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Qi-Kun Xue

Publications and source records attributed to Qi-Kun Xue.

At least 19 recordsLinked to original sources

Intertwined Charge Stripes and Majorana Zero Modes in An Iron-Based Superconductor

In type-II superconductors, magnetic fields modulate the amplitude and phase of the superconducting order parameter, forming quantized vortices where superconductivity is locally suppressed and exotic bound states or competing electronic orders emerge. Using spectroscopic-imaging scanning tunneling microscopy on epitaxial Ba(Fe$_{0.94}Co$_{0.06})$_2$As$_2$ films, we discover an incommensurate charge-stripe order aligned with the Fe-Fe bond direction. These charge modulations become strongly enhanced at the vortex core and extend far into the vortex halo. Strikingly, the charge order modulates Andreev bound states of vortices at non-zero energies, producing abelian vortices with half-odd-integer level quantization and non-abelian vortices with integer-quantized core states that host a Majorana zero mode. The distinct vortex types are distinguished by the registry of their centers relative to the charge-stripe pattern and remain robust in ultrathin (2.5-unit-cell) films. Our findings reveal a density-wave-textured vortex matter and provide fresh insights into intertwined phenomena in iron-based superconductors.

cond-mat.supr-con

Distinct Surface and Bulk Superconductivity in the Kagome Superconductor SrSn$_3$

Surface and bulk superconductivity may possess fundamentally different superconducting properties in quantum materials with nontrivial electronic structures, yet their superimposed spectroscopic signatures often prevent direct experimental access to each superconducting channel. Here we reveal, in epitaxial films of the kagome superconductor SrSn$_3$, distinct surface and bulk superconducting channels with markedly different superconducting gaps, upper critical fields, and vortex-core electronic states by tuning the tunneling junction resistance in scanning tunneling spectroscopy. The surface superconductivity is characterized by a thickness-independent superconducting gap and an enhanced upper critical field, whereas the bulk superconducting channel exhibits a larger superconducting gap that decreases with reducing film thickness and a much lower upper critical field. Within magnetic vortex cores, robust non-split zero-bias conductance peaks are observed exclusively in the surface superconducting channel, while pronounced zero-bias suppression is consistently associated with the bulk superconducting channel. These findings demonstrate that the vortex-core electronic structure depends sensitively on the underlying superconducting channel, providing new insight into vortex-bound states in topological quantum materials.

cond-mat.supr-con

Dual Enhancement of Superconductivity in FeSe/SrTiO3 via Orbital and Correlation Synergy

In iron-based superconductors, the dz2 orbital band typically resides far below the Fermi level and has not been considered to participate in Cooper pairing. Here, using monolayer FeSe/SrTiO3 as a model system, we demonstrate that tip-induced tensile strain controllably shifts the dz2 band toward the Fermi level, driving a two-stage enhancement of superconductivity. In-plane lattice expansion first enhances electronic correlation, amplifying superconductivity in the initial stage. As strain further increases, the upward-shifted dz2 band hybridizes with the dxy band, reconstructing the pairing-active d-orbital bands and inducing a secondary, stronger gap enhancement. Collectively, these two stages enlarge the superconducting gap from 17.8 to 23.6 meV. Throughout this process, invariant Fermi wave vectors confirm that the enhancement originates from band renormalization and reconstruction rather than carrier doping. Our work establishes a route to tailor superconducting states via strain-activated electronic correlations and band engineering, and reveals a previously unrecognized orbital-selective pairing mechanism with broad implications for correlated multiband superconductors.

cond-mat.supr-con

Tip-Tuned Renormalization-Group Spectroscopy Unmasks a False-positive Topological Superconducting Vortex

Clean, nonsplit vortex zero-bias peaks (ZBPs) can be misinterpreted as Majorana zero modes (MZMs), making static scanning tunneling microscopy intrinsically ambiguous. Here we use the STM tip coupling to drive a local boundary-renormalization-group (boundary RG) flow, turning dynamical Coulomb blockade into a falsification test for Majorana-like ZBPs. Experimentally, in a $\mathrm{SrSn}_3$ thin film, normal-state spectra establish an Ohmic dissipative environment, and a common boundary-RG/thermodynamic-Bethe-ansatz analysis of the superconducting-gap and vortex-center spectra yields consistent dissipation strengths within the $r < 1/2$ Majorana-filter regime. Lowering the tip nevertheless drives a clean, non-split vortex-center ZBP into a zero-bias dip, opposite to the protected flow of an isolated MZM, unmasking the peak as a Majorana false positive produced by a conventional vortex-core state. The same flow selectively suppresses the strongly tip-coupled channel, resolving the two-gap superconductivity. Dissipative STM thus tests dynamical protection rather than spectral appearance.

