arXiv subjects

Q. Zhang

Publications and source records attributed to Q. Zhang.

At least 73 records · Page 4Linked to original sources

arXiv2021

Evolution of Magnetic Interactions in Sb-substituted MnBi2Te4

The Mn(Bi$_{1-x}$Sb$_x$)$_2$Te$_4$ series is purported to span from antiferromagnetic (AF) topological insulator at x = 0 to a trivial AF insulator at x = 1. Here we report on neutron diffraction and inelastic neutron scattering studies of the magnetic interactions across this series. All compounds measured possess ferromagnetic (FM) triangular layers and we find a crossover from AF to FM interlayer coupling near x = 1 for our samples. The large spin gap at x = 0 closes rapidly and the average FM exchange interactions within the triangular layer increase with Sb substitution. Similar to a previous study of MnBi$_2$Te$_4$, we find severe spectral broadening which increases dramatically across the compositional series. In addition to broadening, we observe an additional sharp magnetic excitation in MnSb$_2$Te$_4$ that may indicate the development of local magnetic modes based on recent reports of antisite disorder between Mn and Sb sublattices. The results suggest that both substitutional and antisite disorder contribute substantially to the magnetism in Mn(Bi$_{1-x}$Sb$_x$)$_2$Te$_4$.

cond-mat.str-el↗

arXiv2021

The physical and chemical structure of high-mass star-forming regions. Unraveling chemical complexity with the NOEMA large program "CORE"

We use sub-arcsecond resolution ($\sim$0.4$''$) observations with NOEMA at 1.37 mm to study the dust emission and molecular gas of 18 high-mass star-forming regions. We combine the derived physical and chemical properties of individual cores in these regions to estimate their ages. The temperature structure of these regions are determined by fitting H2CO and CH3CN line emission. The density profiles are inferred from the 1.37 mm continuum visibilities. The column densities of 11 different species are determined by fitting the emission lines with XCLASS. Within the 18 observed regions, we identify 22 individual cores with associated 1.37 mm continuum emission and with a radially decreasing temperature profile. We find an average temperature power-law index of q = 0.4$\pm$0.1 and an average density power-law index of p = 2.0$\pm$0.2 on scales on the order of several 1 000 au. Comparing these results with values of p derived in the literature suggest that the density profiles remain unchanged from clump to core scales. The column densities relative to N(C18O) between pairs of dense gas tracers show tight correlations. We apply the physical-chemical model MUSCLE to the derived column densities of each core and find a mean chemical age of $\sim$60 000 yrs and an age spread of 20 000-100 000 yrs. With this paper we release all data products of the CORE project available at https://www.mpia.de/core. The CORE sample reveals well constrained density and temperature power-law distributions. Furthermore, we characterize a large variety in molecular richness that can be explained by an age spread confirmed by our physical-chemical modeling. The hot molecular cores show the most emission lines, but we also find evolved cores at an evolutionary stage, in which most molecules are destroyed and thus the spectra appear line-poor again.

astro-ph.GA↗

arXiv2021

Computational study of simultaneous positive and negative streamer propagation in a twin surface dielectric barrier discharge via 2D PIC simulations

The propagation mechanisms of plasma streamers have been observed and investigated in a surface dielectric barrier discharge (SDBD) using 2D particle in cell simulations. The investigations are carried out under a simulated air mixture, 80\% N$_2$ and 20\% O$_2$, at atmospheric pressure, 100$\,$kPa, under both DC conditions and a pulsed DC waveform that represent AC conditions. The simulated geometry is a simplification of the symmetric and fully exposed SDBD resulting in the simultaneous ignition of both positive and negative streamers on either side of the Al$_2$O$_3$ dielectric barrier. In order to determine the interactivity of the two streamers, the propagation behavior for the positive and negative streamers are investigated both independently and simultaneously under identical constant voltage conditions. An additional focus is implored under a fast sub nanosecond rise time square voltage pulse alternating between positive and negative voltage conditions, thus providing insight into the dynamics of the streamers under alternating polarity switches. It is shown that the simultaneous ignition of both streamers, as well as using the pulsed DC conditions, provides both an enhanced discharge and an increased surface coverage. It is also shown that additional streamer branching may occur in a cross section that is difficult to experimentally observe. The enhanced discharge and surface coverage may be beneficial to many applications such as, but are not limited to: air purification, volatile organic compound removal, and plasma enhanced catalysis.

