization between the f electrons and conduction electrons. The hybridization is further confirmed by the formation of the hybridization gap revealed by temperature-dependent scanning tunneling spectroscopy. Moreover, we find the hybridization strength in CeIn3 is much weaker than that in the more two-dimensional compounds CeCoIn5 and CeIrIn5. Our results may be essential for the complete microscopic understanding of this important compound and the related heavy-fermion systems.

cond-mat.str-el↗

arXiv2017

Direct measurement of the localized-itinerant transition, hybridization and antiferromagnetic transition of 5f electrons

In heavy-fermion compounds, f electrons show both itinerant and localized behaviour depending on the external conditions, and the hybridization between localized f electrons and itinerant conduction bands gives rise to their exotic properties like heavy-fermions, magnetic orders and unconventional superconductivity. Duo to the risk of handling radioactive actinide materials, the direct experimental evidence of the band structure evolution across the localized-itinerant and magnetic transitions for 5f electrons is lacking. Here, by using angle-resolved photoelectron spectroscopy, we revealed the dual nature (localized vs itinerant) and the development of two different kinds of heavy quasi-particle bands of 5f electrons in antiferromagnetic (AFM) USb2. Partially opened energy gaps were observed on one quasi-particle 5f band cross the AFM transition around 203 K, indicating that the magnetic orders in USb2 are of spin density wave (SDW) type similar to Cr. The localized 5f electrons and itinerant conduction bands hybridize to form another heavy quasi-particle band at about 120 K, and then open hybridization gaps at even lower temperature. Our results provide direct spectral demonstration of the localized-itinerant transition, hybridization and SDW transition of 5f electrons for uranium-based materials.

cond-mat.str-el↗

arXiv2017

Evolution of the Reactor Antineutrino Flux and Spectrum at Daya Bay

The Daya Bay experiment has observed correlations between reactor core fuel evolution and changes in the reactor antineutrino flux and energy spectrum. Four antineutrino detectors in two experimental halls were used to identify 2.2 million inverse beta decays (IBDs) over 1230 days spanning multiple fuel cycles for each of six 2.9 GW$_{\textrm{th}}$ reactor cores at the Daya Bay and Ling Ao nuclear power plants. Using detector data spanning effective $^{239}$Pu fission fractions, $F_{239}$, from 0.25 to 0.35, Daya Bay measures an average IBD yield, $\barσ_f$, of $(5.90 \pm 0.13) \times 10^{-43}$ cm$^2$/fission and a fuel-dependent variation in the IBD yield, $dσ_f/dF_{239}$, of $(-1.86 \pm 0.18) \times 10^{-43}$ cm$^2$/fission. This observation rejects the hypothesis of a constant antineutrino flux as a function of the $^{239}$Pu fission fraction at 10 standard deviations. The variation in IBD yield was found to be energy-dependent, rejecting the hypothesis of a constant antineutrino energy spectrum at 5.1 standard deviations. While measurements of the evolution in the IBD spectrum show general agreement with predictions from recent reactor models, the measured evolution in total IBD yield disagrees with recent predictions at 3.1$σ$. This discrepancy indicates that an overall deficit in measured flux with respect to predictions does not result from equal fractional deficits from the primary fission isotopes $^{235}$U, $^{239}$Pu, $^{238}$U, and $^{241}$Pu. Based on measured IBD yield variations, yields of $(6.17 \pm 0.17)$ and $(4.27 \pm 0.26) \times 10^{-43}$ cm$^2$/fission have been determined for the two dominant fission parent isotopes $^{235}$U and $^{239}$Pu. A 7.8% discrepancy between the observed and predicted $^{235}$U yield suggests that this isotope may be the primary contributor to the reactor antineutrino anomaly.

hep-ex↗

arXiv2017

Electronic structure of FeS

Here we report the electronic structure of FeS, a recently identified iron-based superconductor. Our high-resolution angle-resolved photoemission spectroscopy studies show two hole-like ($α$ and $β$) and two electron-like ($η$ and $δ$) Fermi pockets around the Brillouin zone center and corner, respectively, all of which exhibit moderate dispersion along $k_z$. However, a third hole-like band ($γ$) is not observed, which is expected around the zone center from band calculations and is common in iron-based superconductors. Since this band has the highest renormalization factor and is known to be the most vulnerable to defects, its absence in our data is likely due to defect scattering --- and yet superconductivity can exist without coherent quasiparticles in the $γ$ band. This may help resolve the current controversy on the superconducting gap structure of FeS. Moreover, by comparing the $β$ bandwidths of various iron chalcogenides, including FeS, FeSe$_{1-x}$S$_x$, FeSe, and FeSe$_{1-x}$ Te$_x$, we find that the $β$ bandwidth of FeS is the broadest. However, the band renormalization factor of FeS is still quite large, when compared with the band calculations, which indicates sizable electron correlations. This explains why the unconventional superconductivity can persist over such a broad range of isovalent substitution in FeSe$_{1-x}$Te$_{x}$ and FeSe$_{1-x}$S$_{x}$.

cond-mat.supr-con↗