cond-mat.mes-hall

Presence versus absence of charging energies in PbTe quantum dots

Charging energy ($E_C$) is essential in quantum dot (QD) devices. Previous studies on PbTe QDs have reported both the presence and absence of $E_C$. To resolve this ambiguity, we vary the QD size, i.e. the cross-sectional area of PbTe nanowires, and track the evolution of $E_C$. For large crosssectional areas ($\sim$ 16000 nm$^2$), the PbTe QDs exhibit no measurable $E_C$, while quantized levels are well resolved. Decreasing this area successively to 5000, 1500, and 460 nm$^2$, $E_C$ becomes finite and increases to 80, 160, and 210 $μ$eV, respectively. We further demonstrate the strong tunability of local gates, which can tune the PbTe device from the QD regime to the regime of ballistic transport. These results address concerns regarding the large dielectric constant of PbTe and provide key insights in engineering advanced PbTe quantum devices.

cond-mat.mes-hall

Probing PbTe-Pb nanowire devices with radio-frequency reflectometry

We report the implementation of radio-frequency (rf) reflectometry on selective-area-grown PbTe-Pb nanowire devices on a CdTe substrate. These nanowires are predicted to host Majorana zero modes. We demonstrate the compatibility of the rf technique, including both resistive and capacitive sensing, with these nanowires. The effect of dielectric loss from the CdTe substrate is quantitatively characterized. Furthermore, the feasibility of rf reflectometry is verified under finite magnetic fields where zero-energy modes can emerge. Our results establish the fast control of PbTe quantum devices, paving the way for their applications in topological quantum computation.

cond-mat.mes-hall

Antiferromagnetic Quantum Criticality in Infinite-Layer Cuprates Sr1-xNdxCuO2

The interplay between quantum criticality and Fermi surface reconstruction is central to elucidating the phase diagram of high-temperature cuprate superconductors. While studies on electron-doped T'-structure cuprates suggest an antiferromagnetic origin of this reconstruction, quantitative consensus has been hindered by apical oxygen instabilities and uncontrolled oxygen vacancies. Here, we overcome these limitations by utilizing ozone-assisted molecular beam epitaxy to synthesize high-quality, oxygen-stoichiometric thin films of infinite-layer cuprate Sr1-xNdxCuO2 across its entire superconducting dome. Hall transport measurements reveal a sharp carrier-type transition signaling a Fermi surface reconstruction at a critical doping xc ~ 0.155. We show that a spin-density-wave tight-binding model quantitatively reproduces the transport evolution, supporting an antiferromagnetic origin of this quantum phase transition. Furthermore, upon suppressing superconductivity with magnetic fields, the normal-state resistivity exhibits a pristine strange metal behavior that persists down to 2 K in the vicinity of xc. Our findings establish an intrinsic, universal antiferromagnetic quantum criticality in electron-doped cuprates, positioning the structurally simplest infinite-layer cuprates as a clean benchmark platform for theories of unconventional superconductivity.

cond-mat.supr-con

Bipolar-doped superconducting infinite-layer cuprates

Distilling the intrinsic physics of the superconducting CuO2 plane from the complexities of charge-reservoir layers is a defining challenge in high-temperature superconductivity. While superconducting electron-doped infinite-layer cuprates have been synthesized, controllable and uniform hole doping has long remained elusive despite exploratory attempts, limiting spectroscopic insights. Here, we realize bipolar doping across infinite-layer (Sr,Eu)CuO2 and (Ca,Li)CuO2+δ single-crystalline thin films, mapping the electronic phase diagram. Both electron- and hole-doped films show pronounced electrical resistance anisotropy, indicating the quasi-two-dimensional nature of the CuO2 planes. Angle-resolved photoemission spectroscopy across electron- and hole-doped regimes reveals persistent antiferromagnetic band folding coexisting with superconductivity. Remarkably, at a hole doping ~0.07 determined by Luttinger volume, the antiferromagnetic folding emerges from Fermi arcs within the film's single Fermi surface, with the onset superconducting transition temperature exceeding 60 K. These findings redefine the interplay between magnetic order and superconductivity and establish a definitive platform to investigate the intrinsic mechanism of high-temperature superconducting cuprates.