physics.plasm-ph↗

arXiv2021

Tuning the flat bands of the kagome metal CoSn with Fe, In, or Ni doping

CoSn is a Pauli paramagnet with relatively flat d-bands centered about 100 meV below the Fermi energy Ef. Single crystals of CoSn lightly doped with Fe, In, or Ni are investigated using x-ray and neutron scattering, magnetic susceptibility and magnetization, ac susceptibility, specific heat and resistivity measurements. Within the rigid band approximation, hole doping with a few percent of Fe or In should move the flat bands closer to Ef, whereas electron doping with Ni should move the flat bands further away from Ef. We provide evidence that this indeed occurs. Fe and In doping drive CoSn toward magnetism, while Ni doping suppresses CoSn's already weak magnetic response. The resulting ground state is different for Fe versus In doping. For Fe-doped crystals, Co1-xFexSn, with 0.02 < x < 0.27, the magnetic and specific heat data are consistent with the formation of a spin glass, with a glass transition temperature, Tg, ranging from 1 K for x=0.02 to 10 K for x= 0.27. Powder and single crystal neutron diffraction found no evidence of long-range magnetic order below Tg with x = 0.17. For In-doped crystals, CoSn1-yIny, both the magnetic susceptibility and the Sommerfeld coefficient, gamma, increase substantially relative to pure CoSn, but with no clear indication of a magnetic transition for 0.05 < y < 0.2. CoSn crystals doped with Ni (Co0.93Ni0.07Sn) have a significantly smaller magnetic susceptibility and gamma than pure CoSn, consistent with the flat bands further from Ef.

cond-mat.str-el↗

arXiv2021

Laser-assisted atom probe tomography of c-plane and m-plane InGaN test structures

Laser-assisted atom probe tomography (APT) was used to measure the indium mole fraction x of c-plane, MOCVD-grown, GaN/In(x)Ga(1-x)N/GaN test structures and the results were compared with Rutherford backscattering analysis (RBS). Four sample types were examined with (RBS determined) x = 0.030, 0.034, 0.056, and 0.112. The respective In(x)Ga(1-x)N layer thicknesses were 330 nm, 327 nm, 360 nm, and 55 nm. APT data were collected at (fixed) laser pulse energy (PE) selected within the range of (2-1000) fJ. Sample temperatures were = 54 K. PE within (2-50) fJ yielded x values that agreed with RBS (within uncertainty) and were comparatively insensitive to region-of-interest (ROI) geometry and orientation. By contrast, approximate stoichiometry was only found in the GaN portions of the samples provided PE was within (5-20) fJ and the analyses were confined to cylindrical ROIs (of diameters =20 nm) that were coaxial with the specimen tips. m-plane oriented tips were derived from c-axis grown, core-shell, GaN/In(x)Ga(1-x)N nanorod heterostructures. Compositional analysis along [0 0 0 1] (transverse to the long axis of the tip), of these m-plane samples revealed a spatial asymmetry in charge-state ratio (CSR) and a corresponding asymmetry in the resultant tip shape along this direction; no asymmetry in CSR or tip shape was observed for analysis along [-1 2-1 0]. Simulations revealed that the electric field strength at the tip apex was dominated by the presence of a p-type inversion layer, which developed under typical tip-electrode bias conditions for the n-type doping levels considered. Finally, both c-plane and m-plane sample types showed depth-dependent variations in absolute ion counts that depended upon ROI placement.

cond-mat.mtrl-sci↗

arXiv2020

Widely Spaced Planes of Magnetic Dimers in the Ba6Y2Rh2Ti2O17-δ Hexagonal Perovskite

We report the synthesis and initial characterization of Ba6Y2Rh2Ti2O17-δ, a previously unreported material with a hexagonal symmetry structure. Face-sharing RhO6 octahedra form triangular planes of Rh2O9 dimers that are widely separated in the perpendicular direction. The material displays a small effective magnetic moment, due to the Rh ions present, and a negative Curie-Weiss temperature. The charge transport and optical band gaps are very similar, near 0.16 eV. A large upturn in the heat capacity at temperatures below 1 K, suppressed by applied magnetic fields larger than {μ0H = 2 Tesla, is observed. A large T-linear term in the specific heat (γ=166 mJ/mol f.u-K2) is seen, although the material is insulating at low temperatures. These results suggest the possibility of a spin liquid ground state in this material.

cond-mat.str-el↗

arXiv2020

The role of the magnetic field in the fragmentation process: the case of G14.225-0.506

B-fields are predicted to play a role in the formation of filamentary structures and their fragmentation process. We aim at investigating the role of the B-field in the process of core fragmentation toward the hub-filament systems in the IRDC G14.2, which present different fragmentation level. We performed observations of the thermal dust polarization at 350 μm using the CSO toward the hubs. We applied the polarization--intensity-gradient method to estimate the significance of the B-field over the G-force. The B-field in Hub-N shows a uniform structure along the E-W orientation, perpendicular to the major axis of the hub-filament system. The I-gradient in Hub-N displays a local minimum coinciding with the dust core MM1a detected with interferometric observations. The B-field orientation is perturbed when approaching the dust core. Hub-S shows 2 local minima, reflecting the bimodal distribution of the B-field. In Hub-N, both E and W of the hub-filament system, the I-gradient and the B-field are parallel whereas they tend to be perpendicular when penetrating the filaments and hub. The analysis of the δ- and Σ B-maps indicate that, the B-field cannot prevent the collapse, suggesting that the B-field is initially dragged by the infalling motion and aligned with it, or is channeling material toward the central ridge from both sides. Values of Σ B > 1 are found toward a N-S ridge encompassing the dust emission peak, indicating that in this region B-field dominates over G-force, or that with the current angular resolution we cannot resolve an hypothetical more complex structure. We estimated the B-field strength, the MtF ratio and the A-M number, and found differences between the 2 hubs. The different levels of fragmentation observed in these 2 hubs could arise from the differences in the B-field properties rather than from different intensity of the G-field.

astro-ph.GA↗

arXiv2020

Complex magnetic structure in Ba5Ru3O12 with isolated Ru3O12-trimer

We report detailed magnetic, transport, heat-capacity, and neutron diffraction measurements of Ba5Ru3O12, a compound consisting of isolated Ru3O12 trimers. We show that this system develops long-range antiferromagnetic ordering at 60 K (TN) without structural distortion and metal-insulator-type transition, which is in sharp contrast to other Barium Ruthenate trimer systems such as 9R-BaRuO3 and Ba4Ru3O10. A complex magnetic structure is revealed which is attributable to the magnetic frustration due to competing exchange interactions between Ru ions on different crystallographic sites within the Ru3O12 trimer.

cond-mat.str-el↗

arXiv2020

Helical magnetic order and Fermi surface nesting in non-centrosymmetric ScFeGe

An investigation of the structural, magnetic, thermodynamic, and charge transport properties of non-centrosymmetric hexagonal ScFeGe reveals it to be an anisotropic metal with a transition to a weak itinerant incommensurate helimagnetic state below $T_N = 36$ K. Neutron diffraction measurements discovered a temperature and field independent helical wavevector \textbf{\textit{k}} = (0 0 0.193) with magnetic moments of 0.53 $μ_{B}$ per formula unit confined to the {\it ab}-plane. Density functional theory calculations are consistent with these measurements and find several bands that cross the Fermi level along the {\it c}-axis with a nearly degenerate set of flat bands just above the Fermi energy. The anisotropy found in the electrical transport is reflected in the calculated Fermi surface, which consists of several warped flat sheets along the $c$-axis with two regions of significant nesting, one of which has a wavevector that closely matches that found in the neutron diffraction. The electronic structure calculations, along with a strong anomaly in the {\it c}-axis conductivity at $T_N$, signal a Fermi surface driven magnetic transition, similar to that found in spin density wave materials. Magnetic fields applied in the {\it ab}-plane result in a metamagnetic transition with a threshold field of $\approx$ 6.7 T along with a sharp, strongly temperature dependent, discontinuity and a change in sign of the magnetoresistance for in-plane currents. Thus, ScFeGe is an ideal system to investigate the effect of in-plane magnetic fields on an easy-plane magnetic system, where the relative strength of the magnetic interactions and anisotropies determine the topology and magnetic structure.