cond-mat.supr-con

Atomically resolved intrinsic superconducting gap in (La,Pr)3Ni2O7 films

Ruddlesden-Popper bilayer nickelates provide an emerging platform for studying high-temperature superconductivity, yet the superconducting pairing symmetry remains under debate. Here, we use atomic-resolution scanning tunnelling microscopy and spectroscopy to investigate superconducting 1.5-unit-cell (La,Pr)3Ni2O7 films grown on SrLaAlO4. A cryogenic ultrahigh-vacuum (UHV) sample transfer preserves an ordered sqrt(2) * sqrt(2) surface and yields reproducible U-shaped spectra with two gap scales of ~14 and ~20 meV and extended flat zero-conductance bottoms. By contrast, samples exposed for a longer time in UHV without cooling during transfer show V-shaped spectra despite retaining the surface reconstruction and a transport superconducting transition onset above 40 K. Wide-energy-range spectra indicate that oxygen loss can mix density-wave-related spectral weight. Our measurements provide an atomic-scale observation of the intrinsic nodeless superconducting gap in bilayer nickelate ultrathin films.

cond-mat.supr-con

$3d_{z^2}$ orbital delocalization and magnetic collapse in superconducting (La,Pr)$_3$Ni$_2$O$_{7-δ}$ films

The recent discovery of Ruddlesden--Popper (RP) nickelate thin-film superconductors has opened a new frontier in unconventional superconductivity. Its realization requires both compressive epitaxial strain and highly oxidative growth conditions, yet the microscopic pathway from the parent phase to the superconducting phase remains elusive. Here, X-ray absorption spectra and resonant inelastic X-ray scattering are employed to track this evolution by independently tuning strain and oxygen content in (La,Pr)$_3$Ni$_2$O$_{7-δ}$ thin films. We uncover a remarkable two-step narrative. First, signatures of delocalization emerge in the same way upon two independent tunings: Spectral weight transfers from a ''Upper Hubbard''-like peak to the hole-like peak associated with O $2p_z$ state, and in parallel, the initially localized Ni $3d_{z^2}$ orbital becomes more itinerant followed by the broadening and weakening of $dd$ orbital excitations. Second, as itinerancy increases, long-range spin-density-wave (SDW) order is suppressed in both intensity and correlation length, indicating direct competition with superconductivity. Yet, short-range magnons persist: they become damped but their bandwidth stays unchanged. Our results paint a coherent picture that both strain and oxygenation drive the RP bilayer nickelates towards the superconducting instability, where the O $2p_z$ and Ni $3d_{z^2}$ orbitals become delocalized. Concomitantly, the long-range magnetic order loses coherence and gets suppressed. These findings establish an orbital-selective route to RP nickelate superconductivity, in which the delocalization of the $2p_z$ and $3d_{z^2}$ orbitals and the robust short-range magnons upon the melting of SDW order are prerequisites, providing strong constraints for theory and the roadmap for designing nickelate superconductors.

cond-mat.supr-con

Electronic structures across superconductor-insulator transition in Ruddlesden-Popper bilayer nickelate films

High-transition-temperature ($T_{C}$) superconductivity is recently discovered in Ruddlesden-Popper (RP) nickelate films with extraordinarily strong oxidation. While investigating phase diagrams is essential for uncovering the superconducting mechanism, the oxygen-tuned superconductor-insulator transition (SIT) in RP nickelates differs fundamentally from that in cuprates or iron-based systems. Here, we unveil the evolution of electronic structure in RP bilayer nickelate thin films across the SIT, combining angle-resolved photoemission spectroscopy (ARPES) and X-ray absorption spectroscopy (XAS) for both occupied and unoccupied states. In the superconducting state, a coherent quasiparticle band near Fermi level ($E_{F}$) coexists with an incoherent waterfall feature at high energy, paralleling that in cuprates. Approaching the insulating state with oxygen deficiency, the spectral weight of the occupied coherent quasiparticle band is gradually suppressed, accompanied by pronounced density of states redistribution and orbital reconfiguration in unoccupied states. These results reveal the electronic origin of the SIT in the phase diagram, which transcends carrier doping effects and oxygen vacancy states. Our findings point to a decisive role of oxygen in shaping the essential electronic landscape of RP bilayer nickelates, offering crucial insights into the superconducting mechanism.