cond-mat.mtrl-sci↗

arXiv2020

The chemical structure of young high-mass star-forming clumps: (II) parsec-scale CO depletion and deuterium fraction of $\rm HCO^+$

The physical and chemical properties of cold and dense molecular clouds are key to understanding how stars form. Using the IRAM 30 m and NRO 45 m telescopes, we carried out a Multiwavelength line-Imaging survey of the 70 $μ$m dark and bright clOuds (MIAO). At a linear resolution of 0.1--0.5 pc, this work presents a detailed study of parsec-scale CO depletion and $\rm HCO^+$ deuterium (D-) fractionation toward four sources (G11.38+0.81, G15.22-0.43, G14.49-0.13, and G34.74-0.12) included in our full sample. In each source with $\rm T<20$ K and $n_{\rm H}\rm\sim10^4$--$\rm 10^5 cm^{-3}$, we compared pairs of neighboring 70 $μ$m bright and dark clumps and found that (1) the $\rm H_2$ column density and dust temperature of each source show strong spatial anticorrelation; (2) the spatial distribution of CO isotopologue lines and dense gas tracers, such as 1--0 lines of $\rm H^{13}CO^+$ and $\rm DCO^+$, are anticorrelated; (3) the abundance ratio between $\rm C^{18}O$ and $\rm DCO^+$ shows a strong correlation with the source temperature; (4) both the $\rm C^{18}O$ depletion factor and D-fraction of $\rm HCO^+$ show a robust decrease from younger clumps to more evolved clumps by a factor of more than 3; and (5) preliminary chemical modeling indicates chemical ages of our sources are ${\sim}8\times10^4$ yr, which is comparable to their free-fall timescales and smaller than their contraction timescales, indicating that our sources are likely dynamically and chemically young.

astro-ph.GA↗

arXiv2020

On Spectral Peak Energy of Swift Gamma-Ray Bursts

Owing to narrow energy band of \textit{Swift}/BAT, several urgent issues are required to pay more attentions but unsolved so far. We systematically study the properties of a refined sample of 283 \textit{Swift}/BAT gamma-ray bursts with well-measured spectral peak energy ($E_{\text p}$) at a high confidence level larger than 3$σ$. It is interestingly found that duration ($T_{90}$) distribution of \textit{Swift} bursts still exhibits an evident bimodality with a more reliable boundary of $T_{90}\simeq$1.06 s instead of 2 s for previously contaminated samples including bursts without well-peaked spectra, which is very close to $\sim$1.27 s and $\sim$0.8 s suggested by some authors for Fermi/GBM and \textit{Swift}/BAT catalogs, respectively. The \textit{Swift}/BAT short and long bursts have comparable mean $E_{\text p}$ values of $87^{+112}_{-49}$ and $85^{+101}_{-46}$ keV in each, similar to what found for both types of BATSE bursts, which manifests the traditional short-hard/long-soft scheme may not be tenable for the certain energy window of a detector. In statistics, we also investigate the consistency of distinct methods for the $E_{\text p}$ estimates and find that Bayesian approach and BAND function can always give consistent evaluations. In contrast, the frequently-used cut-off power-law model matches two other methods for lower $E_{\text p}$ and will overestimate the $E_{\text p}$ more than 70\% as $E_{\text p}>$100 keV. Peak energies of X-ray flashes, X-ray rich bursts and classical gamma-ray bursts could have an evolutionary consequence from thermal-dominated to non-thermal-dominated radiation mechanisms. Finally, we find that the $E_{\text p}$ and the observed fluence ($S_γ$) in the observer frame are correlated as $E_p\simeq [S_γ/(10^{-5} erg\ cm^{-2})]^{0.28}\times 117.5^{+44.7}_{-32.4}$ keV proposed to be an useful indicator of GRB peak energies.

astro-ph.HE↗

arXiv2020

Observation of Photoinduced Terahertz Gain in GaAs Quantum Wells: Evidence for Radiative Two-Exciton-to-Biexciton Scattering

We have observed photoinduced negative optical conductivity, or gain, in the terahertz frequency range in a GaAs multiple-quantum-well structure in a strong perpendicular magnetic field at low temperatures. The gain is narrow-band: it appears as a sharp peak (linewidth $<$0.45 meV) whose frequency shifts with applied magnetic field. The gain has a circular-polarization selection rule: a strong line is observed for hole-cyclotron-resonance-active polarization. Furthermore, the gain appears only when the exciton $1s$ state is populated, which rules out intraexcitonic transitions to be its origin. Based on these observations, we propose a possible process in which the stimulated emission of a terahertz photon occurs while two free excitons scatter into one biexciton in an energy and angular-momentum conserving manner.

cond-mat.mes-hall↗

arXiv2020

Cloud-cloud collision as drivers of the chemical complexity in Galactic Centre molecular clouds

G+0.693-0.03 is a quiescent molecular cloud located within the Sagittarius B2 (Sgr B2) star-forming complex. Recent spectral surveys have shown that it represents one of the most prolific repositories of complex organic species in the Galaxy. The origin of such chemical complexity, along with the small-scale physical structure and properties of G+0.693-0.03, remains a mystery. In this paper, we report the study of multiple molecules with interferometric observations in combination with single-dish data in G+0.693-0.03. Despite the lack of detection of continuum source, we find small-scale (0.2 pc) structures within this cloud. The analysis of the molecular emission of typical shock tracers such as SiO, HNCO, and CH$_3$OH unveiled two molecular components, peaking at velocities of 57 and 75 km s$^{-1}$. They are found to be interconnected in both space and velocity. The position-velocity diagrams show features that match with the observational signatures of a cloud-cloud collision. Additionally, we detect three series of class \rom{1} methanol masers known to appear in shocked gas, supporting the cloud-cloud collision scenario. From the maser emission we provide constraints on the gas kinetic temperatures ($\sim$30-150 K) and H$_2$ densities (10$^4$-10$^5$ cm$^{-2}$). These properties are similar to those found for the starburst galaxy NGC253 also using class \rom{1} methanol masers, suggested to be associated with a cloud-cloud collision. We conclude that shocks driven by the possible cloud-cloud collision is likely the most important mechanism responsible for the high level of chemical complexity observed in G+0.693-0.03.

astro-ph.GA↗

arXiv2020

Crystal and Magnetic Structure of Polar Oxide HoCrWO$_6$

Polar magnetic oxide HoCrWO$_6$ is synthesized and its crystal structure, magnetic structure, and thermodynamic properties are investigated. HoCrWO$_6$ forms the polar crystal structure (space group Pna2$_1$ (#33)) due to the cation ordering of W$^{6+}$ and Cr$^{3+}$. There is an antiferromagnetic transition at TN = 24.5 K along with the magnetic entropy change (~5 J.Kg.$^{-1}$K$^{-1}$ at 70 kOe). Neutron diffraction measurement indicates that both Cr and Ho sublattices are ordered with the moment of 2.32(5)$μ_B$ and 8.7(4)$μ_B$ at 2 K, respectively. While Cr forms A-type collinear antiferromagnetic (AFM) structure with magnetic moment along the $b$ axis, Ho sublattice orders in a non-coplanar AFM arrangement. A comparison with isostructural DyFeWO$_6$ and DyCrWO$_6$ indicates that the magnetic structure of this family of compounds is controlled by the presence or absence of eg electrons in the transition metal sublattice.

cond-mat.mtrl-sci↗

arXiv2020

Observation of a $\bar{K}NN$ bound state in the $^3{\rm He} (K^-, Λp)n$ reaction

We have performed an exclusive measurement of the $K^{-}+\! ~^{3}{\rm He} \to Λpn$ reaction at an incident kaon momentum of $1\ {\rm GeV}/c$.In the $Λp$ invariant mass spectrum, a clear peak was observed below the mass threshold of $\bar{K}\!+\!N\!+\!N$, as a signal of the kaonic nuclear bound state, $\bar{K}NN$.The binding energy, decay width, and $S$-wave Gaussian reaction form-factor of this state were observed to be $B_{K} = 42\pm3({\rm stat.})^{+3}_{-4}({\rm syst.})\ {\rm MeV}$, $Γ_{K} = 100\pm7({\rm stat.})^{+19}_{-9}({\rm syst.})\ {\rm MeV}$, and $Q_{K} = 383\pm11({\rm stat.})^{+4}_{-1}({\rm syst.})\ {\rm MeV}/c$, respectively. The total production cross-section of $\bar{K}NN$, determined by its $Λp$ decay mode, was $σ^{tot}_{K} \cdot BR_{Λp} = 9.3\pm0.8({\rm stat.})^{+1.4}_{-1.0}({\rm syst.})\ μ{\rm b}$.We estimated the branching ratio of the $\bar{K}NN$ state to the $Λp$ and $Σ^{0}p$ decay modes as $BR_{Λp}/BR_{Σ^{0}p} \sim 1.7$, by assuming that the physical processes leading to the $ΣN\!N$ final states are analogous to those of $Λpn$.