cond-mat.supr-con

Atomic-scale visualization of d-wave altermagnetism

Altermagnetism is a newly identified magnetic phase, distinct from conventional ferromagnetism and antiferromagnetism. It exhibits no net magnetization while breaking time-reversal symmetry. Although its momentum-space signatures are established, direct real-space visualization of its defining rotational-symmetry breaking remains missing. Here, using scanning tunnelling microscopy, we provide atomic-scale real-space evidence for altermagnetism in CsV2Se2O. Utilizing intrinsic spin defects as probes, we directly visualize the hallmark symmetry breaking through unidirectional electronic patterns and elliptical charging rings, both tied to the alternating spin texture. Moreover, adjacent spin-defect lines exhibit opposite spins and long-range antiferromagnetic coupling, hinting at a novel spin order. Our work moves the field from momentum-space probes to direct real-space visualization, opening a path to explore how this unconventional magnetic order couples to other quantum states.

cond-mat.mtrl-sci

Superconductivity and Electronic Structures of Nickelate Thin Film Superstructures

Ruddlesden-Popper (RP) nickelates have emerged as a crucial platform for exploring the mechanisms of high-temperature superconductivity. However, the Fermi surface topology required for superconductivity remains elusive. Here, beyond the superconducting pure bilayer (2222) phase, we report the thin film growth and ambient-pressure superconductivity of monolayer-bilayer (1212) and bilayer-trilayer (2323) superstructures, together with the absence of superconductivity in monolayer-trilayer (1313) superstructure, under identical compressive epitaxial strain. The onset superconducting transition temperatures range from 46 to 50 K, exceeding the McMillan limit. Angle-resolved photoemission spectroscopy reveals key Fermi surface differences in these atomically-engineered structures. In superconducting 1212 and 2222 films, a dispersive hole-like band ($γ^{\mathrm{II}}$) forms an underlying Fermi pocket, surrounding the Brillouin zone corner. In contrast, the top of the flat band ($γ^{\mathrm{III}}$) is observed ~70 meV below $E_\text{F}$ in the non-superconducting 1313 films. Particularly, the superconducting 2323 films host both $γ^{\mathrm{II}}$ and $γ^{\mathrm{III}}$ bands. The polarization dependence of the $γ$ bands reveals their Ni $d_{z^2}$ origin. Our findings expand the family of ambient-pressure nickelate superconductors and establish a connection between structural configuration, electronic structure, and the emergence of superconductivity in nickelates.

cond-mat.supr-con

Three-Dimensional Electronic Structures in Superconducting Ruddlesden-Popper Bilayer Nickelate Films

Beyond the quasi-two-dimensional (2D) paradigm of cuprates, the role of the third dimension of the Ruddlesden-Popper bilayer nickelates is essential to decoding their superconducting mechanism. Here, using angle-resolved photoemission spectroscopy (ARPES) with varied photon energies, we systematically investigate the electronic band structures in three dimensions for superconducting (La,Pr,Sm)$_3$Ni$_2$O$_7$/SrLaAlO$_4$ thin films (superconducting onset temperature $T_c^{\text{onset}} \sim 48$ K) transferred via a cryogenic ultra-high vacuum suitcase. We reveal an orbital-dependent dimensionality: while the $d{x^2-y^2}$-dominant bands exhibit a quasi-2D character, the $d{z^2}$-dominant band displays a finite $k_z$ dispersion. Finite energy gaps are identified on all observed bands across multiple high-symmetry directions. Systematic temperature-dependent analysis characterizes the superconducting nature of the gap on the $d{z^2}$-derived band, revealing a large gap $Δ\sim 18$ meV and a ratio $2Δ/k_BT_c\sim 8$ exceeding the weak-coupling BCS limit. The suppression of spectral weight near the Fermi level persists above the superconducting transition temperature. Ubiquitous waterfall-like spectral features evidence the presence of electron interactions. These results underscore the role of the $d_{z^2}$ orbital and correlations, placing constraints on theoretical models for nickelate superconductivity.

cond-mat.supr-con

Multimodal Terahertz Spectroscopy of the Pairing Symmetry and Normal-State Pseudogap in (La,Pr)$_3$Ni$_2$O$_7$ Films

The discovery of ambient-pressure superconductivity in compressively strained (La,Pr)$_3$Ni$_2$O$_7$ thin films has intensified efforts to identify the pairing mechanism. However, the symmetry of the superconducting order parameter and the character of the normal state remain unsettled. Here we combine bulk-sensitive terahertz (THz) time-domain spectroscopy with THz third-harmonic generation to present spectroscopic insights into these issues. Linear THz spectroscopy reveals a bulk superconducting response in the (La,Pr)$_3$Ni$_2$O$_7$ films, evidenced by the suppression of low-frequency spectral weight below the onset critical temperature, $T_\mathrm{c}^{\mathrm{onset}}$. A weak coherence peak near $T_\mathrm{c}^{\mathrm{onset}}$, together with substantial residual low-frequency conductivity as $T\to 0$, is consistent with disordered $s_{\pm}$-wave pairing. In the nonlinear regime, the third-harmonic signal rises sharply on cooling through $T_\mathrm{c}^{\mathrm{onset}}$, providing an independent signature of the transition. Strikingly, the nonlinear response persists above $T_\mathrm{c}^{\mathrm{onset}}$, pointing to either disorder-enhanced nonlinearity or a distinct correlated normal state. Motivated by angle-resolved photoemission spectroscopy on similarly grown films that identifies a comparable temperature scale, we associate the anomalous normal-state terahertz nonlinearity with a pseudogap. These results establish (La,Pr)$_3$Ni$_2$O$_7$ as a bulk superconductor with $s_{\pm}$-like pairing that coexists with, and may compete with, a distinct ordered state, providing a platform for exploring unconventional superconductivity beyond cuprates and pnictides.

cond-mat.supr-con

Strong enhancement of g-factor in PbTe-Pb hybrid nanowires

We report large Lande g-factors observed in PbTe-Pb hybrid nanowires. The g-factor can reach 83, significantly larger than those in bare PbTe nanowires (typically below 20). We attribute this enhancement to orbital effects in the superconducting film, particularly when the magnetic field is nearly perpendicular to the Pb film. This enhancement is beneficial for the search for topological superconductivity by reducing the critical magnetic field required for the phase transition.

cond-mat.mes-hall

Pressure-enhanced superconductivity and its correlation with suppressed resistance dip in (La,Pr)3Ni2O7 films

The discovery of superconductivity with a transition temperature (Tc) exceeding 40 K in La3Ni2O7 and (La,Pr)3Ni2O7 thin films at ambient pressure provides a viable platform for the experiments that can only be conducted under ambient-pressure conditions, and for the theoretical investigations aimed at understanding the commonalities and peculiarities of the behaviors related to the superconductivity between the film and the compressed bulk systems - including the effects of oxygen vacancies and strain. Consequently, it is crucial to determine whether Tc can be further enhanced and to uncover the underlying physics that controls the Tc value in these ambient-pressure superconducting thin films. Here, we report a systematic study of hydrostatic pressure effects on the superconducting properties of (La,Pr)3Ni2O7 thin films. We find that external pressure universally enhances Tc of the film samples regardless of their initial Tc value. The onset Tc of 68.5 K at 2.0 GPa demonstrates a notable increase from 62 K at 0.3 GPa. Furthermore, we observe that the samples without zero resistance show a resistance dip just above the superconducting transition, whereas the samples that exhibit zero resistance do not display this dip. Applying pressure can suppress the dips and drive the system toward zero resistance. Based on our results, we propose that this feature is associated with oxygen vacancies and that the depth of the dip can serve as an indicator of the concentration of the vacancies. It is plausible that the dip is caused by the localization of mobile electrons at the vacancy sites. Applying pressure can delocalize these electrons, which in turn may contribute to the increase in Tc.

cond-mat.supr-con

Spectroscopic Studies of two-dimensional Superconductivity

Two-dimensional superconductivity has become a major frontier in condensed matter physics. It holds the key to the mechanism of high-temperature superconductors and offers an exceptional arena to stabilize emergent quantum states enabled by enhanced electron correlations in reduced dimensionality. These states are frequently characterized by spatial modulations and intertwined with competing orders, calling for studies that combine real-space imaging with local spectroscopy. Scanning tunneling microscopy and spectroscopy meets this need by directly accessing local density of states with lattice-scale resolution. In this review, we summarize recent advances of the study on several representative unconventional superconductors using this technique, focusing on direct characterization of high-temperature superconducting planes, pair-density waves, and topological superconductivity in both artificial heterostructures and intrinsic materials. We conclude by outlining current challenges and future directions motivated by the microscopic insights.

cond-mat.supr-con