nucl-ex↗

arXiv2020

ALMA reveals the coherence of the magnetic field geometry in OH 231.8+4.2

In a continuing effort to investigate the role of magnetic fields in evolved low and intermediate mass stars (principally regarding the shaping of their envelopes), we present new ALMA high resolution polarization data obtained for the nebula OH 231.8+4.2. We found that the polarized emission likely arises from aligned grains in the presence of magnetic fields rather than radiative alignment and self scattering. The ALMA data show well organized electric field orientations in most of the nebula and the inferred magnetic field vectors (rotated by 90 degrees) trace an hourglass morphology centred on the central system of the nebula. One region in the southern part of OH 231.8+4.2 shows a less organized distribution probably due to the shocked environment. These findings, in conjunction with earlier investigations (maser studies and dust emission analysis at other scales and wavelengths) suggest an overall magnetic hourglass located inside a toroidal field. We propose the idea that the magnetic field structure is closely related to the architecture of a magnetic tower and that the outflows were therefore magnetically launched. While the current dynamical effect of the fields might be weak in the equatorial plane principally due to the evolution of the envelope, it would still be affecting the outflows. In that regard, the measurement of the magnetic field at the stellar surface, which is still missing, combined with a full MHD treatment are required to better understand and constrain the events occurring in OH 231.8+4.2.

astro-ph.SR↗

arXiv2020

Domain alignment within ferroelectric/dielectric PbTiO$_3$/SrTiO$_3$ superlattice nanostructures

The ferroelectric domain pattern within lithographically defined PbTiO3/SrTiO3 ferroelectric/dielectric heteroepitaxial superlattice nanostructures is strongly influenced by the edges of the structures. Synchrotron x-ray nanobeam diffraction reveals that the spontaneously formed 180° ferroelectric stripe domains exhibited by such superlattices adopt a configuration in rectangular nanostructures in which domain walls are aligned with long patterned edges. The angular distribution of x-ray diffuse scattering intensity from nanodomains indicates that domains are aligned within an angular range of approximately 20° with respect to the edges. Computational studies based on a time-dependent Landau-Ginzburg-Devonshire model show that the preferred direction of the alignment results from lowering of the bulk and electrostrictive contributions to the free energy of the system due to the release of the lateral mechanical constraint. This unexpected alignment appears to be intrinsic and not a result of distortions or defects caused by the patterning process. Our work demonstrates how nanostructuring and patterning of heteroepitaxial superlattices allow for pathways to create and control ferroelectric structures that may appear counterintuitive.

cond-mat.mes-hall↗

arXiv2020

Edge Temperature Ring Oscillation Modulated by Turbulence Transition for Sustaining Stationary Improved Energy Confinement Plasmas

A reproducible stationary improved confinement mode (I-mode) has been achieved recently in the Experimental Advanced Superconducting Tokamak, featuring good confinement without particle transport barrier, which could be beneficial to solving the heat flux problem caused by edge localized modes (ELM) and the helium ash problem for future fusion reactors. The microscopic mechanism of sustaining stationary I-mode, based on the coupling between turbulence transition and the edge temperature oscillation, has been discovered for the first time. A radially localized edge temperature ring oscillation (ETRO) with azimuthally symmetric structure ($n=0$,$m=0$) has been identified and it is caused by alternative turbulence transitions between ion temperature gradient modes (ITG) and trapped electron modes (TEM). The ITG-TEM transition is controlled by local electron temperature gradient and consistent with the gyrokinetic simulations. The self-organizing system consisting with ETRO, turbulence and transport transitions plays the key role in sustaining the I-mode confinement. These results provide a novel physics basis for accessing, maintaining and controlling stationary I-mode in the future.

physics.plasm-ph↗